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Tailored design of novel Co0-Coδ+dual phase nanoparticles for selective CO2 hydrogenation to ethanol

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Journal of Environmental Sciences 2025年第3期149卷 598-615页

作者： Subhasis das Ganapati d.Yadav department of Chemical Engineering Institute of Chemical TechnologyNathalal Parekh MargMatunga 400019MumbaiIndia

Catalytic hydrogenation of CO_(2)to ethanol is a promising solution to address the greenhouse gas(GHG)emissions,but many current catalysts face efficiency and cost *** based catalysts are frequently examined due to their abundance,cost-efficiency,and effectiveness in the reaction,where managing the Co^(0)to Co^(δ+)ratio is *** this study,we adjusted support nature(Al_(2)O_(3),MgO-MgAl_(2)O_(4),and MgO)and reduction conditions to optimize this balance of Co^(0)to Co^(δ+)sites on the catalyst surface,enhancing ethanol *** selectivity of ethanol reached 17.9%in a continuous flow fixed bed micro-reactor over 20 mol%Co@MgO-MgAl_(2)O_(4)(CoMgAl)catalyst at 270°C and 3.0 MPa,when reduced at 400°C for 8 *** results coupled with activity analysis confirmed that mild reduction condition(400°C,10%H_(2)balance N_(2),8 h)with intermediate metal support interaction favoured the generation of partially reduced Co sites(Co^(δ+)and Co^(0)sites in single atom)over MgO-MgAl_(2)O_(4)surface,which promoted ethanol synthesis by coupling of dissociative(CHx^(∗))/non-dissociative(CHxO^(∗))intermediates,as confirmed by density functional theory ***,the CoMgAl,affordably prepared through the coprecipitation method,offers a potential alternative for CO_(2)hydrogenation to yield valuable chemicals.

关键词： CO_(2)hydrogenation Ethanol Co-based catalysts Metal support ineraction dFT analysis

Biochemical dissection of STAT3 signaling in amyotrophic lateral sclerosis

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Neural Regeneration Research 2025年第11期20卷 3229-3230页

作者： Savina Apolloni Nadia d’Ambrosi department of Biology University of Rome Tor VergataRomeItaly

Amyotrophic lateral sclerosis(ALS)is a progressive neurodegenerative disease characterized by the loss of upper and lower motor neurons,clinically marked by muscle atrophy and *** the clinical course is highly variable,the average time from the onset of symptoms to the need for respiratory support or death is 3-5 *** is the most prevalent motor neuron disease in adults,occurring at a rate of 2 per 100,000 individuals and affecting 5.4 per 100,000 individuals overall.

关键词： STAT3 dissection sclerosis

From Imperfection to Perfection: Advanced 3d Facial Reconstruction Using MICA Models and Self-Supervision Learning

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Computer Modeling in Engineering & Sciences 2025年第2期142卷 1459-1479页

作者： Thinh d.Le duong Q.Nguyen Phuong d.Nguyen H.Nguyen-Xuan CIRTECH Institute HUTECH UniversityHo Chi Minh City72308Viet Nam

Research on reconstructing imperfect faces is a challenging *** this study,we explore a data-driven approach using a pre-trained MICA(MetrIC fAce)model combined with 3d printing to address this *** propose a training strategy that utilizes the pre-trained MICA model and self-supervised learning techniques to improve accuracy and reduce the time needed for 3d facial structure *** results demonstrate high accuracy,evaluated by the geometric loss function and various statistical *** showcase the effectiveness of the approach,we used 3d printing to create a model that covers facial *** findings indicate that our method produces a model that fits well and achieves comprehensive 3d facial *** technique has the potential to aid doctors in treating patients with facial injuries.

关键词： 3d face reconstruction self-supervised learning face defect 3d printed prototypes

Anti-amyloid antibodies in Alzheimer’s disease: what did clinical trials teach us?

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Neural Regeneration Research 2025年第4期20卷 1092-1093页

作者： danko Jeremic Lydia Jiménez-díaz Juan d.Navarro-López NeuroPhysiology&Behavior Lab University of Castilla-La ManchaBiomedical Research Center(CRIB)School of Medicine of Ciudad RealCiudad RealSpain

Although many causes of Alzheimer’s disease(Ad)may exist,both the original amyloid cascade and tau hypotheses posit that abnormal misfolding and accumulation of amyloid-β(Aβ)and tau protein is the central event causing the ***,that conclusion could be only partly true,and there is conflicting evidence about the role of both proteins in Ad,being able to precede and influence one *** researchers argue that these proteins are mere executors rather than primary causes of ***,there have been continuing refinements of both hypotheses,with alternative explanations proposed.Aβand tau proteins may be independently involved in specific neurotoxic pathways;yet there may be other crucial processes going on in early ***,accumulating evidence suggests that Aβand tau act synergistically,rather than additively in disease onset(Jeremic et al.,2021,2023a).

关键词： amyloid Alzheimer additive

Remaking a connection:molecular players involved in post-injury synapse formation

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Neural Regeneration Research 2025年第6期20卷 1719-1720页

作者： diogo Tomé Ramiro d.Almeida iBiMEd-Institute of Biomedicine Department of Medical SciencesUniversity of AveiroAveiroPortugal CNC-Center for Neuroscience and Cell Biology University of CoimbraCoimbraPortugal

Functional recovery from central nervous system(CNS)trauma depends not only on axon regeneration or compensatory sprouting of uninjured fibers but also on the ability of newly grown axons to establish functional synapses with appropriate *** several studies have successfully promoted long-distance axonal regeneration in distinct CNS injury models,none of them have resulted in a viable therapeutic approach for patient recovery.A possible reason may be the lack of new synaptogenesis for reestablishing the circuitry lost after ***,we discuss how our understanding of the mechanisms that instruct synapse formation in the injured nervous system may contribute to the design of new strategies to promote functional restoration in traumatic CNS disorders.

关键词： viable injury instru

Finding the balance: Modifying the cholesterol and steroidal glycoalkaloid synthesis pathway in tomato(Solanum lycopersicum L.) for human health, fruit flavor, and plant defense

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Horticultural Plant Journal 2025年第1期11卷 42-56页

作者： Vincenzo Averello IV Adrian d.Hegeman Changbin Chen department of Horticultural Science University of Minnesota1970 Folwell AvenueSt.PaulMN 55108USA School of Life Sciences Arizona State University427 E Tyler MalTempeAZ 85287USA

Unlike most plants, members of the genus Solanum produce cholesterol and use this as a precursor for steroidal glycoalkaloids. The production of the compounds begins as a branch from brassinosteroid biosynthesis, which produces cholesterol that is further modified to produce steroidal glycoalkaloids. during the cholesterol biosynthesis pathway, genetic engineering could alter the formation of cholesterol from provitamin d3(7-dehydrocholesterol) and produce vitamin d3. Cholesterol is a precursor for many steroidal glycoalkaloids, including a-tomatine and esculeoside A. Alpha-tomatine is consumed by mammals and it can reduce cholesterol content and improve LdL:HdL ratio. When there is a high a-tomatine content, the fruit will have a bitter flavor, which together with other steroidal glycoalkaloids serving as protective and defensive compounds for tomato against insect, fungal, and bacterial pests. These compounds also affect the rhizosphere bacteria by recruiting beneficial bacteria. One of the steroidal glycoalkaloids, esculeoside A increases while fruit ripening. This review focuses on recent studies that uncovered key reactions of the production of cholesterol and steroidal glycoalkaloids in tomato connecting to human health, fruit flavor, and plant defense and the potential application for tomato crop improvement.

关键词： Cholesterol Steroidal glycoalkaloids Tomato Biosynthesis a-tomatine Sterols Terpenoids Plant defense

Treating amyotrophic lateral sclerosis with allogeneic Schwann cell-derived exosomal vesicles: a case report

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Neural Regeneration Research 2025年第4期20卷 1207-1216页

作者： Pascal J.Goldschmidt-Clermont Aisha Khan George Jimsheleishvili Patricia Graham Adriana Brooks Risset Silvera Alexander J.P.Goldschmidt damien d.Pearse W.dalton dietrich Allan d.Levi James d.Guest Miller School of Medicine University of MiamiMiamiFLUSA Stem Cell Institute Miller School of MedicineUniversity of MiamiMiamiFLUSA The Miami Project to Cure Paralysis Miller School of MedicineUniversity of MiamiMiamiFLUSA Alzady International LLC MiamiFLUSA Neurological Surgery Miller School of MedicineUniversity of MiamiMiamiFLUSA

Schwann cells are essential for the maintenance and function of motor neurons,axonal networks,and the neuromuscular *** amyotrophic lateral sclerosis,where motor neuron function is progressively lost,Schwann cell function may also be ***,important signaling and potential trophic activities of Schwann cell-derived exosomal vesicles have been *** case report describes the treatment of a patient with advanced amyotrophic lateral sclerosis using serial intravenous infusions of allogeneic Schwann cell-derived exosomal vesicles,marking,to our knowledge,the first instance of such *** 81-year-old male patient presented with a 1.5-year history of rapidly progressive amyotrophic lateral *** initial diagnosis,the patient underwent a combination of generic riluzole,sodium phenylbutyrate for the treatment of amyotrophic lateral sclerosis,and *** patient volunteered to participate in an FdA-approved single-patient expanded access treatment and received weekly intravenous infusions of allogeneic Schwann cell-derived exosomal vesicles to potentially restore impaired Schwann cell and motor neuron *** confirmed that cultured Schwann cells obtained from the amyotrophic lateral sclerosis patient via sural nerve biopsy appeared impaired(senescent)and that exposure of the patient’s Schwann cells to allogeneic Schwann cell-derived exosomal vesicles,cultured expanded from a cadaver donor improved their growth capacity in *** a period of observation lasting 10 weeks,during which amyotrophic lateral sclerosis Functional Rating Scale-Revised and pulmonary function were regularly monitored,the patient received weekly consecutive infusions of 1.54×1012(×2),and then consecutive infusions of 7.5×1012(×6)allogeneic Schwann cell-derived exosomal vesicles diluted in 40 mL of dulbecco’s phosphate-buffered *** of the infusions were associated with adverse events such as infusion reactions(allergic or otherwise)or

关键词： allogeneic amyotrophic lateral sclerosis exosomes infusion neuromuscular junction Schwann cell

Cyclic loading of marble: Correlating the attenuation of the electric and acoustic activities and highlighting criticality indices in terms of natural time

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International Journal of Mining Science and Technology 2025年第2期35卷 159-174页

作者： Triantis, dimos Stavrakas, Ilias Pasiou, Ermioni d. Kourkoulis, Stavros K. University of West Attica Department of Electrical & Electronics Engineering Electronic Devices and Materials Laboratory Ancient Olive Grove Campus Athens12244 Greece National Technical University of Athens School of Applied Mathematical and Physical Sciences Department of Mechanics Laboratory for Testing and Materials Athens15773 Greece

The attenuation of the acoustic activity in marble specimens under uniaxial compressive loading-unloading loops is quantified in juxtaposition to that of the electric activity. In parallel, the existence of "pre-failure indices" warning about entrance into a critical stage, that of impending fracture, is explored. The acoustic activity is quantified in terms of the normalized number of acoustic hits, their average rate of production and their cumulative energy, and, the cumulative counts and their average rate of change. The electric activity is studied in terms of the pressure stimulated currents and the electric charge released. The analysis revealed that the acoustic and electric activities are linearly correlated to each other, suggesting that they are different manifestations of the same damage mechanisms. In addition, Kaiser's effect, governing the acoustic activity, is found to govern, also, the electric activity. Moreover, it is concluded that entrance into the critical stage is safely predicted by means of a simple criterion, based on the evolution of the average rate of change of the normalized cumulative counts in the natural time domain. These predictions are almost identical with those of the criterion based on the "variance" and the "entropies" of the time series of acoustic events in this domain. © 2025

关键词： Acoustic emissions

Embeddings of Generalised Morrey Smoothness Spaces

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Acta Mathematica Sinica,English Series 2025年第1期41卷 413-456页

作者： dorothee d.Haroske Zhen Liu Susana d.Moura Leszek Skrzypczak Institute of Mathematics Friedrich Schiller University JenaJena 07737Germany University of Coimbra Department of MathematicsCMUCCoimbra 3000-143Portugal Faculty of Mathematics&Computer Science Adam Mickiewicz Universityul.Uniwersytetu Pozna´nskiego 4Pozna´n 61-614Poland

We study embeddings between generalised Triebel–Lizorkin–Morrey spacesε_(ϕ,p,q)^(s)(R^(d))and within the scales of further generalised Morrey smoothness spaces like N_(ϕ,p,q)^(s)(R^(d)),B_(p,q)^(s,ϕ)(R^(d))and F_(p,q)^(s,ϕ)(R^(d)).The latter have been investigated in a recent paper by the first two authors(2023),while the embeddings of the scale N_(ϕ,p,q)^(s)(R^(d))were mainly obtained in a paper of the first and last two authors(2022).Now we concentrate on the characterisation of the spacesε_(ϕ,p,q)^(s)(R^(d)).Our approach requires a wavelet characterisation of those spaces which we establish for the system of daubechies’*** we prove necessary and sufficient conditions for the embeddingε_(ϕ1,p1,q1)^(s1)(R^(d))→ε_(2ϕ2,p2,q2)^(s)(R^(d)).We can also provide some almost final answer to the question whenε_(ϕ,p,q)^(s)(R^(d))is embedded into C(R^(d)),complementing our recent findings in case of N_(ϕ,p,q)^(s)(R^(d)).

关键词： Generalised Morrey spaces generalised Besov-type space generalised Triebel–Lizorkintype space generalised Besov–Morrey space generalised Triebel-Lizorkin-Morrey space embeddings wavelet decompositions