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Unveiling the tailorable electrochemical properties of zeolitic imidazolate framework-derived Ni-doped LiCoO_(2) for lithium-ion batteries in half/full cells

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Journal of Energy Chemistry 2024年第6期93卷 229-242,I0006页

作者： Jian-En Zhou Yiqing Liu Zhijian Peng Quanyi ye hua Zhong Xiaoming Lin Ronghua Zeng Yongbo Wu Jiaye ye Guangdong Provincial International Joint Research Center for Energy Storage Materials Key Laboratory of Theoretical Chemistry of EnvironmentMinistry of EducationSchool of ChemistrySouth China Normal UniversityGuangzhou 510006GuangdongChina School of Chemistry and Physics Faculty of ScienceQueensland University of TechnologyBrisbaneQLD 4001Australia Key Laboratory of Atomic and Subatomic Structure and Quantum Control(Ministry of Education) Guangdong Basic Research Center of Excellence for Structure and Fundamental Interactions of MatterSchool of PhysicsSouth China Normal UniversityGuangzhou 510006GuangdongChina Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials Guangdong-Hong Kong Joint Laboratory of Quantum MatterSouth China Normal UniversityGuangzhou 510006GuangdongChina

As a prevailing cathode material of lithium-ion batteries(LIBs),LiCoO_(2)(LCO)still encounters the tricky problems of structural collapse,whose morphological engineering and cation doping are crucial for surmounting the mechanical strains and alleviating phase degradation upon ***,we propose a strategy using a zeolitic imidazolate framework(ZIF)as the self-sacrificing template to directionally prepare a series of LiNi_(0.1)Co_(0.9)O_(2)(LNCO)with tailorable electrochemical *** rational selection of sintering temperature imparts the superiority of the resultant products in lithium storage,during which the sample prepared at 700℃(LNCO-700)outperforms its counterparts in cyclability(156.8 mA h g^(-1)at 1 C for 200 cycles in half cells,1 C=275 mA g^(-1))and rate capability due to the expedited ion/electron transport and the strengthen mechanical *** feasibility of proper Ni doping is also divulged by half/full cell tests and theoretical study,during which LNCO-700(167 mA h g^(-1)at 1 C for 100 cycles in full cells)surpasses LCO-700 in battery performance due to the mitigated phase deterioration,stabilized layered structu re,ameliorated electro nic co nductivity,a nd exalted lithium sto rage *** work systematically unveils tailorable electrochemical behaviors of LNCO to better direct their practical application.

关键词： Lithium-ion batteries Zeolitic imidazolate framework LiNi_(0.1)Co_(0.9)O_(2) Electrochemical properties

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On some new fuzzy entropy measure of Pythagorean fuzzy sets for decision-making based on an extended TOPSIS approach

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Journal of Management Analytics 2024年第1期11卷 87-109页

作者： h.d.Arora Anjali Naithani department of Mathematics Amity Institute of Applied SciencesAmity University Uttar PradeshNoidaIndia

Fuzzy entropy measures are valuable tools in decision-making when dealing with uncertain or imprecise *** exist many entropy measures for Pythagorean Fuzzy Sets(PFS)in the literature that fail to deal with the problem of providing reasonable or consistent results to the *** deal with the shortcomings of the existing measures,this paper proposes a robust fuzzy entropy measure for PFS to facilitate decision-making under *** usefulness of the measure is illustrated through an illustration of decision-making in a supplier selection problem and compared with existing fuzzy entropy *** Technique for Order Performance by Similarity to Ideal Solution(TOPSIS)approach is also explored to solve the decision-making *** results demonstrate that the proposed measure can effectively capture the degree of uncertainty in the decision-making process,leading to more accurate decision outcomes by providing a reliable and robust ranking of alternatives.

关键词： Pythagorean fuzzy sets entropy measures multi criteria decision analysis TOPSIS method supplier selection

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Preparation and Characterization of ph-Responsive Charge Reversal Nanocomposite for miRNA delivery

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 1048-1052页

作者：余丹 ye Liyuan LI Binbin MOU Fangzhi 殷义霞 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China hainan Institute Wuhan University of TechnologySanya 572000China Biomedical Materials and Engineering Research Center of hubei Province Wuhan University of TechnologyWuhan 430070China

ph-responsive charge reversal loaded miRNA nanocomposite was prepared by electrostatic *** morphology,particle size and zeta potential of the nanocomposites were analyzed by transmission electron microscopy and dynamic light *** synthesis of the polymer was analyzed by^(1)*** zeta-potential changes and cellular uptake effects of the nanocomplexes under different ph environments were *** experimental results show that the surface morphology of the nanocomposite is spherical,and the average particle size is about 135 *** the ph value of the solution gradually decreases,the surface charge of the nanocomposite reverses from negative charge to positive charge(from-9.4 to+17.1 mV).Cellular uptake mediated by ph-responsive nanocomposite is selective for tumor cells,and the cellular uptake effect in tumor cells at ph 6.5 was approximately 3 times higher than that at ph *** ph responsive charge reversal nanocomposite has promising application prospects for gene delivery in the weak acid environment of tumors.

关键词： charge conversion siRNA delivery ph responsive cancer therapy

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The Extension dimension of Subcategories and Recollements of Abelian Categories

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Acta Mathematica Sinica,English Series 2024年第4期40卷 1042-1058页

作者： Xin MA ye Yang PENG Zhao Yong hUANG College of Science Henan University of EngineeringZhengzhou 451191P.R.China department of Mathematics Nanjing UniversityNanjing 210093P.R.China

We investigate the behavior of the extension dimension of subcategories of abelian categories under ***Λ',Λ,Λ"be art in algebras such that(modΛ',mod A,modΛ")is a recollement,and let d'and d"be subcategories of modΛand modΛ"*** any n,m≥0,under some conditions,we get dimΩ^(k)(d)≤dimΩ^(n)(d')+dimΩ^(m)(d")+1,where k=max{m,n}and d is the subcategory of modΛglued by d'and d";moreover,we give a sufficient condition such that the converse inequality holds *** applications,some results for Igusa-Todorov subcategories and syzygy finite sub categories are obtained.

关键词： Recollements extension dimension Igusa–Todorov subcategories syzygy finite subcategories

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Clinical observation on 90 cases of primary dysmenorrhea treated by buccal acupuncture therapy:a randomized controlled study

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Journal of Traditional Chinese Medicine 2024年第1期44卷 172-181页

作者： YANG Yi ye huijun ZhENG huiling JIN Lihua department of Obstetrics and Gynecology the Second Affiliated Hospital of Zhejiang Chinese Medical UniversityXinhua Hospital of Zhejiang ProvinceHangzhou 310005China

OBJECTIVE:To explore the short-term and long-term efficacy of buccal acupuncture therapy in the treatment of patients with primary dysmenorrhea(Pd).METhOdS:A total of 90 patients with Pd who were admitted to the Second Affiliated.h.spital of Zhejiang University of Traditional Chinese Medicine from January 2020 to december 2021 were included in this study and randomly divided into three groups,including the observation group,the control group,and the placebo group,with 30 patients in each *** in the observation group were treated according to the syndrome types of Traditional Chinese Medicine,those in the control group were treated with Saridon,and those in the placebo group received a *** visual analog scale(VAS)scores of these patients were evaluated at different time points(before treatment,5 min after needle retention,30 min after needle retention,1 h after treatment,2 h after treatment,1 d after treatment,and 2 d after treatment).The Cox Menstrual Symptom Scale(CMSS)scores were assessed before the treatment and after three courses of ***,these two scales were also evaluated during ***,the pain score and adverse reactions of these patients were assessed during ***:After treatment,the VAS and CMSS scores in the observation group decreased significantly(Pd 30 min after needle retention and after ***:Buccal acupuncture therapy is verified to have short-term efficacy in the treatment of *** addition,this therapy has an immediate analgesic effect and long-term efficacy in reducing the severity and frequency of Pd.

关键词： buccal acupuncture therapy primary dysmenorrhea pain score randomized controlled trial

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The multi-impurity system in CdSe nanoplatelets:electronic structure and thermodynamic properties

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Communications in Theoretical Physics 2024年第3期76卷 165-173页

作者： d A Baghdasaryan V A harutynyan E M Kazaryan h A Sarkisyan Russian-Armenian University H Emin 1230051YerevanArmenia Institute of Applied Problems of Physics 25 Nersisyan St0014YerevanArmenia

This paper theoretically studies the impurity states and the effects of impurity concentration and configuration on the optical,electrical,and statistical properties of CdSe nanoplatelets(NPLs).An image charge-based model of electron-impurity interaction is *** charge-carrier energy spectra and corresponding wave functions depending on the impurity number and configuration are *** electron binding energies are calculated for different NPL *** is shown that the image charge-based interaction potential that arises due to the dielectric constants mismatch is much stronger than the interaction potential that does not take such a mismatch into ***,it is demonstrated that the binding energies are increasing with the number of *** calculate the canonical partition function using the energy levels of the electron,which in turn is used to obtain the mean energy,heat capacity,and entropy of the non-interacting electron *** thermodynamic properties of the non-interacting electron gas that depend on the geometric parameters of the NPL,impurity number,configuration,and temperature are studied.

关键词： nanoplateletes thermodynamic properties impurity states

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Influence of vibration on the lubrication effect of a splash-lubricated gearbox

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第4期25卷 324-339页

作者： Yi LIU Kailin ZhANG Shuai ShAO hongxu XIANG Zhijian ye State Key Laboratory of Rail Transit Vehicle System Southwest Jiaotong UniversityChengdu 610031China

In this study,we investigate the effect of rail vibrations on the lubrication and efficiency of a splash-lubricated gearbox;specifically,the gearbox of a rail-transit vehicle.A high-fidelity 3d numerical model of the gearbox in a moving reference system is described,as well as computational fluid dynamics(CFd)simulations of the gearbox with different vibration *** effects of rotational speed,oil-immersion depth,and different oil-injection volume rates on lubrication and efficiency are *** propose a method of evaluating the internal lubrication condition of a splash-lubricated gearbox and quantitatively compare the effects of different operating parameters on lubrication and ***,our experiment to verify the feasibility of the simulation method is *** results show that with vibration,the churning loss and oil supply for the bearings are significantly higher than those under static *** addition,among different vibrational directions,lateral vibration has the greatest influence on the lubrication condition and efficiency of the *** the studied railway-vehicle gearbox,the best lubrication condition is achieved at a rotational speed of 1600 r/min and an oil-immersion depth of two times the tooth height(***).Rotational speed is the operating parameter that has the most significant effect on the lubrication and efficiencyofthegearbox.

关键词： Comprehensive lubrication evaluation Churning loss Moving reference system Splash lubrication Vibrational excitation Gearbox

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Rapid Energy Exchange between In Situ Formed Bromine Vacancies and CO_(2)Molecules Enhances CO_(2)Photoreduction

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Research 2024年第2期2023卷 763-771页

作者： Qin Ren ye he hong Wang Yanjuan Sun Fan dong Research Center for Environmental and Energy Catalysis Institute of Fundamental and Frontier SciencesUniversity of Electronic Science and Technology of ChinaChengdu 611731China School of Resources and Environment University of Electronic Science and Technology of ChinaChengdu 611731China

Photocatalytic reduction of CO_(2)into fuels provides a prospective tactic for regulating the global carbon balance utilizing renewable solar ***,CO_(2)molecules are difficult to activate and reduce due to the thermodynamic stability and chemical *** this work,we develop a novel strategy to promote the adsorption and activation of CO_(2)molecules via the rapid energy exchange between the photoinduced Br vacancies and CO_(2)*** in situ continuous wave-electron paramagnetic resonance(cw-EPR)and pulsed EPR technologies,we observe that the spin-spin relaxation time(T_(2))of BiOBr is decreased by 198 ns during the CO_(2)photoreduction reaction,which is further confirmed by the broadened EPR *** result reveals that there is an energy exchange interaction between in situ formed Br vacancies and CO_(2)molecules,which promotes the formation of high-energy CO_(2)molecules to facilitate the subsequent reduction *** addition,theoretical calculations indicate that the bended CO_(2)adsorption configuration on the surface of BiOBr with Br vacancies caused the decrease of the lowest unoccupied molecular orbital of the CO_(2)molecule,which makes it easier for CO_(2)molecules to acquire electrons and get *** situ diffuse reflectance infrared Fourier transform spectroscopy further shows that the activated CO_(2)molecules are favorably converted to key intermediates of COOh*,resulting in a CO generation rate of 9.1μmol g^(-1)h^(-1)and a selectivity of 100%.This study elucidates the underlying mechanism of CO_(2)activation at active sites and deepens the understanding of CO_(2)photoreduction reaction.

关键词： reaction. adsorption activation

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Estimation of the anisotropy of hydraulic conductivity through 3d fracture networks using the directional geological entropy

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International Journal of Mining Science and Technology 2024年第2期34卷 137-148页

作者： Chuangbing Zhou Zuyang ye Chi Yao Xincheng Fan Feng Xiong School of Infrastructure Engineering Nanchang UniversityNanchang 330031China b School of Resource and Environmental Engineering Wuhan University of Science and TechnologyWuhan 430081China School of Engineering China University of GeosciencesWuhan 430074China

With an extension of the geological entropy concept in porous media,the approach called directional entrogram is applied to link hydraulic behavior to the anisotropy of the 3d fracture networks.A metric called directional entropic scale is used to measure the anisotropy of spatial order in different *** with the traditional connectivity indexes based on the statistics of fracture geometry,the directional entropic scale is capable to quantify the anisotropy of connectivity and.h.draulic conductivity in heterogeneous 3d fracture *** to the numerical analysis of directional entrogram and fluid flow in a number of the 3d fracture networks,the hydraulic conductivities and entropic scales in different directions both increase with spatial order(i.e.,trace length decreasing and spacing increasing)and are independent of the dip *** a result,the nonlinear correlation between the hydraulic conductivities and entropic scales from different directions can be unified as quadratic polynomial function,which can shed light on the anisotropic effect of spatial order and global entropy on the heterogeneous hydraulic behaviors.

关键词： 3d fracture network Geological entropy directional entropic scale Anisotropy hydraulic conductivity

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Clifford deformations of Koszul Frobenius Algebras and Noncommutative Quadrics

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Algebra Colloquium 2024年第1期31卷 63-82页

作者： Jiwei he Yu ye department of Mathematics Hangzhou Normal UniversityHangzhou 311121China School of Mathematical Sciences University of Science and Technology of China Hefei 230026China

A Clifford deformation of a Koszul Frobenius algebra E is a finite dimensional Z_(2)-graded algebra E(θ),which corresponds to a noncommutative quadric hypersurface E^(!)/(z)for some central regular element z∈E_(2)^(!).It turns out that the bounded derived category d^(b)(gr_(Z_(2))E(θ))is equivalent to the stable category of the maximal Cohen-Macaulay modules over E^(!)/(z)provided that E!is *** a consequence,E^(!)/(z)is a noncommutative isolated singularity if and only if the corresponding Clifford deformation E(θ)is a semisimple Z_(2)-graded *** preceding equivalence of triangulated categories also indicates that Clifford deformations of trivial extensions of a Koszul Frobenius algebra are related to Knörrer's periodicity theorem for quadric *** an application,we recover Knörrer's periodicity theorem without using matrix factorizations.

关键词： Koszul Frobenius algebra Clifford deformation noncommutative quadric hypersurface maximal Cohen-Macaulay module

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