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Journal of Materiomics 2024年第2期10卷 423-430页

作者： Yiwen Liu Hulei Yu Hong Meng Yanhui chu School of Materials Science and Engineering South China University of TechnologyGuangzhou510641China

Understanding the initial oxidation mechanism is critical for studying the oxidation resistance of high-entropy ***,related studies are ***,the initial oxidation mechanism of(Zr_(0.25)Ti_(0.25)Nb_(0.25)Ta_(0.25))B_(2)high-entropy diborides(HEB_(2)-1)is investigated by first-principles calculations at the atomic *** employing the two-region model method,the most stable surface of HEB_(2)-1 is determined to be(1120)*** dissociative adsorption process of the oxygen molecule on the HEB_(2)-1-(1120)surface is predicted to proceed spontaneously,where OeO bond breaks and each oxygen atom is chemisorbed on the most preferable hollow *** adsorption energy and the diffusion barrier of the oxygen atom on the(1120)surface of HEB_(2)-1 are in the vicinity of the average level of the cor-responding four individual *** addition,ab initio molecular dynamics simulations indicate a high initial oxidation resistance of HEB_(2)-1 at 1000 *** results are beneficial to further designing the high-entropy diborides with excellent oxidation resistance.

关键词： High-entropy diborides Oxidation First-principles calculations

Enzyme-driven Nanorobots Walking Along Predesigned Tracks on the DNA Origami for Cargo Transport and Catalysis

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Chemical Research in Chinese Universities 2024年第2期40卷 333-342页

作者： NIE Cunpeng MA Tianran CHEN Tingting chu Xia State Key Laboratory of Chemo/Bio-Sensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha410082P.R.China

In molecular engineering,designing and synthesizing molecular machines with capable of performing complex tasks,remains a formidable *** is an excellent candidate for building molecular robots because it is highly ***,we present an artificial nanorobot,in which a DNA cube serves as the inert‘body’,and nucleic acid catalysts based on an enzymatic nicking reaction act as the‘legs’for *** nanorobot can execute a series of actions,such as‘start’,‘turn’,and‘stop’when it walks along a predefined *** performance could be confirmed and monitored by using an atomic force microscope(AFM)and fluorescence *** by biological machines,we artificially designed a series of specialized tasks that combined walking with control of cargo transport and ***-time fluorescence kinetics curves provide monitoring signals for cargo transport and catalytic *** work can enrich the toolbox of DNA machinery and has great potential for engineering molecular nanofactories.

关键词： DNA origami DNA nanorobot Controlled cargo transport DNAzyme catalysis

Single-atom Co alloyed Ru for electrocatalytic nitrite reduction to ammonia

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Nano Research 2024年第5期17卷 3660-3666页

作者： Fuzhou Wang Jiaqi Xiang Guike Zhang Kai Chen Ke chu School of Materials Science and Engineering Lanzhou Jiaotong UniversityLanzhou 730070China

Electrochemical converting NO_(2)^(-)into NH_(3)(NO_(2)RR)holds an enormous prospect to attain efficient NH_(3) electrosynthesis and polluted NO_(2)^(-)***,we report single-atom Co alloyed Ru(Co_(1)Ru)as an efficient and durable NO_(2)RR *** experimental and theoretical investigations reveal that single-atom Co alloying of Ru enables the construction of Co_(1)-Ru heteronuclear active sites to synergistically promote NO_(2)^(-)activation/hydrogenation while suppressing the competitive H_(2) evolution,rendering the greatly enhanced activity and selectivity of Co_(1)Ru towards the NO_(2)***,Co_(1)Ru assembled within a flow cell exhibits an impressive NH_(3) yield rate of 2379.2μmol·h^(-1)·cm^(-2) with an NH_(3)-Faradaic efficiency of 92%at a high current density of 415.9 mA·cm^(-2),which is among the highest NO_(2)RR performances reported to date.

关键词： electrochemical converting NO_(2)-into NH3 single-atom alloys theoretical computations industrial-level current density

ED-Ged:Nighttime Image Semantic Segmentation Based on Enhanced Detail and Bidirectional Guidance

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Computers, Materials & Continua 2024年第8期80卷 2443-2462页

作者： Xiaoli Yuan Jianxun Zhang Xuejie Wang Zhuhong chu College of Computer Science and Engineering Chongqing University of TechnologyChongqing400054China

Semantic segmentation of driving scene images is crucial for autonomous *** deep learning technology has significantly improved daytime image semantic segmentation,nighttime images pose challenges due to factors like poor lighting and overexposure,making it difficult to recognize small *** address this,we propose an Image Adaptive Enhancement(IAEN)module comprising a parameter predictor(Edip),multiple image processing filters(Mdif),and a Detail Processing Module(DPM).Edip combines image processing filters to predict parameters like exposure and hue,optimizing image *** adopt a novel image encoder to enhance parameter prediction accuracy by enabling Edip to handle features at different *** strengthens overlooked image details,extending the IAEN module’s *** the segmentation network,we integrate a Depth Guided Filter(DGF)to refine segmentation *** entire network is trained end-to-end,with segmentation results guiding parameter prediction optimization,promoting self-learning and network *** lightweight and efficient network architecture is particularly suitable for addressing challenges in nighttime image *** experiments validate significant performance improvements of our approach on the ACDC-night and Nightcity datasets.

关键词： Night driving semantic segmentation nighttime image processing adverse illumination differentiable filters

YOLO-O2E:A Variant YOLO Model for Anomalous Rail Fastening Detection

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Computers, Materials & Continua 2024年第7期80卷 1143-1161页

作者： Zhuhong chu Jianxun Zhang Chengdong Wang Changhui Yang Department of Computer Science and Engineering Chongqing University of TechnologyChongqing400054China Institute of Flexible Electronics(Future Technologies) Xiamen UniversityXiamen361000China College of Mechanical Engineering Chongqing University of TechnologyChongqing400054China

Rail fasteners are a crucial component of the railway transportation safety *** fasteners,distinguished by their high length-to-width ratio,frequently encounter elevated failure rates,necessitating manual inspection and *** inspection not only consumes time but also poses the risk of potential *** the advancement of deep learning technology in rail fasteners,challenges such as the complex background of rail fasteners and the similarity in their states are *** have proposed an efficient and high-precision rail fastener detection algorithm,named YOLO-O2E(you only look once-O2E).Firstly,we propose the EFOV(Enhanced Field of View)structure,aiming to adjust the effective receptive field size of convolutional kernels to enhance insensitivity to small spatial ***,The OD_MP(ODConv and MP_2)and EMA(EfficientMulti-Scale Attention)modules mentioned in the algorithm can acquire a wider spectrum of contextual information,enhancing the model’s ability to recognize and locate ***,we collected and prepared the GKA dataset,sourced from real train *** testing on the GKA dataset and the publicly available NUE-DET dataset,our method outperforms general-purpose object detection *** the GKA dataset,our model achieved a mAP 0.5 value of 97.6%and a mAP 0.5:0.95 value of 83.9%,demonstrating excellent inference ***-O2E is an algorithm for detecting anomalies in railway fasteners that is applicable in practical industrial settings,addressing the industry gap in rail fastener detection.

关键词： Rail fastening detection deep learning anomalous rail fastening variant YOLO feature reinforcement

To be or not to be direct:The role of neuromedin U in neuro-eosinophil crosstalk

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Science Bulletin 2024年第2期69卷 148-150页

作者： Ruichao Liu Wenhao Shao Jun Xu Coco chu SXMU-Tsinghua Collaborative Innovation Center for Frontier Medicine Taiyuan 030001China Insttute for Immunogy Department of Basic Medical SciencesSchool of Medicinesinghua UnierstyBejing 100084China Tsinghua-Peking Center for Life Sciences Tsinghua UniversityBeijing 100084China Shanxi Medical University Taiyuan 030012China Department of Surgery First Hospital of Shanxi Medical UniversityShanxi Provincial Key Laboratory for Digestive Diseases and Organ TransplantationTaiyuan 030001China Beijing Key Laboratory for Immunological Research on Chronic Diseases Tsinghua UniversityBejing 100084China

With the development of new experimental techniques(e.g.,single-cell RNA sequencing(scRNA-seq),light sheet microscopy,and clustered regularly interspaced palindromic repeats(CRISPR)/CRISPR-associated protein 9(Cas9),emerging studies have begun to uncover the interactions between the nervous system and the immune system,both in health and *** example,in mucosal tissues such as the lung and the intestine,neurotransmitters including acetylcholine[1]and adrenaline[2]can directly regulate the immune cell functions thus affect the results of allergy,asthma,and anti-pathogen host defense[3].

关键词： intestine lung asthma

Partially-hiding functional encryption for degree-2 polynomials with fine-grained access control

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Frontiers of Computer Science 2024年第3期18卷 231-233页

作者： Haifeng QIAN Cheng LIN Qiaohan chu Jie CHEN Shanghai Key Laboratory of Trustworthy Computing Software Engineering InstituteEast China Normal UniversityShanghai 200062China

1 Introduction Boneh et al.[1]first systematically introduce the concept of Functional Encryption(FE)which overcomes all-or-nothing limitation of traditional public key ***,FE hides a potential problem:even if the secret key is obtained legitimately,once it is released,it can be used *** leads to that the secret key may leak information *** deal with this problem and make FE more practical,Abdalla et al.[2]recently constructed inner-product FE(IPFE)with fine-grained access control achieving strong security guarantees under standard assumptions.

关键词： grain Encryption encryption

A review of CFD simulation in pressure driven membrane with fouling model and anti-fouling strategy

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Frontiers of Environmental Science & Engineering 2024年第8期18卷 1-29页

作者： Shiyong Miao Jiaying Ma Xuefei Zhou Yalei Zhang Huaqiang chu State Key Laboratory of Pollution Control and Resource Reuse Tongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Tongji UniversityShanghai 200092China

Pressure-driven membrane filtration systems are widely utilized in wastewater treatment,desalination,and water reclamation and have received extensive attention from *** fluid dynamics(CFD)offers a convenient approach for conducting mechanistic studies of flow and mass transfer characteristics in pressure-driven *** a signature phenomenon in membrane systems,the concentration polarization that accompanies the permeation process is a key factor in membrane performance degradation and membrane fouling *** fouling models(scaling,biofouling and colloidal particle fouling)based on CFD theory have been constructed,and considerable research has been *** representative antifouling strategies with special simulation methods,including patterned membranes,vibration membranes,rotation membranes,and pulsatile flows,have also been *** studies should focus on refining fouling models while considering local hydrodynamic characteristics;experimental observation tools focusing on the internal structure of inhomogeneous fouling layers;techno-economic model of antifouling strategies such as vibrational,rotational and pulsatile flows;and unfavorable hydraulic phenomena induced by rapidly changing flows in simulations.

关键词： Computational fluid dynamics Membrane Fouling model Concentration polarization

Microstructure optimization and electrochemical behavior of in-situ growth Ramsdellite-MnO_(2)@NCA-LDH@CC for supercapacitors and oxygen evolution reaction catalysts

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Journal of Materiomics 2024年第3期10卷 552-565页

作者： Xinpeng Huang Yanli Li Xuehua Yan Feng Zhang chu chu Jili Wu Jianmei Pan Zohreh Shahnavaz Jamile Mohammadi Moradian School of Materials Science and Engineering Jiangsu UniversityZhenjiang212013JiangsuChina Institute for Advanced Materials Jiangsu UniversityZhenjiang212013JiangsuChina

Supercapacitors are electrochemical energy storage devices with great potential ***-while,the oxygen evolution reaction(OER)determines the efficiency of some electrochemical energy *** study aims at constructing,exploring,and optimizing Ramsdellite-MnO_(2)@NiCoAl-LDH@CC(R-MNCA@CC)*** effect of microstructure and Al role on the performance is investigated when R-MNCA@CC was used as supercapacitor electrode material and OER ***-like R-MNCA@CC in-situ growth composites were synthesized by a two-step hydrothermal method.R-MNCA@CC-2(molar ratio of Ni:Co:Al is 1:1:1)performs the best with the largest specific capacitance,1,742 F/g at 1 A/g,increased by 797%and 1,489%compared to that of NiCoAl-LDH and Ramsdellite-MnO_(2).The capacitance retention rate of the R-MNCA@CC-2//AC@CC supercapacitor is 80.1%after 5,000 cycles at 0.8 A/*** overpotential for driving an OER to reach 10 m/cm^(2)is only 276 mV,which is lower than that of commercial IrO_(2)(300 mV).Noteworthy,we propose a view that is“competing to trigger redox re-action”of electrochemical active sites in LDH during electrochemical processes derived from a discrepancy between theory and experimental results.

关键词： Supercapacitors Oxygen evolution reaction MnO_(2)@NiCoAl-LDH composites Microstructure optimization Electrochemical mechanism

Alterations of soil aggregates and intra-aggregate organic carbon fractions after soil conversion from paddy soils to upland soils:Distribution,mineralization and driving mechanism

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Pedosphere 2024年第1期34卷 121-135页

作者： Longfei KANG Jiamei WU chunfeng ZHANG Baoguo ZHU Guixin chu College of Life Science Shaoxing UniversityShaoxing 312000China The Key Laboratory of Oasis Eco-agriculture Xinjiang Production and Construction Group/Department of Resources and Environmental SciencesAgronomy CollegeShihezi UniversityShihezi 832000China Hunan Institute of Agricultural Environment and Ecology Changsha 410000China Jiamusi Branch Heilongjiang Academy of Agricultural SciencesJiamusi 154007China

Investigating the impacts of soil conversion on soil organic carbon(OC) content and its fractions within soil aggregates is essential for defining better strategies to improve soil structure and OC sequestration in terrestrial ecosystems. However, the consequences of soil conversion from paddy soil to upland soil for soil aggregates and intra-aggregate OC pools are poorly understood. Therefore, the objective of this study was to quantify the effects of soil conversion on soil aggregate and intra-aggregate OC pool distributions. Four typical rice-producing areas were chosen in North and South China, paired soil samples(upland soil converted from paddy soil more than ten years ago vs. adjacent paddy soil) were collected(0–20 cm) with three replicates in each area. A set of core parameters(OC preservation capacity, aggregate carbon(C) turnover, and biological activity index) were evaluated to assess the responses of intra-aggregate OC turnover to soil conversion. Results showed that soil conversion from paddy soil to upland soil significantly improved the formation of macro-aggregates and increased aggregate stability. It also notably decreased soil intra-aggregate OC pools, including easily oxidized OCa(EOCa), particulate OCa(POCa), and mineral-bound(MOCa) OC, and the sensitivity of aggregate-associated OC pools to soil conversion followed the order: EOCa(average reduction of 21.1%) > MOCa(average reduction of 15.4%) > POCa(average reduction of 14.8%). The potentially mineralizable C(C_(0)) was significantly higher in upland soil than in paddy soil, but the corresponding decay constant(k) was lower in upland soil than in paddy soil. Random forest model and partial correlation analysis showed that EOCa and pH were the important nutrient and physicochemical factors impacting k of C mineralization in paddy soil,while MOCa and C-related enzyme(β-D-cellobiohydrolase) were identified as the key factors in upland soil. In conclusion, this study evidenced that soil conversion

关键词： decay constant easily oxidized organic C macro-aggregate meso-aggregate micro-aggregate mineral-bound organic C particulate organic C potentially mineralizable C