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Theoretical studies of two-dimensional structure design and topological electronic properties of organic Dirac materials

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ChemPhysMater

ChemPhysMater 2024年第3期3卷 241-251页

作者： Aizhu Wang Wei tan Hongbo zhao Hongguang Wang Na Ren Longhua Ding Xin Yu Jingyang Peng Institute for Advanced Interdisciplinary Research University of JinanJinan 250022China Institute of Photonic Chips University of Shanghai for Science and TechnologyShanghai 200093China

Owing to the significant development in graphene,an increasing number of studies have been conducted to identify novel two-dimensional(2D)organic materials with Dirac cones and topological *** a series of toy models based on specific lattice patterns has been proposed and demonstrated to possess a Dirac cone,realistic materials corresponding to the lattice models must be identified to achieve excellent properties for practical *** understand factors contributing to the rarity of 2D organic Dirac materials and provide guidance for identifying novel organic Dirac systems,we review recent theoretical studies pertaining to various 2D Dirac models and their corresponding organic Dirac materials,including the Haldane,Kagome,Libe,linecentered honeycomb,and Cairo pentagonal ***,the corresponding structural and topological electronic properties are ***,we investigate the relationship between the existence of Dirac cones and their structural features,as well as the manner by which Dirac points emerge and propagate in these systems.

关键词： Two-dimensional Dirac models Organic Dirac materials Covalent-organic frameworks Metal-organic frameworks Topological electronic properties

One dimensional CeO_(2) nanorods/poly(ethylene oxide) solid composite electrolyte for all-solid-state lithium-ion batteries

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Journal of Rare Earths 2024年第3期42卷 570-577,I0005页

作者： Yudi Guo Erqing zhao Xiaofang zhao Shuailei Liu School of Chemistry and Materials Engineering Xinxiang UniversityXinxiang453003China School of Chemistry and Chemical Engineering Henan Institute of Science and TechnologyXinxiang453003China

The research of poly(ethylene oxide)(PEO)-based solid composite electrolyte with high ionic conductivity and excellent interfacial stability is the key to the development of all-solid-state lithium-ion batteries(ASSLIBs). Herein, uniform nanorod structured CeO_(2) fillers were controllably synthesized by electrospinning, which were subsequently filled into PEO polymer to prepare CeO_(2)/PEO solid composite electrolyte. The addition of CeO_(2) nanorods can reduce both the glass transition temperature and the melting point of PEO polymer, and also interact with PEO and lithium bis(trifluoromethanesulphonyl)imide(LITFSI) by Lewis acid—base reaction. Therefore, the solid composite electrolyte exhibits a high ionic conductivity of 4.52 × 10^(-4)S/cm, a wide electrochemical stability window of about 4.8 V, and a good interfacial stability with Li at 55℃. Moreover, the LiFePO_4/Li ASSLIB divulges the discharging specific capacity of 165, 162, 156 and 146 mA,h/g at 0.2, 0.5, 1 and 2 C, respectively, and achieves the capacity retention of 90.3% after 150 cycles at 0.5 C. Consequently, one dimensional CeO_(2) nanorods can be considered as an alternative filler for polymeric solid electrolyte.

关键词： Poly(ethylene oxide) Solid composite electrolyte CeO_(2)nanorods Ionic conductivity Rare earths

Design of weak current measurement system and research on temperature impact

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Nuclear Science and Techniques 2024年第4期35卷 46-56页

作者： Chu-Xiang zhao San-Gang Li Rong-Rong Su Li Yang Ming-Zhe Liu Qing-Yue Xue Shan Liao Zhi Zhou Qing-Shan tan Xian-Guo Tuo Yi Cheng College of Nuclear Technology and Automation Engineering Chengdu University of Technology1#DongsanluErxianqiaoChengdu 610059China Applied Nuclear Technology in Geosciences Key Laboratory of Sichuan Province Chengdu University of Technology1#DongsanluErxianqiaoChengdu 610059China University of Science and Technology of China Hefei 230026China School of Physics and Electronic Engineering Sichuan University of Science and EngineeringZigong 643000China

A dedicated weak current measurement system was designed to measure the weak currents generated by the neutron ionization *** system incorporates a second-order low-pass filter circuit and the Kalman filtering algorithm to effectively filter out noise and minimize interference in the measurement *** conducted under normal temperature conditions has demonstrated the system's high precision ***,it was observed that temperature variations can affect the measurement *** were collected across temperatures ranging from -20 to 70℃,and a temperature correction model was established through linear regression fitting to address this *** feasibility of the temperature correction model was confirmed at temperatures of -5 and 40℃,where relative errors remained below 0.1% after applying the temperature *** research indicates that the designed measurement system exhibits excellent temperature adaptability and high precision,making it particularly suitable for measuring weak currents.

关键词： Weak current measurement system Neutron ionization chamber Kalman filter algorithm Temperature correction model

The trajectory of rice from wild to domesticated:A new chapter in the study of origins of agriculture

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Science China Earth Sciences 2024年第9期67卷 3011-3012页

作者： Zhijun zhao Institute of Cultural Heritage Shandong UniversityQingdao 266237China

Rice(Oryza sativa)is one of the most important food crops in the world today,feeding more than one-third of the global *** domestication of rice has always been an international research topic(Gross and zhao,2014).When,where,and how rice was cultivated and eventually domesticated has been a hot issue in many research fields such as archaeology,biology,and agronomy(Fuller et al.,2009).

关键词： sativa Oryza crops

Genomes of Meniocus linifolius and Tetracme quadricornis reveal the ancestral karyotype and genomic features of core Brassicaceae

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Plant Communications 2024年第7期5卷 68-89页

作者： Jie Liu Shi-zhao Zhou Yun-Long Liu Bin-Yan zhao Dongmei Yu Mi-Cai Zhong Xiao-Dong Jiang Wei-Hua Cui Jiu-Xia zhao Juan Qiu Liang-Min Liu Zhen-Hua Guo Hong-Tao Li Dun-Yan tan Jin-Yong Hu De-Zhu Li CAS Key Laboratory for Plant Diversity and Biogeography of East Asia&Yunnan Key Laboratory of Crop Wild Relatives Omics Kunming Institute of BotanyChinese Academy of SciencesKunming 650201China Germplasm Bank of Wild Species&Yunnan Key Laboratory for Crop Wild Relatives Omics Kunming Institute of BotanyChinese Academy of SciencesKunming 650201China College of Life Sciences Xinjiang Agricultural UniversityÜrümqi 830052China University of Chinese Academy of Sciences Beijing 100049China These authors contributed equally to this article

Brassicaceae represents an important plant family from both a scientific and economic ***,genomic features related to the early diversification of this family have not been fully characterized,especially upon the uplift of the Tibetan Plateau,which was followed by increasing aridity in the Asian interior,intensifying monsoons in Eastern Asia,and significantly fluctuating daily ***,we reveal the genomic architecture that accompanied early Brassicaceae diversification by analyzing two high-quality chromosome-level genomes for Meniocus linifolius(Arabodae;clade D)and Tetracme quadricornis(Hesperodae;clade E),together with genomes representing all major Brassicaceae clades and the basal *** reconstructed an ancestral core Brassicaceae karyotype(CBK)containing 9 pseudochromosomes with 65 conserved syntenic genomic blocks and identified 9702 conserved genes in *** detected pervasive conflicting phylogenomic signals accompanied by widespread ancient hybridization events,which correlate well with the early divergence of core *** identified a successive Brassicaceae-specific expansion of the class I TREHALOSE-6-PHOSPHATE SYNTHASE 1(TPS1)gene family,which encodes enzymes with essential regulatory roles in flowering time and embryo *** TPS1s were mainly randomly amplified,followed by expression *** results provide fresh insights into historical genomic features coupled with Brassicaceae evolution and offer a potential model for broad-scale studies of adaptive radiation under an ever-changing environment.

关键词： Cruciferae genomic features ancient hybridization core Brassicaceae karyotype CBK TREHALOSE-6-PHOSPHATE SYNTHASE 1 genes TPS1s

Identification of new cotton fiber-quality QTL by multiple genomic analyses and development of markers for genomic breeding

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The Crop Journal 2024年第3期12卷 866-879页

作者： Haozhe tan Binghui tang Mengling Sun Qiulu Yin Yizan Ma Jianying Li Pengcheng Wang Zhonghua Li Guannan zhao Maojun Wang Xianlong Zhang Chunyuan You Lili Tu National Key Laboratory of Crop Genetic Improvement Hubei Hongshan LaboratoryHuazhong Agricultural UniversityWuhan 430070HubeiChina Cotton Research Institute Shihezi Academy of Agriculture ScienceShihezi 832000XinjiangChina

Cotton fiber is one of the main raw materials for the textile *** recent years,many cotton fiber quality QTL have been identified,but few were applied in *** this study,a genome wide association study(GWAS)of fiber-quality traits in 265 upland cotton breeding intermediate lines(GhBreeding),combined with genome-wide selective sweep analysis(GSSA)and genomic selection(GS),revealed 25 *** of these QTL were ignored by only using *** CRISPR/Cas9 mutants of GhMYB_D13 had shorter fiber,which indicates the credibility of QTL to a certain *** these QTL were verified in other cotton natural populations,5 stable QTL were found having broad potential for application in ***,among these 5 stable QTL,superior genotypes of 4 showed an enrichment in most improved new varieties widely cultivated *** findings provide insights for how to identify more QTL through combined multiple genomic analysis to apply in breeding.

关键词： Cotton fiber quality breeding GWAS Genome-wide selective sweep analysis Genomic selection InDel markers

A DIRECT DISCONTINUOUS GALERKIN METHOD FOR TIME FRACTIONAL DIFFUSION EQUATIONS WITH FRACTIONAL DYNAMIC BOUNdaRY CONDITIONS

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Journal of Computational Mathematics 2024年第1期42卷 156-177页

作者： Jingjun zhao Wenjiao zhao Yang Xu School of Mathematics Harbin Institute of TechnologyHarbin 150001China

This paper deals with the numerical approximation for the time fractional diffusion problem with fractional dynamic boundary *** well-posedness for the weak solutions is studied.A direct discontinuous Galerkin approach is used in spatial direction under the uniform meshes,together with a second-order Alikhanov scheme is utilized in temporal direction on the graded mesh,and then the fully discrete scheme is ***,the stability and the error estimate for the full scheme are analyzed in *** experiments are also given to illustrate the effectiveness of the proposed method.

关键词： Time fractional diffusion equation Numerical stability Convergence

A water-stable high-voltage P3-type cathode for sodium-ion batteries

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Chinese Chemical Letters 2024年第9期35卷 507-513页

作者： Shengyu zhao Xuan Yu Yufeng zhao Institute for Sustainable Energy&College of Sciences Shanghai UniversityShanghai 200444China

The Na-deficient P3-type layered oxide cathode material usually experience complex in-plane Na^(+)/vacancy ordering rearrangement and undesirable P3-O3 phase transitions in the high-voltage region,leading to inferior cycling ***,they exhibit unsatisfactory stability when exposed to water for extended *** address these challenges,we propose a Cu/Ti co-doped P3-type cathode material(Na_(0.67)Ni_(0.3)Cu_(0.03)Mn_(0.6)Ti_(0.07)O_(2)),which effectively mitigates Na^(+)/vacancy ordering and suppresses P3-O3 phase transitions at high *** a result,the as-prepared sample exhibited outstanding cyclic performance,with 81.9%retention after 500 cycles within 2.5–4.15 V,and 75.7%retention after300 cycles within 2.5–4.25 ***,it demonstrates enhanced Na^(+)transport kinetics during desodiation/sodiation and reduced growth of charge transfer impedance(R_(ct))after various ***,the sample showed superb stability against water,exhibiting no discernible degradation in structure,morphology,or electrochemical *** co-doping strategy provides new insights for innovative and prospective cathode materials.

关键词： Sodium ion batteries P3-type materials Phase transition Na^(+)/vacancy ordering Water-stable cathode

Challenges and recent advances in HfO_(2)-based ferroelectric films for non-volatile memory applications

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Chip 2024年第3期3卷 50-72页

作者： Ming-Hao Shao Rui-Ting zhao Houfang Liu Wen-Jia Xu Yi-da Guo da-Peng Huang Yu-Zhe Yang Xin-Ru Li Wancheng Shao Peng-Hui Shen Junwei Liu Kuanmao Wang Jinguo Zheng zhao-Yi Yan Jian-Lan Yan Tian Lu Yi Yang Tian-Ling Ren School of Integrated Circuits and Beijing National Research Center for Information Science and Technology(BNRist) Tsinghua UniversityBeijing 100084China

The emergence of data-centric applications such as artificial intelligence(AI),machine learning,and the Internet of Things(IoT),has promoted surges in demand for storage memories with high operating speed and nonvolatile ***_(2)-based ferroelectric memory technologies,which emerge as a promising alternative,have attracted considerable attention due to their high performance,energy efficiency,and full compatibility with the standard complementary metal-oxide-semiconductors(CMOS)*** nonvolatile storage elements,such as ferroelectric random access memory(FeRAM),ferroelectric field-effect transistors(FeFETs),and ferroelectric tunnel junctions(FTJs),possess different data access mechanisms,individual merits,and specific application boundaries in next-generation memories or even beyond von Neumann *** paper provides an overview of ferroelectric HfO2 memory technologies,addresses the current challenges,and offers insights into future research directions and prospects.

关键词： Ferroelectric memory Ferroelectric random-access memory Ferroelectricﬁeld effect transistor Ferroelectric tunneling junction Hafnium oxide