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Membrane-less MoO_(3-x)@TiO_(2)-bromine battery with excellent rate capability and cyclic stability

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Journal of Energy Chemistry 2024年第6期93卷 316-321,I0008页

作者： Wenjie Huang hui Wang Bin Yuan Liuzhang ouyang Lichun Yang Min Zhu School of Materials Science and Engineering Guangdong Provincial Key Laboratory of Advanced Energy Storage MaterialsSouth China University of TechnologyGuangzhou 510640GuangdongChina

Bromine has attracted significant attention as a cathode material for aqueous batteries due to its high reduction potential of 1.05 V(Br_(3)^(-)+2e~-■3Br~-),impressive theoretical specific capacity of 223 mA h g^(-1),and rapid reaction kinetics in the ***,searching for compatible anode materials to match with bromine has posed a challenge due to its highly corrosive *** this study,we developed oxygen-deficient MoO_(3) with TiO_(2) coating(referred to as MoO_(3-x)@TiO_(2))as an anode material to pair with a bromine cathode in static full *** oxygen deficiency contributes to enhanced electronic and protonic diffusion within the MoO_(3-x)lattice,while the TiO_(2) coating mitigates structural dissolution and proton trapping during *** MoO_(3-x)@TiO_(2) demonstrates fast charge storage kinetics and excellent resistance to bromine *** impressive compatibility between MoO_(3-x)@TiO_(2) and bromine enables the construction of membrane-less full batteries with exceptional rate capability and cyclic *** MoO_(3-x)@TiO_(2)-bromine battery achieves an energy density of70.8 W h kg^(-1)at a power density of 328.1 W kg^(-1),showcasing an impressive long-term cyclic life of 20,000 *** study provides valuable insights for the development of high-performance aqueous secondary batteries.

关键词： Molybdenum trioxide Oxygen deficiency TiO_(2)coating Compatibility Bromine-based battery

Enhanced hydrogen storage properties of MgH_(2) with the co-addition of LiBH_(4) and YNi_(5) alloy

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Journal of Materials Science & Technology 2024年第11期178卷 90-99页

作者： Shaoyang Shen Wenfang Liao Zhijie Cao Jiangwen Liu hui Wang Liuzhang ouyang Guangdong Engineering Research Center for Advanced Energy Storage Materials School of Materials Science and EngineeringSouth China University of TechnologyGuangzhou 510641China New Energy Materials Laboratory School of PhysicsNingxia UniversityYinchuan 750021China

MgH_(2),as one of the typical solid-state hydrogen storage materials,has attracted extensive ***,the slow kinetics and poor cycle stability limit its *** this work,LiBH_(4) and YNi_(5) alloy were co-added as additives to MgH_(2) via ball milling,thereby realizing an excellent dehydrogenation per-formance and good cycle stability at 300 ℃.The MgH_(2)-0.04LiBH_(4)-0.01YNi_(5) composite can release 7 wt.%of hydrogen in around 10 min at 300 ℃ and still have a reversible hydrogen storage capacity of 6.42 wt.%after 110 cycles,with a capacity retention rate as high as 90.3%based on the second dehydrogenation *** FTIR results show that LiBH_(4) can reversibly absorb and desorb hydrogen throughout the hydrogen ab/desorption process,which contributes a portion of the reversible hydrogen storage capacity to the MgH_(2)-0.04LiBH_(4)-0.01YNi_(5) *** to the small amount of LiBH_(4) and YNi_(5),the dehydro-genation activation energy of MgH_(2) did not decrease significantly,nor did the dehydrogenation enthalpy(△H)***,the MgNi3B2 and in-situ formed YH3 during the hydrogen absorption/desorption cycles is not only beneficial to the improvement of the kinetics performance for MgH_(2) but also improves its cycle *** work provides a straightforward method for developing high reversible hydrogen capacity on Mg-based hydrogen storage materials with moderate kinetic performance.

关键词： Hydrogen storage Magnesium hydride Lithium borohydride YNi5 alloy High reversible capacity

Identification of a dual functional betulinic acid analog for the treatment of osteoarthritis by phenotypic screening

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Science China Life Sciences 2025年第1期 300-302页

作者： Ze-Min Lin Mai Xiang Wen-hui Wei Shu-hui Fan Li Chen Jie Wang Xiao-Qian Yang chun-Hao Yang Shi-Jun He Jian-Ping Zuo Laboratory of Immunopharmacology State Key Laboratory of Drug ResearchShanghai Institute of Materia MedicaChinese Academy of Sciences School of Pharmacy University of Chinese Academy of Sciences School of Pharmacy Nanjing University of Chinese Medicine State Key Laboratory of Drug Research Department of Medicinal ChemistryShanghai Institute of Materia MedicaChinese Academy of Sciences Innovation Research Institute of Traditional Chinese Medicine Shanghai University of Traditional Chinese Medicine Experiment Center for Science and Technology Shanghai University of Traditional Chinese Medicine

Dear Editor, Phenotypic drug discovery, which observes compound effects on physiology,has given way to targeting specific molecules, but has revived by using modern methods to find drugs based on therapeutic outcomes in disease models(Vincent et al., 2022). Osteoarthritis(OA) is a prevalent chronic joint disorder, primarily affecting knee joints, with osteoclast activation due to low-grade inflammation resulting in increased bone resorption and structural changes in the joint(Katz et al.,2021).

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Anomalous response to creep deformation from dislocation density during electrically assisted creep aging

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Rare Metals 2024年第10期43卷 5268-5283页

作者： Chang Zhou Li-Hua Zhan chun-hui Liu Ming-hui Huang College of Mechanical and Electrical Engineering Central South UniversityChangsha 410083China Light Alloys Research Institute State Key Laboratory of Precision Manufacturing for Extreme Service PerformanceCentral South UniversityChangsha 410083China

Adding numerous dislocations into metallic materials before the forming stage significantly enhances their ***,this beneficial effect of dislocation defects may not have a simple monotonic relationship with increased dislocation density during electroplastic *** is due to the complex interactions among the drifting electrons,dislocations and solute *** study explores the effect of diverse initial dislocation densities on creep deformation during electrically aided creep aging of an aluminum-lithium ***,we discovered a threshold value for the dislocation density that affects electroplastic creep,i.e.,an enhanced effect from dislocations weakens when exceeding this density threshold(an anomalous response to creep).Microstructural data also reveal that such an anomalous response originates mainly from differences in various dislocation density-tailored configurations,which can influence the dislocation motions and precipitation kinetics of the strengthening T1precipitates under the same action of pulsed *** study provides important insights into the dislocation density-mediated electroplastic creep of an aluminum-lithium alloy.

关键词： Creep aging Dislocation density Al-Cu-Li alloy Pulsed currents

Risk Assessment of Tsunamis Along the Chinese Coast Due to Earthquakes

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International Journal of Disaster Risk Science 2022年第2期13卷 275-290页

作者： chun hui Lixin Ning Changxiu Cheng Key Laboratory of Environmental Change and Natural Disaster Beijing Normal UniversityBeijing 100875China State Key Laboratory of Earth Surface Processes and Resource Ecology Beijing Normal UniversityBeijing 100875China Faculty of Geographical Science Beijing Normal UniversityBeijing 100875China National Tibetan Plateau Data Center Beijing 100101China

China’s coastal areas are densely populated,economically developed, and located in close proximity to several potential tsunami sources;therefore, tsunami risk cannot be ignored. This study assessed tsunami risk in coastal areas of China by developing a framework for tsunami risk assessment from the perspectives of hazards,vulnerability, and exposure. First, a probabilistic tsunami hazard assessment(PTHA) model was applied to estimate the potential tsunami sources in both local crustal faults and circum-Pacific subduction zones based on numerical simulations. The output of the PTHA includes tsunami wave height distributions along the coast. Then, an indicator system reflecting exposure and vulnerability to tsunamis in the coastal areas of China was established by using the entropy method and analytic hierarchy *** PTHA findings show that the tsunami wave height is close to 3 m on the southern coast of the Bohai Sea, the Pearl River Estuary, and the Yangtze River Delta and exceeds 2 m near the Taiwan Strait for the 2000-year return period. The results of the tsunami risk assessment show that the cities at the highest risk level(level I) include Tangshan, Yantai, and Hong Kong, while cities at the high risk level(level II) include Fuzhou, Xiamen, and Quanzhou near the Taiwan Strait and many cities on the Yangtze River Delta, the Pearl River Estuary, and the southern coast of the Bohai Sea. Our findings can provide an understanding of differences in tsunami risk between Chinese coastal cities that may be affected by tsunamis in the future.

关键词： China coast Earthquakes Probabilistic tsunami hazard assessment Tsunami exposure Tsunami risk Vulnerability

Compositional tuning of A_(2)B_(7)-type La_(0.7-x)Y_(x)Mg_(0.3)Ni_(3.5)alloys for gaseous hydrogen storage

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Journal of Rare Earths 2024年第10期42卷 1912-1919页

作者： Junkun Du hui Wang Renheng Tang Jiangwen Liu Liuzhang ouyang Min Zhu School of Materials Science and Engineering Guangdong Engineering Technology Research Center of Advanced Energy Storage MaterialsSouth China Universityof TechnologyGuangzhou510640China

Rare earth-based superlattice alloys have great potential for gaseous hydrogen storage,as well as successful application as nickel-metal hydride batteries *** this work,Y substitution was carried out to adjust the gaseous hydrogen storage properties of A_(2)B_(7)-type La_(0.7)Mg_(0.3)Ni_(3.5)*** results indicate a multiphase structure in the alloys comprised of the main rhombohedral Gd_(2)Co_(7)and PuNi_(3)phases,with a small amount of CaCu_(5)***,the Y substitution results in higher abundance of the Gd_(2)Co_(7)*** alloy La_(0.42)Y_(0.28)Mg_(0.3)Ni_(3.5)exhibits a hydrogen storage cap acity of 1.55 wt%at 298 K and a desorption plateau pressure of 0.244 *** addition,this alloy demonstrates a stable cycle life by a capacity retention of 94.2%after 50 cycles,with the main capacity degradation occurring during the initial 20 *** work accentuates the potential of the La-Y-Mg-Ni-based superlattice alloys for applications in solid-state hydrogen storage.

关键词： Hydrogen storage A_(2)B_(7)-type La-Mg-Ni alloys Y substitution Desorption plateau pressure Cycle performance Rare earths

High-speed train positioning based on a combination of Beidou navigation, inertial navigation and an electronic map

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Science China(Information Sciences) 2023年第7期66卷 237-252页

作者： hui YANG Shuai-Qiang DONG chun-Hua XIE School of Electrical and Automation Engineering East China Jiaotong University Key Laboratory of Advanced Control & Optimization of Jiangxi Province East China Jiaotong University State Key Laboratory of Performance Monitoring Protecting of Rail Transit Infrastructure East China Jiaotong University

To date, the studies on the combination positioning of high-speed trains have made great progress, but the positioning accuracy of these methods is relatively low. Map-matching positioning can improve positioning accuracy, but information transmission is time-consuming. Few studies incorporate it into combination positioning. To solve the problem, this paper proposes a high-speed train positioning method based on combining a Beidou navigation system, an inertial navigation system, and an electronic map. First, the combination positioning problem is transformed into a multi-objective optimization problem, which weights the direction similarity and distance error to form a fitness function and converts the railway line and the maximum error range of each positioning system into constraints. Second, an improved differential evolution algorithm is proposed to solve this problem. By referencing the gray wolf algorithm,the differential evolution algorithm updates individuals by varying toward the direction of multiple optimal values. Then, a new combination positioning algorithm for high-speed trains is proposed. In the simulation,the increase in positioning speed and accuracy is analyzed and validated. Compared to the current algorithms, the proposed algorithm performs better. The proposed method has practical value for improving the reliability and safety of train operations.

关键词： electronic map multi-objective optimization differential evolution algorithm Beidou navigation system high-speed train positioning

T-cell immunoglobulin mucin molecule-3, transformation growth factor β, and chemokine-12 and the prognostic status of diffuse large B-cell lymphoma

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World Journal of Clinical Cases 2022年第32期10卷 11804-11811页

作者： Hao Wu hui-Cong Sun Gui-Fang ouyang Department of Hematology Ningbo First HospitalNingbo Clinical Research Center for Hematologic MalignanciesNingbo 315010Zhejiang ProvinceChina Department of Adult Internal Medicine Ningbo Women and Children's HospitalNingbo 315012Zhejiang ProvinceChina

BACKGROUND The effects of T-cell immunoglobulin mucin molecule-3(Tim-3),transforming growth factor β(TGF-β),and chemokine-12(CXCL12) expression on the prognosis of patients with diffuse large B-cell lymphoma(DLBCL) have not been *** To examine the correlation between Tim-3,TGF-β and CXCL12 expression and DLBCL *** Lymph node tissues of 97 patients with DLBCL and 93 normal-response hyperplastic lymph node tissues treated from January 2017 to May 2019 were selected as the DLBCL and control groups,*** expression of Tim-3,TGF-β,and CXCL12 was detected *** were followed up for 3 years,and progression-free survival was *** mult-ifactorial analysis was performed to analyze the risk factors for poor *** The positive expression rates of Tim-3,TGF-β,and CXCL12 were higher in DLBCL tissues than in non-cancerous(control) tissues(P < 0.05).One-year postsurgery,the positive expression rates of Tim-3,TGF-β,and CXCL12 were higher in patients with effective treatment than in those with ineffective treatment(P < 0.05).The 3-year progression-free survival of 97 patients with DLBCL was 67.01%(65/97).Univariate analysis revealed that clinical stage,bone marrow infiltration,International Prognostic Index(IPI) score,Tim-3 positivity,TGF-β positivity,and CXCL12 positivity were associated with poor prognosis(P < 0.05).Multivariate Cox regression analysis demonstrated that clinical stage Ⅲ–Ⅳ,bone marrow infiltration,mediate-to-high-risk IPI scores,Tim-3 positivity,TGF-β positivity,and CXCL12 positivity were independent risk factors affecting prognosis(P < 0.05).CONCLUSION DLBCL tissues exhibit high positive expression of Tim-3,TGF-β,and CXCL12,and a high expression of all three indicates a poor prognosis.

关键词： T-cell immunoglobulin mucin molecule-3 Transforming growth factorβ Chemokine-12 Diffuse large B-cell lymphoma

Cocatalysts in photocatalytic methane conversion: recent achievements and prospects

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Science China Chemistry 2023年第9期66卷 2532-2557页

作者： Chengcheng Zhang Jing Wang Shenshen ouyang hui Song Jinhua Ye Li Shi School of Materials Science and Chemical Engineering Ningbo UniversityNingbo 315211China Zhejiang Key Laboratory of Bio-based Polymeric Materials Technology and Application Ningbo Key Laboratory of Polymer MaterialsNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China International Center for Materials Nanoarchitectonics(WPI-MANA) National Institute for Materials Science(NIMS)Tsukuba 305-0044Japan TJU-NIMS International Collaboration Laboratory School of Material Science and EngineeringTianjin UniversityTianjin 300072China

Photocatalysis, which performed under mild conditions by utilizing solar energy, has become a desirable technology to convert methane into highly valuable chemicals, such as methanol, ethane, and other hydrocarbons. However, pristine photocatalysts still suffer from the low utilization efficiency of solar light and the high recombination rate of photogenerated charge carriers, which exhibit the low activity and selectivity for photocatalytic methane conversion. Loading cocatalysts on photocatalysts is an attractive strategy to manipulate the products' yield and selectivity of photocatalytic methane conversion due to the enhanced charge carrier separation efficiency, extended light absorption and promoted reactant adsorption/desorption kinetics. This review discusses the recent achievements of the cocatalysts for photocatalytic methane conversion reactions. Moreover, the challenges and perspectives for the development of efficient cocatalysts are presented. This review provides considerable guidelines for the design and construction of efficient cocatalysts for photocatalytic methane conversion reactions.

关键词： photocatalysis methane conversion cocatalysts valuable chemicals