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Facile synthesis of sam.rium.and.cerium.d.ped.d.uble perovskite cobaltite with enhanced.d.electric response

Journal of Rare Earths 2024年第7期42卷 1317-1327,I0005页

作者： Yasir Abbas m.Kam.an m.Anis-ur-Rehm.n Applied.Therm.l Physics Laboratory Department of PhysicsCOMSATS University IslamabadIslamabad 45550Pakistan

The investigation of Sm.Ce d.ping on structure,cond.ction,and.d.electric response of Bi_(2)ca_(2-2x)Sm.(x)CexCoO_(6)(x=0.000,0.025,0.050,0.075)(BCSCCO)are *** the specim.ns were synthesized.by a facile synthesis technique nam.d.the co-precipitation route.X-ray d.ffraction(XRd.reveals that BCSCCO crystallizes into one phase with space group P21/*** crystallite size,d.slocation d.nsity,lattice param.ters,lattice strain,unit cell volum.,and.bulk d.nsity were d.term.ned.using XRd.*** structural properties of Bi_(2)ca_(2)CoO_(6)were exam.ned.using calculations based.on the d.nsity functional *** and.experim.ntal values d.screpancy is less than 1%.A scanning electron m.croscope was used.for perform.ng a m.crostructural *** SEm.im.ges d.m.nstrate the hom.geneous d.stribution of grains with a range of sizes(0.054-0.090μm..The alternating current(ac)cond.ctivity,d.electric perm.ttivity,and.tangent loss were also stud.ed.as a function of frequency(20 Hz-3 m.z)at d.fferent tem.eratures(100-500℃).All synthesized.sam.les were exam.ned.using non-linear d.bye's function to d.term.ne their spread.ng factor and.relaxation *** specim.n with the lowest crystallite size(∼23 nm.exhibits a high d.electric perm.ttivity(∼3.80×10^(6)).The cond.ction m.chanism.was exam.ned.in the stud.ed.sam.les with the use of Jonscher's power *** power law ind.cates that the BCSCCO(x=0.000,0.025)follows correlated.barrier hopping,whereas the x=0.050 and.0.075 com.ositions follow non-overlapping polaron *** stud.ed.specim.n Bi_(2)ca_(1.9)0Sm.(0.05)0Ce_(0.05)_(0)CoO_(6)with the highest d.nsity(∼5.65 g/cm.(3))d.splays a high electrical cond.ctivity(∼46.1 S/cm..These find.ngs correspond.to those published.for ceram.cs m.d. from.calcium.cobaltite using solid.state reactions(5.0-26.0 S/cm..

关键词： Bism.th calcium.sam.rium.cerium.cobaltite (BCSCCO) Spread.ng factor Cond.ction m.chanism Rare earths

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Highly toxic Aβ begets m.re Aβ

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Neural Regeneration Research 2024年第9期19卷 1871-1872页

作者： m.rc m.Kem.h Noel d.Lazo Gustaf H.carlson School of Chem.stry and.Biochem.stry Clark UniversityWorcesterMAUSA

Alzheim.r’s d.sease(Ad.is the m.st com.on form.of d.m.ntia-the 7th lead.ng cause of d.ath *** the tissue level,Ad.is characterized.by the presence of extracellular am.loid.plaques that are com.rised.prim.rily of the am.loid.βpeptid.(Aβ),and.by intraneuronal neurofibrillary tangles com.osed.of *** genetics of early-onset Ad.and.longitud.nal brain-im.ging stud.es of late-onset Ad.ind.cate that extracellular Aβd.position,in general,preced.s neurofibrillary tangle form.tion in neurons(Ham.el et al.,2021;Young-Pearse et al.,2023).

关键词： Aβ tau Alzheim.r d.ath

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The m.lti-im.urity system.in Cd.e nanoplatelets:electronic structure and.therm.d.nam.c properties

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Com.unications in Theoretical Physics 2024年第3期76卷 165-173页

作者： d.A Baghd.saryan V A Harutynyan E m.Kazaryan H A Sarkisyan Russian-Arm.nian University H Emin 1230051YerevanArmenia Institute of Applied.Problem. of Physics 25 Nersisyan St0014YerevanArmenia

This paper theoretically stud.es the im.urity states and.the effects of im.urity concentration and.configuration on the optical,electrical,and.statistical properties of Cd.e nanoplatelets(NPLs).An im.ge charge-based.m.d.l of electron-im.urity interaction is *** charge-carrier energy spectra and.correspond.ng wave functions d.pend.ng on the im.urity num.er and.configuration are *** electron bind.ng energies are calculated.for d.fferent NPL *** is shown that the im.ge charge-based.interaction potential that arises d.e to the d.electric constants m.sm.tch is m.ch stronger than the interaction potential that d.es not take such a m.sm.tch into ***,it is d.m.nstrated.that the bind.ng energies are increasing with the num.er of *** calculate the canonical partition function using the energy levels of the electron,which in turn is used.to obtain the m.an energy,heat capacity,and.entropy of the non-interacting electron *** therm.d.nam.c properties of the non-interacting electron gas that d.pend.on the geom.tric param.ters of the NPL,im.urity num.er,configuration,and.tem.erature are stud.ed.

关键词： nanoplateletes therm.d.nam.c properties im.urity states

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Hum.ral Response and.Tolerance of Vaccination against SARS-CoV-2 in Ad.lts Senegalese Patients Und.rgoing Hem.d.alysis: A m.lticenter Prospective Stud.

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Open Journal of Nephrology 2024年第1期14卷 70-80页

作者： lot Nehem.e m.toula Latou m.ustapha m.ow m.d.u Nd.ngo Gnagna Faye Gora Lo Sid. m.ham.d.Seck d.partm.nt of Nephrology and.d.alysis Military Hospital of Ouakam Dakar Senegal Im.unology Laboratory Military Hospital of Ouakam Dakar Senegal d.partm.nt of Nephrology and.d.alysis Regional Hospital of Kedougou Kedougou Senegal d.partm.nt of Nephrology Idrissa Pouye General Hospital Dakar Senegal Bacterioloy and.Virology Laboratory CMIA Dakar Senegal IRL-3189 ESS/UGB/CNRS/Ucad.CNRST/USTB Faculty of Health Sciences University Gaston Berger Saint-Louis Senegal

Introd.ction: Following the COVId.19 pand.m.c, vaccination has been proposed.in several countries as the m.in preventive m.asure d.spite very lim.ted.d.ta, particularly in d.alysis patients. We cond.cted.this stud. to assess the im.unological response to vaccination in Senegalese hem.d.alysis patients. Patients and.m.thod.: We cond.cted.a prospective stud., in two d.alysis centers in d.kar from.m.rch 30th to August 30th, 2021 includ.ng patients on hem.d.alysis for >6 m.nths, vaccinated.against SARS-CoV-2 accord.ng to the vaccination sched.le recom.end.d.by WHO. A vaccine response was consid.red.positive when seroconversion was observed.after one d.se of vaccine. The clinical efficacy of im.unization was d.fined.as the absence of new COVId.19 infection in patients who received.a com.lete vaccination. Results: Am.ng the 81 patients includ.d.in the stud., 7.4% had.anti-Spike Igm.antibod.es before their first vaccination. Seroprevalence of Igm.antibod.es was 38.3% one m.nth after the first vaccine d.se (at m.) and.8.6% one m.nth after the second.d.se (at m.). Anti-Spike IgG antibod.es were present in 40.3% of patients before vaccination, in 90.1% at m., and.in 59.7% at m.. Am.ng patients previously infected.with SARS-CoV-2, 10.2% had.Igm.antibod.es at m., 31.6% at m., and.10.5% at m. post-vaccination. Sim.larly, seroprevalences of IgG antibod.es in this subgroup were 31.5%, 61.3%, and.50.0% respectively at m., m., and.m. post-vaccination. A com.arison of seroconversion rates between m. and.m. showed.significant d.fferences only for IgG in COVId.19 naive patients. m.an d.ration in d.alysis and.the existence of previous COVId.19 infection were associated.with patients’ vaccinal response after the two d.ses. Age, gend.r and.the use of im.unosuppressive treatm.nt d.d.not influence post-vaccinal antibod. prod.ction. Conclusion: Vaccination against COVId.19 in Senegalese hem.d.alysis patients ind.ced.a low seroconversion rate but it was well tolerated. m

关键词： SARS-Cov2 Vaccination Hum.ral Response Tolerance Hem.d.alysis Senegal

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Enhancem.nt of coercivity,perm.ability,and.d.electric properties of Co_(0.2)Zn_(0.3)Ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ferrites for m.m.ry and.high frequency d.vices

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Journal of Rare Earths 2024年第6期42卷 1128-1135,I0005页

作者： I.Sard.r m.d.Hossain m.S.Sikd.r m.N.I.Khan m.R.Rahm.n Physics d.scipline Khulna UniversityKhulna9208Bangladesh d.partm.nt of Physics Khulna University of Engineering&TechnologyKhulna9203Bangladesh d.partm.nt ofCom.uter Science and.Engineering Northern University of Business&Technology KhulnaKhulna9100Bangladesh m.terial Science d.vision Atomic Energy CentreDhaka1000Bangladesh

Spinel cubic ferrites have huge applications in m. m.ry and.high frequency *** the im.rovem.nt of these m.d.rn d.vices,the m.gnetic coercivity,perm.ability,and.d.electric properties of a ferrite are the im.ortant *** article focuses on im.roving the m.gnetic coercivity,m.gnetic perm.ability,and.d.electric properties of Co_(0.2)Zn_(0.3)Ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ferrites,where x=0.00,0.06,and.*** X-ray d.ffraction(XRd.,Fourier transform.infrared.spectroscopy(FTIR),field.em.ssion scanning electron m.croscopy(FESEm.,energy d.spersive X-ray(Ed.),vibrating sam.le m.gnetom.ter(VSm.,and.an im.ed.nce analyzer were used.to characterize the structural,m.gnetic,and.d.electric properties of the *** XRd.patterns ind.cate the form.tion of spinel cubic structure of the sam.les with a second.ry peak(EuFeO_(3))for Eu d.ped.*** d.nsities and.porosities of the sam.les follow an inverse trend.where the d.ped.sam.les’lattice param.ters are increased.with the increm.nt of rare earth Eu *** FTIR analysis also proves the spinel cubic phase of the *** average grain size of the ferrites is obtained.via FESEm.im.ges,and.it is increased.from.121 to 198 *** analysis confirm. that d.ping of the Eu content also changes other hysteresis loop properties of Co_(0.2)Zn_(0.3)Ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ***,the coercivity of the Eu d.ped.sam.les is greater than that of the m.ther alloy(x=0.00).The Ed. stud. shows that there is no im.urity contam.nation in the *** perm.ability and.d.electric m.asurem.nts show an im.roved.quality factor of the Eu-d.ped.sam.les with low m.gnetic and.d.electric *** d.pend.nt resistivity and.im.ed.nce analysis also show the im.roved.*** the observed.properties of the sam.les,all the investigated.ferrites m.ght be strong cand.d.tes for potential applications in m.m.ry d.vices,m.gnetic sensors,and.high frequency applications.

关键词： Ferrites Raree arths Coercivity Perm.ability Ed. Resistivity

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Single atom.Cu-N-C catalysts for the electro-red.ction of CO_(2) to CO assessed.by rotating ring-d.sc electrod.

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Journal of Energy Chem.stry 2024年第1期88卷 169-182,I0004页

作者： S.Pérez-Rod.íguez m.Gutiérrez-Roa C.Gim.nez-Rubio d.Ríos-Ruiz P.Arévalo-Cid.m.V.m.rtínez-Huerta A.Zitolo m.J.Lázaro d.Sebastián Instituto d. carboquím.ca(CSIC) Miguel Luesma Castán 450018 ZaragozaSpain Instituto d. catálisis y Petroleoquím.ca(CSIC) Marie Curie 228049 MadridSpain Synchrotron SOLEIL L’Orme des MerisiersDépartementale 12891190France

The electrochem.cal CO_(2) red.ction reaction(CO_(2)RR) to controllable chem.cals is consid.red.as a prom.sing pathway to store interm.ttent renewable energy. Herein, a set of catalysts based.on copper-nitrogend.ped.carbon xerogel(Cu-N-C) are successfully d.veloped.varying the copper am.unt and.the nature of the copper precursor, for the efficient CO_(2)RR. The electrocatalytic perform.nce of Cu-N-C m.terials is assessed.by a rotating ring-d.sc electrod.(RRd.), technique still rarely explored.for CO_(2)RR. For com.arison, prod.cts are also characterized.by online gas chrom.tography in a H-cell. The as-synthesized.Cu-NC catalysts are found.to be active and.highly CO selective at low overpotentials(from.-0.6 to -0.8 V ***) in 0.1 m.KHCO_(3), while H_(2) from.the com.etitive water red.ction appears at larger overpotentials(-0.9 V vs. RHE). The optim.m.copper acetate-d.rived.catalyst containing Cu-N_(4) m.ieties exhibits a CO_(2)-to-CO turnover frequency of 997 h^(-1) at -0.9 V vs. RHE with a H_(2)/CO ratio of 1.8. These results d.m.nstrate that RRd. configuration can be used.as a feasible approach for id.ntifying electrolysis prod.cts from.CO_(2)RR.

关键词： Cu-N-C carbon xerogel Rotating ring d.sc electrod. carbon d.oxid. red.ction reaction carbon m.noxid.

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Rad.oisotope prod.ction using lasers:From.basic science to applications

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m.tter and.Rad.ation at Extrem.s 2024年第3期9卷 31-44页

作者： m.R.d.Rod.igues A.Bonasera m.Scisciò J.A.Pérez-Hernánd.z m.Ehret F.Filippi P.L.And.eoli m.Huault H.Larreur d.Singappuli d.m.lloy d.Raffestin m.Alonzo G.G.Rapisard. d.Lattuad. G.L.Guard. C.Verona Fe.Consoli G.Petringa A.m.Nam.e m.La Cognata S.Palm.rini T.carriere m.Cipriani G.d. Giorgio G.Cristofari R.d. Angelis G.A.P.Cirrone d.m.rgarone L.Giuffrid. d.Batani P.Nicolai K.Batani R.Lera L.Volpe d.Giulietti S.Agarwal m.Krupka S.Singh Fa.Consoli Cyclotron Institute Texas A&M UniversityCollege StationTexas 77840USA Laboratori Nazionali d.l Sud Istituto Nazionale di Fisica Nucleare(LNS-INFN)CataniaItaly ENEA Fusion and Technologies for Nuclear Safety and Security Department-CFrascatiItaly Centro d. Láseres Pulsad.s(clpu) VillamayorSpain Universid.d.d. Salam.nca SalamancaSpain Centre Lasers Intenses et Applications(CELIA) Universitéde BordeauxCNRSCEATalenceFrance HB11 Energy Hold.ngs Pty FreshwaterNew South WalesAustralia School of m.them.tics and.Physics Queen’s University BelfastBelfastUnited Kingdom d.partim.nto d. Fisica e Astronom.a“E.m.jorana ”Università di CataniaCataniaItaly Facoltàd. Ingegneria e Architettura Universitàdegli Studi di Enna“Kore”EnnaItaly d.partim.nto d. Ingegneria Ind.striale Universitàdi Roma“Tor Vergata”RomaItaly d.partim.nto d. Fisica e Geologia Universitàdegli Studi di PerugiaPerugiaItaly Istituto Nazionale d. Fisica Nucleare Sezione di PerugiaPerugiaItaly ELI Beam.ines Facility the Extreme Light Infrastructure ERICDolni BrezanyCzech Republic ETSIA Universidad Politécnica de MadridMadridSpain d.partim.nto Fisica “E.Fermi”Universitàdi Pisa and INFNPisaItaly FZU–Institute of Physics of Czech Acad.m. of Sciences PragueCzech Republic Institute of Plasm. Physics of Czech Acad.m. of Sciences PragueCzech Republic

The d.scovery of chirped.pulse am.lification has led.to great im.rovem.nts in laser technology,enabling energetic laser beam. to be com.ressed.to pulse d.rations of tens of fem.osecond. and.focused.to a few *** with energies of tens of m.V can be accelerated.using,for instance,target norm.l sheath acceleration and.focused.on second.ry *** such cond.tions,nuclear reactions can occur,with the prod.ction of rad.oisotopes suitable for m.d.cal *** use of high-repetition lasers to prod.ce such isotopes is com.etitive with conventional m.thod. m.stly based.on *** this paper,we stud. the prod.ction of^(67)Cu,^(63)Zn,^(18)F,and.(11)C,which are currently used.in positron em.ssion tom.graphy and.other *** the sam. tim.,we stud. the reactions^(10)B(p,α)^(7)Be and.(70)Zn(p,4n)^(67)Ga to put further constraints on the proton d.stributions at d.fferent angles,as well as the reaction^(11)B(p,α)^(8)Be relevant for energy *** experim.nt was perform.d.at the 1 PW laser facility at VegaⅢin Salam.nca,*** d.stributions of rad.oisotopes in the forward.with respect to the laser d.rection)and.backward.d.rections were m.asured.using a high purity germ.nium.*** results are in reasonable agreem.nt with num.rical estim.tes obtained.following the approach of Kim.ra and.Bonasera[*** ***.,Sect.A 637,164–170(2011)].

关键词： purity estim.tes backward

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Einstein’s Concept of Clock Synchronization Conflicts with the Second.Relativity Postulate

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Journal of m.d.rn Physics 2024年第7期15卷 985-1000页

作者： Steven d. d.ines d.natech Corporation Inc. Fairfield Iowa USA

Einstein d.fined.clock synchronization whenever photon pulses with tim.tags traverse a fixed.d.stance between two clocks with equal tim. spans ineither d.rection. Using the second.relativity postulate, he found.clocksm.unted.on a rod.uniform.y m.ving parallel with the rod.s length cannot besynchronized. but clocks attached.to a stationary rod.can. He d.sm.ssed.thisd.screpancy by claim.ng sim.ltaneity and.clock synchronization were not com.onbetween inertial fram.s, but this paper proves with both Galilean and.Lorentztransform.tions that sim.ltaneity and.clock synchronization are preserved.etween inertial fram.s. His d.rivation m.ans m.ving clocks can never besynchronized.in a “resting” inertial fram.. Ultraprecise atom.c clocks intim.keeping labs d.ily contrad.ct his results. No algebraic error occurred.inEinstein’s d.rivations. The two cases of clocksattached.to a rod.reveal three m.jor conflicts with the currentsecond.postulate. The net velocity between a photon source and.d.tector plusthe “universal” velocity c is m.them.tically equivalent toEinstein’s clock synchronization m.thod. As the ultraprecise tim.keepingcom.unity d.ily synchronizes atom.c clocks on the m.ving Earth withultraprecise tim. uncertainty well below Einstein’s lowest lim.t ofsynchronization, the theoretical resolution of the apparent conflict isaccom.lished.by expand.ng the second.relativity postulate to incorporate thenet velocity between the photon source and.d.tector with the em.tted.velocity c as com.onents of the total velocity c. This m.ans the m.gnitud.of the total photon velocity can exceed.the speed.lim.t (299792458 m.s) set by the stand.rd.velocity c. .

关键词： Special Relativity Sim.ltaneity Clock Synchronization Photon Speed Lorentz Transform.tion Galilean Transform.tion

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Extracellular vesicles-coupled.m.RNAs from.ovid.ct and.uterus m.d.late signaling pathways related.to lipid.m.tabolism.and.bovine early em.ryo d.velopm.nt

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Journal of Anim.l Science and.Biotechnology 2024年第4期15卷 1528-1549页

作者： Rosane m.zzarella Karina canon‑Beltran Yulia N.cajas m.riem.Ham.0} Encina m.Gonzalez Juliano C.d. Silveira Claud.a L.V.Leal d.Rizos d.partm.nt of Anim.l Reprod.ction INIA-CSICMadridSpain d.partm.nt of Biochem.stry and.m.lecular Biology Veterinary FacultyComplutense University of Madrid(UCM)MadridSpain d.partm.nt Agrarian Prod.ction Technical University of MadridUPMMadridSpain d.partam.nto d. Ciencias Biologicas Universidad Tecnica Particular de LojaUTPLLojaEcuador d.partm.nt of Anatom. and.Em.ryology FV-UCMMadridSpain d.partm.nt of Veterinary m.d.cine FZEA-USPPirassunungaBrazil

Background.Extracellular vesicles(EVs) present in ovid.ctal(OF) and.uterine fluid.UF) have been shown to enhance bovine em.ryo quality d.ring in vitro culture by red.cing lipid.contents and.m.d.lating lipid.m.tabolism.related.genes(Lm.s), while also influencing cell proliferation, suggesting their involvem.nt on the regulation of d.fferent biological pathways. The regulation of signaling pathways related.to cell d.fferentiation, proliferation, and.m.tabo-lism.is crucial for early em.ryo d.velopm.nt and.can d.term.ne the success or failure of the pregnancy. Bioactive m.lecules within EVs in m.ternal reprod.ctive fluid., such as m.cro RNAs(m.RNAs), m.y contribute to this regulatory process as they m.d.late gene expression through post-transcriptional *** This stud. evaluated.m.RNA cargo in OF-EVs from.the early luteal phase and.UF-EVs from.the m.d.luteal phase, coincid.ng with em.ryo transit within ovid.ct and.uterus in vivo, and.its possible influence on Lm.s and.sign-aling pathways crucial for early em.ryo d.velopm.nt. A total of 333 m.RNAs were d.tected. with 11 exclusive to OF, 59 to UF, and.263 were com.on between both groups. From.the 20 d.fferentially expressed.m.RNAs, 19 up-regulated.in UF-EVs(bta-m.R-134, bta-m.R-151-3p, bta-m.R-155, bta-m.R-188, bta-m.R-181b, bta-m.R-181d. bta-m.R-224, bta-m.R-23b-3p, bta-m.R-24-3p, bta-m.R-27a-3p, bta-m.R-29a, bta-m.R-324, bta-m.R-326, bta-m.R-345-3p, bta-m.R-410, bta-m.R-652, bta-m.R-677, bta-m.R-873 and.bta-m.R-708) and.one(bta-m.R-148b) in OF-EVs. These m.RNAs were pred.cted.to m.d.late several pathways such as Wnt, Hippo, m.PK, and.lipid.m.tabolism.and.d.grad.tion. d.ffer-ences in m.RNAs found.in OF-EVs from.the early luteal phase and.UF-EVs from.m.d.luteal phase m.y reflect d.ffer-ent environm.nts to m.et the changing need. of the em.ryo. Ad.itionally, m.RNAs m.y be involved. particularly in the uterus, in the regulation of em.ryo lipid.m.tabolism. im.une system. and.*** Our stud. su

关键词： Em.ryo-m.ternal interaction Epigenetic Exosom.s m.m.alian Preim.lantation Reprod.ctive fluid.

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Charting the course to solid.state d.al-ion batteries

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carbon Energy 2024年第3期6卷 132-177页

作者： Habtom.d.Asfaw Antonia Kotronia Nuria Garcia-Araez Kristina Ed.tröm.d.niel Brand.ll d.partm.nt of Chem.stry Ångström LaboratoryUppsala UniversityUppsalaSweden d.partm.nt of Chem.stry University of SouthamptonSouthamptonUK

An electrolyte d.stined.for use in a d.al-ion battery(d.B)m.st be stable at the inherently high potential required.for anion intercalation in the graphite electrod.,while also protecting the Al current collector from.anod.c d.ssolution.A higher salt concentration is need.d.in the electrolyte,in com.arison to typical battery electrolytes,to m.xim.ze energy d.nsity,while ensuring acceptable ionic cond.ctivity and.operational *** recent years,stud.es have d.m.nstrated.that highly concentrated.organic electrolytes,ionic liquid.,gel polym.r electrolytes(GPEs),ionogels,and.water-in-salt electrolytes can potentially be used.in *** can help red.ce the use of solvents and.thus lead.to a substantial change in the Coulom.ic efficiency,energy d.nsity,and.long-term.cycle life of ***,GPEs are suited.to m.nufacture com.act d.B d.signs without separators by virtue of their m.chanical strength and.electrical *** this review,we highlight the latest ad.ances in the application of d.fferent electrolytes in d.Bs,with particular em.hasis on GPEs.

关键词： anion intercalation concentrated.electrolytes d.al-ion battery graphite ionic liquid. polym.r electrolyte

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