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Interface terminal group regulated organic phototransistors with tunable persistent and switchable photoconductivity

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Science China Chemistry 2022年第12期65卷 2567-2575页

作者： di xue Yingying Zhang Weijie Gong Yao Yin Zi Wang Lizhen Huang Lifeng Chi Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou215123China Gusu Laboratory of Materials Suzhou215123China Macao Institute of Materials Science and Engineering(MIMSE) MUST-SUDA Joint Research Center for Advanced Functional MaterialsMacao University of Science and TechnologyTaipaMacao999078China

With both light detection and intrinsic amplification functions,organic phototransistors have demonstrated promising applications,including photodetection and photomemory.To achieve excellent photoresponse and superior photogain,a common and effective strategy is to modulate the trapping effect with the purpose of reducing recombination or prolonging the lifetime of the photogenerated charge carriers.However,introducing trapping sites delicately is challenging and might sacrifice the response rate together with a typical persistent photoconductivity.Here,we demonstrate a facile strategy for achieving high photo-responsive organic phototransistors with both persistent and switchable photoconductivity features via interface terminal group regulation.By varying the terminate groups of self-assembled monolayer(SAMs)from the strong electron withdrawing group-F,neutral−CH_(3) to electron donating−NH_(2) on the dielectric surface,we realize both minority carrier trapping and majority carrier trapping in the organic phototransistor based on the C8-BTBT active layer.The electron withdrawing effect of F significantly enhances the minority carrier trapping process and yields a high photoresponsivity with a long-lasting persistent photoconductivity.In contrast,the electron donating group−NH_(2) with a distinct majority carrier trapping ability causes switchable photoconductivity so that the photocurrent can rise pronouncedly and fully decay along with light on/off.Attractively,both cases can deliver high performance with photoresponsivities higher than 104 A W^(−1) together with a photosensitivity in the level of 107 and a detectivity of approximately 10^(15)–10^(16) Jones.Such a tunable,excellent photoresponse property enables the convenient exploration of organic phototransistors to satisfy different application requirements.

关键词： organic phototransistor surface modification trapping persistent photoconductivity

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Green Construction of Belt and Road Initiative

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China News Release 2022年第12期 9-13页

作者： di xue 不详

In 2013,Chinese President Xi Jinping put forward the Belt and Road Initiative(BRI).In the past nine years,the construction of the BRI has gradually deepened and solidified,and has become a common road of opportunity and prosperity for all countries.The joint construction of the BRI has become a popular international public product and a platform for international cooperation.

关键词： Road Belt construction

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Growth Behavior of Rubrene Thin Films on Hexagonal Boron Nitride in the Early Stage

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Chinese Journal of Chemistry 2022年第11期40卷 1298-1304,I0002页

作者： Yujia Wei di xue Lianlian Ji Jie Lu Qi Wang Xingyu Jiang Yinghui Sun Zi Wang Lizhen Huang Lifeng Chi Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesCollaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhouJiangsu 215123China College of Energy Soochow Institute for Energy and Materials InnovationsKey Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceSoochow UniversitySuzhouJiangsu 215006China Gusu Laboratory of Materials SuzhouJiangsu 215123China

Two-dimensional materials,with an in-plane ordered and dangling-bonding-free surface,are ideal substrates for fabricating high-quality crystalline thin films.Here,we show a systematic study on the growth of a benchmark organic semiconductor,rubrene,on hexagonal boron nitride(h-BN)substrate via physical vapor deposition from the initial amorphous phase to the final crystalline phase;the role of temperature in such transition and the epitaxy relationship between rubrene and h-BN are revealed.With the increase of substrate temperature,the critical thickness of amorphous-crystalline-transition decreases and the morphology of crystalline phase also evolves from porous to terrace-like.When substrate temperature reaches>100℃,the critical thickness reduces to only 0.5 nm and a precise layer-by-layer growth from the very first layer is achieved,which is quite rare for rubrene growing on other substrates.The high ordering can be attributed to the fine epitaxy relationship between rubrene films and the h-BN surface lattice,and this film demonstrates good charge transport ability with a p-type field-effect mobility of>1 cm^(2)·V^(-1)·s^(-1).

关键词： Thin films Crystal growth Organic thin film transistors 2D materials Molecular electronics

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Construction of a High-Quality Organic-Inorganic Hybrid Heterostructure and Its Photo-response Performance

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Chinese Journal of Chemistry 2023年第1期41卷 50-56页

作者： Yadan Zhang Guanghua Yu di xue Jie Lu Xing Meng Yao Yin Qi Wang Zi Wang Lizhen Huang Lifeng Chi Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow University199 Ren'ai RoadSuzhouJiangsu 215123China Gusu Laboratory of Materials 388 Ruoshui RoadSuzhouJiangsu 215123China Macao Institute of Materials Science and Engineering(MIMSE) MUST-SUDA Joint Research Center for Advanced Functional MaterialsMacao University of Science and TechnologyTaipa 999078MacaoChina

The combination of metal oxide and organic semiconductor for constructing organic-inorganic hybrid heterostructure is promising to offer unique optoelectronic properties.However,the distinct difference in electron structure and processing technology of the two types of materials makes it usually difficult to fully deliver their complementary advantages.Herein,we report the construction of a high quality organic/In_(2)O_(3) hybrid heterostructure presenting a good ambipolar transport with average electron mobility>1 cm^(2)V^(-1)·s^(-1) and hole mobility up to 0.4 cm^(2)·V^(-1)·s^(-1),respectively,together with a high-gain inverter.In addition,the incorporation with organic film on top of In_(2)O_(3) remarkably reduces the dark current,enabling the realization of high photoconductivity response with photo-sensitivity of two magnitudes higher than that of pure In2O3.The photoconductor and phototransistor of the hybrid structure demonstrate high photoresponsivity>10^(3) AW^(-1) and detectivity up to 10^(14) Jones,demonstrating the promising functionality of such a high quality hybrid heterostructure.

关键词： Sol-gel process Thin films Semiconductors Phthalocyanines Hybrid heterostructure

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防治煤自燃的高堆积固化泡沫的制备及应用

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煤炭科学技术 2024年第2期52卷 159-170页

作者：胡相明王凯薛迪孙公正山东科技大学安全与环境工程学院山东青岛266590 山东科技大学矿山灾害预防控制省部共建国家重点实验室培育基地山东青岛266590

漏风是引发矿井煤自燃的重要原因,而煤自燃火灾影响了矿井的正常生产。为解决传统无机固化泡沫(TISF)在充填堵漏过程中存在胶凝时间长、堆积能力弱的问题,提出经液态硅酸钠(LSS)改性制备的速凝无机固化泡沫(RISF)。研究了不同掺量的LSS... 详细信息

漏风是引发矿井煤自燃的重要原因,而煤自燃火灾影响了矿井的正常生产。为解决传统无机固化泡沫(TISF)在充填堵漏过程中存在胶凝时间长、堆积能力弱的问题,提出经液态硅酸钠(LSS)改性制备的速凝无机固化泡沫(RISF)。研究了不同掺量的LSS对泡沫浆液胶凝时间、堆积能力等性能的影响规律,采用抗压强度、稳定性测试等表征手段,确定了LSS的最优添加量为5%(质量分数),RISF的28 d抗压强度达2.49 MPa,是TISF的1.7倍,最大密度比R为1.11,稳定性提升20%左右;胶凝时间和堆积能力的测试结果表明,与TISF相比,RISF的凝结时间大幅缩短(从683 s缩短到52 s),堆积能力提升(最大堆积高度提高1.9倍)。基于此,结合扫描电子显微镜(SEM)和X射线衍射(XRD)对RISF的速凝固化机理进行了探究。试验结果表明,RISF具有更多的水化产物且不同的水化产物紧密交织,颗粒水化过程中,LSS水解生成原硅酸根与溶液中的钙离子结合,加快水化反应,缩短了泡沫浆液的胶凝时间。但也发现,当LSS添加量超过5%时,RISF的抗压强度降低,稳定性下降,这主要是因为过量的LSS使溶液中的钙硅比例低于1.0,导致生成了低强度的水化产物。堵漏风试验和灭火试验结果表明,与TISF相比,RISF具有较高的堵漏效率和优良的防灭火性能,堵漏效率最高提升26.3%,并且在扑灭煤火时未出现复燃。RISF在利民煤矿矸石山的现场应用表明,其具有良好的降温灭火效果,有效解决了矸石山的高温难题,确保了矿井的正常生产。

关键词：煤自燃无机固化泡沫快速凝固机理充填堵漏材料

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Process analysis of PM_(2.5) pollution events in a coastal city of China using CMAQ

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Journal of Environmental Sciences 2019年第5期31卷 225-238页

作者： Qiang Zhang di xue Xiaohuan Liu Xiang Gong Huiwang Gao College of Environmental Science and Engineering Ocean University of China Key Laboratory of Marine Environment and Ecology Ministry of Education Ocean University of China Laboratory for Marine Ecology and Environmental Sciences Qingdao National Laboratory for Marine Science and Technology Qingdao University of Science and Technology

US EPA's Community Multiscale Air Quality modeling system(CMAQ) with Process Analysis tool was used to simulate and quantify the contribution of individual atmospheric processes to PM_(2.5) concentration in Qingdao during three representative PM_(2.5) pollution events in the winter of 2015 and 2016. Compared with the observed surface PM_(2.5) concentrations, CMAQ could reasonably reproduce the temporal and spatial variations of PM_(2.5) during these three events. Process analysis results show that primary emissions accounted for 72.7%–93.2% of the accumulation of surface PM_(2.5) before and after the events.When the events occurred, primary emissions were still the major contributor to the increase of PM_(2.5) in Qingdao, however the contribution percentage reduced significantly,which only account for 51.4%–71.8%. Net contribution from horizontal and vertical transport to the accumulation of PM_(2.5) was also positive and its percentage increased when events occurred. Only 1.1%–4.6% of aerosol accumulation was due to PM processes and aqueous chemical processes before and after events. When the events occurred,contribution from PM processes and aqueous chemistry increased to 6.0%–11.8%. Loss of PM_(2.5) was mainly through horizontal transport, vertical transport and dry deposition, no matter during or outside the events. Wet deposition would become the main removal pathway of PM_(2.5), when precipitation occurred.

关键词： CMAQ Process analysis PM2.5 Qingdao

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Neuroprotective mechanism of Kai Xin San: upregulation of hippocampal insulin-degrading enzyme protein expression and acceleration of amyloid-beta degradation

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Neural Regeneration Research 2017年第4期12卷 654-659页

作者： Na Wang Yong-ming Jia Bo Zhang di xue Maharjan Reeju Yan Li Shu-ming Huang xue-wei Liu Institute of Medicine Qiqihar Medical University Department of Neuroscience Institute of Traditional Chinese MedicineHeilongjiang University of Chinese Medicine

Kai Xin San is a Chinese herbal formula composed of Radix Ginseng, Poria, Radix Polygalae and Acorus Tatarinowii Rhizome. It has been used in China for many years for treating amnesia. Kai Xin San ameliorates amyloid-β （Aβ） induced cognitive dysfunction and is neuroprotective in vivo, but its precise mechanism remains unclear. Expression of insulin-degrading enzyme （IDE）, which degrades Aβ, is strongly correlated with cognitive function. Here, we injected rats with exogenous Aβ42 （200 μM, 5 μL） into the hippocampus and subsequently administered Kai Xin San （0.54 or 1.08 g/kg/d） intragastrically for 21 consecutive days. Hematoxylin eosin and Nissl staining revealed that Kai Xin San protected neurons against Aβ-induced damage. Furthermore, enzyme linked immunosorbent assay, western blot and polymerase chain reaction results showed that Kai Xin San decreased Aβ42 protein levels and increased expression of IDE protein, but not mRNA, in the hippocampus. Our findings reveal that Kai Xin San facilitates hippocampal Aβ degradation and increases IDE expression, which leads, at least in part, to the alleviation of hippocampal neuron injury in rats.

关键词： nerve regeneration neurodegeneration traditional Chinese medicine Kai Xin San insulin-degrading enzyme amyloid-β Alzheimer＇sdisease Chinese herbal compound Aβ-degrading enzymes neurons Radix Ginseng Radix Polygalae Acorus Tatarinowii Rhizoma neuralregeneration

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特征追踪心脏MRI定量评估非梗阻性肥厚型心肌病左房功能的应用研究

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放射学实践 2024年第4期39卷 479-487页

作者：薛迪吴江李璇梁秀琴山西医科大学医学影像学院山西太原030001 山西省心血管病医院磁共振室山西太原030024

目的:应用特征追踪心脏MRI(FT-cMRI)对非梗阻性肥厚型心肌病(NOHCM)患者进行左房应变分析来评估左心房功能,并探究NOHCM对左心结构和功能的影响。方法:回顾性分析2020年1月-2022年12月本院58例非梗阻性肥厚型心肌病患者(NOHCM组)和30例... 详细信息

目的:应用特征追踪心脏MRI(FT-cMRI)对非梗阻性肥厚型心肌病(NOHCM)患者进行左房应变分析来评估左心房功能,并探究NOHCM对左心结构和功能的影响。方法:回顾性分析2020年1月-2022年12月本院58例非梗阻性肥厚型心肌病患者(NOHCM组)和30例健康对照者(HC组)的临床和MRI资料。MRI扫描序列主要为单次激发FSE亮血序列,扫描平面包括两腔、四腔和短轴位。应用CVI42软件测量左房容积指数(LAVI)和左房整体功能参数,后者包括心肌储备功能参数[总应变(εs)、峰值正向应变率(SRs)、左房总射血分数(LATEF)]、导管功能参数[主动应变(εe)、峰值早期负向应变率(SRe)、左房被动射血分数(LAPEF)]和升压泵功能参数[被动应变(εa)、峰值晚期负向应变率(SRa)、左房主动射血分数(LAAEF)],以及左室的功能[左室射血分数(LVEF)、左室心输出量(LVCO)和左室心脏指数(LVCI)]和大小参数[左室最大室壁厚度(LVWT_(max))、左室心肌质量(LVM)、左室质量指数(LVMI)、左室舒张末期容积指数(LVEDVi)和左室收缩末期容积指数(LVESVi)]。采用两样本t检验、Mann-Whitney U检验等统计学方法比较两组间各项定量参数值的差异,并采用Pearson或Spearman相关系数分析左房功能参数与左室的结构和功能参数之间的相关性。结果:NOHCM组的LVWT_(max)、LVM、LVMI和LAVI值均显著高于HC组(P0.05)。左房大小正常的NOHCM患者的LATEF、LAPEF、εs、εe、SRs和SRe值均显著低于HC组(P0.05)。所有受试者的LATEF与εs、LAPEF与εe、LAAEF与εa之间均具有显著相关性(r>0.70)。结论:与健康对照组相比,NOHCM患者各时相左房功能均下降。在左房增大之前,左房的心肌储备和导管功能下降,而升压泵功能正常。各时相左房功能受损与左室的肥厚部位无显著相关性。各时相左房的LAEF与各项应变参数之间具有较强的相关性。

关键词：肥厚型心肌病左房应变左房功能特征追踪技术心脏磁共振成像

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保温型聚氨酯/氢氧化镁复合材料力学性能和燃烧行为的研究

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塑料科技 2024年第5期52卷 104-106页

作者：陈海霞洪学娣唐山工业职业技术学院建筑工程学院河北唐山063000

用钛酸酯偶联剂对氢氧化镁(MH)进行改性,并制备聚氨酯/氢氧化镁(PU/MH)复合材料,研究了复合材料的力学性能和燃烧行为。结果表明:随着MH掺量增加,复合材料的压缩强度逐渐增大,复合材料的抗拉强度和弯曲变形逐渐降低。随着MH掺量增加,复... 详细信息

用钛酸酯偶联剂对氢氧化镁(MH)进行改性,并制备聚氨酯/氢氧化镁(PU/MH)复合材料,研究了复合材料的力学性能和燃烧行为。结果表明:随着MH掺量增加,复合材料的压缩强度逐渐增大,复合材料的抗拉强度和弯曲变形逐渐降低。随着MH掺量增加,复合材料的点燃时间(TTI)和质量残余率(MLR)逐渐增大,总热释放量(THR)、总烟释放量(TSR)、CO生成量和CO_(2)生成量逐渐降低,复合材料的燃烧等级从V-2提高到V-0。MH掺量为30%时,复合材料的力学性能和阻燃性能均较好。4#复合材料的抗压强度比纯PU提高45.0%,抗拉强度和弯曲变形分别降低10.0%和5.3%,燃烧等级从V-2提高到V-0,CO和CO_(2)总生成量分别降低50.0%和22.2%。

关键词：氢氧化镁聚氨酯力学性能燃烧行为

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智能数据可视分析技术综述

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软件学报 2024年第1期35卷 356-404页

作者：骆昱宇秦雪迪谢宇鹏李国良清华大学计算机科学与技术系北京100084 青海大学计算机技术与应用系青海西宁810016

如何从海量数据中快速有效地挖掘出有价值的信息以更好地指导决策,是大数据分析的重要目标.可视分析是一种重要的大数据分析方法,它利用人类视觉感知特性,使用可视化图表直观呈现复杂数据中蕴含的规律,并支持以人为本的交互式数据分析.... 详细信息

如何从海量数据中快速有效地挖掘出有价值的信息以更好地指导决策,是大数据分析的重要目标.可视分析是一种重要的大数据分析方法,它利用人类视觉感知特性,使用可视化图表直观呈现复杂数据中蕴含的规律,并支持以人为本的交互式数据分析.然而,可视分析仍然面临着许多挑战,例如数据准备代价高、交互响应高延迟、可视分析高门槛和交互模式效率低.为应对这些挑战,研究者从数据管理、人工智能等视角出发,提出一系列方法以优化可视分析系统的人机协作模式和提高系统的智能化程度.系统性地梳理、分析和总结这些方法,提出智能数据可视分析的基本概念和关键技术框架.然后,在该框架下,综述和分析国内外面向可视分析的数据准备、智能数据可视化、高效可视分析和智能可视分析接口的研究进展.最后,展望智能数据可视分析的未来发展趋势.

关键词：数据可视化可视分析智能数据可视分析数据管理人工智能

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