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Surface analysis of tablets with and without coating film for common cold based on laser-induced breakdown spectroscopy

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Optoelectronics Letters 2025年

作者： YAO Lixing LI Jingwen liu Yu ShEn Li WAnG cong Tianjin Key Laboratory of Quantum Optics and Intelligent Photonics， School of Science， Tianjin University of Technology

Medications for common cold are used routinely in daily life， and most of these are compounded to be more effective for people suffering from common cold. The composition and quality of the coating， a common component of tablets， have been of great concern. In this paper， laser-induced breakdown spectroscopy (LIBS)， with advantages of rapid， real-time， and in-situ analysis， was used for surface analysis of tablets with and without coating film for common cold. Firstly， the spectra of compound paracetamol and amantadine hydrochloride tablets (CPAhT) and compound diclofenac sodium and chlorphenamine maleate tablets (CDSCMT)， without and with coating film， respectively， were analyzed. Secondly， two kinds of tablets were investigated in-situ at depth to analyze the changes of atomic and molecular spectral line intensities under different number of laser pulses and verified using LIBS imaging method. Finally， the Ca and Ti elements in CDSCMT were analyzed by calibration free LIBS (CF-LIBS) to further verify the elemental content differences at different depth in the tablets with coating film. These results indicate that the LIBS technology can be used in fast， in-situ， depth， and multi-element detection for cold medication tablets.

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Oxidation Resistance of Form-stable hightemperature Phase Change Thermal Energy Storage Materials Doped by Impregnated Graphite

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Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 1-12页

作者： LI Baorang DAI Jianhuan ZhAnG Wei liu Xiangchen YAnG liu School of Energy Power and Mechanical Engineering North China Electric Power UniversityBeijing 102206China School of Ener-gy and Environment Southeast UniversityNanjing 210096China

We adopted the solution impregnation route with aluminum dihydrogen phosphate solution as liquid medium for effective surface modification on graphite *** mass ratio of graphite to Al(h_(2)PO_(4))_(3) changed from 0.5:1 to 4:1,and the impregnation time changed from 1 to 7 *** typical composite phase change thermal storage materials doped with the as-treated graphite were fabricated using form-stable *** investigate the oxidation and anti-oxidation behavior of the impregnated graphite at high temperatures,the samples were put into a muffle furnace for a cyclic heat *** on SEM,EDS,DSC techniques,analyses on the impregnated technique suggested an optimized processing conditions of a 3 h impregnation time with the ratio of graphite:Al(h_(2)PO_(4))_(3) as 1:3 for graphite impregnation *** investigations on high-temperature phase change heat storage materials doped by the treated graphite suggested excellent oxidation resistance and thermal cycling performance.

关键词： phase change materials graphite impregnation method oxidation,sintering thermal analysis

基于长/短视距多模型自适应交互的高速无人车避障规划研究

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北京理工大学学报 2025年第1期45卷 42-51页

作者：刘聪陈雪梅梁玮北京理工大学前沿技术研究院山东济南250307 北京理工大学机械车辆学院北京100081

在低附着、高速紧急避障工况下无人驾驶车辆需要充分考虑到路径规划效率和车辆动力学特性,以保障规划的路径满足车辆高速行驶跟踪精度要求.文中针对无人车紧急避障中路径规划与跟踪控制之间存在的耦合干预问题,提出一种基于长/短视距多... 详细信息

在低附着、高速紧急避障工况下无人驾驶车辆需要充分考虑到路径规划效率和车辆动力学特性,以保障规划的路径满足车辆高速行驶跟踪精度要求.文中针对无人车紧急避障中路径规划与跟踪控制之间存在的耦合干预问题,提出一种基于长/短视距多层融合的高速紧急避障局部路径规划算法.根据不同风险值障碍物分布的密集程度细化障碍物的风险值,分别设计了可跨/绕障碍物群的风险势场和环境风险状态采样空间,从而构建一种基于偏向性采样的长视距局部路径规划算法.提出了一种基于交互式多模型预测控制的短视距局部路径重规划,建立模型概率实时在线更新规则,实现了极限工况下车辆快速行驶的局部路径规划,同时满足计算实时性、避障安全性和跟踪稳定性的路径规划设计需求.仿真试验验证了所提多层融合局部路径规划方法的有效性和优越性.

关键词：紧急避障无人驾驶车辆多层融合规划偏向性采样

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职业教育发展对实体经济的影响研究

黑龙江高教研究 2025年第1期43卷 147-154页

作者：刘聪阮晓文曹辉南京工业职业技术大学江苏南京210023 江苏大学江苏镇江212013

基于2005一2021年的省际面板数据,采用双向固定效应模型,实证分析了职业教育发展对实体经济的影响效应和作用机制。研究发现,职业教育发展会显著促进实体经济增长,且该结论在替换变量和工具变量估计的稳健性检验下依然成立;异质性分析表... 详细信息

基于2005一2021年的省际面板数据,采用双向固定效应模型,实证分析了职业教育发展对实体经济的影响效应和作用机制。研究发现,职业教育发展会显著促进实体经济增长,且该结论在替换变量和工具变量估计的稳健性检验下依然成立;异质性分析表明,职业教育发展对经济发展程度和教育发展水平欠发达地区的实体经济促进效应更大;机制验证表明,职业教育发展会通过培育匠心劳动者、提高新质生产力和繁荣创业活跃度促进实体经济增长。未来,为更好建设以实体经济为支撑的现代化产业体系,应加快推进中国式职业教育现代化建设,并注重发展策略的精准性。

关键词：职业教育实体经济新质生产力

Low-cost and fluoride-free synthesis of MFI zeolite nanosheets with enhanced stability for benzene alkylation with ethanol

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Journal of Energy Chemistry 2025年第1期100卷 458-468页

作者： Peng Zhu Cun liu Yiren Yu Guoshu Gao Yumeng Zhao Xiongfu Zhang Guodong liu Guohui Yang State Key Laboratory of Fine Chemicals School of Chemical Engineering Dalian University of Technology State Key Laboratory of Catalysis Dalian Institute of Chemical Physics Chinese Academy of Sciences

Zeolite nanosheets with a short b-axis thickness are highly desirable in lots of catalytic reactions due to their reduced diffusion resistance. nevertheless, conventional synthesis methods usually require expensive structure-directing agents(SDAs), pricey raw materials, and eco-unfriendly fluorine-containing additives. here, we contributed a cost-effective and fluoride-free synthesis method for synthesizing high-quality MFI zeolite nanosheets through a Silicalite-1(Sil-1) seed suspension and urea cooperative strategy, only with inexpensive colloidal silica as the Si source. Our approach was effective for synthesizing both Sil-1 and aluminum-containing ZSM-5 nanosheets. By optimizing key synthesis parameters,including seed aging time, seed quantity, and urea concentration, we achieved precise control over the crystal face aspect ratio and b-axis thickness. We also revealed a non-classical oriented nanosheet growth mechanism, where Sil-1 seeds induced the formation of quasi-ordered precursor particles, and the(010)crystal planes of these particles facilitated urea adsorption, thereby promoting c-axis-oriented *** obtained ZSM-5 nanosheets exhibited exceptional catalytic performance in the benzene alkylation with ethanol, maintaining stability for over 500 h, which is 5 times longer than traditional ZSM-5 catalysts. Furthermore, large-scale production of ZSM-5 nanosheets was successfully carried out in a 3 L highpressure autoclave, yielding samples consistent with those from laboratory-scale synthesis. This work marks a significant step forward in the sustainable and efficient production of MFI nanosheets using inexpensive and environmentally friendly raw materials, offering the broad applicability in catalysis.

关键词： Aspect ratio

Formal Modeling and Discovery of Multi-instance Business Processes: A Cloud Resource Management Case Study

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IEEE/CAA Journal of Automatica Sinica 2022年第12期9卷 2151-2160页

作者： cong liu IEEE School of Computer Science and Technology Shandong University of TechnologyZibo 255000 College of Computer Science and Engineering Shandong University of Science and TechnologyQingdao 266590China

Process discovery, as one of the most challenging process analysis techniques, aims to uncover business process models from event logs. Many process discovery approaches were invented in the past twenty years;however, most of them have difficulties in handling multi-instance sub-processes. To address this challenge, we first introduce a multi-instance business process model(MBPM) to support the modeling of processes with multiple sub-process instantiations. Formal semantics of MBPMs are precisely defined by using multi-instance Petri nets(MPns)that are an extension of Petri nets with distinguishable ***, a novel process discovery technique is developed to support the discovery of MBPMs from event logs with sub-process multi-instantiation information. In addition, we propose to measure the quality of the discovered MBPMs against the input event logs by transforming an MBPM to a classical Petri net such that existing quality metrics, e.g., fitness and precision, can be *** proposed discovery approach is properly implemented as plugins in the Pro M toolkit. Based on a cloud resource management case study, we compare our approach with the state-of-theart process discovery techniques. The results demonstrate that our approach outperforms existing approaches to discover process models with multi-instance sub-processes.

关键词： Cloud resource management process multi-instance Petri nets(MPns) multi-instance sub-processes process discovery quality evaluation

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A quantum-search-based multi-classifier for image recognition

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 21-31页

作者： Lu liu Xingyu Wu Lufan Zhang Chuan Wang School of Artificial Intelligence Beijing Normal University Applied Optics Beijing Area Major Laboratory Beijing Normal University

The multi-class classification of images is a pivotal challenge within the realm of image processing. As the volume of visual data continues to expand, there is a burgeoning interest in harnessing the unique capabilities of quantum computation to augment the efficiency of classification tasks. however, many existing methods for training quantum image multi-classifiers parallel classical machine learning techniques, where the requisite circuit measurements increase linearly with the volume of training data. This work introduces a novel approach for training a quantum image multi-classifier based on the quantum search algorithm. We have meticulously conducted rigorous experiments on a handwritten digit dataset, a classic benchmark in the field. The results have been meticulously compared with previous works, and the comparative analysis not only validates the efficiency of our proposed approach, requiring only O(n/b) measurements during training, but also highlights a significant quadratic speedup of the algorithm.

关键词： quantum computation image recognition quantum search algorithm

Engineering atomic Rb-n configurations to tune radical pathways for highly selective photocatalytic h2O2 synthesis coupled with biomass valorization

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Journal of Energy Chemistry 2025年第1期100卷 215-225页

作者： Jiaye Li Shuang Pan Yihuang Chen Qiong liu College of Chemistry and Materials Engineering Wenzhou University Guangdong Provincial Key Laboratory of Chemical Measurement and Emergency Test Technology (China) Institute of Analysis Guangdong Academy of Sciences (China National Analytical CenterGuangzhou)

Photocatalytic oxygen reduction for hydrogen peroxide （h2O2） synthesis presents a green and costeffective production ***,achieving highly selective h2O2synthesis remains challenging,necessitating precise control over free radical reaction pathways and minimizing undesirable oxidative ***,we report for the visible light-driven simultaneous co-photocatalytic reduction of O2to h2O2and oxidation of biomass using the atomic rubidium-nitride modified carbon nitride（CnRb）.The optimized CnRb catalyst demonstrates a record photoreduction rate of 8.01 mM h-1for h2O2generation and photooxidation rate of 3.75 mM h-1for furfuryl alcohol to furoic acid,achieving a remarkable solar-to-chemical conversion （SCC） efficiency of up to 2.27%.Experimental characterizations and DFT calculation disclosed that the introducing atomic Rb–n configurations allows for the high-selective generation of superoxide radicals while suppressing hydroxyl free radical *** is because the Rb–n serves as the new alternative site to perceive a stronger connection position for O2adsorption and reinforce the capability to extract protons,thereby triggering a high selective redox product *** study holds great potential in precisely regulating reactive radical processes at the atomic level,thereby paving the way for efficient synthesis of h2O2coupled with biomass valorization.

关键词： Free radical reactions

Molecular simulation study of the microstructures and properties of pyridinium ionic liquid[hPy][BF_(4)]mixed with acetonitrile

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原子与分子物理学报 2025年第4期42卷 27-32页

作者： XU Jian-Qiang MA Zhao-Peng ChEnG Si liu Zhi-cong ZhU Guang-Lai Department of Physics School of Physics and Electronic InformationAnhui Normal UniversityWuhu 241002China

The microstructures and thermodynamic properties of mixed systems comprising pyridinium ionic liquid[hPy][BF_(4)]and acetonitrile at different mole fractions were studied using molecular dynamics simulation in this *** following properties were determined:density,self-diffusion coefficient,excess molar volume,and radial distribution *** results show that with an increase in the mole fraction of[hPy][BF_(4)],the self-diffusion coefficient ***,the excess molar volume initially decreases,reaches a minimum,and then *** rules of radial distribution functions(RDFs)of characteristic atoms are *** increasing the mole fraction of[hPy][BF_(4)],the first peak of the RDFs of hA1-F decreases,while that of CT6-CT6 rises at first and then *** indicates that the solvent molecules affect the polar and non-polar regions of[hPy][BF_(4)]differently.

关键词： Pyridinium ionic liquids Thermodynamic properties Molecular dynamics simulation Radial distribution functions

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