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Smartphone-assisted electrochemiluminescence imaging test strips towards dual-signal visualized and sensitive monitoring of aflatoxin B1 in corn samples

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Chinese Chemical Letters 2025年第1期36卷 464-468页

作者： Miao-Miao Chen Min-ling Zhang Xiao Song Jun jiang Xiaoqian Tang Qi Zhang Xiuhua Zhang Peiwu li Key Laboratory of Biology and Genetic Improvement of Oil Crops Ministry of Agriculture and Rural AffairsLaboratory of Risk Assessment for Oilseed Products(Wuhan)Quality Inspection and Test Center for Oilseed ProductsOil Crops Research InstituteChinese Academy of Agricultural SciencesWuhan 430062China Food Safety Research Institute Hubei UniversityWuhan 430062China Hubei Hongshan Laboratory Wuhan 430070China Xianghu Laboratory Hangzhou 311231China College of Chemistry and Chemical Engineering Hubei UniversityWuhan 430062China

Aflatoxins B1(AFB1)contamination in agro-food holds great threaten to human and animal *** test strips for rapid AFB1 visualized monitoring remains challenged by improvement of sensitivity and matrix interference *** this case,we developed a portable electrochemiluminescence(ECL)imaging test strip with dual-signal outputs for AFB1 quantification in corn ***@SiO_(2)@Au nanospheres were synthesized for bonding with anti-AFB1 antibody and then colorimetrical signal-reported on test line through the capillary flow at ***,ECL imaging signal of the constructed carbon-ink-based working electrode on polyvinyl chloride substrate of strips was exported under an applied potential of 1.25 *** whole ECL test strips not only endowed convenient colorimetric responses but guaranteed quick-witted ECL image distinguishment even at extremely low AFB1 *** detection limit of this ECL imaging-integrated mode was 10-fold lower than that of only colorimetric ***,satisfactory selectivity,reliability and practicability of the as-proposed ECL test strips were *** work offered a promising platform for on-site,accurate and sensitive detection of pollutants in foods.

关键词： Electrochemiluminescence imaging Test strips Nanomaterials Dual-signal outputs Aflatoxin B1 Food safety

Petrogenesis of late Cretaceous high Ba-Sr granodiorites,SE Lhasa block,China:implications for the reworking of juvenile crust and continental growth

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Acta Geochimica 2025年第1期44卷 86-111页

作者： li-Hang lin Ren-Zhi Zhu Shao-Cong Lai jiang-Feng Qin Yu Zhu Shao-Wei Zhao Min liu State Key Laboratory of Continental Dynamics Department of GeologyNorthwest UniversityXi’an 710069China Ministry of Education Key Laboratory of Western China’s Mineral Resources and Geological Engineering School of Earth Science and ResourcesChang’an UniversityXi’an 710054China

The high Ba-Sr rocks can provide significant clues about the evolution of the continent lithosphere,but their petrogenesis remains *** the Late Cretaceous high Ba–Sr granodiorites in the SE Lhasa Block could potentially provide valuable insights into the continent evolution of the Qinghai-Tibet *** U–Pb ages suggest that the granodiorites were emplaced at 87.32±0.43 ***,the high Ba–Sr granodiorites are characterized by elevated K_(2)O+Na_(2)O contents(8.18-8.73 wt%)and K_(2)O/Na_(2)O ratios(0.99-1.25,mostly>1),and belong to high-K calc-alkaline to shoshonitic *** Yonglaga granodiorites show notably high Sr(653-783 ppm)and Ba(1346-1531 ppm)contents,plus high Sr/Y(30.92-38.18)and(La/Yb)_(N)(27.7-34.7)ratios,but low Y(20.0-22.8 ppm)and Yb(1.92-2.19 ppm)contents with absence of negative Eu anomalies(δEu=0.83-0.88),all similar to typical high Ba–Sr *** variable zirconεHf(t)values of-4.58 to+12.97,elevated initial^(87)Sr/^(86)Sr isotopic ratios of 0.707254 to 0.707322 and lowεNd(t)values of-2.8 to-3.6 with decoupling from the Hf system suggest that a metasomatized mantle source included significant recycled ancient *** occurrence of such high Ba–Sr intrusions indicates previous contributions of metasomatized mantle-derived juvenile material to the continents,which imply the growth of continental crust during the Late Cretaceous in the SE *** with regional data,we infer that the underplated mafic magma provides a significant amount of heat,which leads to partial melting of the juvenile *** melting of the metasomatized mantle could produce a juvenile mafic lower crust,from which the high Ba–Sr granitoids were derived from reworking of previous mafic crust during the Late Cretaceous(ca.100-80 Ma)in the SE Lhasa.

关键词： Late Cretaceous High Ba-Sr granodiorites SE Lhasa Growth of continental crust Juvenile crust

ZmADT2 regulates maize kernel development via the auxin signaling pathway

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Crop Journal 2025年第1期13卷 181-191页

作者： Ren, Ruchang jiang, Xin Zheng, Guangming Zhao, Yajie li, Jun Zhang, Xiansheng Zhao, Xiangyu State Key Laboratory of Wheat Improvement College of Life Sciences Shandong Agricultural University Shandong Tai'an 271018 China Sanya Institute of China Agricultural University Hainan Sanya 572025 China

Arogenate dehydratase (ADT) catalyzes the final step in phenylalanine synthesis and is crucial for plant development and metabolism. Previously, we demonstrated that the ADT/prephenate dehydratase ZmADT2 is essential for maize resistance to Ustilago maydis and for overall plant development. In this study, we explored the role of ZmADT2 in maize kernel development. The mmsu mutant, a dysfunctional ZmADT2 variant, exhibits delayed embryo and endosperm development, along with deficiencies in carbohydrate and protein storage. Transcriptome analysis revealed differential expression of many kernel compartment-specific genes between mmsu and wild-type (WT) kernels, with impaired nutrient accumulation and auxin signaling pathway in the mmsu endosperm. Compared to WT, ZmADT2 mutation led to reduced auxin levels and smaller endosperm cell size. Exogenous auxin rescued the small kernel phenotype of mmsu. Additionally, auxin distribution was reduced in the basal endosperm transfer layer (BETL), causing defects in its development and function, including reduced transfer cell elongation, cell wall ingrowth and nutrient uptake. These findings suggest that ZmADT2 mediated mediates an auxin signaling pathway that is essential for maize kernel development. © 2024 Crop Science Society of China and Institute of Crop Science, CAAS

关键词： Arogenate dehydratase Auxin Basal endosperm transfer layer Kernel development Maize

The comprehensive assessment of epigenetics changes during skin development

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Fundamental Research 2025年第1期5卷 228-240页

作者： Lei, li jiang, ling Hu, Yibo Chen, Menglu Huang, Jinhua Chen, Jing Zeng, Qinghai department of dermatology Third Xiangya Hospital Central South University Changsha 410013 China

Epigenetic regulation is critical to multiple physiological and pathological processes. However, little is known regarding the epigenetic changes during neonatal skin development and skin aging, and in response to ultraviolet (UV) exposure. The transcriptomes of human skin samples from different ages or irradiated with different types and doses of UV light were analyzed using R (version 4.0.3) software. The epigenetic landscape of the skin, including histone modifications, genetic imprinting and m6A modification, which are mainly involved in collagen formation, extracellular matrix organization, immune function and keratinization, underwent significant changes during neonatal to adult development. Epigenetic effectors such as IGF2BP2, GATA2, GATA3, CPA4 and CDK1 were significantly correlated with extracellular matrix organization, and VEGFA, CDK1 and PRKCB with skin immune function. The m6A readers such as IGF2BP2, IGF2BP3, HNRNPA2B1 and EIF3G showed significant correlation with extracellular matrix organization, metabolism, or antigen processing and presentation. Small doses of UV exposure only induced changes in the expression levels of some epigenetic effectors, without any significant effect on the overall epigenetic landscape. However, the minimal erythema dose of UV exposure altered multiple epigenetic effectors regulating extracellular matrix organization, cell-matrix adhesion, innate immune response, mitochondrial function and mRNA processing. In addition, epigenetic changes following UV exposure were more pronounced in the elderly skin compared to the younger skin. In conclusion, histone modifications, genetic imprinting and m6A modification play critical roles during skin development, and a large dose of UV exposure can significantly change the expression of multiple epigenetic effectors. © 2022

关键词： Aging Epigenetics m6A Skin development Ultraviolet

Chlorination of benzyl group on the terminal unit of A_(2)-A_1-D-A_1-A_(2) type nonfullerene acceptor for high-voltage organic solar cells

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Chinese Chemical Letters 2025年第1期36卷 312-317页

作者： Jinge Zhu Ailing Tang Leyi Tang Peiqing Cong Chao li Qing Guo Zongtao Wang Xiaoru Xu jiang Wu Erjun Zhou School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China National Center for Nanoscience and Technology Beijing 100190China Zhongyuan Critical Metals Laboratory Zhengzhou UniversityZhengzhou 450001China Henan Institute of Advanced Technology Zhengzhou UniversityZhengzhou 450003China

Benzotriazole(BTA)-based A_(2)-A_1-D-A_1-A_(2)type wide-bandgap(WBG)non-fullerene acceptors(NFAs)have shown promising potential in indoor photovoltaic,and in-depth investigation of their structure-property relationship is of great ***,we explored the chlorination effect of the side chain on the *** introduced Cl atoms into the benzyl side chains in parent BTA5 to synthesize two NFAs,BTA5-Cl with mono-chlorinated benzyl groups and BTA5-2Cl containing bi-chlorinated benzyl *** chose D18-Cl with deep-energy levels and strong crystallinity to pair with these three acceptors,affording high photovoltage and *** the stepwise chlorination,the open-circuit voltage(V_(OC))values decrease from 1.28,1.22,to 1.20 V,while the corresponding power conversion efficiencies(PCEs)improve from 5.07%,9.15%,to 10.96%.Compared with BTA5-based OSCs,introducing Cl atoms downshifts the energy levels and slightly increases the non-radiative energy loss(0.14decrease in VO ***,more chlorine atom replacements produce more effective exciton dissociation,higher charge transfer,and balanced carrier mobility in the blend films,ultimately achieving better *** work indicates that chlorination of the benzyl group on the terminals can improve the device's performance,implying good application potential in indoor photovoltaics.

关键词： High open-circuit voltage Benzotriazole Non-fullerene acceptor Terminal engineering Chlorination

Melon2K array:A versatile 2K liquid SNP chip for melon genetics and breeding

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Horticultural Plant Journal 2025年第1期11卷 314-322页

作者： Qing Yu Shuai li Xiaofeng Su Xinxiu Chen Yuanhua Dong Zhiwang Yao Naiyu jiang Sen Chai Zhonghua Zhang Kuipeng Xu Engineering Laboratory of Genetic Improvement of Horticultural Crops of Shandong Province College of HorticultureQingdao Agriculture UniversityQingdaoShandong 266109China Key Laboratory of Special Food Proceing(Coconstructionby Ministry and Province) Ministryof Agriculture Rural AairsQingdao Agriculural UniversityQingdaoShandong 266109China Shandong Technology Innovation Center of Special Food QingdaoShandong 266109China Qingdao Special Food Research Institute QingdaoShandong 266109China Genome Analysis Laboratory of the Ministry of Agriculture Agricultural Genomics Institute at ShenzhenChinese Academy of Agricultural SciencesShenzhenGuangdong 518124China Institute of Vegetables and Flowers Chinese Academy of Agricultural SciencesKey Laboratory of Biology and Genetic Improvement of Horticultural Crops of the Ministry of AgricultureSino-Dutch Joint Laboratory of Horticultural GenomicsBeijing 100081China

High-throughput genotyping tools can effectively promote molecular breeding in *** this study,genotyping by target sequencing(GBTS)system was utilized to develop a genome-wide liquid SNP chip for facilitating genetics and breeding in melon(Cucumis melo L.),a globally cultivated economically important horticultural *** on over eight million SNPs derived from 823 representative melon accessions,16K,8K,4K,2K,1K,500,250 and 125 informative SNPs were screened and evaluated for their polymorphisms,conservation of flanking sequences,and *** set of 2K SNPs was found to be optimal for representing the maximum diversity with the lowest number of SNPs,and it was selected to develop the liquid chip,named“Melon2K”.Using Melon2K,more than 1500 SNPs were detected across 17 samples of five melon cultivars,and the phylogenetic relationships were clearly *** the same cultivar,genetic differences were also assessed between different *** evaluated the performance of Melon2K in genetic background selection during the breeding process,obtaining the introgression lines of interested trait with more than 97%genetic background of elite variety by only two rounds of *** results suggest that Melon2K provides a cost-effective,efficient and reliable platform for genetic analysis and molecular breeding in melon.

关键词： Melon Cucumis melo L. Melon2K liquid SNP chip Cultivar identification Background selection

Impact of Spinal Manipulative Therapy on Brain Function and Pain Alleviation in Lumbar Disc Herniation:A Resting-State fMRI Study

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Chinese Journal of Integrative Medicine 2025年第2期31卷 108-117页

作者： ZHOU Xing-chen WU Shuang WANG Kai-zheng CHEN Long-hao WEI Zi-cheng li Tao HUA Zi-han XIA Qiong LYU Zhi-zhen LYU li-jiang department of Spine The Third Affiliated Hospital of Zhejiang Chinese Medicine UniversityHangzhou(310053)China department of Spine The Third School of Clinical MedicineZhejiang Chinese Medicine UniversityHangzhou(310053)China Research Institute of Tuina(Spinal Disease) Zhejiang Chinese Medicine UniversityHangzhou(310053)China

Objective:To elucidate how spinal manipulative therapy(SMT)exerts its analgesic effects through regulating brain function in lumbar disc herniation(LDH)patients by utilizing resting-state functional magnetic resonance imaging(rs-f MRI).Methods:From September 2021 to September 2023,we enrolled LDH patients(LDH group,n=31)and age-and sex-matched healthy controls(HCs,n=28).LDH group underwent rs-f MRI at 2 distinct time points(TPs):prior to the initiation of SMT(TP1)and subsequent to the completion of the SMT sessions(TP2).SMT was administered once every other day for 30 min per session,totally 14 treatment sessions over a span of 4 *** did not receive SMT treatment and underwent only one f MRI ***,participants in LDH group completed clinical questionnaires on pain using the Visual Analog Scale(VAS)and the Japanese Orthopedic Association(JOA)score,whereas HCs did not undergo clinical scale *** effects on the brain were jointly characterized using the amplitude of low-frequency fluctuations(ALFF)and regional homogeneity(Re Ho).Correlation analyses were conducted between specific brain regions and clinical ***:Following SMT treatment,pain symptoms in LDH patients were notably alleviated and accompanied by evident activation of effects in the *** comparison to TP1,TP2 exhibited the most significant increase in ALFF values for Temporal_Sup_R and the most notable decrease in ALFF values for Paracentral_Lobule_L(voxelwise P30;FDR correction).Additionally,the most substantial enhancement in Re Ho values was observed for the Cuneus_R,while the most prominent reduction was noted for the Olfactory_R(voxelwise P30;FDR correction).Moreover,a comparative analysis revealed that,in contrast to HCs,LDH patients at TP1 exhibited the most significant increase in ALFF values for Temporal_Pole_Sup_L and the most notable decrease in ALFF values for Frontal_Mid_L(voxelwise P30;FDR correction).Fur

关键词： functional magnetic resonance imaging lumbar disc herniation spinal manipulative therapy pain

Cascade degradation and electrocatalytic upcycling of waste poly(ethylene terephthalate)to valued products

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Nano Research 2025年第1期18卷 76-93页

作者： Xin li Zirui jiang Zongkui Kou John Wang Shiyou Zheng School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai 200093China School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China department of Materials Science and Engineering National University of SingaporeSingapore 117574Singapore

The global annual production of poly(ethylene terephthalate)(PET)has reached 82 million tons,yet only a small fraction(less than 20%)is *** ultra-slow degradation rate of PET results in the accumulation of PET waste in the environment,causing serious plastic pollution and posing severe challenges to *** response,great efforts have been directed toward developing a cascade degradation and electrocatalytic upcycling strategy,which serves as a“waste-towealth”*** strategy involves electro-reforming PEThydrolyzed intermediates or using PET pyrolyzed products as electrocatalysts to generate high-value *** review provides an overview of the state-of-the-art strategies for the“degradation-electrocatalytic upcycling(de-eUp)”of PET ***,an introduction to the strategy is provided,categorizing it into two main frameworks:“pyrolysis-electrocatalytic upcycling”and“hydrolysis-electrocatalytic upcycling”.The section on“pyrolysis-electrocatalytic upcycling”delves into the degradation methods for designing derived carbon nanomaterials and their utilization as high-performance ***“hydrolysis-electrocatalytic upcycling”section discusses recent advancements in electro-reforming of PET hydrolyzed intermediates for the production of C_(1) and C_(2) *** review concludes by examining the challenges and future prospects in developing an efficient and economical PET upcycling *** is anticipated that this review will stimulate further progress in plastic waste valorization.

关键词： poly(ethylene terephthalate)waste electrocatalytic upcycling pyrolysis hydrolysis ethylene glycol oxidation reaction

Microstructure characterization and hydrogen desorption behaviors of Mg-Al-H powders prepared by reactive milling in hydrogen

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Transactions of Nonferrous Metals Society of China 2013年第10期23卷 3112-3118页

作者：王瑶曾小勤邹建新李德江吴晓梅丁文江上海交通大学材料科学与工程学院上海镁材料及应用工程技术研究中心上海200240 上海交通大学材料科学与工程学院金属基复合材料国家重点实验室上海200240

Microstructure and phase evolutions of Mg-A1 powders ball milled in hydrogen atmosphere were investigated. Both in Mg-3%A1 （mass fraction） and Mg-9%AI systems, fl-MgH2 phase was observed upon a short milling time of 4 h and its maximum content of-80% was reached after 32 h. Neither as-milled powders of the in the two systems contain Mgl7All2. However, heating the milled powders of Mg-9%AI powders to 350 ~C resulted in the precipitation of Mg17A112. DTA/TG analyses of those powders milled for 8-40 h showed that either well-developed peak doublets or shoulders were observed, which plausibly corresponded to the separate hydrogen desorption from different particle fractions offl-MgH2.

关键词： Mg alloy reaction milling hydriding nanocrystalline magnesium hydride peak doublets