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Bifunctional passivation by lewis-base molecules for efficient printable mesoscopic perovskite solar cells

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Journal of Energy Chemistry 2024年第9期96卷 177-184页

作者： Hang Yang Jianhong Zhao Xiaodong Ren Tong Zhou Henbing zhang Weilong zhang Jin zhang Guangzhi Hu Yuming zhang Wen-Hua zhang Qingju Liu Yunnan Key Laboratory for Micro/Nano Materials & Technology National Center for International Research on Photoelectric and Energy Materials School of Materials and Energy Yunnan UniversityKunming 650091YunnanChina Institute for Ecological Research and Pollution Control of Plateau Lakes School of Ecology and Environmental Science Yunnan UniversityKunming 650091YunnanChina

Printable mesoscopic perovskite solar cells(PM-PSCs)possess notable merits in terms of cost-effectiveness,easy manufacturing,and large scale ***,the absence of a hole transport layer contributes to the exacerbation of carrier recombination,and the defects between the perovskite and electron transport layer(ETL)interfaces significantly decrease the efficiency of the *** this study,a bifunctional surface passivation approach is proposed by applying a thioacetamide(TAA)surfactant on the mesoporous TiO_(2)*** results demonstrate that TAA molecules could interact with TiO_(2),thereby diminishing the oxygen vacancy ***,the amino group and sulfur atoms in TAA molecules act as Lewis base to effectively passivate the uncoordinated Pb^(2+)in perovskite and improve the morphology of perovskite,and decrease the trap-state density of *** TAA passivation mechanism improves the alignment of energy levels between TiO_(2)and perovskite,facilitating electron transport and reducing carrier ***,the TAA-passivated device achieved a champion power conversion efficiency(PCE)of 17.86%with a high fill factor(FF)of 79.16%and an open-circuit voltage(V_(OC))of 0.971 *** investigation presents a feasible strategy for interfacial passivation of the ETL to further improve the efficiency of PM-PSCs.

关键词： Perovskite solarcells Carbon electrode Thioacetamide Interfacial passivation

A hierarchical enhanced data-driven battery pack capacity estimation framework for real-world operating conditions with fewer labeled data

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Journal of Energy Chemistry 2024年第4期91卷 417-432页

作者： Sijia Yang Caiping zhang Haoze Chen Jinyu Wang Dinghong Chen Linjing zhang Weige zhang National Active Distribution Network Technology Research Center(NANTEC) Beijing Jiaotong UniversityBeijing 100044China

Battery pack capacity estimation under real-world operating conditions is important for battery performance optimization and health management,contributing to the reliability and longevity of batterypowered ***,complex operating conditions,coupling cell-to-cell inconsistency,and limited labeled data pose great challenges to accurate and robust battery pack capacity *** address these issues,this paper proposes a hierarchical data-driven framework aimed at enhancing the training of machine learning models with fewer labeled *** traditional data-driven methods that lack interpretability,the hierarchical data-driven framework unveils the“mechanism”of the black box inside the data-driven framework by splitting the final estimation target into cell-level and pack-level intermediate targets.A generalized feature matrix is devised without requiring all cell voltages,significantly reducing the computational cost and memory *** generated intermediate target labels and the corresponding features are hierarchically employed to enhance the training of two machine learning models,effectively alleviating the difficulty of learning the relationship from all features due to fewer labeled data and addressing the dilemma of requiring extensive labeled data for accurate *** only 10%of degradation data,the proposed framework outperforms the state-of-the-art battery pack capacity estimation methods,achieving mean absolute percentage errors of 0.608%,0.601%,and 1.128%for three battery packs whose degradation load profiles represent real-world operating *** high accuracy,adaptability,and robustness indicate the potential in different application scenarios,which is promising for reducing laborious and expensive aging experiments at the pack level and facilitating the development of battery technology.

关键词： Lithium-ion battery pack Capacity estimation Label generation Multi-machine learning model Real-world operating

Bayesian ensemble methods for predicting ground deformation due to tunnelling with sparse monitoring data

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Underground Space 2024年第3期16卷 79-93页

作者： Zilong zhang Tingting zhang Xiaozhou Li Daniel Dias School of Civil Engineering Central South UniversityChangshaHunan 410075China Laboratory 3SR Grenoble Alpes UniversityCNRS UMR 5521Grenoble 38000France

Numerous analytical models have been developed to predict ground deformations induced by tunneling,which is a critical issue in tunnel ***,the accuracy of these predictions is often limited by errors and uncertainties resulting from model selection and parameter fittings,given the paucity of monitoring data in field *** paper proposes a novel approach to estimate tunnelling-induced ground deformations by applying Bayesian model averaging to several representative prediction *** accounting for both model and parameter uncertainties,this approach enables more realistic predictions of ground deformations than individual ***,our results indicate that the Gonzalez-Sagaseta model outperforms other models in predicting ground surface settlements,while the Loganathan-Poulos model is most suitable for predicting subsurface vertical and horizontal ***,our analysis reveals that when monitoring data are sparse,model uncertainties may contribute up to 78.7%of the total ***,obtaining sufficient data for parameter fitting is crucial for accurate *** proposed method in this study offers a more realistic and efficient prediction of tunnelling-induced ground deformations.

关键词： Tunnelling-induced ground deformations Sparse data Model uncertainties Bayesian model averaging

Strategies to achieve effective nitrogen activation

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Carbon Energy 2024年第5期6卷 137-163页

作者： Bin Chang Huabin zhang Shuhui Sun Gaixia zhang KAUST Catalysis Center(KCC) King Abdullah University of Science and Technology(KAUST)ThuwalKingdom of Saudi Arabia Institut National de la Recherche Scientifique(INRS) CentreÉnergie Matériaux TélécommunicationsVarennesQuébecCanada Department of Electrical Engineering École de Technologie Supérieure(ÉTS)MontréalQuébecCanada

Ammonia serves as a crucial chemical raw material and hydrogen energy *** electrocatalytic nitrogen reduction reaction(NRR),powered by renewable energy,has attracted tremendous interest during the past few *** some achievements have been revealed in aqueous NRR,significant challenges have also been *** activity and selectivity are fundamentally limited by nitrogen activation and competitive hydrogen *** review focuses on the hurdles of nitrogen activation and delves into complementary strategies,including materials design and system optimization(reactor,electrolyte,and mediator).Then,it introduces advanced interdisciplinary technologies that have recently emerged for nitrogen activation using high-energy physics such as plasma and *** a better understanding of the corresponding reaction mechanisms in the coming years,these technologies have the potential to be extended in further *** review provides further insight into the reaction mechanisms of selectivity and stability of different reaction *** then recommend a rigorous and detailed protocol for investigating NRR performance and also highlight several potential research directions in this exciting field,coupling with advanced interdisciplinary applications,in situ/operando characterizations,and theoretical calculations.

关键词： activation via mediators catalyst optimization electrochemical nitrogen fixation high-energy activation of nitrogen nitrogen

Interface Engineering of Titanium Nitride Nanotube Composites for Excellent Microwave Absorption at Elevated Temperature

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Nano-Micro Letters 2024年第9期16卷 147-160页

作者： Cuiping Li Dan Li Shuai zhang Long Ma Lei zhang Jingwei zhang Chunhong Gong College of Chemistry and Molecular Sciences Henan UniversityKaifeng 475004People’s Republic of China National and Local Joint Engineering Research Center for Applied Technology of Hybrid Nanomaterials Henan UniversityKaifeng 475004People’s Republic of China

Currently,the microwave absorbers usually suffer dreadful electromagnetic wave absorption(EMWA)performance damping at elevated temperature due to impedance mismatching induced by increased conduction ***,the development of high-performance EMWA materials with good impedance matching and strong loss ability in wide temperature spectrum has emerged as a top ***,due to the high melting point,good electrical conductivity,excellent environmental stability,EM coupling effect,and abundant interfaces of titanium nitride(TiN)nanotubes,they were designed based on the controlling kinetic diffusion procedure and Ostwald ripening *** from boosted heterogeneous interfaces between TiN nanotubes and polydimethylsiloxane(PDMS),enhanced polarization loss relaxations were created,which could not only improve the depletion efficiency of EMWA,but also contribute to the optimized impedance matching at elevated ***,the TiN nanotubes/PDMS composite showed excellent EMWA performances at varied temperature(298-573 K),while achieved an effective absorption bandwidth(EAB)value of 3.23 GHz and a minimum reflection loss(RLmin)value of−44.15 dB at 423 *** study not only clarifies the relationship between dielectric loss capacity(conduction loss and polarization loss)and temperature,but also breaks new ground for EM absorbers in wide temperature spectrum based on interface engineering.

关键词： TiN nanotubes Interface engineering Polarization loss Impedance matching Electromagnetic wave absorption performance

Protective benefit of folded linear HDPE board sand fences along the Golmud-Korla Railway,China:Field observation and wind tunnel study

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Journal of Mountain Science 2024年第7期21卷 2206-2219页

作者： zhang Kai TIAN Jianjin WANG Zhenghui zhang Hailong zhang Xingxin College of Civil Engineering Lanzhou Jiaotong UniversityLanzhou 730000China Key Laboratory of Desert and Desertification Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China College of Civil Engineering Chongqing UniversityChongqing 400045China

The Milan Gobi area of the Golmud-Korla Railway in northwest China is located in the lower dispersal area of the mountain pass and has strong winds with evident double wind direction *** study introduced a novel sand fence deployment technique,termed‘folded linear deployment',designed to position the sand fence orthogonally to the two predominant wind directions for optimal *** study used wind tunnel and field tests to evaluate the wind and sand flow characteristics,as well as the windproof and sandresistant performance of folded linear HDPE(Highdensity polyethylene)board sand *** results suggest that the airflow around the fence creates clear zoning *** deceleration area on the BSF(backwind side of the sand fence)is much larger than that on the DSF(downwind side of the sand fence).Thus,sand particles are primarily deposited on the *** different wind speeds,the airflow at 2 and 5 h on the DSF is not *** WSP(wind speed profile)presents a logarithmic *** airflow is disturbed at 1-20 h on the BSF,and the WSP gradually deviates from the logarithmic ***,as the airflow moves away from the fence,the WSP gradually approaches a logarithmic ***,the WPE(windproof efficiency)and SRE(sand-resistant efficiency)of the sand fence exceed 80%.In addition,the results of wind tunnel tests are compared with those of field *** overall dispersion is good,and the best dispersion is found at z/H=2.00,indicating good agreement between the two test *** study provides a scientific basis for the design of sand hazard control measures,similar to the railway project in the Gobi Gale area.

关键词： Folded linear HDPE board sand fence Double wind direction Gobi area Protection benefit

Multicolor upconversion reversible modulations in YNbO_(4):Er^(3+)/Tm^(3+)/Yb^(3+) photochromic materials

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Journal of Rare Earths 2024年第2期42卷 270-277,I0002页

作者： Zhen zhang Peng Li Ziyi Xu Zhihao zhang Qiwei zhang Haiqin Sun Xihong Hao Inner Mongolia Key Laboratory of Ferroelectric-related New Energy Materials and Devices Schoolof Materials and MetallurgyInner Mongolia University of Science and TechnologyBaotou014010China College of Physics and Technology Guangxi Normal UniversityGuilin541004China

Photochromic materials with multicolor upconversion reversible modulations are attractive in optical switching ***,the fabricated YNbO_(4):Er^(3+)/Tm^(3+)/Yb^(3+) materials exhibit excellent photochromism and multicolor upconversion properties from green,red to near infrared(NIR) emissions with increasing Yb *** multiband upconversion modulations are achieved by alternating light(365 and 405 nm) or thermal *** 365 nm irradiation,the luminescence color changes from yellow to red,the luminescent photoswitching contrast reaches up to 86.21%(green),82.12%(red) and 77.38%(NIR) in the Y_(0.83)Er_(0.01)Tm_(0.01)NbO_(4):0.15 Yb ***,the upconversion emission intensity before and after photochromic reaction shows remarkable change in a wide temperature range of 298-718 *** results indicate that the Er^(3+)/Tm^(3+)/Yb^(3+) tri-doped YNbO_(4) materials can be a good candidate in optical switching and data storage applications.

关键词： Photochromic materials Luminescence modulation Multicolor emission Photoswitching contrast Rare earths

Neighbor Sum Distinguishing Total Choosability of Planar Graphs with Maximum Degree at Least 10

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Acta Mathematicae Applicatae Sinica 2024年第1期40卷 211-224页

作者： Dong-han zhang You Lu Sheng-gui zhang Li zhang School of Mathematics and Statistics Northwestern Polytechnical UniversityXi’an710129China School of Mathematics and Computer Application Shangluo UniversityShangluo726000China

A neighbor sum distinguishing(NSD)total coloringφof G is a proper total coloring of G such thatΣz∈EG(u)U{u}φ(z)≠Σz∈EG(v)U{v}φ(z)for each edge uv∈E(G),where EG(u)is the set of edges incident with a vertex *** 2015,Pilśniak and Wozniak conjectured that every graph with maximum degreeΔhas an NSD total(Δ+3)-***,Yang et *** that the conjecture holds for planar graphs withΔ≥10,and Qu et *** that the list version of the conjecture also holds for planar graphs withΔ≥*** this paper,we improve their results and prove that the list version of the conjecture holds for planar graphs withΔ≥10.

关键词： planar graphs neighbor sum distinguishing total choosibility combinatorial nullstellensatz discharging method

Anisotropic phonon dynamics in Dirac semimetal PtTe2 thin films enabled by helicity-dependent ultrafast light excitation

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Light(Science & Applications) 2024年第9期13卷 1888-1897页

作者： Ziyang Li Yequan Chen Anke Song Jinzhong zhang Rong zhang Zongzhi zhang Xuefeng Wang Key Laboratory of Micro and Nano Photonic Structures(MOE) School of Information Science and TechnologyFudan UniversityShanghaiChina Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials State Key Laboratory of Spintronics Devices and TechnologiesSchool of Electronic Science and EngineeringCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjingChina Department of Physics School of Physics and Electronic ScienceEast China Normal UniversityShanghaiChina Department of Physics Xiamen UniversityXiamenChina

Coherent phonons have aroused considerable attention in condensed matter physics owing to their extraordinary capacity of reflecting and controlling the physical properties of ***,the investigation on the interaction between coherent phonons and other microscopic particles on the ultrafast timescale within topological systems continues to be an active and unresolved ***,we show the energy transfer of coherent optical phonons(COP)in Dirac semimetal PtTe2 thin films using ultrafast optical pump-probe ***,the helicitydependent light-driven anisotropic COP signals disclose their direct connection with the light-excited anisotropic spinpolarized electrons via an angular momentum ***,we observe the notable decreases in the COP oscillation frequency and the decay rate with increasing temperatures due to the anharmonic phonon-phonon scattering and electron-phonon scattering in the COP dissipation process,*** work paves the way for uncovering the coherent phonons in Dirac semimetals for the potential applications in optoelectronics and optospintronics.

关键词： spectroscopy. phonon Dirac