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Chinese Journal of Polymer Science 2020年第5期38卷 531-539,I0007页

作者： Gui-Qing Wu Xin-Yu Yang Jia-Hui Li Nan Sheng cheng-yi hou Yao-Gang Li Hong-Zhi Wang State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China School of Materials Science and Engineering Nanyang Technological University639798Singapore

The development of lightweight,flexible,and stretchable energy storage systems is essential for state-of-the-art electronic *** propose a new and broad strategy to fabricate a stretchable and conductive GO/CNTs-TPU fiber electrode by direct wet spinning,from which a flexible fibrous supercapacitor is *** fibrous electrode exhibits a high strength of 11.68 MPa,high conductivity of 342 S/cm,and high specific capacitances(21.8 mF/cm,36.45 F/cm^3,and 95 F/g).The specific capacitance of the assembled all-solid-state hybrid fiber-shaped supercapacitor reaches 14.3 F/cm^*** 5000 charge-discharge cycles,97%of the capacitance of the hybrid supercapacitor is *** high-strength electrochemical electrode materials could be potential candidates for applications in practical and large-scale energy storage systems and textile clothes.

关键词： Graphene Carbon nanotubes Thermoplastic polyurethane Supercapacitor Flexibility

The usually caloric and protein percentage of nutritional support on day 4 would predict better prognosis of ICU patients:a retrospective observational study in Taiwan

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The usually caloric and protein percentage of nutritional su...

Identifying the dynamic behaviors in complete reconstruction of Co-based complex precatalysts during electrocatalytic oxygen evolution

第五届两岸四地营养改善学术会议

作者： yi-cheng hou Yan-Chen Su Pei-Chen Weng Hao-Wen Liu Department of Nutrition Taipei Tzu Chi Hospital Buddhist Tzu Chi Medical Foundation

目的:There were no published studies describing the impacts of nutritional support on the prognosis of patients from all kinds of ICU(intensive care unit),including MICU(medical intensive care unit),RCC(respiratory care center)and SlCU(surgical intensive care unit).To determine whether different patterns of nutritional support have relationship with length of stay at ICU.

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Journal of Energy Chemistry 2025年第1期100卷 226-233页

作者： Jingfang Zhang Danyang Wu Linke Cai Youluan Lu Fanpeng cheng Lijuan Shi Qun yi Yao Liu yi Huang Key Laboratory of Green Chemical Engineering Process of Ministry of Education Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education Hubei Key Laboratory of Novel Reactor and Green Chemical Technology School of Chemical Engineering & Pharmacy Wuhan Institute of Technology Key Laboratory of Pesticide & Chemical Biology of Ministry of Education Engineering Research Center of Photoenergy Utilization for Pollution Control and Carbon Reduction of Ministry of Education College of Chemistry Central China Normal University College of Materials Science and Engineering Fuzhou University

Transition metal-based nanomaterials have emerged as promising electrocatalysts for oxygen evolution reaction（OER）. Considerable research efforts have shown that self-reconstruction occurs on these nanomaterials under operating conditions of OER process. However, most of them undergo incomplete reconstruction with limited thickness of reconstruction layer, leading to low component utilization and arduous exploration of real catalytic mechanism. Herein, we identify the dynamic behaviors in complete reconstruction of Co-based complexes during OER. The hollow phytic acid（PA） cross-linked CoFe-based complex nanoboxes with porous nanowalls are designed because of their good electrolyte penetration and mass transport ability, in favor of the fast and complete reconstruction. A series of experiment characterizations demonstrate that the reconstruction process includes the fast substitution of PA by OH-to form Co（Fe）(OH)xand subsequent potential-driven oxidation to Co（Fe）OOH. The obtained CoFeOOH delivers a low overpotential of 290 mV at a current density of 10 mA cm-2and a long-term *** experiment results together with theory calculations reveal that the Fe incorporation can result in the electron rearrangement of reconstructed CoFeOOH and optimization of their electronic structure,accounting for the enhanced OER activity. The work provides new insights into complete reconstruction of metal-based complexes during OER and offers guidelines for rational design of high-performance electrocatalysts.

关键词： Oxygen evolution reaction

Crystallization Modulation and Holistic Passivation Enables Efficient Two‑Terminal Perovskite/CuIn(Ga)Se_(2)Tandem Solar Cells

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Nano-Micro Letters 2025年第1期17卷 205-215页

作者： Cong Geng Kuanxiang Zhang Changhua Wang Chung Hsien Wu Jiwen Jiang Fei Long Liyuan Han Qifeng Han yi‑Bing cheng Yong Peng State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070People’s Republic of China Triumph Photovoltaic Materials Co. Ltd.No.1001 Yannan AvenueHigh‑Tech Development DistrictBengbuAnhui 233000People’s Republic of China College of Materials Science and Engineering Guilin University of TechnologyGuilin 541004People’s Republic of China State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China

Two-terminal(2-T)perovskite(PVK)/CuIn(Ga)Se_(2)(CIGS)tandem solar cells(TSCs)have been considered as an ideal tandem cell because of their best bandgap matching regarding to Shockley–Queisser(S–Q)***,the nature of the irregular rough morphology of commercial CIGS prevents people from improving tandem device *** this paper,D-homoserine lactone hydrochloride is proven to improve coverage of PVK materials on irregular rough CIGS surfaces and also passivate bulk defects by modulating the growth of PVK *** addition,the minority carriers near the PVK/C60 interface and the incompletely passivated trap states caused interface recombination.A surface reconstruction with 2-thiopheneethylammonium iodide and N,N-dimethylformamide assisted passivates the defect sites located at the surface and grain ***,LiF is used to create this field effect,repelling hole carriers away from the PVK and C60 interface and thus reducing *** a result,a 2-T PVK/CIGS tandem yielded a power conversion efficiency of 24.6%(0.16 cm^(2)),one of the highest results for 2-T PVK/CIGS TSCs to our *** validation underscores the potential of our methodology in achieving superior performance in PVK/CIGS tandem solar cells.

关键词： PVK/CIGS TSCs Irregular rough surfaces Modulating the growth PVK/C60 interface recombination

Spin-modulated near-infrared-Ⅰ emission in a xanthene-decorated Fe(Ⅱ) spin-crossover complex

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Science China Chemistry 2025年

作者： cheng yi Duyong Chen Shihui Zhang Rui Cai Chunying Duan yinshan Meng Tao Liu State Key Laboratory of Fine Chemicals Frontier Science Center for Smart Materials and Chemical Engineering School of Chemical Engineering Dalian University of Technology Instrumental Analysis Center Dalian University of Technology School of Chemistry Dalian University of Technology Liaoning Binhai Laboratory

Molecular materials showing synergetic coupling of near-infrared （NIR） fluorescence and spin-crossover （SCO） are promisingly applicable in in-vivo bioimaging,temperature sensing,and spintronic *** the related study faces formidable *** this work we graft the NIR fluorophore xanthene onto the dipyridyl substituted triazole ligand and construct a new Febased SCO material,{FeⅡ（ddxc-abpt）2[N（CN）2]2}(1,ddxc-abpt:（E）-4-(((3,5-di（pyridin-2-yl）-4H-1,2,4-triazol-4-yl)imino)methyl)-N,N-diethyl-2,3-dihydro-1H-xanthen-6-amine).Magnetic studies indicate that compound 1 exhibits thermally induced SCO property in both the solid and solution ***-temperature fluorescence emission spectra reveal a remarkable 7-fold increase in photoluminescence intensity upon the transition from the low-spin state at 110 K to the high-spin state at 280 K,which is the record of all reported coupled fluorescence-SCO ***-temperature ultraviolet-visible （UV-Vis）absorption spectra show a significant change in absorption intensity within the fluorescence emission window,consistent with the F?rster resonance energy transfer （FRET） ***-dependent density functional theory （TD-DFT） calculations demonstrate that the strong coupling is attributed to disrupted energy transfer between the xanthene fluorophore and high-spin *** work provides a feasible approach for expanding the synergetic SCO-fluorescence materials to the NIR-Iwavelength region,and hopefully contributes to the applications of tunable NIR-SCO molecule-based sensors and devices.

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磁控溅射法生长Bi2Te3/CoFeB双层异质结太赫兹发射

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物理学报 2020年第20期69卷 76-81页

作者：张帆许涌柳洋程厚义张晓强杜寅昌吴晓君赵巍胜北京航空航天大学微电子学院大数据科学与脑机智能高精尖创新中心北京100191 北京航空航天大学北航合肥创新研究院合肥230012 北京航空航天大学电子信息工程学院北京100191

自旋太赫兹源作为一种新型太赫兹辐射源,以其高效率、超宽带、低成本、易集成等优点已成为太赫兹科学与应用领域的研究热点.本实验报道了晶圆级磁控溅射生长的多晶拓扑绝缘体Bi2Te3和铁磁体CoFeB双层异质结纳米薄膜发射太赫兹电磁波,并... 详细信息

自旋太赫兹源作为一种新型太赫兹辐射源,以其高效率、超宽带、低成本、易集成等优点已成为太赫兹科学与应用领域的研究热点.本实验报道了晶圆级磁控溅射生长的多晶拓扑绝缘体Bi2Te3和铁磁体CoFeB双层异质结纳米薄膜发射太赫兹电磁波,并对太赫兹辐射特性进行了深入而系统的实验研究.在飞秒激光放大级脉冲作用下,该异质结呈现出高效率的太赫兹发射,且辐射偏振可通过外加磁场方向控制.通过与Pt/CoFeB对比,研究发现Bi2Te3/CoFeB的发射性能与Pt/CoFeB双层异质结相当.实验还对生长在不同衬底上的Bi2Te3/CoFeB的发射性能进行了对比研究,发现MgO衬底上制备的样品具有相对较好的太赫兹辐射性能.本实验研究不仅对自旋太赫兹发射机理有更加深入的认识,而且通过样品和结构的优化,有望获得更高的发射效率,且该发射器具有大尺寸批量生长、成本较低的优势,具备商业化应用的潜力.

关键词：太赫兹辐射拓扑绝缘体/铁磁异质结飞秒激光

Catalytic atroposelective synthesis of indolyl quinazolinones bearing N-N/C-C diaxes

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Science China Chemistry 2025年

作者： Ning-yi Wang Shuo Gao Zhu-Di Shu Bei-Bei cheng Chun Ma Yu-Chen Zhang Feng Shi Research Center of Chiral Functional Heterocycles School of Chemistry and Materials Science Jiangsu Normal University School of Petrochemical Engineering Changzhou University School of Chemistry and Chemical Engineering Henan Normal University

The first catalytic atroposelective synthesis of indole derivatives bearing N-N/C-C diaxes has been established by the strategy of de novo ring formation. By this strategy, various indolyl quinazolinones bearing vicinal N-N/C-C diaxes were synthesized in high yields with overall good diastereoselectivities and excellent enantioselectivities via chiral phosphoric acid-catalyzed onepot asymmetric formal (5+1) cycloaddition/oxidation reaction. Moreover, such indolyl quinazolinones bearing vicinal N-N/CC diaxes have good configurational stability and could be converted into new chiral ligands with applications in asymmetric catalysis. Therefore, this work not only offered a new member for the family of diaxial atropisomers, but also provided a powerful strategy for catalytic asymmetric synthesis of atropisomers bearing N-N/C-C diaxes.

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Smart molecular crystal switches

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Smart Molecules

Smart Molecules 2024年第1期2卷 9-24页

作者： Ian cheng-yi hou Liang Li Hongyu Zhang Panče Naumov Smart Materials Lab New York University Abu DhabiAbu DhabiUnited Arab Emirates State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchunChina Center for Smart Engineering Materials New York University Abu DhabiAbu DhabiUnited Arab Emirates Research Center for Environment and Materials Macedonian Academy of Sciences and ArtsSkopjeMacedonia Department of Chemistry Molecular Design InstituteNew York UniversityNew YorkUSA

The multifaceted switches are part of our everyday life from the macroscopic to the molecular world.A molecular switch operating in the solution and in the crystalline state is very *** this review,we summarize the state-of-the-art of smart molecular crystal switches based on molecular *** crystal switches respond to external stimuli and reversibly change between states,retaining their macroscopic *** operation of the switches predominantly relies on temperature alterations or mechanical stress,with emerging methods based on photothermal effects,photoisomerization,and host-guest *** capability of changing the molecular orientation and interaction in smart molecular crystal switches offers opportunities in several applications,including actuators,reversibly shaping structural materials,optoelectronic and magnetic materials,as well as switchable porous *** molecular crystal switches have vast potential in modern scientific and technological *** ongoing research shapes a rich landscape for innovation and future scientific exploration across diverse disciplines.

关键词： martensitic transition molecular switch phase transition single crystal smart material

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新时代高校师德失范行为惩戒的法治化构造

黑龙江高教研究 2025年第1期43卷 15-21页

作者：王羿程中国人民公安大学北京100038

高校师德失范行为惩戒既是新时代师德师风建设的核心部分,更是推进教育治理现代化的关键命题。当前高校师德失范行为惩戒面临两个方面困境:一是制度层面的供给不足;二是在实施机制中存在参与通道不畅、教师权利的实效性救济困难等问题... 详细信息

高校师德失范行为惩戒既是新时代师德师风建设的核心部分,更是推进教育治理现代化的关键命题。当前高校师德失范行为惩戒面临两个方面困境:一是制度层面的供给不足;二是在实施机制中存在参与通道不畅、教师权利的实效性救济困难等问题。应当明确,法治既是新时代教育治理现代化的基本目标与重要内容,也是高校教育治理现代化的基本路径,更是高校进行师德失范行为惩戒必须遵循的基本模式。通过法治化的建构路径,于静态维度准确界定惩戒的启动条件,划定惩戒的适用范围;于动态维度畅通多元主体的利益诉求表达通道。进而,在实践维度强化高校自主化、专业化实施师德失范行为惩戒的能力,在中国式现代化的时代格局下,有力推进高校教育治理现代化。

关键词：教育治理现代化师德失范行为惩戒制度困境法治化建构阶层化构造

Effects of coal seam dip angle on the outburst in coal roadway excavation

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International Journal of Mining Science and Technology 2019年第5期29卷 757-764页

作者： cheng hou yinghua Zhang yi Yan University of Science and Technology Beijing Beijing 100083China Department of Mechanical Engineering McGill UniversityMontrealQC H3A 0C3Canada

The prevention and forecast of coal and gas outburst has always been one of the key issues in coal mining *** simulating the process of tunneling in coal seam with different dip angle through FLAC3D software,the dangerous zone in which outburst may occur and the probability of outburst near the working face were predicted through the distribution of stress,displacement and plastic *** we discussed the size of unstable area in the surrounding rock through the distribution of stress and the variation curve of the displacement on the roadway *** results show that,with an increase of the coal seam dip angle,the risk of outburst in the working face rises *** the dangerous areas in which may outburst occur moves to the upper part of coal *** size of unstable area in the surrounding rock increases with the increase of coal seam dip angle.

关键词： Dip angle Stress concentration Plastic zone Displacement Coal and gas outburst