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Palladium-assisted Metal Patterning on Polyimide Surfaces

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Chinese Journal of Polymer Science 2022年第10期40卷 1287-1296,I0011页

作者： Shi-Long Zhong Bai-Yang Zhou Xi-Rui Gu ding-shan yu Xu-Dong Chen Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education Key Laboratory of High Performance Polymer-based Composites of Guangdong Province School of Chemistry Sun Yat-sen UniversityGuangzhou 510275China

A novel method of patterning high precision copper conductive micropatterns on flexible polymer substrate(polyimide)is *** utilized the coordination effect between palladium salts and pyridine structures to fix the palladium chloride(PdCl_(2))on the surface of polymer film while the 2,6-dimethylpyridine structures formed in the specific areas under ultraviolet light guaranteed the resolution of final *** thermal reduction of PdCl_(2) on the surface can be achieved in the process of thermal cyclization of the polymer *** a consequence,the obtained polyimide(PI)film can be patterned with conductive copper micropatterns directly by electroless *** particular,we accomplished the deposition of high precision copper pattern with a minimum line width of 50μm and minimum line spacing of 20μm on PI thin films(thickness~10μm)by electroless *** prepared conductive copper micropatterns exhibit a low resistivity of 1.78μΩ·cm the same as the pure block *** the relationship between the structures of the polymer chains and the physical properties of polymer substrates,such as the dimensional stability,mechanical and dielectric properties were also discussed in *** simple and novel method of patterning metal on the polymer surface does not need to achieve the catalytic metal adhesion required for electroless plating at the cost of destroying the substrate surface and avoiding the introduction of unstable *** patterning method is compatible with the current roll-to-roll production process and can be used to develop high-performance micro-integrated circuits.

关键词： Polyimide Metal patterning Electroless plating Palladium chloride Coordination effect

Graphene-based materials for polymer solar cells

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Chinese Chemical Letters 2016年第8期27卷 1259-1270,1468页

作者： Xiao-Feng Lin Zi-Yan Zhang Zhong-Ke yuan Jing Li Xiao-Fen Xiao Wei Hong Xu-Dong Chen ding-shan yu Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education of China School of Chemistry and Chemical EngineeringSun Yat-sen University Key Laboratory of High Performance Polymer-based Composites of Guangdong Province School of Chemistry and Chemical Engineering Sun Yat-sen University

Due to the remarkable electronic,optical,thermal,and mechanical properties,graphene-based materials have shown great potential in a wide range of technique ***,the high transparency,conductivity,flexibility,and abundance make graphene materials highly attractive for polymer solar cells（PSCs）.Graphene-based materials have been regarded as one promising candidate used in various parts in PSCs not only as electrodes,but also as interfacial layers and active layers with an aim to boost the power conversion efficiency of the *** this review,we summarize the recent progress about the design and synthesis of graphene-based materials for efficient PSCs along with the related challenges and future perspectives.

关键词： Graphene Polymer solar cells Electrodes Interfacial layers Active layers

Side-Chain-Type Polyimide-Cu Complexes with Suppressed Activation Energy of Relaxation for Advanced High-Temperature Capacitor

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Chinese Journal of Polymer Science 2024年第8期42卷 1038-1048页

作者： Bai-Yang Zhou Ze-Tong Ma Shi-Long Zhong Zhen-Jie Huang Qi Guo Deng-Chong Feng Zhong-Ke yuan Shao-Lin Lu yu-Zhao Yang Cheng Wang ding-shan yu Xu-Dong Chen Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education Guangdong Engineering Technology Research Centre for High Performance Organic and Polymer Photoelectric Functional FilmsSchool of ChemistrySun Yat-sen UniversityGuangzhou 510275China School of Chemical Engineering and Light Industry Guangdong University of TechnologyGuangzhou 510006China Guangdong Provincial Laboratory of Chemistry and Fine Chemical Industry Jieyang Centre Jieyang 515200China Chemistry and Chemical Engineering Guangdong Laboratory Shantou 515031China

The burgeoning growth of the new energy vehicles and aviation industry has escalated the need for energy storage capacitors capable of stable operation in harsh *** advent of metal-polyimide complexes has illuminated a novel approach for preparing tem perature-resistant ***,the general application of these metal-polyimide com plexes is impeded by the high dielectric loss and low breakdown strength,consequences of main-chain coordination and excessive metal ions ***,our study proposes a novel polyimideCu complex material(POP-Cu)predicated on side-chain-type pyridine-Cu coordination,utilizing the structural backbone PMDA-ODA of mature commercial PI(Kapton)with reliable *** to the high degree of freedom afforded by the side chain with suppressed relaxation activation energy and the long-range electron delocalization formed by d-πcoordination,the dielectric constant of this material containing merely 2.7 mol%Cu increases from 3.25(POPI)to 5.58,while maintaining a remarkably low dielectric loss of ***,this material exhibits a substantial DC breakdown strength of 436.2 MV·m^(-1)and a high energy density of 5.42 J·cm^(-3),coupled with superior mechanical and thermal *** at 150℃,it retains over 90%of its room-temperature energy density,demon strating notable dielectric stability under high *** attributes underscore its promising application for capacitors operating in harsh environments.

关键词： Dielectric performance Polyimide complexes Side-Chain-Type High-temperature capacitor

A Major QTL, Ghd8, Plays Pleiotropic Roles in Regulating Grain Productivity, Plant Height, and Heading Date in Rice

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Molecular Plant 2011年第2期4卷 319-330页

作者： Wen-Hao Yan Peng Wang Hua-Xia Chen Hong-Ju Zhou Qiu-Ping Li Chong-Rong Wang Ze-Hong ding yu-shan Zhang Si-Bin yu Yong-Zhong Xing Qi-Fa Zhang National Key Laboratory of Crop Genetic Improvement and National Center of Plant Gene Research (Wuhan) Huazhong Agricultural University Wuhan430070 China

Rice yield and heading date are two distinct traits controlled by quantitative trait loci （QTLs）. The dissection of molecular mechanisms underlying rice yield traits is important for developing high-yielding rice varieties. Here, we report the cloning and characterization of Ghd8, a major QTL with pleiotropic effects on grain yield, heading date, and plant height. Two sets of near isogenic line populations were developed for the cloning of GhdS. Ghd8 was narrowed down to a 20-kb region containing two putative genes, of which one encodes the OsHAP3 subunit of a CCAAT-box binding protein （HAP complex）; this gene was regarded as the Ghd8 candidate. A complementary test confirmed the identity and pleiotropic effects of the gene; interestingly, the genetic effect of Ghd8 was dependent on its genetic background. By regulating Ehdl, RFT1, and Hd3a, Ghd8 delayed flowering under long-day conditions, but promoted flowering under short-day conditions. Ghd8 up-regulated MOC1, a key gene controlling tillering and branching; this increased the number of tillers, primary and secondary branches, thus producing 50% more grains per plant. The ectopic expression of Ghd8 in Arabidopsis caused early flowering by 10 d-a situation similar to the one observed by its homolog AtHAP3b, when compared to wild-type under long-day conditions; these findings indicate the conserved function of Ghd8 and AtHAP3b in flowering in Arabidopsis. Our results demonstrated the important roles of Ghd8 in rice yield formation and flowering, as well as its opposite functions in flowering between rice and Arabidopsis under long-day conditions.

关键词： Near isogenic lines CCAAT-box binding protein ectopic expression flowering pathway yield formation

进化伦理学与自然主义谬误——理查兹对进化伦理学的辩护是否成功

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科学技术哲学研究 2024年第6期41卷 1-7页

作者：丁雨姗武汉大学哲学学院武汉430072

一般认为,进化伦理学尝试从进化生物学事实中推出规范性结论,犯了自然主义谬误。然而,作为进化伦理学的主要代表,理查兹认为自然主义谬误不是谬误。对此,乔伊斯进行了反驳。但他的反驳不能真正驳倒理查兹。一方面,身份或职位(是)与相应... 详细信息

一般认为,进化伦理学尝试从进化生物学事实中推出规范性结论,犯了自然主义谬误。然而,作为进化伦理学的主要代表,理查兹认为自然主义谬误不是谬误。对此,乔伊斯进行了反驳。但他的反驳不能真正驳倒理查兹。一方面,身份或职位(是)与相应的义务和规范(应当)同时被设立,“是”与“应当”没有鸿沟;另一方面,理查兹将“应当”定义成连接属性和期待,而属性本质也是一种“是”,因而,从“是”可以推出“应当”。通过对推断原则内容和功用的澄清,以及对“应当”不同意义的区分,一些可能的反驳也不成立。理查兹对进化伦理学的辩护为消解自然主义谬误提供了一种可能性。

关键词：进化伦理学自然主义谬误理查兹乔伊斯是与应当

基于声学数据反演定量评价致密砂岩储层微裂隙应力敏感性新方法

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岩土力学 2017年第2期38卷 409-418页

作者：尹帅丁文龙单钰铭周文谢润成中国地质大学能源学院北京100083 中国地质大学海相储层演化与油气富集机理教育部重点实验室北京100083 中国地质大学页岩气资源战略评价国土资源部重点实验室北京100083 成都理工大学油气藏地质及开发工程国家重点实验室四川成都610059

设计试验方法流程对塔中地区深层致密砂岩储层岩样进行不同围压条件下声学测试,提出基于声学数据反演定量研究致密砂岩储层微裂隙应力敏感性的评价方法。通过Biot相洽理论和DEM理论组合模型分别对岩石裂隙密度?和孔隙纵横比?进行反演,... 详细信息

设计试验方法流程对塔中地区深层致密砂岩储层岩样进行不同围压条件下声学测试,提出基于声学数据反演定量研究致密砂岩储层微裂隙应力敏感性的评价方法。通过Biot相洽理论和DEM理论组合模型分别对岩石裂隙密度?和孔隙纵横比?进行反演,探讨了不同围压条件下岩石?、?的变化规律,并对微裂隙应力敏感性进行评价。结果表明:?随围压的增加而降低,?随围压的增加而增加,这主要是由于微裂隙的闭合引起的;根据不同围压条件下?值降低幅度可以确定发生闭合的裂隙或依然保持张开的裂隙所占的百分比;在较高围压条件下依然具有较大?值的样品应力敏感性较弱,反之,应力敏感性较强;定义试验中岩石内部孔裂隙性质发生急剧变化的点为转折点,发现该点对应的?值相差不大,该值可视为该致密砂岩储层的裂隙共性特征,并可作为裂隙相对发育程度的对比指标;分别探讨了?值(围压65 MPa)及所定义转折压力与岩石孔隙度间的相关性,结果表明,两者正相关性均非常好,对于该地区深层低渗致密砂岩储层而言,存在低应力敏感性的有利类型裂隙受岩石物理性质影响程度最大。

关键词：塔中地区声学反演致密砂岩储层微裂隙应力敏感性

Acute and chronic excitotoxicity in ischemic stroke and late-onset Alzheimer's disease

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Neural Regeneration Research 2025年第7期20卷 1981-1988页

作者： shan Ping yu Emily Choi Michael QJiang Ling Wei Department of Anesthesiology Emory University School of MedicineAtlantaGAUSA Center for Visual and Neurocognitive Rehabilitation Atlanta Veterans Affairs Medical CenterDecaturGAUSA

Stroke and Alzheimer's disease are common neurological disorders and often occur in the same *** comorbidity of the two neurological disorders represents a grave health threat to older *** review presents a brief background of the development of novel concepts and their clinical *** activity of glutamatergic N-methyl-D-aspartate receptors and N-methyl-D-aspartate receptor-mediated Ca^(2+)influx is critical for neuronal *** ischemic insult induces prompt and excessive glutamate release and drastic increases of intracellular Ca^(2+)mainly via N-methyl-D-aspartate receptors,particularly of those at the extrasynaptic *** Ca^(2+)-evoked neuronal cell death in the ischemic core is dominated by necrosis within a few hours and days known as acute ***,mild but sustained Ca^(2+)increases under neurodegenerative conditions such as in the distant penumbra of the ischemic brain and early stages of Alzheimer's disease are not immediately toxic,but gradually set off deteriorating Ca^(2+)-dependent signals and neuronal cell loss mostly because of activation of programmed cell death *** on the Ca^(2+)hypothesis of Alzheimer's disease and recent advances,this Ca^(2+)-activated“silent”degenerative excitotoxicity evolves from years to decades and is recognized as a unique slow and chronic *** N-methyl-D-aspartate receptor subunit GluN3A,primarily at the extrasynaptic site,serves as a gatekeeper for the N-methyl-D-aspartate receptor activity and is neuroprotective against both acute and chronic *** stroke and Alzheimer's disease,therefore,share an N-methyl-D-aspartate receptor-and Ca^(2+)-mediated mechanism,although with much different time *** is thus proposed that early interventions to control Ca^(2+)homeostasis at the preclinical stage are pivotal for individuals who are susceptible to sporadic late-onset Alzheimer's disease and Alzheimer's disease-related

关键词： Ca^(2+)hypothesis cognitive deficits hyperactivity late-onset Alzheimer's disease neurodegeneration N-methyl-D-aspartate receptors N-methyl-D-aspartate receptor subunits pathogenesis preventive treatment

Surface micro-arrays enhancing electromagnetic interference shielding of polydimethylsiloxane/multiwalled carbon nanotubes nanocomposites

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Nano Research 2025年第1期18卷 508-519页

作者： Ke Jiang Zhi Chen Ji yu Chen Zheng shan Huang Ming Wang Chongqing Key Laboratory of Soft-Matter Material Manufacturing School of Chemistry and Chemical EngineeringSouthwest UniversityChongqing 400715China School of Mechanics Civil Engineering and ArchitecturesNorthwestern Polytechnical UniversityXi’an 710072China Jieyang Branch of Chemistry and Chemical Engineering Guangdong Laboratory(Rongjiang Laboratory) Jieyang 515200China

Herein,the electromagnetic shielding performance of surface concave-convex(SC)and zig-zag micro-arrays was studied by using a simulation prediction and a three-dimensional(3D)printing custom ***,surface stripe concaveconvex(SSC)and surface cylindrical concave-convex(SCC)micro-arrays with or without zig-zag micro-arrays are designed,and their shielding performance is simulated in multi-bands(C-,X-band).The multiwalled carbon nanotubes/polydimethylsiloxane composites(MWCNT/PDMS)with different SC structures and different electrical conductivity are molded in acrylonitrile-butadiene-styrene copolymer(ABS)molds which are printed by a 3D *** results show that the electromagnetic interference shielding effectiveness(EMI SE)of the samples can be enhanced by constructing the SC micro-arrays with zig-zag micro-arrays,and improving with the increase of conductivity and *** addition,the shielding mechanism of the SC-MWCNT/PDMS composites is investigated and discussed by an electromagnetic simulation.

关键词： surface micro-arrays electrical properties electromagnetic interference(EMI)shielding three-dimensional(3D)printing

Successful emergency surgical intervention in acute non-STsegment elevation myocardial infarction with rupture:A case report

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World Journal of Clinical Cases 2025年第4期13卷 41-47页

作者： Xing-Po Li Zi-shan Wang Hong-Xia yu shan-shan Wang Department of Cardiovascular Medicine Huantai County Hospital of Traditional Chinese MedicineZibo 256400Shandong ProvinceChina Department of Cardiovascular Medicine Zibo Hospital of Integrated Traditional Chinese and Western MedicineZibo 255500Shandong ProvinceChina

BACKGROUND The incidence of acute myocardial infarction(AMI)is rising,with cardiac rupture accounting for approximately 2%of deaths in patients with acute ST-segment elevation myocardial infarction(STEMI).Ventricular free wall rupture(FWR)occurs in approximately 2%of AMI patients and is notably rare in patients with *** of cardiac rupture include left ventricular FWR,ventricular septal rupture,and papillary muscle *** FWR usually leads to acute cardiac tamponade or electromechanical dissociation,where standard resuscitation efforts may not be *** septal rupture and papillary muscle rupture often result in refractory heart failure,with mortality rates over 50%,even with surgical or percutaneous repair *** SUMMARY We present a rare case of an acute non-STEMI patient who suffered sudden FWR causing cardiac tamponade and loss of consciousness immediate before undergoing coronary *** resuscitation and emergency open-heart repair along with coronary artery bypass grafting resulted in successful patient *** This case emphasizes the risks of AMI complications,shares a successful treatment scenario,and discusses measures to prevent such complications.

关键词： Acute non-ST segment elevation myocardial infarction Cardiac rupture Acute myocardial infarction Free wall rupture Case report