检索结果-南通市图书馆

Towards adaptable synchrotron image restoration pipeline

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

NUCLEAR SCIENCE AND TECHNIQUES 2024年第10期35卷 1-13页

作者： Li, chun Bi, Xiao-Xue Zhang, yu-Jun Zhang, Zhen Wang, Li-Wen Zhuang, Jian Chen, Dong-Liang Dong, yu-Hui Zhang, Yi Chinese Acad Sci Inst High Energy Phys Beijing Synchrotron Radiat Facil Beijing 100049 Peoples R China Spallat Neutron Source Sci Ctr Dongguan 523803 Peoples R China Univ Chinese Acad Sci Beijing 100049 Peoples R China Univ Sci & Technol China Natl Synchrotron Radiat Lab Hefei 230029 Peoples R China

Synchrotron microscopic data commonly suffer from poor image quality with degraded resolution incurred by instrumentation defects or experimental conditions. Image restoration methods are often applied to recover the reduced resolution, providing improved image details that can greatly facilitate scientific discovery. Among these methods, deconvolution techniques are straightforward, yet either require known prior information or struggle to tackle large experimental data. Deep learning (DL)-based super-resolution (SR) methods handle large data well, however data scarcity and model generalizability are problematic. In addition, current image restoration methods are mostly offline and inefficient for many beamlines where high data volumes and data complexity issues are encountered. To overcome these limitations, an online image-restoration pipeline that adaptably selects suitable algorithms and models from a method repertoire is promising. In this study, using both deconvolution and pretrained DL-based SR models, we show that different restoration efficacies can be achieved on different types of synchrotron experimental data. We describe the necessity, feasibility, and significance of constructing such an image-restoration pipeline for future synchrotron experiments.

关键词： Synchrotron Deconvolution Deep learning Super-resolution Pipeline SUPERRESOLUTION REGULARIZATION DECONVOLUTION SOFTWARE

The impact of female sex hormones on cardiovascular disease:from mechanisms to hormone therapy

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Geriatric Cardiology 2024年第6期21卷 669-681页

作者： Yi KAN yu-Lu PENG Ze-Hao ZHAO Shu-Tong DONG yin-Xiao XU Xiao-Teng MA Xiao-Li LIU yu-Yang LIU yu-Jie ZHOU Department of Cardiology Beijing Anzhen HospitalCapital Medical UniversityBeijing Institute of Heart Lung and Blood Vessel DiseaseBeijing Key Laboratory of Precision Medicine of Coronary Atherosclerotic DiseaseClinical Center for Coronary Heart DiseaseCapital Medical UniversityBeijingChina

Cardiovascular disease remains the leading cause of mortality in women,yet it has not raised the awareness from the *** pathogenesis of cardiovascular disease differs significantly between females and males concerning the effect of sex *** and progestogen impact cardiovascular system through genomic and non-genomic *** menopause,cardiovascular protective effects of estrogens have been well *** were often used in combination with estrogens in hormone *** in sex hormone levels,particularly estrogen deficiency,were considered the specific risk factor in women’s cardiovascular ***,considerable heterogeneity in the impact of hormone therapy was observed in clinical *** heterogeneity is likely closely associated with factors such as the initial time,administration route,dosage,and formulation of hormone *** review will delve into the pathogenesis and hormone therapy,summarizing the effect of female sex hormones on hypertension,pre-eclampsia,coronary heart disease,heart failure with preserved ejection fraction,and cardiovascular risk factors specific to women.

关键词： impact dosage protective

Electron push-pull effects induced performance promotion in covalent organic polymer thin films-based memristor for neuromorphic application

在线全文

学校读者我要写书评

暂无评论

Chinese Chemical Letters 2024年第5期35卷 227-231页

作者： Panke Zhou Hong yu Mun yin Chee Tao Zeng Tianli Jin Hongling yu Shuo Wu Wen Siang Lew Xiong Chen State Key Laboratory of Photocatalysis on Energy and Environment College of ChemistryFuzhou UniversityFuzhou 350116China School of Physical and Mathematical Sciences Nanyang Technological UniversitySingapore 637371Singapore Department of Materials Science and Engineering National University of SingaporeSingapore 117575Singapore

Covalent organic polymer(COP)thin film-based memristors have generated intensive research interest,but the studies are still in their ***,by controlling the content of hydroxyl groups in the aldehyde monomer,Py-COP thin films with different electronic push-pull effects were fabricated bearing distinct memory performances,where the films were prepared by the solid-liquid interface method on the ITO substrates and further fabricated as memory devices with ITO/Py-COPs/Ag *** Py-COP-1-based memory device only exhibited binary memory behavior with an ON/OFF ratio of 1:10^(1.87).In contrast,the device based on Py-COP-2 demonstrated ternary memory behavior with an ON/OFF ratio of 1:10^(0.6):10^(3.1) and a ternary yield of 55%.The ternary memory mechanism of the ITO/Py-COP-2/Ag memory device is most likely due to the combination of the trapping of charge carriers and conductive ***,the Py-COPs-based devices can successfully emulate the synaptic potentiation/depression behavior,clarifying the programmability of these devices in neuromorphic *** results suggest that the electronic properties of COPs can be precisely tuned at the molecular level,which provides a promising route for designing multi-level memory devices.

关键词： Covalent organic polymers Push-pull effects Multi-level memory Memristor

Enhanced energy density and fast-charging ability via directional particle configuration

在线全文

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2024年第3期90卷 152-164,I0005页

作者： Xiongwei Wu Shanguang lv Jiabao Li Xingrong yin Xuewen Wu Jun Liu Jie Zhang yuhan yu Bei Long Hunan yinfeng New Energy Co.Ltd. Changsha 410019HunanChina

The limited energy density of lithium-ion capacitors poses a significant obstacle to their widespread application,primarily stemming from the inability of the electrodes to simultaneously fulfill both high energy density and rapid charging *** data demonstrate that a directional particle configuration can enhance charging speed while maintaining high-capacity density,but it is rarely ***,we have developed a particle-level electrochemical model capable of reconstructing an electrode with a directional particle *** employing this method,an investigation was conducted to explore how the spatial morphology characteristics of particle configuration impact the energy storage characteristics of *** demonstrate that rational particle configuration can effectively enhance the transport of lithium ions and create additional space for lithium-ion *** the same particle size distribution,the best electrode can increase the discharge capacity by up to132.4% and increase the charging SOC by 11.3% compared to the ordinary electrode under the condition of 6 *** findings provide a further understanding of the energy storage mechanism inside the anisotropic particle distribution electrode,which is important for developing high-performance lithium-ion capacitors.

关键词： Supercapacitor Gradient design strategies Energy storage Charge transport

Co-adsorption and selective-adsorption of heavy metals and dyes from aqueous solution by bio-based humus/chitosan hydrogels

在线全文

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2024年第11期145卷 193-204页

作者： Rongping Chen Chenghao Gan Bingcai Cai Ruxue Liu Wenjie Xu Weize yin Hongyi Li Lei yu Qiang Yong College of Biology and the Environment Nanjing Forestry UniversityNanjing 210037China College of Chemical Engineering Nanjing Forestry UniversityNanjing 210037China

An eco-friendly adsorbent was prepared by reverse suspension crosslinking method to remove multiple pollutants from aqueous *** raw materials,derived from humus(HS)and chitosan(CS),are biodegradable and low-cost natural *** combining HS with CS,the adsorption capacity was significantly improved due to compensation effects between the two ***/CS exhibited the features of amphoteric adsorption through pH adjustment,enabling it to adsorb not only anionic pollutants(Methyl Orange(MO)and Cr(VI)),but also cationic ones(Methylene Blue(MB)and Pb(II)).The adsorption capacities were approximately 242 mg/g,69 mg/g,188 mg/g and 57 mg/g for MO,Cr(VI),MB and Pb(II),***/CS showed a slight preference for MO in MO/Cr(VI)co-adsorption system,whereas strong selectivity for MB over Pb(II)in MB/Pb(II)system under acidic condition(pH<3.0).This selective behavior would allow for potential applications in separating MB/Pb(II)effluents and selectively recycling Pb(II)in acidic *** isothermal and kinetic adsorption behaviors followed Langmuir model and pseudo-second-order model,*** density functional theory(DFT)confirmed that the interaction between metal ions and adsorbents was primarily attributed to chelation and electrostatic adsorption,owing to nitric and oxygenic functional ***,the adsorption mechanisms for dyes were involved in electrostatic attraction,H-bond andπ-πbond,due to available hydrogen,oxygen,nitrogen atoms and aromatic groups on the surface of adsorbent and *** adsorbent could be efficiently regenerated and retained over 90%of its adsorption capacity after five cycles,which has a potential for practical applications in water treatment.

关键词： Adsorption Density functional theory(DFT) Humus Chitosan

One-step conversion of methane and formaldehyde to ethanol over SA-FLP dual-active-site catalysts: A DFT study

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Chemical Letters 2024年第4期35卷 544-548页

作者： Tao Ban Xi-Yang yu Hai-Kuo Tian Zheng-Qing Huang chun-Ran Chang Shaanxi Key Laboratory of Energy Chemical Process Intensification School of Chemical Engineering and TechnologyXi'an Jiaotong UniversityXi'an 710049China Shaanxi Key Laboratory of Low Metamorphic Coal Clean Utilization School of Chemistry and Chemical EngineeringYulin UniversityYulin 719000China

One-step conversion of methane and formaldehyde into ethanol is a 100% atom-efficient process for carbon resources utilization and environment protection but still faces eminent challenges due to the lacking of efficient catalysts. Therefore, developing active and stable catalysts is crucial for the co-conversion of methane and formaldehyde. Herein, twelve kinds of “Single-Atom”-“Frustrated Lewis Pair”(SA-FLP)dual-active-site catalysts are designed for the direct conversion of methane and formaldehyde to ethanol based on density functional theory(DFT) calculations and microkinetic simulations. The results show that the SA-FLP dual active sites can simultaneously activate methane at the SA site and activate formaldehyde at the FLP site. Among the twelve designed SA-FLP catalysts, Fe1-FLP shows the best performance in the co-conversion of methane and formaldehyde to ethanol with the rate-determining barrier of 1.15 e *** is proved as the main product with the turnover frequency of 1.32 × 10^(-4)s^(-1)at 573 K and 3 *** work provides a universal strategy to design dual active sites on metal oxide materials and offers new insights into the effective conversion of methane and formaldehyde to desired C_(2) chemicals.

关键词： Single-atom Frustrated Lewis pairs Methane conversion Dual active sites Ethanol synthesis

Te-doped Fe3O4 flower enabling low overpotential cycling of Li-CO2 batteries at high current density

在线全文

学校读者我要写书评

暂无评论

Effective strategies to promote Z(S)-scheme photocatalytic water splitting

结构化学 2024年第3期43卷 25-32页

作者： Huyi yu Renshu Huang Qian Liu Xingfa Chen Tianqi yu Haiquan Wang Xincheng Liang Shibin yin Guangxi Key Laboratory of Electrochemical Energy Materials School of Chemistry and Chemical EngineeringGuangxi University100 Daxue RoadNanning530004China

Li-CO2 batteries(LCBs)suffer from high overpotentials caused by sluggish CO2 reaction *** work designs a Te-doped Fe3O4(Te-Fe3O4)flower-like microsphere catalyst to lower the overpotential and improve the reversibility of *** results reveal that Te doping modifies the electronic structure of Fe3O4 and reduces the *** stable Te-O bond between Te and C2O4-could effectively inhibit the dispro-portionation reaction of the latter,enabling the Te-Fe3O4 cathodes to exhibit a remarkable capacity(9485 mAh g-1)and a long cycling life(155 cycles)with an overpotential of 1.21 V and an energy efficiency of about 80％at a high current density(2000 mA g-1).Through the interaction between Te and Li2C2O4 to inhibit the dispro-portionation reaction,this work successfully achieves long-term cycling of LCBs with low overpotential at high current density.

关键词： Li-CO_2 batteries Catalyst Tellurium Li_2C_2O_4 Large current density

来源：评论

学校读者我要写书评

暂无评论

Chinese Chemical Letters 2024年第3期35卷 27-39页

作者： Ye yuan Junan Pan Weinan yin Haoxuan yu Fengshun Wang Weifeng Hu Longlu Wang Dafeng Yan College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology) Nanjing University of Posts&Telecommunications(NUPT)Nanjing 210023China College of Chemistry and Chemical Engineering Hubei UniversityWuhan 430062China

Artificial Z(S)-scheme photocatalytic water splitting systems have attracted extensive attention due to their advantages such as wide light absorption range,high charge separation efficiency and strong carrier redox ***,it is still challenging to design and prepare Z(S)-scheme photocatalysts with low-cost and highly stability for efficiently photocatalytic overall water splitting using solar *** review mainly introduces various strategies to improve the photocatalytic water splitting performance of Z(S)-scheme *** strategies mainly focus on enhancing or extending the range of light absorption,promoting charge separation,and enhancing surface redox reaction in Z(S)-scheme ***,the main challenges of Z(S)-scheme photocatalytic water splitting systems and their future development directions are pointed *** review would be beneficial to understanding the challenges and opportunities faced by the research field of Z(S)-scheme photocatalytic systems,and has important guiding significance for the development and utilization of high-performance Z(S)-scheme photocatalytic reaction system in the future.

关键词： Z(S)-scheme Overall water splitting Light absorption Charge separation Loading co-catalyst

Atherosis-associated lnc_000048 activates PKR to enhance STAT1-mediated polarization of THP-1 macrophages to M1 phenotype

在线全文

学校读者我要写书评

暂无评论

Neural Regeneration Research 2024年第11期19卷 2488-2498页

作者： yuanyuan Ding yu Sun Hongyan Wang Hongqin Zhao Ruihua yin Meng Zhang Xudong Pan Xiaoyan Zhu Department of Neurology The Affiliated Hospital of Qingdao UniversityQingdaoShandong ProvinceChina Qingdao Cadre Health Care Service Center The Affiliated Hospital of Qingdao UniversityQingdaoShandong ProvinceChina Department of Critical Care Medicine The Affiliated Hospital of Qingdao UniversityQingdaoShandong ProvinceChina

Our previous study has demonstrated that lnc_000048 is upregulated in large-artery atherosclerotic stroke and promotes atherosclerosis in ApoE^(-/-)***,little is known about the role of lnc_000048 in classically activated macrophage(M1)*** this study,we established THP-1-derived testing state macrophages(M0),M1 macrophages,and alternately activated macrophages(M2).Real-time fluorescence quantitative PCR was used to verify the expression of marker genes and the expression of lnc_000048 in *** cytometry was used to detect phenotypic proteins(CD11b,CD38,CD80).We generated cell lines with lentivirus-mediated upregulation or downregulation of lnc_*** cytometry,western blot,and real-time fluorescence quantitative PCR results showed that down-regulation of lnc_000048 reduced M1 macrophage polarization and the inflammation response,while over-expression of lnc_000048 led to the opposite *** blot results indicated that lnc_000048 enhanced the activation of the STAT1 pathway and mediated the M1 macrophage ***,catRAPID prediction,RNA-pull down,and mass spectrometry were used to identify and screen the protein kinase RNA-activated(PKR),then catRAPID and RPIseq were used to predict the binding ability of lnc_000048 to ***(IF)-RNA fluorescence in situ hybridization(FISH)double labeling was performed to verify the subcellular colocalization of lnc_000048 and PKR in the cytoplasm of M1 *** speculate that lnc_000048 may form stem-loop structure-specific binding and activate PKR by inducing its phosphorylation,leading to activation of STAT1 phosphorylation and thereby enhancing STAT1 pathway-mediated polarization of THP-1 macrophages to M1 and inflammatory factor *** together,these results reveal that the lnc_000048/PKR/STAT1 axis plays a crucial role in the polarization of M1 macrophages and may be a novel therapeutic target for atherosclerosis alleviation in stroke.

关键词： atherosclerosis inflammation lnc_000048 lncRNA macrophage polarization protein kinase RNA-activated(PKR) STAT1