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Strain‑Induced Surface Interface Dual Polarization Constructs PML‑Cu/Bi_(12)O_(17)Br_(2) High‑Density Active Sites for CO_(2) Photoreduction

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Nano-Micro Letters 2024年第5期16卷 169-183页

作者： yi Zhang Fangyu Guo Jun di Keke Wang Molly Meng‑Jung Li Jiayu Dai Yuanbin She Jiexiang Xia Huaming Li School of Chemistry and Chemical Engineering Institute for Energy ResearchSchool of the Environment and Safety EngineeringJiangsu UniversityZhenjiang 212013People’s Republic of China State Key Laboratory Breeding Base of Green Chemistry‑Synthesis Technology College of Chemical EngineeringZhejiang University of TechnologyHangzhou 310014People’s Republic of China College of Science and Hunan Key Laboratory of Extreme Matter and ApplicationsNational University of Defense TechnologyChangsha 410073People’s Republic of China Department of Applied Physics The Hong Kong Polytechnic UniversityHung HomHong KongPeople’s Republic of China School of Chemistry and Chemical Engineering National Special Superfine Powder Engineering Research CenterNanjing University of Science and TechnologyNanjing 210094People’s Republic of China Key Laboratory of the Ministry of Education for Advanced Catalysis Materials Zhejiang Normal UniversityJinhua 321004People’s Republic of China

The insufficient active sites and slow interfacial charge trans-fer of photocatalysts restrict the efficiency of CO_(2) *** synchronized modulation of the above key issues is demanding and ***,strain-induced strategy is developed to construct the Bi–O-bonded interface in Cu porphyrin-based monoatomic layer(PML-Cu)and Bi_(12)O_(17)Br_(2)(BOB),which triggers the surface interface dual polarization of PML-Cu/BOB(PBOB).In this multi-step polarization,the built-in electric field formed between the interfaces induces the electron transfer from con-duction band(CB)of BOB to CB of PML-Cu and suppresses its reverse ***,the surface polarization of PML-Cu further promotes the electron converge in Cu *** introduction of PML-Cu endows a high density of dispersed Cu active sites on the surface of PBOB,significantly promoting the adsorption and activation of CO_(2) and CO *** conversion rate of CO_(2) photoreduction to CO for PBOB can reach 584.3μmol g-1,which is 7.83 times higher than BOB and 20.01 times than *** work offers valuable insights into multi-step polarization regulation and active site design for catalysts.

关键词： Bi_(12)O_(17)Br_(2) Porphyrin CO_(2)photoreduction Polarization Active sites

Controlling hydrogenation of C=C and C=O bonds in cinnamaldehyde using Pt_(1)/Ni and Pt_(1)/Co single-atom alloy catalysts

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Rare Metals 2024年第6期43卷 2859-2868页

作者： Huan-Shi Lan yi-Da Yang Qing-di Sun Hao Zhang ying Zhang Qian He Ran Chen Guo-yi Bai Xiao-Hui He Hong-Bing Ji School of Chemistry and Chemical Engineering Guangxi UniversityNanning 530004China Key Laboratory of Bioinorganicand Synthetic Chemistry of Ministry of Education Fine Chemical Industry Research InstituteSchool of ChemistryIGCMESun Yat-sen UniversityGuangzhou510275China UBFC CNRSENSMMFEMTO-ST Institute25030 Besancon CEDEXFrance College of Chemistry and Materials Science Hebei UniversityBaoding 071002China State Key Laboratory Breeding Base of Green-Chemical Synthesis Technology Institute of Green Petroleum Processing and Light Hydrocarbon ConversionCollege of Chemical EngineeringZhejiang University of TechnologyHangzhou 310014China

Selective hydrogenation of C=C and C=O bonds in cinnamaldehyde(CAL)to produce desired products is a challenging task due to the complex conjugate system of the two unsaturated functional *** this study,a simple ball milling method is presented for synthesizing Pt-based single-atom alloy catalysts(SAAs)that can function as a control switch for the selective hydrogenation of CAL into highly valuable products.

关键词： alloy hydrogenation conjugate

New food sources and production systems:a comparison of international regulations and China’s advancements in novel foods with synthetic biology

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Food Science and Human Wellness 2024年第5期13卷 2519-2542页

作者： Xin Liu di Wu yi Shao Yongning Wu Key Laboratory for Deep Processing of Major Grain and Oil(The Chinese Ministry of Education) College of Food Science and EngineeringWuhan Polytechnic UniversityWuhan 430023China Institute for Global Food Security School of Biological SciencesBelfast B795DLUnited Kingdom NHC Key Laboratory of Food Safety Risk Assessment China National Center for Food Safety Risk AssessmentBeijing 100021China Department of Nutrition and Food Safety Peking Union Medical CollegeResearch Unit of Food SafetyChinese Academy of Medical SciencesBeijing 100021China

The global shift towards sustainable food systems has sparked innovations in food sources and production systems,including cell-based meat,plant-based food products,precision fermentation,and 3D food *** advancements pose regulatory challenges and opportunities,with China emerging as a critical player in adopting and regulating new food *** review explores the international landscape of new food sources and production systems(NFPS),focusing on China’s role and regulatory approaches compared to global *** this comparative analysis,we aim to contribute to the ongoing dialogue on food safety regulation,offering insights and recommendations for policymakers,industry stakeholders,and researchers engaged in the global food system’s *** comprehensive overview underscores the dynamic nature of regulatory frameworks governing NFPS,highlighting the international efforts to ensure food safety,consumer protection,and the sustainable evolution of the food industry.

关键词： New food sources Food production system Food safety International regulation Synthetic biology China

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Deletion of Axin1 in aggrecan-expressing cells leads to growth plate cartilage defects in adult mice

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Genes & diseases 2024年第4期11卷 149-151页

作者： Dan yi Hongting Jin William W.Lu Chunxiang Zhang Guozhi Xiao Liping Tonag di Chen Research Center for Computer-aided Drug discovery Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenGuangdong 518055China PFaculty of Pharmaceutical Sciences Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenGuangdong 518055China The First College of Clinical Medicine Zhejiang Chinese Medical UniversityHangzhouZhejiang 310053China Department of Cardiology Basic Medicine Innovation Centerfor Cardiometabolic Diseases of Ministry of EducationInstitute of Cardiovascular ResearchThe Affiliated HospitalSouthwest Medical UniversityLuzhouSichuan 646000China School of Medicine Southern University of Science and TechnologyShenzhenGuangdong 518055China

In mammals,skeletal bone development begins at hyaline cartilage formation at the early embryonic stage.1Then osteoblasts from the periosteum,which are distributed surrounding the hyaline cartilage,build up compact bone to formdiaphysis and spongy bone known as primary ossification center.1 Next,osteoclasts from the hematopoietic system destroy spongy bone to generate a medullary cavity.

关键词： cartilage skeletal medullary

Microstructure and corrosion behaviors of friction stir-welded Q235 low-carbon steel joint

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Journal of Iron and Steel Research International 2023年第12期30卷 2517-2530页

作者： Hong-duo Wang Zhi-yong Zhou Kuai-she Wang Wen Wang Peng Han Cheng-wen Zhang Yong-xin Lu Guang Li yi-di Lu Xiao Li Yan-ming Liu Xiao-yong Zhang School of Materials Science and Engineering Xi’an Shiyou UniversityXi’an710065ShaanxiChina School of Metallurgical Engineering National and Local Joint Engineering Research Center for Functional Materials ProcessingXi’an University of Architecture and TechnologyXi’an710055ShaanxiChina

Friction stir welding(FSW)was used to prepare Q235 low-carbon steel joint,and the microstructure of different zones of the joint was *** electrochemical corrosion behavior of different macroscopic zones of the joint was evaluated in 3.5 wt.%NaCl *** results showed that the retreated-side heat-affected zone(HAZRS)and the advanced-side heat-affected zone(HAZAS)did not undergo phase transformation during FSW,and their microstructures were similar to those of the base material(BM),which was mainly composed of blocky ferrite and *** retreated-side thermo-mechanical affected zone(TMAZRS),the stirring zone(SZ),and the advanced-side thermo-mechanical affected zone(TMAZAS)underwent phase transformation,and the microstructure was mainly composed of proeutectoid ferrite and *** order of the corrosion resistance of different micro-zones from high to low was:HAZRS>BM>HAZAS>TMAZRS>SZ>*** corrosion mechanism for BM,HAZRS,and HAZAS was mainly the dissolution of *** contrast,the corrosion mechanism for TMAZRS,SZ,and TMAZAS was mainly galvanic corrosion between proeutectoid ferrite and pearlite.

关键词： Q235 low-carbon steel Friction stir welding Microstructure Electrochemistry.Corrosion resistance

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中文非功能需求描述的识别与分类方法研究

软件学报 2019年第10期30卷 3115-3126页

作者：贾一荻刘璘清华大学软件学院

非功能需求描述系统质量相关的属性,是软件设计决策的重要依据和评估标准.与功能需求的描述相比,非功能需求描述通常比较分散,且往往是隐含的.当采集到的需求原始描述内容较多时,逐一进行人工判别和整理需要耗费大量的时间和精力.针对... 详细信息

非功能需求描述系统质量相关的属性,是软件设计决策的重要依据和评估标准.与功能需求的描述相比,非功能需求描述通常比较分散,且往往是隐含的.当采集到的需求原始描述内容较多时,逐一进行人工判别和整理需要耗费大量的时间和精力.针对中文自然语言描述的需求文本,提出了自动化的非功能需求识别和分类方法.其中,识别过程旨在从文本中提取出可能包含非功能需求的语句,尽可能地缩小人工检查的范围.分类过程则进一步将包含非功能需求的语句划分到性能、可靠性、可用性、安全性、可维护性这五大类非功能需求类型之中.分类训练和实验测试基于课题组工作项目整理的实验数据集进行,最终,基于一个工业界的实际应用案例数据,验证了方法的有效性.

关键词：需求工程非功能需求中文文本分类需求识别特征词提取

Highly soluble dendritic fullerene derivatives as electron transport material for perovskite solar cells

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Journal of Central South University 2021年第12期28卷 3714-3727页

作者： CHENG Zheng-chun FANG yin-yu WANG Ai-fei MA Tao-tao LIU Fang GAO Song YAN Su-hao di yi QIN Tian-shi Institute of Advanced Materials(IAM) Nanjing Tech UniversityNanjing 210009China Ningbo Institute of Northwestern Polytechnical University Ningbo 315103China Shaanxi Institute of Flexible Electronics Northwestern Polytechnical UniversityXi'an 710072China

A series of shape-persistent polyphenylene dendritic C_(60)derivatives as the electron transport materials were designed and synthesized via a catalyst-free diels-Alder[4+2]cycloaddition *** increasing hyperbranched scaffolds could effectively enhance the solubility;notably,both first and second generation dendrimers,C_(60)-G1 and C_(60)-G2,demonstrated more than 5 times higher solubilities than pristine C_(60).Furthermore,both simulated and experimental data proved their promising solution-processabilities as electron-transporting layers(ETLs)for perovskite solar *** a result,the planar p-i-n structural perovskite solar cell could achieve a maximum power conversion efficiency of 14.7%with C_(60)-G2.

关键词： dendritic structures fullerene C60 electron transport materials enhanced solubility perovskite solar cells

Evaluation of Resistance of different Kiwifruit Varieties (Lines) to Canker disease and Brown Spot disease

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Phyton-International Journal of Experimental Botany 2024年第6期93卷 1249-1261页

作者： Wenwen Su Chongpei Zheng Zhencheng Han Chunguang Ren di Wu Tao Li yi Yang Weijie Li Institute of Mountain Resources of Guizhou Province Guizhou Academy of SciencesGuiyang550001China Guizhou Botanical Garden Guizhou Academy of SciencesGuiyang550001China Key Laboratory of Plant Resource Conservation and Germplasm Innovation in Mountainous Region(Ministry of Education) Institute of Agro-Bioengineering/College of Life SciencesGuizhou UniversityGuiyang550025China

Kiwifruit canker and brown spot are signiﬁcant diseases affecting kiwis,caused by Pseudomonas syringae patho-genic variations(Pseudomonas syringae ***(Psa))and Corynesporapolytica(Corynespora cassiicola).At present,the research on canker disease and brown spot disease mainly focuses on the isolation and identiﬁcation of pathogenic bacteria,drug control,resistance gene mining and functional veriﬁ*** has proved that breeding disease resistant varieties are an effective method to control canker disease and brown spot ***,most existing cultivars lack genes for canker and brown spot *** kiwifruit resources in nat-ure exhibit extensive genetic diversity due to prolonged natural selection,containing numerous resistance ***,due to insufﬁcient understanding of the resistance of most kiwifruit varieties(lines)to canker disease and brown spot disease,some high-quality resources have not been fully *** incidence of canker and brown spot of 18 kiwifruit cultivars(lines)was measured by inoculating isolated branches and leaves,and their resistance to canker and brown spot was analyzed according to the length,disease index,mean diameter,and systematic *** results were as follows:Among 18 different kiwifruit varieties(lines)for canker disease,there were two highly resistant materials,eight disease-resistant materials,four disease-susceptible materials,and two highly susceptible ***,regarding brown spot disease,there were one highly resistant material,ﬁve dis-ease-resistant materials,four susceptible materials,and three highly susceptible ***,four resources were resistant to both *** outcomes provided a theoretical basis for breeding kiwifruit against canker and brown spot.

关键词： Kiwifruit canker disease brown spot resistance evaluation

Electrochemically recycling degraded superalloy and valorizing CO_(2)in the aff ordable borate-modified molten electrolyte

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Tungsten 2024年第2期6卷 382-393页

作者： Xiang Chen Yuan Sun Long Wang Xin Qu Yan Zhao Hong-Wei Xie di-Hua Wang Hua-yi yin Key Laboratory for Ecological Metallurgy of Multimetallic Mineral of Ministry of Education School of MetallurgyNortheastern UniversityShenyang 110819China Institute of Metal Research Chinese Academy of ScienceShenyang 110016China School of Resource and Environmental Science Wuhan UniversityWuhan 430072China

Integrating electrochemical reduction of CO_(2)and electrochemical oxidation to recycle degraded superalloys is a promising solution to ease resource scarcity and safeguard environmental ***,we propose an electrochemical technique for the conversion of bulk superalloy scraps and CO_(2)into oxide powder at the anode and solid carbon at the cathode,*** particular,a borax-modifi ed CaCl_(2)-based molten salt electrolyte is used for enhancing the electrochemical oxidation of superalloy *** a temperature of 700℃and a voltage of 2.8 V,90.55 wt.%of alloy scraps were oxidized in a molten CaCl_(2)–NaCl–CaCO_(3)–Na_(2)B_(4)O_(7)with an acid–base ratio(K_(a/b))of *** synergy of Cl−and B_(4)O_(7)2−of electrolyte prevents the passivation of the alloy anode and enables continuous ***,the Ni and Co in the anode products are recovered by sulfation roasting with recovery efficiencies of 85.58%and 95.27%for Ni and Co,***,modulating the alkalinity of the electrolyte for enhancing oxidation/pulverization of alloy scrap anode provides new insight into electrochemically recovering superalloy scraps.

关键词： Superalloy scraps Recycling Molten salt Alkalinity Electrochemical oxidation Cobalt