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Dielectric metasurface evolution from bulk to monolayer by strong coupling of quasi-BICs for second harmonic boosting

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Photonics Research 2024年第4期12卷 784-792页

作者： YINONG XIE QIANTING chen JIN yao XUEYING LIU ZHAOGANG dong JINFENG ZHU Institute of Electromagnetics and Acoustics and Key Laboratory of Electromagnetic Wave Science and Detection Technology Xiamen UniversityXiamen 361005China Shenzhen Research Institute of Xiamen University Shenzhen 518057China Department of Electrical Engineering City University of Hong KongHong Kong 999077China Institute of Materials Research and Engineering(IMRE) Agency for ScienceTechnology and Research(A*STAR)Singapore 138634Singapore Department of Materials Science and Engineering National University of SingaporeSingapore 117575Singapore

2D materials are promising candidates as nonlinear optical components for on-chip devices due to their ultrathin structure. In general, their nonlinear optical responses are inherently weak due to the short interaction thickness with light. Recently, there has been great interest in using quasi-bound states in the continuum (q-BICs) of dielectric metasurfaces, which are able to achieve remarkable optical near-field enhancement for elevating the second harmonic generation (SHG) emission from 2D materials. However, most studies focus on the design of combining bulk dielectric metasurfaces with unpatterned 2D materials, which suffer considerable radiation loss and limit near-field enhancement by high-quality q-BIC resonances. Here, we investigate the dielectric metasurface evolution from bulk silicon to monolayer molybdenum disulfide (MoS2), and discover the critical role of meta-atom thickness design on enhancing near-field effects of two q-BIC modes. We further introduce the strongcoupling of the two q-BIC modes by oblique incidence manipulation, and enhance the localized optical field on monolayer MoS2dramatically. In the ultraviolet and visible regions, the MoS2SHG enhancement factor of our design is 105times higher than that of conventional bulk metasurfaces, leading to an extremely high nonlinear conversion efficiency of 5.8%. Our research will provide an important theoretical guide for the design of high-performance nonlinear devices based on 2D materials.

关键词： monolayer harmonic quasi

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Investigating the Absorption and Desorption Behavior of Methylene Chloride in the Poly(aryl ether ketone) Film with Different Crystallinities

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Chinese Journal of Polymer Science 2024年第2期42卷 239-246,I0009页

作者： Hong-Ru Yang Jin-dong Zhang dong-Ting Gao Gang Liu Chun-Hai chen Jia-Nan yao Center for Advanced Low-Dimension Materials State Key Laboratory for Modification of Chemical Fibers and Polymer MaterialsCollege of Materials Science and EngineeringDonghua UniversityShanghai201620China

Poly(aryl ether keton e)(PAEK) films with different crystallinities were obtained by controlling the cooling rate,which were subjected to the absorption and desorption of methylene chloride(CH_(2)Cl_(2)).We employed attenuated total reflection Fourier transform infrared(ATR-FTIR)spectroscopy analyses to investigate the diffusion behavior of CH_(2)Cl_(2) in PAEK films with different crystallinities.According to the Fickian diffusion model,the calculated diffu sion coefficients of CH_(2)Cl_(2) in PAEK films were observed to decrease with increasing crystallinity.The effect of CH_(2)Cl_(2)absorption and desorption on the mechanical properties of PAEK films with different crystallinity was further analyzed using tensile tests.The tensile tests exhibited that CH_(2)Cl_(2) has two concurrent effects:plasticization and solvent-induced crystallization.Differential scanning calorimetry(DSC) and wide-angle X-ray diffraction(WXRD) techniques further confirmed solvent-induced crystallization behavior.The results would be beneficial to understand the solvent resistance of PAEK materials and consequently provide the practical application conditions of PAEK with a theoretical basis.

关键词： Poly(aryl ether ketone) Diffusion behavior Infrared spectra Solvent-induced crystallization Mechanical properties

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Investigation into the roles of interfacial H_(2)O structure in catalytic oxidation of HCHO and CO over CuMnO_(2) catalysts

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Journal of Environmental Sciences 2024年第3期137卷 310-320页

作者： Chunyan Ma Jushuang Pan cheng chen Yuanyuan dong Feng yao Fengbang Wang Maoyong Song Key Laboratory of Environmental Nanotechnology and Health Effects Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China No.52 Institute of China North Industries Group Yantai Branch Co.Ltd. Yantai 264000China

The rapid deactivation of cost-effective MnO_(2)-based catalysts in humid air limits their application in practice,and the identification of the role of water in an oxidation process is significant for developing water-resistant MnO_(2)-based catalysts.Here,CuMnO_(2)showed a20.3%HCHO conversion in 10 hr at room temperature in humid air with relative humidity of 40%,but deactivated in 3 hr in dry air.The excellent activity and stability of HCHO oxidation in humid air were attributed to the positive effect of H_(2)O on HCHO oxidation to the H_(2)O-HOCH_(2)OH supermolecule assemblies via hydrogen bonds formed on CuMnO_(2).H_(2)O-HOCH_(2)OH supermolecule assemblies tend to be oxidized to carbonate,which is further oxidized to CO_(2).Furthermore,CuMnO_(2)exhibited a much poorer activity of CO oxidation in humid air,but the CO conversion was still 100%in 10 hr in dry air.H_(2)O showed a competitive adsorption effect to CO on CuMnO_(2).CuMnO_(2)could be applied in HCHO elimination in humid air and CO elimination in dry air.

关键词： H_(2)O-HOCH_(2)OH supermolecule HCHO oxidation Humid air CuMnO_(2) CO oxidation

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Temperature-Dependent Tearing Behavior of Rubber Materials:Characterization and Modeling

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Acta Mechanica Solida Sinica 2024年第2期37卷 316-326页

作者： Qinyuan yao Feilong Zhang Pan dong Ziyuan Zhao Yi He Weiguo Li Liming chen State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing400044China College of Aerospace Engineering Chongqing UniversityChongqing400044China

With the increasingly widespread application of rubber in many fields,there is a growing demand for quantitative characterization of temperature-dependent mechanical properties in high-temperature service environments.The critical tearing energy is an important criterion for determining whether rubber materials will experience tearing instability,while tear strength is a key parameter for rubber materials to resist tearing.It is necessary to quantitatively characterize their evolution with temperature.Current theoretical research mainly relies on fitting a large amount of experimental data,which is not convenient for engineering applications.Therefore,in this work,a temperature-dependent critical tearing energy model is firstly developed based on the force-heat equivalence energy density principle.This model considers the equivalent relationship between the critical tearing energy required for crack instability propagation and the thermal energy stored in the rubber material.It is demonstrated that our model has higher prediction accuracy when compared to other models.Furthermore,combining with the Griffith fracture theory,temperature-dependent tear strength models applicable to three different crack modes are separately established.These models are validated using experimental data for Mode I opening cracks and ModeⅢtearing cracks,and good consistency is achieved.Additionally,a quantitative analysis of the influence of elastic modulus on tear strength at different temperatures is conducted.This work provides a reliable way for predicting temperature-dependent tearing instability behavior and offers beneficial suggestions for improving the tear strength of rubber materials at different temperatures.

关键词： Temperature-dependent Critical tearing energy Tear strength Rubber Theoretical model

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On hypersurfaces of H2×H2

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Science China Mathematics 2024年第2期67卷 339-366页

作者： dong Gao Hui Ma Zeke yao School of Science Beijing University of Civil Engineering and Architecture Department of Mathematical Sciences Tsinghua University

In this paper, we study hypersurfaces of H2× H2. We first classify the hypersurfaces with constant principal curvatures and constant product angle functions. Then we classify homogeneous hypersurfaces and isoparametric hypersurfaces, respectively. Finally, we classify the hypersurfaces with at most two distinct constant principal curvatures, as well as those with three distinct constant principal curvatures under some additional conditions.

关键词： constant principal curvature homogeneous hypersurface isoparametric hypersurface 53C42 53B25 53C40

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Quantum Curve and Bilinear Fermionic Form for the Orbifold Gromov–Witten Theory of P[r]

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Acta Mathematica Sinica,English Series 2024年第1期40卷 43-80页

作者： Chong yao chen Shuai GUO Mathematics Department Duke UniversityBox 90320DurhamNC 27708-0320USA School of Mathematical Sciences Peking UniversityBeijing 100871P.R.China

We construct the quantum curve for the Baker-Akhiezer function of the orbifold Gromov-Witten theory of the weighted projective line P[r].Furthermore,we deduce the explicit bilinear Fermionic formula for the(stationary... 详细信息

关键词： Quantum curve Free Fermions Gromov-Witten invariants Orbifold P^(1)

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Ten-year observation of corneal densitometry and associated factors following small incision lenticule extraction

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International Journal of Ophthalmology(English edition) 2024年第3期17卷 485-490页

作者： Xiao-Song Han Fei Xia Zhuo-Yi chen Pei-Jun yao dong-Mei Yang Jing Zhao Xing-Tao Zhou Eye Institute and Department of Ophthalmology Eye&ENT HospitalFudan UniversityShanghai 200031China NHC Key Laboratory of Myopia(Fudan University) Key Laboratory of MyopiaChinese Academy of Medical SciencesShanghai 200031China Shanghai Research Center of Ophthalmology and Optometry Shanghai 200031China Shanghai Engineering Research Center of Laser and Autostereoscopic 3D for Vision Care(20DZ2255000) Shanghai 200031China

●AIM:To investigate the long-term changes of corneal densitometry(CD)and its contributing elements after small incision lenticule extraction(SMILE).●METHODS:Totally 31 eyes of 31 patients with mean spherical equivalent of-6.46±1.50 D and mean age 28.23±7.38y were enrolled.Full-scale examinations were conducted on all patients preoperatively and during followup.Visual acuity,manifest refraction,axial length,corneal thickness,corneal higher-order aberrations,and CD were evaluated.●RESULTS:All surgeries were completed successfully without complications or adverse events.Ten-year safety index was 1.17±0.20 and efficacy 1.04±0.28.CD value of 0–6 mm zones in central layer was statistically significantly lower 10y postoperatively,compared with preoperative values(0–2 mmΔ=-1.62,2–6 mmΔ=-1.24,P<0.01).There were no correlations between CD values and factors evaluated.●CONCLUSION:SMILE is a safe and efficient procedure for myopia on a long-term basis.CD values get lower 10y postoperatively,whose mechanism is to be further discussed.

关键词： myopia small incision lenticule extraction corneal densitometry

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Numerical Simulation of the Settling Flux of Biodeposition in a Bay with Cage Culture Through Similarity Theory and a Simplified Pollution Source

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Journal of Ocean University of China 2024年第1期23卷 247-254页

作者： LIU yao chen Yifan GE Changzi Marine College Shandong UniversityWeihai 264209China

The settling flux of biodeposition affects the environmental quality of cage culture areas and determines their environmental carrying capacity.Simple and effective simulation of the settling flux of biodeposition is extremely important for determining the spatial distribution of biodeposition.Theoretically,biodeposition in cage culture areas without specific emission rules can be simplified as point source pollution.Fluent is a fluid simulation software that can simulate the dispersion of particulate matter simply and efficiently.Based on the simplification of pollution sources and bays,the settling flux of biodeposition can be easily and effectively simulated by Fluent fluid software.In the present work,the feasibility of this method was evaluated by simulation of the settling flux of biodeposition in Maniao Bay,Hainan Province,China,and 20 sampling sites were selected for determining the settling fluxes.At sampling sites P1,P2,P3,P4,P5,Z1,Z2,Z3,Z4,A1,A2,A3,A4,B1,B2,C1,C2,C3 and C4,the measured settling fluxes of biodeposition were 26.02,15.78,10.77,58.16,6.57,72.17,12.37,12.11,106.64,150.96,22.59,11.41,18.03,7.90,19.23,7.06,11.84,5.19 and 2.57 g d^(−1)m^(−2),respectively.The simulated settling fluxes of biodeposition at the corresponding sites were 16.03,23.98,8.87,46.90,4.52,104.77,16.03,8.35,180.83,213.06,39.10,17.47,20.98,9.78,23.25,7.84,15.90,6.06 and 1.65 g d^(−1)m^(−2),respectively.There was a positive correlation between the simulated settling fluxes and measured ones(R=0.94,P=2.22×10^(−9)<0.05),which implies that the spatial differentiation of biodeposition flux was well simulated.Moreover,the posterior difference ratio of the simulation was 0.38,and the small error probability was 0.94,which means that the simulated results reached an acceptable level from the perspective of relative error.Thus,if nonpoint source pollution is simplified to point source pollution and open waters are simplified based on similarity theory,the setting flux of biodeposition in the open waters can be simply and effectively

关键词： fluent fluid simulation software pollution source simplification posterior difference ratio similarity theory Spear-man correlation

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Tau Accumulation in the Spinal Cord Contributes to Chronic Inflammatory Pain by Upregulation of IL-1βand BDNF

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Neuroscience Bulletin 2024年第4期40卷 466-482页

作者： Shuxia Zhang Yeru chen Yongjie Wang Hongwei Wang Dandan yao Gang chen Department of Anesthesiology School of MedicineSir Run Run Shaw HospitalZhejiang UniversityHangzhou310016China Key Laboratory of Elemene Anti-Cancer Medicine of Zhejiang Province and Holistic Integrative Pharmacy Institutes Hangzhou Normal UniversityHangzhou311121China Engineering Laboratory of Development and Application of Traditional Chinese Medicine from Zhejiang Province Holistic Integrative Pharmacy InstitutesHangzhou Normal UniversityHangzhou311121China

Microtubule-associated protein Tau is responsible for the stabilization of neuronal microtubules under normal physiological conditions.Much attention has been focused on Tau’s contribution to cognition,but little research has explored its role in emotions such as pain,anxiety,and depression.In the current study,we found a significant increase in the levels of p-Tau(Thr231),total Tau,IL-1β,and brain-derived neurotrophic factor(BDNF)on day 7 after complete Freund's adjuvant(CFA)injection;they were present in the vast majority of neurons in the spinal dorsal horn.Microinjection of Mapt-shRNA recombinant adeno-associated virus into the spinal dorsal cord alleviated CFA-induced inflammatory pain and inhibited CFA-induced IL-1βand BDNF upregulation.Importantly,Tau overexpression was sufficient to induce hyperalgesia by increasing the expression of IL-1βand BDNF.Furthermore,the activation of glycogen synthase kinase 3 beta partly contributed to Tau accumulation.These findings suggest that Tau in the dorsal horn could be a promising target for chronic inflammatory pain therapy.

关键词： Tau Inflammatory pain IL-1β BDNF

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A Galaxy Image Augmentation Method Based on Few-shot Learning and Generative Adversarial Networks

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Research in Astronomy and Astrophysics 2024年第3期24卷 180-193页

作者： Yiqi yao Jinqu Zhang Ping Du Shuyu dong School of Artificial Intelligence South China Normal UniversityFoshan 528225China School of Computer Science South China Normal UniversityGuangzhou 510631China Guangdong Construction Vocational Technology Institute Guangzhou 511500China

Galaxy morphology classifications based on machine learning are a typical technique to handle enormous amounts of astronomical observation data,but the key challenge is how to provide enough training data for the machine learning models.Therefore this article proposes an image data augmentation method that combines few-shot learning and generative adversarial networks.The Galaxy10 DECaLs data set is selected for the experiments with consistency,variance,and augmentation effects being evaluated.Three popular networks,including AlexNet,VGG,and ResNet,are used as examples to study the effectiveness of different augmentation methods on galaxy morphology classifications.Experiment results show that the proposed method can generate galaxy images and can be used for expanding the classification model’s training set.According to comparative studies,the best enhancement effect on model performance is obtained by generating a data set that is 0.5–1 time larger than the original data set.Meanwhile,different augmentation strategies have considerably varied effects on different types of galaxies.FSL-GAN achieved the best classification performance on the ResNet network for In-between Round Smooth Galaxies and Unbarred Loose Spiral Galaxies,with F1 Scores of 89.54%and 63.18%,respectively.Experimental comparison reveals that various data augmentation techniques have varied effects on different categories of galaxy morphology and machine learning models.Finally,the best augmentation strategies for each galaxy category are suggested.

关键词： techniques image processing-galaxies structure-galaxies general

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