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Efficient cutting path planning for a non-spherical tool based on an iso-scallop height distance field

Chinese Journal of Aeronautics 2024年第7期37卷 496-510页

作者： Jiancheng HAO dong HE Zhaoyu LI Pengcheng HU Yuanzhi chen Kai TANG Department of Mechanical and Aerospace Engineering Hong Kong University of Science and TechnologyHong Kong 999077China The Hong Kong University of Science and Technology(Guangzhou) Smart Manufacturing ThrustNanshaGuangzhou 511400China HKUST Shenzhen-Hong Kong Collaborative Innovation Research Institute Shenzhen 518057China HKUST Shenzhen Research Institute Shenzhen 518057China

Iso-scallop height machining means,when machining a freeform surface,the scallop height between any two neighboring tool paths on the surface will be a constant(i.e.,the given threshold),which is preferable among various freeform surface machining strategies due to its high machining efficiency as well as better machine tool’s ***,all the existing iso-scallop height path planning methods pertain to only the ball-end or flat-end types of *** recent years,the non-spherical cutting tool has become more and more popular,especially for five-axis machining of complex freeform surfaces,majorly owing to its non-constant curvature which can be utilized to adaptively fit the tool to the surface to both avoid the local gouging and enlarge the cutting ***,there have been no reported works on iso-scallop height five-axis tool path generation for a non-spherical tool,and,in this paper,we present ***,we first define and construct two fields on the surface to be machined-the collision-free tool orientation field(vector)and the iso-scallop height distance field(scalar).The iso-lines of the scalar field and their associated tool orientation field vectors then naturally serve as potential iso-scallop height five-axis tool paths,and we present a propagation-based algorithm to construct the desired tool path from the *** computer simulation and physical cutting experiments confirm that everywhere on the surface,except maybe near the saddle curves of the scalar filed,the scallop height is exactly the given *** adding the saddle curves as extra tool paths,the final machined surface then is assured of the required scallop height requirement.

关键词： Freeform surface machining Iso-scallop tool path Customized tool Five-axis tool path Computer aided manufacturing

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Dynamic lithium-compensation mechanism for densification of garnet-type Li_(7)La_(3)Zr_(2)O_(12)electrolyte by Li_(2)O atmosphere buffer pair

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Nano Research 2024年第7期17卷 6184-6191页

作者： Chujun Zheng Ya chen Haoxin dong Yan Lu Jun Jin Zhaoyin Wen CAS Key Laboratory of Materials for Energy Conversion Shanghai Institute of CeramicsChinese Academy of ScienceShanghai 200050China State Key Lab High Performance Ceram and Superfine Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

Solid-state lithium metal batteries are one of the most promising options for next-generation batteries pursuing high-energy density and ***,the inevitable volatilization of lithium compounds during sintering leads to low relative density and low ionic conductivity of solid-state ***,the dynamic lithium-compensation mechanism is proposed to facilitate the densification of Ta-substituted garnet-type electrolyte(Li_(6.5)La_(3)Zr_(1.5)Ta_(0.5)O_(12)(LLZT))through the reversible manipulating of Li_(2)O ***_(2)ZrO_(3)is used as mother powder additive,which reacts with Li_(2)O in sintering atmosphere and forms Li_(6)Zr_(2)O_(7).Li_(2)ZrO_(3)/Li_(6)Zr_(2)O_(7)buffer pair manipulates the sintering Li_(2)O atmosphere,which is vital for LLZT,within the Li_(2)O partial pressure range corresponding to Li_(2)ZrO_(3)and Li_(6)Zr_(2)O_(7).Furthermore,the reversibility mechanism of buffer pair for Li_(2)O absorption and release is *** obtained LLZT exhibits a relative density of over 96%and an ionic conductivity exceeding 7×10^(−4)S·cm^(−1)with no abnormal grain *** symmetric cell demonstrates an excellent lithium dendrite suppressing ability(stable cycling at a current density of 0.3 mA·cm^(−2)for over 1000 h).Such dynamic lithium-compensation strategy has been successfully applied in atmosphere manipulation of LLZT sintering process,which reduces the dependence of LLZT on the Li_(2)O atmosphere,making it conducive to large-scale preparation of electrolyte ceramics.

关键词： solid-state batteries garnet-type electrolyte high-density electrolyte dynamic lithium-compensation buffer pair

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Memory-enhanced text style transfer with dynamic style learning and calibration

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Science China(Information Sciences) 2024年第4期67卷 181-196页

作者： Fuqiang LIN Yiping SONG Zhiliang TIAN Wangqun chen Diwen dong Bo LIU College of Computer Science and Technology National University of Defense Technology Department of Computer Science and Engineering The Hong Kong University of Science and Technology Strategic Assessments and Consultation Institute Academy of Military Sciences

Text style transfer aims to rephrase a sentence to match the desired style while retaining the original content. As a controllable text generation task, mainstream approaches use content-independent style embedding as control variables to guide stylistic generation. Nonetheless, stylistic properties are contextsensitive even under the same style. For example, “delicious” and “helpful” convey positive sentiments,although they are more likely to describe food and people, respectively. Therefore, desired style signals must vary with the content. To this end, we propose a memory-enhanced transfer method, which learns fine-grained style representation concerning content to assist transfer. Rather than employing static style embedding or latent variables, our method abstracts linguistic characteristics from training corpora and memorizes subdivided content with the corresponding style representations. The style signal is dynamically retrieved from memory using the content as a query, providing a more expressive and flexible latent style space. To address the imbalance between quantity and quality in different content, we further introduce a calibration method to augment memory construction by modeling the relationship between candidate *** results obtained using three benchmark datasets confirm the superior performance of our model compared to competitive approaches. The evaluation metrics and case study also indicate that our model can generate diverse stylistic phrases matching context.

关键词： style transfer memory-enhanced method text generation deep learning text representation

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Insight into the mechanism of 5-hydroxymethylfurfural electroreduction to 2,5-bis(hydroxymethyl)furan over Cu anchored N-doped carbon nanosheets

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Nano Research 2024年第9期17卷 7991-7999页

作者： Haoran Wu Xinwei chen Haishan Xu Runlu Yang Xin Wang Junying chen Zhenbing Xie liang Wu Yiyong Mai School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China School of Chemistry and Chemical Engineering Frontiers Science Center for Transformative MoleculesShanghai Key Laboratory of Electrical Insulation and Thermal AgeingShanghai Jiao Tong UniversityShanghai 200240China Department of Chemistry Tangshan Normal UniversityTangshan 063000China

Design of non-noble metal electrocatalysts for biomass conversion to high-value chemicals and understanding the related catalytic mechanisms are of profound significance but have remained a major ***,we developed a novel biomass-derived electrocatalyst(denoted as Cu/NC),featuring with electron-deficient copper nanoparticles anchored on N-doped carbon nanosheets,for the electrochemical reduction of 5-hydroxymethylfurfural(HMF)to 2,5-bis(hydroxymethyl)furan(BHMF,a vital precursor of functional polymers).The optimized Cu/NC electrocatalyst exhibited an excellent performance with high Faradaic efficiency(89.5%)and selectivity(90.8%)of BHMF at a low concentration of HMF(18.1 mM).Even at a very high HMF concentration(108.6 mM),the Faraday efficiency and selectivity of BHMF could still reach 74.8%and 81.1%,*** performance approached those of the reported noble metal-based *** study revealed that the N doping in the Cu/NC catalyst could regulate the electronic structure of Cu,strengthening the adsorption of the HMF carbonyl group,and thus boosting the selectivity of ***,strong electronic metal-support interactions of Cu and the N-doped carbon support optimized the charge transfer rate,thus promoting the dissociation of water to the active hydrogen(H^(*))species and boosting the reaction kinetic rate of H^(*)and HMF.

关键词： biomass 5-hydroxymethylfurfural electrochemical reduction N-doped carbon materials 2,5-bis(hydroxymethyl)furan

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Impact crater recognition methods:A review

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Science China Earth Sciences 2024年第6期67卷 1719-1742页

作者： dong chen Fan HU Liqiang ZHANG Yunzhao WU Jianli DU Jiju PEETHAMBARAN College of Civil Engineering Nanjing Forestry UniversityNanjing 210037China Department of Geography State Key Laboratory of Remote Sensing ScienceFaculty of Geographical ScienceBeijing Normal UniversityBeijing 100875China Purple Mountain Observatory Chinese Academy of SciencesNanjing 210023China Key Laboratory of Space Object and Debris Observation Chinese Academy of SciencesNanjing 210023China Department of Mathematics and Computing Science Saint Mary’s UniversityHalifaxNS B3H 3C3Canada

Impact craters are formed due to the high-speed collisions between small to medium-sized celestial *** is the most significant driving force in the evolution of celestial bodies,and the impact craters provide crucial insights into the formation,evolution,and impact history of celestial *** this paper,we present a detailed review of the characteristics of impact craters,impact crater remote sensing data,recognition algorithms,and applications related to impact *** first provide a detailed description of the geometric texture,illumination,and morphology characteristics observed in remote sensing data of *** we summarize the remote sensing data and cataloging databases for the four terrestrial planets(i.e.,the Moon,Mars,Mercury,and Venus),as well as the impact craters on ***,we study the advancement achieved in the traditional methods,machine learning methods,and deep learning methods applied to the classification,segmentation,and recognition of impact ***,based on the analysis results,we discuss the existing challenges in impact crater recognition and suggest some ***,we explore the implementation of impact crater detection algorithms and provide a forward-looking perspective.

关键词： Terrestrial planets Deep space exploration Impact crater Impact crater recognition Deep learning

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Quasi-two dimensional Ruddlesden−Popper halide perovskites for laser applications

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Frontiers of physics 2024年第2期19卷 53-71页

作者： Kun chen Qianpeng Zhang Yin liang Jiepeng Song Chun Li Shi chen Fang Li Qing Zhang School of Mechanical and Electrical Engineering Wuhan Institute of TechnologyWuhan 430205China School of Materials Science and Engineering Peking UniversityBeijing 100871China Institute of Applied Physics and Materials Engineering Macao UniversityMacao 999078China

Quasi-two-dimensional(2D)Ruddlesden‒Popper(RP)halide perovskites,as a kind of emerged two-dimensional layered materials,have recently achieved great attentions in lasing materials field owing to their large exciton binding energy,high emission yield,large optical gain,and wide-range tuning of optical *** review will introduce research progresses of RP halide perovskites for lasing applications in aspects of materials,photophysics,and devices with emphasis on emission and lasing properties tailored by the molecular composition and *** materials,structures and fabrications are introduced in the first ***,the optical transitions and amplified spontaneous emission properties are discussed from the aspects of electronic structure,exciton,gain dynamics,and interface ***,the research progresses on lasing devices are summarized and several types of lasers including VCSEL,DFB lasers,microlasers,random lasers,plasmonic lasers,and polariton lasers are *** last,the challenges and perspectives would be provided.

关键词： two-dimensional materials metal halide perovskite Ruddlesden−Popper halide perovskites lasing emission

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Reasonable design a high-entropy garnet-type solid electrolyte for all-solid-state lithium batteries

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Journal of Energy Chemistry 2024年第9期96卷 414-423页

作者： Shiyu Yu Yandi Li Jiaxin Luo Daming chen liang Yang Yaqing Wei De Li Yuanxun Li Yong chen State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science1nd EngineeringHainan Provincial Key Laboratory of Research on Utilization of Si-Zr-Ti ResourcesHainan UniversityHaikou 570228HainanChina State Key Laboratory of Electronic Thin Films1nd Integrated Devices University of Electronic Science1nd Technology of ChinaChengdu 610054SichuanChina Guangdong Key Laboratory for Hydrogen Energy Technologies School of Materials Science1nd Hydrogen EnergyFoshan UniversityFoshan 528000GuangdongChina

Traditional garnet solid electrolyte(Li_(7)La_(3)Zr_(2)O_(12))suffers from low room temperature ionic conductivity,poor air stability,high sintering temperature and energy *** the development prospects of high-entropy materials with high structural disorder and strong component controllability in the field of electrochemical energy storage,herein,a novel high-entropy garnet-type oxide solid electrolyte,Li_(5.75)Ga_(0.25)La_(3)Zr_(0.5)Ti_(0.5)Sn_(0.5)Nb_(0.5)O_(12)(LGLZTSNO)was constructed by partially replacing the Li and Zr sites in Li_(7)La_(3)Zr_(2)O_(12)with Ga and Ti/Sn/Nb elements,*** experimental and density functional theory(DFT)calculation results show that the high-entropy LGLZTSNO electrolyte has preferable room temperature ion conductivity,air stability,interface contact performance with lithium anode,and the ability to suppress lithium *** to the improvement of electrolyte performance,the critical current density of Li/Ag@LGLZTSNO/Li symmetric cell was increased from 0.42 to 1.57 mA cm^(−2),and the interface area specific impedance(IASR)was reduced from 765.2 to 42.3Ωcm^(2).Meanwhile,the Li/Ag@LGLZTSNO/LFP full cell also exhibits excellent rate performance and cycling performance(148 mA h g^(−1)at 0.1 C and 124 mA h g^(−1)at 0.5 C,capacity retention up to 84.8%after 100 cycles at 0.1 C),showing the application prospects of high-entropy LGLZTSNO solid electrolyte in high-performance all solid state lithium batteries.

关键词： Garnet solid electrolyte Dual-site substitution High-entropy all solid-state lithium batteries(ASSLBs)

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Synergistic Brønsted Base/Photoredox-Catalyzed Three-Component Coupling with Malonates to Synthesize δ-Hydroxy Esters and δ-Keto Esters

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Chinese Journal of Chemistry 2024年第9期42卷 957-962页

作者： Ting Li Wei Wang Ming dong Zhije Zhang Sha Yu Zhengchu chen Siping Wei dong Yi Green Pharmaceutical Technology Key Laboratory of Luzhou City Central Nervous System Drug Key Laboratory of Sichuan ProvinceSchoolof PharmacySouthwestMedicalUniversityLuzhouSichuan 646000China Nuclear Medicine and Molecular Imaging Key Laboratory of Sichuan Province LuzhouSichuan 646000China

Multicomponent alkene 1,2-dicarbofunctionalizations(DCFs)have emerged as a powerful strategy to rapidly incorporate both two carbon subunits across one C-C double bond in one step for enhancing molecular complexity and *** the best of our knowledge,there is only one report on photoredox-catalyzed three-component DCFs with malonates through the radical−radical cross-coupling,while photoredox-catalyzed radical-polar crossover(RPC)-type DCFs with malonates were still ***,we describe a redox-neutral RPC-type 1,2-dialkylation of styrenes with malonates and aldehydes through the synergistic Brønsted base/photoredox catalysis *** transition-metal-free strategy provides an efficient and clean approach to a broad variety ofδ-hydroxy esters and also features exceptionally mild conditions,wide compatibility of substrate scope and functional groups,and high atomic ***,three-component 1,2-alkylacylation from the same starting materials was achieved in one-pot manner through such RPC-type coupling and subsequent two-electron oxidation process,providing a set ofδ-keto esters of interest in pharmaceutical research.

关键词： Alkene difunctionalization Photoredox catalysis Malonates Radical reactions C-C coupling Synthetic methods Aldehydes Alkylation Multicomponentreactions

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Circularly polarized light emission and detection by chiral inorganic semiconductors

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Frontiers of Optoelectronics 2024年第2期17卷 43-49页

作者： Zha Li Wancai Li Dehui Li Wei Tang Huageng liang Huaibing Song Chao chen liang Gao Jiang Tang Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China International Health Care Center National Center for Global Health and MedicineTokyo 162‑8655Japan Hepato‑Biliary‑Pancreatic Surgery Division Department of SurgeryThe University of Tokyo HospitalTokyo 113‑8655Japan Department of Urology Union HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430074China Faculty of Materials Science and Chemistry China University of GeosciencesWuhan 430074China

Chiral inorganic semiconductors with high dissymmetric factor are highly desirable,but it is generally difficult to induce chiral structure in inorganic semiconductors because of their structure rigidity and *** this study,we introduced chiral ZnO film as hard template to transfer chirality to CsPbBr_(3) film and PbS quantum dots(QDs)for circularly polarized light(CPL)emission and detection,*** prepared CsPbBr_(3)/ZnO thin film exhibited CPL emission at 520 nm and the PbS QDs/ZnO film realized CPL detection at 780 nm,featuring high dissymmetric factor up to around *** electron transition based mechanism is responsible for chirality transfer.

关键词： High dissymmetric factor Circularly polarized light emission Semiconductor Hard template,Chirality

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Recent progress in online detection methods of bioaerosols

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Fundamental Research 2024年第3期4卷 442-454页

作者： Taicheng An Zhishu liang Zhen chen Guiying Li Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and Health Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlInstitute of Environmental Health and Pollution controlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlSchool of Environmental Science and EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China

The aerosol transmission of coronavirus disease in 2019,along with the spread of other respiratory diseases,caused significant loss of life and property;it impressed upon us the importance of real-time bioaerosol *** complexity,diversity,and large spatiotemporal variability of bioaerosols and their external/internal mixing with abiotic components pose challenges for effective online bioaerosol *** methods focus on directly capturing bioaerosols before subsequent time-consuming laboratory analysis such as culture-based methods,preventing the high-resolution time-based characteristics necessary for an online *** a comprehensive literature assessment,this review highlights and discusses the most commonly used real-time bioaerosol monitoring techniques and the associated commercially available *** applied in online bioaerosol monitoring,including adenosine triphosphate bioluminescence,laser/light-induced fluorescence spectroscopy,Raman spectroscopy,and bioaerosol mass spectrometry are *** working principles,characteristics,sensitivities,and efficiencies of these real-time detection methods are compared to understand their responses to known particle types and to contrast their *** developed to analyze the substantial data sets obtained by these instruments and to overcome the limitations of current real-time bioaerosol monitoring technologies are also ***,an outlook is proposed for future instrumentation indicating a need for highly revolutionized bioaerosol detection technologies.

关键词： Airborne microorganisms Real-time monitoring Adenosine triphosphate luminescence Laser/light-induced fluorescence Raman spectroscopy Bioaerosol mass spectrometry

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