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Chinese Chemical Letters 2025年第1期36卷 6-7页

作者： Qiyan wu Qing Li State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The continuous combustion of unsustainable carbon-based fossil fuels has dramatically accelerated the increase in carbon dioxide(CO_(2))concentration in the atmosphere(from approximately278.3 ppm in 1750 to 417.9 ppm in 2023),which would exacerbate environmental problems such as greenhouse effect[1].The effective electrosynthesis of high value-added multi-carbon(C_(2+))chemicals(e.g.,ethanol,ethylene)from CO_(2) reduction reaction(CO_(2)RR)is a promising strategy to mitigate these environmental issues mentioned above but remains highly challenging due to the competition of hydrogen evolution reaction(HER)and low selectivity of target products.

关键词： intermetallic alloy carbon

Sex-dependent alterations in extracellular vesicles linking chronic spinal cord injury to brain neuroinflammation and neurodegeneration

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Neural Regeneration Research 2025年第2期20卷 483-484页

作者： Yun Li Junfang wu Department of Anesthesiology&Shock Trauma and Anesthesiology Research(STAR)CenterUniversity of Maryland School of MedicineBaltimoreMDUSA

Traumatic spinal cord injury(SCI)is a devastating exogenous injury with long-lasting consequences and a leading cause of death and disability *** in assistive technology,rehabilitative interventions,and the ability to identify and intervene in secondary conditions have significantly increased the long-term survival rate of SCI patients,with some people even living well into their seventh or eighth *** survival changes have led neurotrauma researchers to examine how SCI interacts with brain *** health and epidemiological data showed that patients with long-term SCI can have a lower life expectancy and quality of life,along with a higher risk of comorbidities and complications.

关键词： alterations inflammation injury

A high maneuvering motion strategy and stable control method for tandem twin-rotor aerial-aquatic vehicles near the water surface

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Defence Technology(防务技术) 2025年第2期44卷 206-220页

作者： Sifan wu Maosen Shao Sihuan wu Zhilin He Hui Wang Jinxiu Zhang Yuan Liu School of Aeronautics and Astronautics Sun Yat-sen UniversityShenzhen518107China Southern Marine Science and Engineering Guangdong Laboratory Zhuhai519000China

The maneuverability and stealth of aerial-aquatic vehicles(AAVs)is of significant importance for future integrated air-sea combat *** improve the maneuverability and stealth of AAVs near the water surface,this paper proposed a high-maneuverability skipping motion strategy for the tandem twin-rotor AAV,inspired by the motion behavior of the flying fish to avoid aquatic and aerial predators near the water *** novel tandem twin-rotor AAV was employed as the research subject and a strategybased ADRC control method for validation,comparing it with a strategy-based PID control *** results indicate that both control methods enable the designed AAV to achieve high stealth and maneuverability near the water surface with robust control *** strategy-based ADRC control method exhibits a certain advantage in controlling height,pitch angle,and reducing impact *** motion strategy will offer an inspiring approach for the practical application of AAVs to some extent.

关键词： Tandem twin-rotor Aerial-aquatic vehicle High maneuvering motion strategy Active disturbance rejection controller Skipping on water surface

Dynamic damage characteristics and control mechanism of rocks anchored by constant resistance and energy absorption material

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International Journal of Mining Science and Technology 2025年第1期35卷 57-67页

作者： Bei Jiang Kunbo wu Qi Wang Yetai Wang Wenrui wu Yaoxia Feng Yanbo Zhang State Key Laboratory for Tunnel Engineering China University of Mining&Technology-BeijingBeijing 100083China State Key Laboratory of Explosion Science and Safety Protection Beijing Institute of TechnologyBeijing 100081China Collaborative Innovation Center of Green Development and Ecological Restoration of Mineral Resources North China University of Science and TechnologyTangshan 063210China

With resource exploitation and engineering construction gradually going deeper,the surrounding rock dynamic disaster becomes frequent and *** anchorage support is a common control method of surrounding rock in underground *** study the dynamic damage characteristics of anchored rock and the energy absorption control mechanism of dynamic disasters,a new type of constant resistance and energy absorption(CREA)material with high strength,high elongation and high energy absorption characteristics is developed.A contrast test of rockbursts in anchored rock with different support materials is *** test results show that the surface damage rates and energy release degree of anchored rock with common bolt(CB)and CREA are lower than those of unanchored rock,*** total energy,average energy and maximum energy released by CREA anchored rock are 30.9%,94.3%and 84.4%lower than those of CB anchored *** with unanchored rock,the rockburst peak stress in the CREA anchored rock is increased by 39.9%,and the rockburst time is delayed by 53.2%.Based on the rockburst energy calculation model,the evolution law of rockburst peak stress and energy release is *** control mechanism of CREA support units on rock dynamic failure is clarified.

关键词： Constant resistance and energy absorption Anchored rock Rockburst Peak stress Control mechanism

Potassium-modified carbon nitride photocatalyzed-aminoacylation of N–sulfonyl ketimines

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Chinese Chemical Letters 2025年第2期36卷 406-411页

作者： Cailing wu Shaojie wu Qifei Huang Kai Sun Xianqiang Huang Jianji Wang Bing Yu Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals Key Laboratory of Green Chemical Media and ReactionsMinistry of Education School of Chemistry and Chemical Engineering Henan Normal University College of Chemistry Zhengzhou University School of Chemistry & Chemical Engineering Liaocheng University

The development of innovative and sustainable catalytic strategies for organic synthesis is a pivotal aspect of advancing material science and chemical *** research presents a new catalytic method for the aminoacylation of N–sulfonyl ketimines by utilizing a potassium-doped graphite-like carbon nitride （g-C3N4） *** method not only enhances the catalytic efficiency and broadens the light absorption spectrum of g-C3N4but also significantly reduces the recombination rate of electronhole pairs,thereby increasing the reaction yield and ***,our approach facilitates the synthesis of aminoacylated N-heterocycles,expanding the applicability of potassium-modified g-C3N4in photocatalytic organic synthesis.A notable accomplishment of this study is the unprecedented generation of carbamoyl radicals via heterogeneous photocatalysis,which can be easily recycled after *** advancement highlights the capability of potassium-doped g-C3N4（namely K-CN） as an advanced heterogeneous photocatalyst for the formation of complex organic compounds.

关键词： Amides Aminoacylation K+-modified carbon nitride Oxamic acids Photocatalysis

Enhancement of weathered crust elution-deposited rare earth ores leaching process with PQ-10 addition

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Journal of Rare Earths 2025年第1期43卷 180-190,I0007页

作者： Aoyang Sha Huifang Yang Zhengyan He Zhigao Xu Chenjie wu Ming wu Ru'an Chi Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education Key Laboratory of Resources Conversion and Pollution Control of the State Ethnic Affairs Commission&Hubei Key Laboratory of Catalysis and Materials ScienceCollege of Resources and Environmental ScienceSouth-Central Minzu UniversityWuhan430074China Key Laboratory for Green Chemical Process of Ministry of Education School of Resources&Safety EngineeringWuhan Institute of TechnologyWuhan 430073China

To solve the problems of the long development period,low mass transfer efficiency and high impurity conte nt in the in-situ leaching process of weathe red crust elution-deposited rare earth ores(WCE-DREO),cationic hydroxyethyl cellulose(PQ-10)was composited with conventional leaching agent ammonium sulfate((NH_(4))_(2)SO_(4))to form a novel composite leaching *** effects of PQ-10 concentration,leaching temperature and leaching flow rate of the composite leaching agent on the leaching kinetics and mass transfer processes of rare earth(RE)and aluminum(Al)were *** to the single leaching agent(NH_(4))_(2)SO_(4),the composite leaching agent(2 wt%(NH_(4))_(2)SO_(4)+0.02 wt%PQ-10)can reduce the RE leaching equilibrium time from 465 to 130 min and increase the RE leaching efficiency and decrease the Al leaching *** also facilitates the leaching process of WCE-DREO by increasing the peak concentrations of RE and Al,reducing the theoretical tower plate height(HETP)and improving the leaching mass transfer *** is indicated that PQ-10 can promote the leaching of *** leaching process of the composite leaching system conforms to the diffusion kinetic control *** the PQ-10 concentration is in the range of 0.005 wt%-0.020 wt%,the reaction orders of RE and Al are 0.73 and 0.54,respectively,which shows a positive effect on the leaching velocity;when the PQ-10 concentration is in the range of 0.030 wt%-0.060 wt%,the reaction orders of RE and Al are-1.16 and-0.75,respectively,which show a negative effect on the leaching *** the range of 10-50℃,the apparent activation energies of RE and Al are 15.02 and 17.31 kJ/mol,respectively,and the higher the leaching temperature,the smaller the HETP and the higher the leaching velocity and mass transfer *** increase in leaching flow rate contributes to the increase in the longitudinal diffusion velocity of the leaching agent within WCE-DREO,causing a shorter time for RE

关键词： Cationic hydroxyethyl cellulose Weathered crust elution-deposited rare earthores Leaching Novel compositeagent

PltcRB:a practical distributed randomness beacon with optimal amortized communication complexity

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Science China(Information Sciences) 2025年第2期68卷 269-284页

作者： Zheyi wu Haolin LIU Lei WANG School of Electronic Information and Electrical Engineering Shanghai Jiao Tong University

The distributed randomness beacon(DRB) is a crucial tool for continuously generating unpredictable, bias-resistant,and publicly verifiable random numbers on a regular basis. This is particularly useful for applications such as lotteries, electronic voting, and cryptographic parameter generation. However, existing studies either require complex communication or rely on a public bulletin board to meet security requirements. This brings a performance bottleneck when dealing with a large number of participants. This paper introduces a novel DRB protocol PltcRB based on timed commitments, eliminating the need for a public bulletin board. Our approach achieves optimal communication complexity of O(n) while maintaining the desired properties of a DRB protocol. The computation complexity is also O(n) when n is larger than the security parameter κ. These results demonstrate the practicality and performance of PltcRB, supported by our experimental analysis under various configurations.

关键词： timed commitment randomness beacon random number optimal communication complexity permissionlessłinebreak setting

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Accelerated warming of High Mountain Asia predicted at multiple years ahead

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Science Bulletin 2025年第3期70卷 419-428页

作者： Shuai Hu Tianjun Zhou Bo wu Key Laboratory of Earth System Numerical Modeling and Application Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China University of the Chinese Academy of Sciences Beijing 100049China

High-Mountain Asia(HMA)is an important source of freshwater since it holds the largest reservoir of frozen water outside the polar *** feeds ten great rivers,ultimately supporting more than 2 billion ***,the threat of accelerated glacier melt,which is a consequence of unprecedented global warming since the early 1950s,threatens water resources in the surrounding *** predictions of the near-term temperature change and synergistic mass loss of glaciers are essential but challenging to implement because of the impacts of internal climate ***,based on large ensembles of state-of-the-art decadal climate prediction experiments,we provide evidence that the internally generated surface air temperature variations in HMA can be predicted multiple years in advance,and the model initialization has robust added value to the decadal prediction ***-time decadal forecasts suggest that the HMA will experience accelerated warming in 2025-2032,where the surface warming will increase by 0.98°C(0.67 to 1.33°C;5%to 95%range)relative to the reference period 1991-2020,which is equivalent to 1.75 times the observed warming during *** decadal predictability originates from extratropical Pacific decadal variability modes,which modulate the convective heating in the tropical Pacific and influence HMA via the eastward-propagating atmospheric Kelvin *** warming in the coming decade will likely increase the shrinkage of the glacier volume over the HMA by 1.4%.This change poses unprecedented challenges,including potential water scarcity,ecosystem disruption,and increased risk of natural disasters,to HMA and surrounding regions.

关键词： Decadal prediction High Mountain Asia Surface air temperature Pacific decadal variabilities Glacier

Quantum convolution inequalities on Frobenius von Neumann algebras

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Science China Mathematics 2025年第3期68卷 615-636页

作者： Linzhe Huang Zhengwei Liu Jinsong wu Beijing Institute of Mathematical Sciences and Applications Yau Mathematical Sciences Center and Department of Mathematics Tsinghua University

In this paper, we introduce Frobenius von Neumann algebras and study quantum convolution inequalities. In this framework, we unify quantum Young's inequality on quantum symmetries such as subfactors,and fusion bi-algebras studied in quantum Fourier analysis. Moreover, we prove quantum entropic convolution inequalities and characterize the extremizers in the subfactor case. We also prove quantum smooth entropic convolution inequalities. We obtain the positivity of comultiplications of subfactor planar algebras, which is stronger than the quantum Schur product theorem. All these inequalities provide analytic obstructions of unitary categorification of fusion rings stronger than the Schur product criterion.

关键词： Frobenius von Neumann algebra quantum Young's inequality quantum entropic convolution inequality unitary categorification

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Mechanisms behind the surprising observation of supra-thermal ions in NIF’s fusion burning plasmas

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Science Bulletin 2025年第3期70卷 359-364页

作者： Yuhan Xue Dong wu Jie Zhang Key Laboratory for Laser Plasmas and Department of Physics and Astronomy Collaborative Innovation Center of IFSA(CICIFSA)Shanghai Jiao Tong UniversityShanghai 200240China Institute of Physics Chinese Academy of SciencesBeijing 100190China

Although ignition had been achieved at the National Ignition Facility(NIF),recent observations of the experiments indicate novel physics that beyond theoretical predictions emerge,e.g.,the neutron analysis of experiments has revealed deviations from the Maxwellian distributions in ion relative kinetic energies of burning plasmas,with the surprising emergence of supra-thermal deuterium and tritium(DT)ions that fall outside the predictions of macroscopic statistical hydrodynamic *** our newly developed hybrid-particle-in-cell code,incorporating the newly-proposed model of large-angle collisions,we infer that that this could be attributed to the increased significance of large-angle collisions among DT ions andα-particles in the burning *** and unprecedented kinetic investigations into the implications of large-angle collisions in the burning plasma have yielded several key findings,including an ignition moment promotion by~10 ps,the presence of supra-thermal ions below an energy threshold,and approximately twice the expected deposition ofα-particles *** rationality of our findings is confirmed through the congruency between the neutron spectral moment analyses conducted by the NIF and our kinetic simulations,both highlighting progressively widening disparities between neutron spectral moment analyses and hydrodynamics predictions,which becomes more pronounced as the yield *** kinetic simulations with large-angle collisions not only provide novel insights for experiment interpretation but also open new research opportunities for the largely unexplored regime of the nuclear burning plasmas,which are distinguished by their exceptionally high energy densities and hold immense potential for illuminating the intricate physics that underpins the evolution of the early universe.

关键词： lon kinetics Supra-thermal ions Large-angle collisions Non-equilibrium ignition Inertial confinement fusion Burning plasmas