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Surface-functionalized hole-selective monolayer for high efficiency single-junction wide-bandgap and monolithic tandem perovskite solar cells

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Journal of Energy Chemistry 2024年第1期88卷 317-326,I0008页

作者： Devthade Vidyasagar Yeonghun Yun Jae Yu Cho Hyemin Lee Kyung Won kim Yong Tae kim Sung Woong Yang Jina Jung Won Chang Choi Seonu kim Rajendra Kumar Gunasekaran Seok Beom Kang Kwang Heo dong hoe kim Jaeyeong Heo Sangwook Lee School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Department of Materials Science and Engineering and Optoelectronics Convergence Research CenterChonnam National UniversityGwangju 61186Republic of Korea Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea Department of Nanotechnology and Advanced Materials Engineering Sejong UniversitySeoul 05006Republic of Korea

Carbazole moiety-based 2PACz([2-(9H-carbazol-9-yl)ethyl]phosphonic acid)self-assembled monolayers(SAMs)are excellent hole-selective contact(HSC)materials with abilities to excel the charge-transferdynamics of perovskite solar cells(PSCs).Herein,we report a facile but powerful method to functionalize the surface of 2PACz-SAM,by which reproducible,highly stable,high-efficiency wide-bandgap PSCs can be *** 2PACz surface treatment with various donor number solvents improves assembly of 2PACz-SAM and leave residual surface-bound solvent molecules on 2PACz-SAM,which increases perovskite grain size,retards halide segregation,and accelerates hole *** surface functionalization achieves a high power conversion efficiency(PCE)of 17.62%for a single-junction wide-bandgap(~1.77 e V)*** also demonstrate a monolithic all-perovskite tandem solar cell using surfaceengineered HSC,showing high PCE of 24.66%with large open-circuit voltage of 2.008 V and high fillfactor of 81.45%.Our results suggest this simple approach can further improve the tandem device,when coupled with a high-performance narrow-bandgap sub-cell.

关键词： Perovskite solar cells 2PACz Monolithic tandem solar cells Wide bandgap

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High-throughput compositional mapping of triple-cation tin-lead perovskites for high-efficiency solar cells

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InfoMat 2023年第4期5卷 25-38页

作者： Rajendra Kumar Gunasekaran Jina Jung Sung Woong Yang Jungchul Yun Yeonghun Yun Devthade Vidyasagar Won Chang Choi Chang-Lyoul Lee Jun Hong Noh dong hoe kim Sangwook Lee School of Materials Science and Engineering Kyungpook National UniversityDaeguRepublic of Korea Advanced Photonics Research Institute(APRI) Gwangju Institute of Science and Technology(GIST)GwangjuRepublic of Korea School of Civil Environmental and Architectural EngineeringGreen SchoolKorea UniversitySeoulRepublic of Korea Department of Materials Science and Engineering Korea UniversitySeoulRepublic of Korea

Mixed tin-ead perovskites suffer from structural instability and rapid tin oxidation;thus,the investigation of their optimal composition ranges is important to address these inherent *** critical role of triple cations in mixed Sn–Pb iodides is studied by performing a wide range of compositional screenings over mechanochemically synthesized bulk and solution-processed thin films.A ternary phase map of FA(Sn_(0.6)Pb_(0.4))I_(3),MA(Sn_(0.6)Pb_(0.4))I_(3),and Cs(Sn_(0.6)Pb_(0.4))I_(3)is formed,and a promising composition window of(FA_(0.6-x)MA_(0.4)Cs_(x))Sn_(0.6)Pb_(0.4)I_(3)(0≤x≤0.1)is demonstrated through phase,photoluminescence,and stability *** cell performance and chemical stability across the targeted compositional space are investigated,and FA_(0.55)MA_(0.4)Cs_(0.05)Sn_(0.6)Pb_(0.4)I_(3)with strain-relaxed lattices,reduced defect densities,and improved oxidation stability is *** inverted perovskite solar cells with the optimal composition demonstrate a power conversion efficiency of over 22%with an open-circuit voltage of 0.867 V,which corresponds to voltage loss of 0.363 V,promising for the development of narrow-bandgap perovskite solar cells.

关键词： compositional engineering mixed tin-ead iodides narrow-bandgap perovskites perovskite solar cells strain relaxation ternary phase mapping

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Aligned Ion Conduction Pathway of Polyrotaxane‑Based Electrolyte with Dispersed Hydrophobic Chains for Solid‑State Lithium–Oxygen Batteries

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Nano-Micro Letters 2025年第2期17卷 169-186页

作者： Bitgaram kim Myeong‑Chang Sung Gwang‑Hee Lee Byoungjoon Hwang Sojung Seo Ji‑Hun Seo dong‑Wan kim Department of Materials Science and Engineering Korea University145 Anam‑RoSeongbuk‑GuSeoul 02841Republic of Korea School of Civil Environmental and Architectural EngineeringKorea University145 Anam‑RoSeongbuk‑GuSeoul 02841Republic of Korea Materials Science and Chemical Engineering Center Institute for Advanced Engineering(IAE)Yongin 17180Republic of Korea

A critical challenge hindering the practical application of lithium–oxygen batteries(LOBs)is the inevitable problems associated with liquid electrolytes,such as evaporation and safety *** study addresses these problems by proposing a modified polyrotaxane(mPR)-based solid polymer electrolyte(SPE)design that simultaneously mitigates solvent-related problems and improves ***-SPE exhibits high ion conductivity(2.8×10^(−3)S cm^(−1)at 25℃)through aligned ion conduction pathways and provides electrode protection ability through hydrophobic chain *** this mPR-SPE into solid-state LOBs resulted in stable potentials over 300 *** situ Raman spectroscopy reveals the presence of an LiO_(2)intermediate alongside Li_(2)O_(2)during oxygen *** situ X-ray diffraction confirm the ability of the SPE to hinder the permeation of oxygen and moisture,as demonstrated by the air permeability *** present study suggests that maintaining a low residual solvent while achieving high ionic conductivity is crucial for restricting the sub-reactions of solid-state LOBs.

关键词： Solid polymer electrolyte Lithium-oxygen batteries Polyrotaxane ion conductivity Hydrophobic chain

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A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three‑Dimensionally Conductive MOF Network for Gas and Pressure Sensing

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Nano-Micro Letters 2025年第2期17卷 601-620页

作者： Qingqing Zhou Qihang Ding Zixun Geng Chencheng Hu Long Yang Zitong Kan Biao dong Miae Won Hongwei Song Lin Xu Jong Seung kim State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012People’s Republic of China Department of Chemistry Korea UniversitySeoul 02841Republic of Korea TheranoChem Incorporation Seoul 02856Republic of Korea

The rising flexible and intelligent electronics greatly facilitate the noninvasive and timely tracking of physiological information in telemedicine *** building bionic-sensitive moieties is vital for designing efficient electronic skin with advanced cognitive functionalities to pluralistically capture external ***,realistic mimesis,both in the skin’s three-dimensional interlocked hierarchical structures and synchronous encoding multistimuli information capacities,remains a challenging yet vital need for simplifying the design of flexible logic ***,we construct an artificial epidermal device by in situ growing Cu_(3)(HHTP)_(2) particles onto the hollow spherical Ti_(3)C_(2)T_(x) surface,aiming to concurrently emulate the spinous and granular layers of the skin’s *** bionic Ti_(3)C_(2)T_(x)@Cu_(3)(HHTP)_(2) exhibits independent NO_(2) and pressure response,as well as novel functionalities such as acoustic signature perception and Morse code-encrypted message ***,a wearable alarming system with a mobile application terminal is self-developed by integrating the bimodular senor into flexible printed *** system can assess risk factors related with asthmatic,such as stimulation of external NO_(2) gas,abnormal expiratory behavior and exertion degrees of fingers,achieving a recognition accuracy of 97.6%as assisted by a machine learning *** work provides a feasible routine to develop intelligent multifunctional healthcare equipment for burgeoning transformative telemedicine diagnosis.

关键词： Ti_(3)C_(2)T_(x)@Cu_(3)(HHTP)_(2)composites NO_(2)/pressure flexible sensors Health-monitoring Machine learning

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Risk Analysis of Breakwater Caisson Under Wave Attack Using Load Surface Approximation

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China Ocean Engineering 2014年第6期28卷 739-748页

作者： dong Hyawn kim Department of Ocean Science and Engineering Kunsan National University

A new load surface based approach to the reliability analysis of caisson-type breakwater is proposed. Uncertainties of the horizontal and vertical wave loads acting on breakwater are considered by using the so-called load surfaces, which can be estimated as functions of wave height, water level, and so on. Then, the first-order reliability method（FORM） can be applied to determine the probability of failure under the wave action. In this way, the reliability analysis of breakwaters with uncertainties both in wave height and in water level is possible. Moreover, the uncertainty in wave breaking can be taken into account by considering a random variable for wave height ratio which relates the significant wave height to the maximum wave height. The proposed approach is applied numerically to the reliability analysis of caisson breakwater under wave attack that may undergo partial or full wave breaking.

关键词： failure probability load surface reliability caisson breakwater wave breaking FORM

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Probabilistic Distribution of the Maximum Wave Heigh

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China Ocean Engineering 2014年第5期28卷 579-586页

作者： dong Hyawn kim Taerim kim Department of Ocean Science and Engineering Kunsan National University

A new method of treating maximum wave height as a random variable in reliability analysis of breakwater caissons isproposed. The maximum wave height is expressed as the significant wave height multiplied by the so-called wave height *** proposed wave height ratio is a type of transfer function from the significant wave height to the maximum wave *** the condition of a breaking wave, the ratio is intrinsically nonlinear. Therefore, the probability density function for thevariable cannot be easily defined. In this study, however, it can be derived from the relationship between the maximum andsignificant waves in a nonbreaking environment. Some examples are shown to validate the derived probability density functionfor the wave ratio parameter. By introducing the wave height ratio into reliability analysis of caisson breakwater, the maximumwave height can be used as an independent and primary random variable, which means that the risk of caisson failure during itslifetime can be evaluated realistically.

关键词： maximum wave height wave height ratio reliability caisson breakwater wave breaking

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Experimental Study on the Inlet Fogging System Using Two-Fluid Nozzles

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Journal of Thermal Science 2010年第2期19卷 132-135页

作者： Abhilash Suryan dong Sun kim Heuy dong kim School of Mechanical Engineering Andong National University FMTRC Daejoo Machinery Co.

Large-capacity compressors in industrial plants and the compressors in gas turbine engines consume a considerable amount of power. The compression work is a strong fimction of the ambient air temperature. This increase in compression work presents a significant problem to utilities, generators and power producers when electric demands are high during the hot months. In many petrochemical process industries and gas turbine engines, the in- crease in compression work curtails plant output, demanding more electric power to drive the system. One way to counter this problem is to directly cool the inlet air. Inlet fogging is a popular means of cooling the inlet air to air compressors. In the present study, experiments have been performed to investigate the suitability of two-fluid nozzle for inlet fogging. Compressed air is used as the driving working gas for two-fluid nozzle and water at am- bient conditions is dragged into the high-speed air jet, thus enabling the entrained water to be atomized in a very short distance from the exit of the two-fluid nozzle. The air supply pressure is varied between 2.0 and 5.0 bar and the water flow rate entrained is measured. The flow visualization and temperature and relative humidity measurements are carried out to specify the fogging characteristics of the two-fluid nozzle.

关键词： Evaporative Cooling Inlet Fogging Energy Savings Two-fluid Nozzles

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Expected Sliding Distance of Vertical Slit Caisson Breakwater

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China Ocean Engineering 2017年第3期31卷 317-321页

作者： dong Hyawn kim Department of Ocean Science & Engineering Ktmsan National University Daehakro 558 Kunsan Jeormuk 54150 Republic of Korea

Evaluating the expected sliding distance of a vertical slit caisson breakwater is proposed. Time history for the wave load to a vertical slit caisson is made. It consists of two impulsive wave pressures followed by a smooth sinusoidal pressure. In the numerical analysis, the sliding distance for an attack of single wave was shown and the expected sliding distance during 50 years was also presented. Those results were compared with a vertical front caisson breakwater without slit. It was concluded that the sliding distance of a vertical slit caisson may be over-estimated if the wave pressure on the caisson is evaluated without considering vertical slit.

关键词： breakwater vertical slit caisson expected sliding distance reliability performance based design

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Preparation and characterization of 3-dimensionally ordered macroporous SiC

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Science China(Technological Sciences) 2006年第1期49卷 1-9页

作者： kim dong-pyo Department of Fine Chemical Engineering and Chemistry of Chungnam National University Taejon 305-764 South Korea

Three-dimensionally (3D) long range ordered macroporous SiC ceramics were prepared through infiltrating polymethylsilane (PMS) into the 3D ordered sacrificial silica template, pyrolysis and the template removal. It was found that the pore size (84―658 nm), BET surface area (299.44―584.64 m2/g) and micropore volume (0.25―0.64 cm3/g) of the achieved porous SiC can be tailored by utilizing different sizes silica sphere templates. There exist three kinds of pores in the porous ceramics: sphere inversed pores, windows and mesopores (2―5 nm). The sphere inversed pores were packed as hcp structure and three dimensionally penetrated through the windows, and the mesopores endowed the porous ceramics surprising high BET surface areas and micropore volumes.

关键词： three-dimensionally ordered materials, templated technique, preceramic polymer conversion technique, SiC ceramic.

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China’s Changing Economic Structure and Implications for Regional Patterns of Trade,Production and Integration

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China & World Economy 2006年第6期14卷 1-19页

作者： kim Song Tan hoe Ee Khor Practice Associate Professor Singapore Management University Singapore. Email: kstan@smu.edu.sg Assistant Managing Director Monetary Authority of Singapore. Email: hkhor@mas.gov.sg

Without intending to do so, China has in recent years played a major role in East Asia＇s economic integration. It has done so mainly through the production and supply chain networks it has spun across the region. This paper argues that given the developmental trends in the Chinese economy, the Chinese government should pursue a more active strategy towards a broader and more balanced economic integration with the region. The emergence of a multi-track production structure, increased importance of domestic consumption and the services sector, together with faster integration of the domestic economy, will fundamentally change China＇s trade and investment relationships with the rest of East Asia and necessitate a review of China＇s economic integration strategy. The paper also argues that ASEAN can play a useful role in facilitating the region-wide integration process.

关键词： China East Asia economic integration production networks

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