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Unique double-layer solid electrolyte interphase formed with fluorinated ether-based electrolytes for high-voltage lithium metal batteries

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Journal of Energy Chemistry 2024年第1期88卷 532-542,I0012页

作者： Ruo Wang Jiawei Li bing Han Qingrong Wang Ruohong Ke Tong Zhang Xiaohu Ao Guangzhao Zhang Zhongbo Liu Yunxian Qian Fangfang Pan Iseult Lynch Jun Wang Yonghong deng Department of Materials Science&Engineering School of Innovation and EntrepreneurshipSouthern University of Science and TechnologyShenzhen 518055GuangdongChina School of Geography Earth and Environmental SciencesUniversity of BirminghamEdgbastonBirmingham B152TTUK Key Laboratory of Marine Environmental Corrosion and Bio-Fouling Institute of OceanologyChinese Academy of SciencesQingdao 266071ShandongChina Shenzhen CAPCHEM Technology Co. Ltd.Shenzhen 518118GuangdongChina CALB Group Co. Ltd.Changzhou 213200JiangsuChina

Li metal batteries using high-voltage layered oxides cathodes are of particular interest due to their high energy ***,they suffer from short lifespan and extreme safety concerns,which are attributed to the degradation of layered oxides and the decomposition of electrolyte at high voltage,as well as the high reactivity of metallic *** key is the development of stable electrolytes against both highvoltage cathodes and Li with the formation of robust interphase films on the ***,we report a highly fluorinated ether,1,1,1-trifluoro-2.[(2.2.2.trifluoroethoxy)methoxy]ethane(TTME),as a cosolvent,which not only functions as a diluent forming a localized high concentration electrolyte(LHCE),but also participates in the construction of the inner solvation *** TTME-based electrolyte is stable itself at high voltage and induces the formation of a unique double-layer solid electrolyte interphase(SEI)film,which is embodied as one layer rich in crystalline structural components for enhanced mechanical strength and another amorphous layer with a higher concentration of organic components for enhanced *** Li||Cu cells display a noticeably high Coulombic efficiency of 99.2.%after 300 cycles and Li symmetric cells maintain stable cycling more than 32.0 h at 0.5 mA/cm^(2. and 1.0m Ah/cm^(2..In addition,lithium metal cells using LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2. and Li CoO_(2. cathodes(both loadings~3.0 m Ah/cm^(2.)realize capacity retentions of>85%over 2.0 cycles with a charge cut-off voltage of 4.4 V and 90%for 170 cycles with a charge cut-off voltage of 4.5 V,*** study offers a bifunctional ether-based electrolyte solvent beneficial for high-voltage Li metal batteries.

关键词： Lithium metal batteries High-voltage layered oxides Fluorinated ether-based electrolytes Solid electrolyte interphase Cathode electrolyte interphase

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高压电脉冲刺激对于热处理花岗岩影响的实验研究

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Journal of Central South University 2024年第5期31卷 1526-1541页

作者：尹土兵刘程辉庄登登李夕兵 School of Resources and Safety Engineering Central South UniversityChangsha 410083China Oulu Mining School University of OuluOulu FI-90014Finland

高压电脉冲技术作为一种环保、可控、高效的破碎坚硬岩石的方法,其潜在应用场景值得进一步深入发掘。本文研究了高压电脉冲诱导干热岩产生预损伤和劣化方法的效果。对热处理后花岗岩薄片试样施加了不同峰值电压的高压电脉冲刺激,探讨了... 详细信息

高压电脉冲技术作为一种环保、可控、高效的破碎坚硬岩石的方法,其潜在应用场景值得进一步深入发掘。本文研究了高压电脉冲诱导干热岩产生预损伤和劣化方法的效果。对热处理后花岗岩薄片试样施加了不同峰值电压的高压电脉冲刺激,探讨了高压电脉冲对于热处理花岗岩的影响。此外,还研究了初始温度对高压电脉冲刺激花岗岩的影响。结果表明:当外加峰值电压超过96 kV时,热处理花岗岩试样发生贯穿性的破裂,峰值电压越高,贯穿裂纹网络越复杂。当电压从96 kV增加到144kV时,花岗岩试样的微裂纹密度从8.63 mm/mm^(2.增加到13.2. mm/mm^(2.。随着热处理温度的升高,花岗岩发生电击穿的难度逐渐降低。在12. kV电脉冲放电刺激3次后,所有热处理温度高于400℃的花岗岩试样均能发生贯穿破裂。高压电脉冲刺激造成花岗岩产生的最大损伤发生在300~400℃的温度区间内。通过扫描电子显微镜观察到,随着试样处理温度的升高,内部孔隙和裂缝的发育情况逐渐加剧,孔隙大小、裂缝宽度和深度也随之增加。这项研究有望为建造干热岩人工储层提供新的见解。

关键词：干热岩高压电脉冲破岩技术温度断裂模式岩石结构

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基于注汞法的液冷花岗岩微观特性实验研究

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Journal of Central South University 2024年第1期31卷 169-181页

作者：尹土兵苏巨振庄登登李夕兵 School of Resources and Safety Engineering Central South UniversityChangsha 410083China Oulu Mining School University of OuluFI-90014 OuluFinland

在开采高温储层的过程中,微观特征变化重要影响深部热储层人工裂隙网络的建立。因此,研究该过程中微观特征的变化对深部地热能的安全高效开采具有重要意义。采用液体冷却(包括酸冷却和水冷却)处理高温花岗岩,模拟向高温储层注酸情况,以... 详细信息

在开采高温储层的过程中,微观特征变化重要影响深部热储层人工裂隙网络的建立。因此,研究该过程中微观特征的变化对深部地热能的安全高效开采具有重要意义。采用液体冷却(包括酸冷却和水冷却)处理高温花岗岩,模拟向高温储层注酸情况,以获取相应条件下的花岗岩试样。随后,使用扫描电子显微镜-能量散射谱(SEM-EDS)和高压注汞法对样品进行测试。SEM-EDS结果显示,水冷却几乎不会影响元素的组成,酸冷却导致氧、硅和金属元素减少。在两种情况下,都观察到了孔隙和裂缝的形成。此外,与水冷却相比,酸冷却的样品表面更加不平整、疏松和粗糙。注汞法测试结果显示,随着处理温度的升高,液冷花岗岩样品的孔隙率、孔隙体积和比表面积有增加,但分形维数呈相反的趋势。研究结果表明,与水冷却相比,酸冷却条件对花岗岩的腐蚀作用使各项参数的变化更加显著,在酸冷却过程中产生更多的孔隙,提供更好的运输空间,使孔隙结构的复杂性降低。在高温储层的地热能有效提取方面,酸冷却具有更大应用潜力。

关键词：孔隙结构微观结构液体冷却土酸溶液注汞法花岗岩分形理论

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A seismic elastic moduli module for the measurements of low-frequency wave dispersion and attenuation of fluid-saturated rocks under different pressures

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Petroleum Science 2024年第1期21卷 162-181页

作者： Yan-Xiao He Shang-Xu Wang Gen-Yang Tang Chao Sun Hong-bing Li San-Yi Yuan Xian Wei Li-deng Gan Xiao-Feng Dai Qiang Ge Peng-Peng Wei Hui-Qing Zhang National Key Laboratory of Petroleum Resources and Engineering CNPC Key Lab of Geophysical ExplorationCollege of GeophysicsChina University of Petroleum(Beijing)Beijing102249China School of Resources and Geosciences China University of Mining and TechnologyXuzhou221116JiangsuChina Research Institute of Petroleum Exploration and Development CNPCBeijing100083China Beijing Vocational College of Labour and Social Security Beijing100029China PetroChina Dagang Oilfield Exploration and Development Research Institute CNPCTianjin300280China

Knowledge about the seismic elastic modulus dispersion,and associated attenuation,in fluid-saturated rocks is essential for better interpretation of seismic observations taken as part of hydrocarbon identification and time-lapse seismic surveillance of both conventional and unconventional reservoir and overburden performances.A Seismic Elastic Moduli Module has been developed,based on the forced-oscillations method,to experimentally investigate the frequency dependence of Young's modulus and Poisson's ratio,as well as the inferred attenuation,of cylindrical samples under different confining pressure *** with three standard samples showed that the measured elastic moduli were consistent with the published data,indicating that the new apparatus can operate reliably over a wide frequency range of f∈[1-2.00,10^(6)]*** Young's modulus and Poisson's ratio of the shale and the tight sandstone samples were measured under axial stress oscillations to assess the frequency-and pressure-dependent *** dry condition,both samples appear to be nearly frequency independent,with weak pressure dependence for the shale and significant pressure dependence for the *** particular,it was found that the tight sandstone with complex pore microstructure exhibited apparent dispersion and attenuation under brine or glycerin saturation conditions,the levels of which were strongly influenced by the increased effective *** addition,the measured Young's moduli results were compared with the theoretical predictions from a scaled poroelastic model with a reasonably good agreement,revealing that the combined fluid flow mechanisms at both mesoscopic and microscopic scales possibly responsible for the measured dispersion.

关键词： Low-frequency measurements Dispersion and attenuation Rock physics Fluid flow

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Novel PIKfyve/Tubulin Dual-target Inhibitor as a Promising Therapeutic Strategy for B-cell Acute Lymphoblastic Leukemia

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Current Medical Science 2024年第2期44卷 298-308页

作者： Zhen LU Qian LAI Zhi-feng LI Meng-ya ZHONG Yue-long JIANG Li-ying FENG Jie ZHA Jing-wei YAO Yin LI Xian-ming deng bing XU Department of Hematology The First Affiliated Hospital of Xiamen University and Institute of HematologySchool of MedicineXiamen UniversityXiamen361005China Key Laboratory of Xiamen for Diagnosis and Treatment of Hematological Malignancy Xiamen361005China Department of Oncology The First Affiliated Hospital of Jinan UniversityJinan UniversityGuangzhou510630China State Key Laboratory of Cellular Stress Biology Innovation Center for Cell Signaling NetworkSchool of Life SciencesXiamen UniversityXiamen361003China

Objective:In B-cell acute lymphoblastic leukemia(B-ALL),current intensive chemotherapies for adult patients fail to achieve durable responses in more than 50%of cases,underscoring the urgent need for new therapeutic regimens for this patient *** present study aimed to determine whether HZX-02.059,a novel dual-target inhibitor targeting both phosphatidylinositol-3-phosphate 5-kinase(PIKfyve)and tubulin,is lethal to B-ALL cells and is a potential therapeutic for B-ALL ***:Cell proliferation,vacuolization,apoptosis,cell cycle,and in-vivo tumor growth were *** addition,Genome-wide RNA-sequencing studies were conducted to elucidate the mechanisms of action underlying the anti-leukemia activity of HZX-02.059 in ***:HZX-02.059 was found to inhibit cell proliferation,induce vacuolization,promote apoptosis,block the cell cycle,and reduce in-vivo tumor *** of the p53 pathway and suppression of the phosphoinositide 3-kinase(PI3K)/AKT pathway and the downstream transcription factors c-Myc and NF-κB were responsible for these ***:Overall,these findings suggest that HZX-02.059 is a promising agent for the treatment of B-ALL patients resistant to conventional therapies.

关键词： B-cell acute lymphoblastic leukemia dual-target inhibitor NF-kB c-Myc PI3K/AKT p53

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Research of caged dynamics of clusters center atoms in Pd_(82.Si_(18) amorphous alloy

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Chinese Physics B 2024年第4期33卷 623-629页

作者：邓永和陈贝祁清华李兵兵高明文大东王小云彭平 School of Computational Science and Electronics Hunan Institute of EngineeringXiangtan 411104China School of Physics and Mechanical&Electrical Engineering Jishou UniversityJishou 416000China School of Materials Science and Engineering Hunan UniversityChangsha 410082China

To date,there is still a lack of a comprehensive explanation for caged dynamics which is regarded as one of the intricate dynamic behaviors in amorphous *** study focuses on Pd_(82.Si_(18)as the research object to further elucidate the underlying mechanism of caged dynamics from multiple perspectives,including the cage's lifetime,atomic local environment,and atomic potential *** results reveal that Si atoms exhibit a pronounced cage effect due to the hindrance of Pd atoms,resulting in an anomalous peak in the non-Gaussian *** in-depth investigation was conducted on the caged dynamics differences between fast and slow Si *** comparison to fast Si atoms,slow Si atoms were surrounded by more Pd atoms and occupied lower potential energy states,resulting in smaller diffusion displacements for the slow Si ***,slow Si atoms tend to be in the centers of smaller clusters with coordination numbers of 9 and *** the isothermal relaxation process,clusters with coordination numbers 9 and 10 have longer lifetimes,suggesting that the escape of slow Si atoms from their cages is more *** findings mentioned above hold significant implications for understanding the caged dynamics.

关键词： caged dynamics Pd_(82.Si_(18) amorphous alloy fast and slow atoms clusters lifetime

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Seven-years post allogeneic hematopoietic stem cell transplantation pure red cell aplastic anemia cured with daratumumab:A case report and review of literature

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World Journal of Clinical Cases 2024年第24期12卷 5604-5612页

作者： Bo deng Rui Gao bing Yang Wen-bing Lei Ming-Fang Xue Ji-Shi Wang Peng Zhao Department of Haematology Guizhou HospitalThe First Affiliated Hospital of Sun Yat-sen UniversityGuiyang 550001Guizhou ProvinceChina Department of Hematology The Affiliated Hospital of Guizhou Medical UniversityGuiyang 550001Guizhou ProvinceChina School of Clinical Medicine Guizhou Medical UniversityGuiyang 550001Guizhou ProvinceChina Department of Hematology The Affiliated Hospital of Guizhou Medical UniversityHematological Institute of Guizhou ProvinceGuiyang 550001Guizhou ProvinceChina

BACKGROUND Allogeneic hematopoietic stem cell transplantation(Allo-HSCT)is currently the only viable method of curing patients with acute myeloid *** 30%to 50%of patients,donors and recipients have some level of ABO blood group *** blood group incompatibility can cause antibodies against the donor's red blood cells to persist in the recipient's body,resulting in a delay of several months in the recovery of red blood cells.A number of different treatments have been reported for post-transplant pure red cell aplastic anaemia(PRCA),such as plasmapheresis,donor lymphocyte infusions,anti-thymocyte globulin,rituximab and *** SUMMARY A 41-year-old female diagnosed with acute myeloid leukaemia underwent peripheral blood allogeneic haematopoietic stem cell transplantation in November 2.13 from an HLA matched unrelated *** donor was AB-positive and the recipient was *** patient was diagnosed with PRCA three months after receiving the donor stem cell *** failing multiple lines of therapy,the patient applied for *** receiving three doses of daratumumab,the patient developed a reticulocyte response and no longer required CONCLUSION The use of daratumumab anti-CD38 for the remove of plasma cells is safe and effective and may be tried for refractory patients with PRCA after undergoing allo-HSCT for ABO incompatibility.

关键词： Transplantation PRCA Daratumumab Leukemia blood-group Case report

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Global epidemiology of mental disorder in atrial fibrillation between 1998-2.2.:A systematic review and meta-analysis

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World Journal of Psychiatry 2024年第1期14卷 179-193页

作者： Shuai Zhang Na Zhang Liu Liu Wang Zheng Zi-Lin Ma Si-Yu Qiao Ying-Li Zhao Yi-Hong Wei Gang Wu Qiu-Ting Yu bing deng Lin Shen Department of Cardiology LongHua Hospital Shanghai University of Traditional Chinese MedicineShanghai 200032China Department of Dermatology Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghai 200437China

BACKGROUND As the burden of mental disorders among patients with atrial fibrillation(AF)increases,researchers are beginning to pay close attention to the risk and prevalence of these *** studies have independently analyzed the risk of comorbidity with depression and anxiety in patients with AF,no study has systematically focused on the global epidemiology of these two mental *** To explore the prevalence of depression and anxiety in patients with *** Five databases were searched from their date of establishment until January *** studies reporting the comorbidity of AF with depression and anxiety,were included in this *** information,such as the first author/publication year,study year,study type,and prevalence of depression and anxiety,were *** SE 15.1 was used to analyze the ***,meta-regression,and sensitivity analyses were performed to estimate study *** After a thorough search,2. studies were identified and included in this *** prevalence rates of depression and anxiety in adults with AF were 2..3%and 14.5%,*** adult males with AF,the prevalence was 11.7%and 8.7%,respectively,whereas in females it was 19.8%and 10.1%,*** older adults with AF,the prevalence rates of depression and anxiety were 40.3%and 33.6%,*** highest regional prevalence of depression and anxiety was observed in European(30.2.)and North American(19.8%)patients with *** In this study,we found that the prevalence of depression and anxiety among patients with AF varies with sex,region,and evaluation scales,suggesting the need for psychological interventions for patients with AF in clinical practice.

关键词： Atrial fibrillation Depression Anxiety Prevalence

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快速城镇化地区生态系统服务时空演变及权衡协同分析:以黄河下游地区为例

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环境科学 2024年第9期45卷 5372-5384页

作者：李欣陈登帅张冰冰曹建荣聊城大学地理与环境学院聊城252000

作为实现我国“黄河重大国家战略”的前沿地区,黄河下游地区在加快推进城镇化进程的同时,对区域自然生态系统及生态功能造成了不可逆转的“建设性破坏”,成为流域生态保护与高质量发展的矛盾尖锐区.对此,研究基于ArcGIS和MATLAB软件,运... 详细信息

作为实现我国“黄河重大国家战略”的前沿地区,黄河下游地区在加快推进城镇化进程的同时,对区域自然生态系统及生态功能造成了不可逆转的“建设性破坏”,成为流域生态保护与高质量发展的矛盾尖锐区.对此,研究基于ArcGIS和MATLAB软件,运用InVEST和RUSLE模型对1990~2.2.年黄河下游地区的产水量、生境质量和土壤保持服务进行定量化评估,并分析其时空变化特征及各项生态系统服务之间的权衡协同关系.结果表明:①1990~2.2.年的土地城镇化进程显著加快,建设用地扩张增幅高达39.89%,其他主要地类的面积则呈现不同程度的下降.②1990~2.2.年,黄河下游地区县域尺度与格网尺度的分布规律较为一致;产水量和土壤保持经历了先减后增的变动趋势,产水量的空间分布格局逐渐转变为东多西少;而土壤保持和生境质量的空间分布格局在整个时期内基本保持不变,高值分布在地势较高的丘陵或山区,低值主要分布在地形和缓的平原地区.③生态系统服务间的权衡协同关系呈现空间异质性,相互作用关系以协同关系为主,存在少部分区县为权衡关系,如产水与生境质量之间的微山县和槐荫区为显著的强权衡关系.研究量化黄河下游地区生态系统服务时空演变特征,明晰生态系统服务之间的权衡协同关系,可为快速城镇化进程下的生态保护和流域治理提供科学依据.

关键词：生态系统服务时空特征权衡与协同快速城镇化黄河下游地区

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毫米波通信的低复杂度时变信道估计算法

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控制工程 2024年第4期31卷 738-744页

作者：邓芳刘兵无锡科技职业学院物联网技术学院江苏无锡214028

当毫米波通信系统工作于时变信道场景中时,为解决通信用户快速位移导致的方位角计算误差和信道估计算法精度下降等问题,通常要消耗大量计算资源。因此,基于用户在快时变信道场景下的信号传输特征,首先在确定毫米波传输信号方位时采用对... 详细信息

当毫米波通信系统工作于时变信道场景中时,为解决通信用户快速位移导致的方位角计算误差和信道估计算法精度下降等问题,通常要消耗大量计算资源。因此,基于用户在快时变信道场景下的信号传输特征,首先在确定毫米波传输信号方位时采用对角加载方法,根据高斯白噪声先验信息得到对角加载方法的参数;然后采用对角带矩阵分解方法对所得到的信道干扰矩阵模型进行处理,从而降低信道估计与均衡算法的复杂度。仿真结果表明,所提算法能够使工作在时变信道条件下的通信系统以低于常规算法的运算复杂度处理系统中的干扰,且不降低传输性能。

关键词：发射角(angle of departure,AoD) 移动通信计算复杂度

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