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Global paleobiogeography of Albian—Cenomanian(mid-Cretaceous)marine ostracods

Journal of Palaeogeography 2024年第2期13卷 212-236页

作者： Bernardo vázquez-García Jorge villegas-Martín Gerson Fauth Leonardo Borghi Aristóteles de Moraes Rios Netto Post-Graduate Program in Geology Unisinos UniversitySao LeopoldoRSBrazil Technological Institute of Paleoceanography and Climate Change-Itt Oceaneon Unisinos UniversitySao LeopoldoRSBrazil Laboratory of Sedimentary Geology(Lagesed) Department of GeologyInstitute of GeosciencesUFRJ-Federal Universityof Riode JaneiroBrazil Labmicro Department of GeologyInstitute of GeosciencesUFRJ-Federal University of Rio de JaneiroBrazil

despite their potential for providing important information for paleobiogeography,studies using ostracod assemblages compiled from global datasets have been scarce so *** this study,the paleogeographic implications of the relationship between different ostracod assemblages are analyzed and discussed for the Albian and *** compiled an ostracod dataset at the genus level,with 168 genera for the Albian and 174 for the Cenomanian,to which different multivariate statistical methods of grouping were *** affinity between different ostracod assemblages from different regions allowed for the delineation of 30 operational geographic units(OGUs)for the Albian,and 32 OGUs for the Cenomanian,grouped in three paleobiogeographic units(PBUs;Megatethys,Persia,and Austral)and one sub-unit(PBSU;Maghreb associated to the Megatethys).The Maghreb PBSU showed minor changes between the Albian and *** relationship among the OGUs grouped in each PBU is related to different factors,such as eustatic sea level events,similar climatic zones,and marine current circulation patterns.A relationship was observed between the Gabon and Nigeria OGUs with the Persia PBU,which suggests a direct east—west connection between them during the *** affinity observed in the Austral PBU between the South American,South African,and Australian regions during the Albian can be explained by their relative geographic isolation due to the Walvis Ridge *** eventual flooding of this barrier led to the relationship observed between the SE Brazilian and Bolivian regions with the Austral ***,the data also suggested that the separation of the Indian subcontinent from the Austral PBU took place during the Cenomanian.

关键词： Operational geographic units Paleobiogeographic units Albian Cenomanian Marine ostracods

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A combined computational/experimental study of anode-concerned voltage drop in aqueous primary Mg-air batteries

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Journal of Magnesium and Alloys 2024年第5期12卷 1854-1866页

作者： Wen Xu Min deng darya Snihirova Linqian Wang Yulong Wu Sviatlana v.Lamaka Mikhail L.Zheludkevich daniel Hoche Institute of Surface Science Helmholtz-Zentrum Hereon21502 GeesthachtGermany School of Materials Science and Engineering Hebei University of Technology300000TianjinChina Institute for Materials Science Faculty of EngineeringKiel University24143 KielGermany

The voltage drop appearing at Mg anode-electrolyte interface is a critical issue for the battery power and energy density of aqueous primary Mg-air *** respective voltage loss is typically assigned to the deposits layer forming on the anode surface during *** this work,we experimentally and computationally investigate the critical factors affecting the voltage drop at Mg anode towards a deeper understanding of the contribution of deposit and its growth.A two-dimensional(2d)mathematical model is proposed to compute the voltage drop of Mg-0.15Ca wt.%alloy(Mg-0.15Ca)by means of a semi-empirical formulas and experiments-based modification model,considering the effect of discharge current density,the negative difference effect(NdE)and surface deposits layer *** model is utilized to simulate the discharge potential of the anode at predefined experimental current *** computed voltage drop(half-cell voltage)is in good agreement with the experimental *** applicability of the mathematical model is successfully validated on the second material(namely high-purity Mg).

关键词： Aqueous Mg-air battery voltage drop NdE Charge transfer deposits-related resistances

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Heavy metal pollution of river water and eco-friendly remediation using potent microalgal species

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Water Science and Engineering 2024年第1期17卷 41-50页

作者： Amudham Radha Amal Raj Prabhakaran Mylsamy v.Sivasankar B.Sathish Kumar Kiyoshi Omine T.G.Sunitha Phycological Research Laboratory Research Department of BotanyPachaiyappa's College(Affiliated to University of Madras)Chennai 600030India Research department of Chemistry Pachaiyappa's College(Affiliated to University of Madras)Chennai 600030India department of Botany Sri Vidya Mandir Arts&Science College(Autonomous)KatteriUthangarai 636902India department of Civil Engineering School of Engineering.Nagasaki UniversityNagasaki-Daigaku1-14 Bunkyo-machiNagasaki 8528521Japan

Pollution of rivers is mainly caused by anthropogenic activities such as discharge of effluent from industrial facilities,maintenance of sewage/effluent treatment plants,and dumping of solid waste on river *** study dealt with the pollution issues of the Cooum River in the well-known city of Chennai in South *** samples from 27 locations were collected and analyzed for 12 elements,including Ba,B,and Al,as well as heavy metals such as Pb,Cr,Mn,Fe,Co,Ni,Cu,Zn,and *** samples showed levels of these elements that exceeded World Health Organization *** correlation analysis revealed the inter-dependency among elements,and the contribution of each element based on factor loadings showed its percentage contribution compared to *** samples from six significant locations were chosen for remediation with three algae:Chlorella vulgaris,Scenedesmus dimorphus,and Phormedium *** uptake of pollutants led to the continuous growth of algae during the incubation period of 15 d,effectively removing heavy metals from the river *** increasing levels of algal counts and the chlorophyll a content confirmed the algal growth during the incubation period,followed by a declining stage after the incubation *** scanning electron microscopic images of algae before and after the remediation showed no remarkable modification of morphological *** study showed that the uptake of heavy metals using algae is an effective water pollution remediation measure,making the process practicable in the field on a large scale in the near future.

关键词： Heavy metal Cooum river Phycoremediation Microalgae Factor analysis

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Stroke depression:a concept with clinical applicability

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Stroke & vascular Neurology 2024年第3期9卷 189-193页

作者： Jun Mu Arun v Ravindran Pim Cuijpers Yiqing Shen Wensong Yang Qi Li Xinyu Zhou Peng Xie department of Neurology The First Affiliated Hospital of Chongqing Medical UniversityChongqingChina Campbell Family Mental Health Research Centre Centre for Addiction and Mental HealthDepartment of PsychiatryUniversity of TorontoTorontoOntarioCanada department of Clinical Neuro and Developmental PsychologyAmsterdam Public Health research instituteVrije Universiteit AmsterdamAmsterdamThe Netherlands NHC Key Laboratory of diagnosis and Treatment on Brain Functional diseases The First Affiliated Hospital of Chongqing Medical UniversityChongqingChina department of Psychiatry The First Affiliated Hospital of Chongqing Medical UniversityChongqingChina

Stroke is a common neurological condition and among the leading causes of death and disability *** is both a risk factor for and complication of stroke,and the two conditions may have a complex reciprocal relationship over ***,the secondary effects of depression on stroke are often overlooked,resulting in increased morbidity and *** the previous concept of‘poststroke depression’,stroke and depression were considered as two independent *** often delays the diagnosis and treatment of *** concept‘stroke depression’proposed in this article will emphasise more the necessity of aggressive treatment of depression in the overall management of stroke,thus to reduce the incidence of stroke and in the meantime,improve the prognosis of ***,it will lead us into a new era of acute stroke intervention.

关键词： diagnosis mortality acute

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H_(2)mediated mixed culture microbial electrosynthesis for high titer acetate production from CO_(2)

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Environmental Science and Ecotechnology 2024年第3期19卷 125-131页

作者： Yanhong Bian Aaron Leininger Harold d.May Zhiyong Jason Ren department of Civil and Environmental Engineering Princeton University86 Olden StPrincetonNJ08544United States Andlinger Center for Energy and the Environment Princeton University86 Olden St.PrincetonNJ08544United States

Microbial electrosynthesis(MES)converts CO_(2)into value-added products such as volatile fatty acids(vFAs)with minimal energy use,but low production titer has limited scale-up and *** electron transfer via H_(2)on the MES cathode has shown a higher conversion rate than the direct biofilm-based approach,as it is tunable via cathode potential control and accelerates electrosynthesis from CO_(2).Here we report high acetate titers can be achieved via improved in situ H_(2)supply by nickel foam decorated carbon felt cathode in mixed community MES *** concentration of 12.5 g L^(-1)was observed in 14 days with nickel-carbon cathode at a poised potential of-0.89 v(*** hydrogen electrode,SHE),which was much higher than cathodes using stainless steel(5.2 g L^(-1))or carbon felt alone(1.7 g L^(-1))with the same projected surface area.A higher acetate concentration of 16.0 g L^(-1)in the cathode was achieved over long-term operation for 32 days,but crossover was observed in batch operation,as additional acetate(5.8 g L^(-1))was also found in the abiotic anode *** observed the low Faradaic efficiencies in acetate production,attributed to partial H_(2)utilization for *** selective acetate production with high titer demonstrated in this study shows the H_(2)-mediated electron transfer with common cathode materials carries good promise in MES development.

关键词： Microbial electrosynthesis Indirect electron transfer CO_(2)electrolysis vFAs production

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Anomalies in the short-range local environment and atomic diffusion in single crystalline equiatomic CrMnFeCoNi highentropy alloy

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Nano Research 2024年第6期17卷 5336-5348页

作者： Alevtina Smekhova daniel Gaertner Alexei Kuzmin Ana Guilherme Buzanich Goetz Schuck Ivo Zizak Gerhard Wilde Kirill v.Yusenko Sergiy divinski Helmholtz-Zentrum Berlin für Materialien und Energie(HZB) D-12489 BerlinGermany Institute of Materials Physics University of MünsterD-48149 MünsterGermany Institute of Solid State Physics University of LatviaLV-1063 RigaLatvia Bundesanstalt für Materialforschung und–prüfung(BAM) D-12489 BerlinGermany

Multi-edge extended X-ray absorption fine structure(EXAFS)spectroscopy combined with reverse Monte Carlo(RMC)simulations was used to probe the details of element-specific local coordinations and component-dependent structure relaxations in single crystalline equiatomic CrMnFeCoNi high-entropy alloy as a function of the annealing *** representative states,namely a high-temperature state,created by annealing at 1373 K,and a low-temperature state,produced by long-term annealing at 993 K,were compared in *** features identified in atomic configurations of particular principal components indicate variations in the local environment distortions connected to different degrees of compositional disorder at the chosen representative *** detected changes provide new atomistic insights and correlate with the existence of kinks previously observed in the Arrhenius dependencies of component diffusion rates in the CrMnFeCoNi high-entropy alloy.

关键词： high-entropy alloys diffusion short-range order extended X-ray absorption fine structure(EXAFS) reverse Monte Carlo

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Synergistic Co-doping effect of CNTs and PvP in Na_(4)MnCr(PO_(4))3 cathode as a strategy for improving the electrochemical performance of SIBs

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Chinese Chemical Letters 2024年第2期35卷 539-543页

作者： Ruoyu Chen denys S.Butenko Shilin Li Xinyu Zhang Guangshe Li Igor v.Zatovsky Wei Han College of Physics State Key Laboratory of Inorganic Synthesis and Preparative ChemistryInternational Center of Future ScienceJilin UniversityChangchun 130012China Academy for Advanced Interdisciplinary Studies Southern University of Science and TechnologyShenzhen 518055China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China F.d.Ovcharenko Institute of Biocolloidal Chemistry NAS UkraineKyiv 03142Ukraine

In order to solve the contradiction between the rapidly growing energy demand and the excessive exploitation of fossil fuels,it is urgent to research and develops more environmentally friendly and efficient energy storage ***,the development of high-performance cathode materials to enhance the energy density of SIB is currently one of the most important topics of scientific *** high-voltage and low-cost cathode material for SIBs,a composite of carbon-coated Na_(4)MnCr(PO_(4))_(3)(NASICON-type),polyvinylpyrrolidone(PvP),and modified carbon nanotubes(CNTs)is prepared by sol-gel and freeze-drying *** to the high conductivity of CNTs,the conductivity of the composite is significantly improved,and its initial capacity is increased to 114 mAh/g at 0.5 C and 96 mAh/g at 5 C(Mn^(2+)/Mn^(4+)conversion for voltage windows 1.4-4.3 v).Moreover,the multi-electrons transfer of Cr^(3+)/Cr^(4+) and Mn^(2+)/Mn^(4+) can provide a high capacity of 165 mAh/g at 0.1 C and 102 mAh/g at 5 C in the high voltage window of 1.4-4.6 ***,PvP can effectively inhibit the Jahn-Teller effect caused by Mn ion,making the composite have more excellent high-rate performance and *** addition,GITT,EIS and Cv curves were drawn to better reveal the excellent kinetic properties of Na_(4)MnCr(PO_(4))_(3)@C@PvP@CNT cathode,and the mechanism of its performance improvement is deeply studied and ***,the co-doping of CNTs and PvP is a simple way to high conductivity and fast charging of cathode materials for SIBs.

关键词： Sodium-ion batteries Na_(4)MnCr(PO_(4))_(3) Carbon nanotubes Polyvinylpyrrolidone Synergistic effect

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Expanded Porphyrin Exhibiting Off-Centered Out-of-Plane Coordination to dysprosium

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CCS Chemistry 2024年第7期6卷 1731-1738页

作者： dmitry I.Nazarov Jorge Labella Alexey v.Kuzmin Maxim A.Faraonov Evgenii N.Ivanov Salavat S.Khasanov Tomas Torres Mikhail K.Islyaikin dmitri v.Konarev Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry RAS 142432 Chernogolovka department of Organic Chemistry Universidad Autonoma de Madrid28049 Madrid Institute of Solid-State Physics RAS 142432 Chernogolovka Research Institute of Macroheterocycles Ivanovo State University of Chemistry and Technology15300 Ivanovo G.A.Krestov Institute of Solution Chemistry of the Russian Academy of Sciences 153045 Ivanovo Institute for Advanced Research in Chemical Sciences Universidad Autonoma de Madrid28049 Madrid IMdEA-Nanociencia 28049 Madrid

The complexation of high-spin lanthanides to porphyrinoids is a powerful strategy for the development of advanced molecular *** this context,the use of expanded porphyrinoids remains elusive since their coordination chemistry is challenging to ***,taking inspiration from on-surface chemistry,we explored the coordination of dy^(3+)to a six-membered porphyrinoid,namely,the hemihexaphyrazine ***,we observed the selective formation of a mono-nuclear off-centered,out-of-plane H_(2)Hhp-dy^(3+)complex when performing the complexation under reductive *** this reaction,the oxidation state of the macrocycle did not *** X-ray diffraction analysis,we found that the coordination number of dy in this complex was *** macrocycle cocrystallized with decamethylcobaltocene(Cp_(2)^(*)Co)molecules,giving rise to a wellordered solid-state packing,governed byπ-π*** a result of this organization,a small magnetic coupling between the neighboring molecules was *** in all,this work provides key insights into the coordination of magnetically active metals with expanded porphyrinoids,thus motivating the development of advanced spintronic devices.

关键词： porphyrins dysprosium macrocycle coordination chemistry magnetism

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Interaction of photons with silver and indium nuclei at energies up to 20 Mev

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Chinese Physics C 2024年第2期48卷 135-140页

作者： J.H.Khushvaktov M.A.demichev d.L.demin S.A.Evseev M.I.Gostkin v.v.Kobets F.A.Rasu-lova S.v.Rozov E.T.Ruziev A.A.Solnyshkin T.N.Tran E.A.Yakushev B.S.Yuldashev Joint Institute for Nuclear Research(JINR) DubnaRussia Institute of Nuclear Physics of the Academy of Sciences of the Republic of Uzbekistan(INP ASRU) TashkentUzbekistan Institute of Physics of the vietnam Academy of Science and Technology(IP vAST) HanoiVietnam

The yields of photonuclear reactions in the 107Ag,113In,and 115In nuclei were *** Carlo simulations were performed using the Geant4 code,and the results were compared with the experimental *** isomeric ratios of the yields in the reactions 107Ag(γ,n)106m,gAg and 113In(γ,m)112m,gIn were determined,and the cross sections for the reactions 107Ag(γ,n)106gAg and 107Ag(γ,2n)105Ag at an energy of 20 Mev were calculated based on the experimental data.

关键词： 107Ag(γ,n)10mgAg and I13In(γ,n)12m-2In reactions cross section yield isomeric ratio simula-tion Geant4 TALYS

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Rigidity Symmetry Line for Thermodynamic Fluid Equations-of-State

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Journal of Modern Physics 2024年第5期15卷 613-633页

作者： Leslie v. Woodcock department of Physics University of Algarve Faro Portugal

We report progress towards a modern scientific description of thermodynamic properties of fluids following the discovery (in 2012) of a coexisting critical density hiatus and a supercritical mesophase defined by percolation transitions. The state functions density ρ(p,T), and Gibbs energy G(p,T), of fluids, e.g. CO2, H2O and argon exhibit a symmetry characterised by the rigidity, ω = (dp/dρ)T, between gaseous and liquid states along any isotherm from critical (Tc) to Boyle (TB) temperatures, on either side of the supercritical mesophase. Here, using experimental data for fluid argon, we investigate the low-density cluster physics description of an ideal dilute gas that obeys dalton’s partial pressure law. Cluster expansions in powers of density relate to a supercritical liquid-phase rigidity symmetry (RS) line (ω = ρrs(T) = RT) to gas phase virial coefficients. We show that it is continuous in all derivatives, linear within stable fluid phase, and relates analytically to the Boyle-work line (BW) (w = (p/ρ)T = RT), and to percolation lines of gas (PB) and liquid (PA) phases by: ρBW(T) = 2ρPA(T) = 3ρPB(T) = 3ρRS(T)/2 for T TB. These simple relationships arise, because the higher virial coefficients (bn, n ≥ 4) cancel due to clustering equilibria, or become negligible at all temperatures (0 T TB) within the gas phase. The Boyle-work line (p/ρBW)T is related exactly at lower densities as T → TB, and accurately for liquid densities, by ρBW(T) = −(b2/b3)T. The RS line, ω(T) = RT, defines a new liquid-density ground-state physical constant (ρRS(0) = (2/3)ρBW(0) for argon). Given the gas-liquid rigidity symmetry, the entire thermodynamic state functions below TB are obtainable from b2(T). A BW

关键词： Liquid-State Theory Cluster Physics Percolation Lines Fluid Thermodynamics Boyle Line Rigidity-Symmetry Line

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