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Spontaneous Orientation Polarization of Anisotropic Equivalent Dipoles Harnessed by Entropy Engineering for Ultra‑Thin Electromagnetic Wave Absorber

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Nano-Micro Letters 2025年第1期17卷 424-438页

作者： Honghan Wang Xinyu Xiao Shangru Zhai Chuang Xue Guangping Zheng Deqing Zhang Renchao che Junye cheng Liaoning Key Lab of Lignocellulose chemistry and BioMaterials Liaoning Collaborative Innovation Center for Lignocellulosic BiorefinerySchool of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034People’s Republic of China School of Life Science and Biotechnology Dalian University of TechnologyDalian 116024People’s Republic of China Department of Mechanical Engineering Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China School of Materials Science and Engineering Qiqihar UniversityQiqihar 161006People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Department of Materials Science Shenzhen MSU-BIT UniversityShenzhen 517182People’s Republic of China

The synthesis of carbon supporter/nanoscale high-entropy alloys(HEAs)electromagnetic response composites by carbothermal shock method has been identified as an advanced strategy for the collaborative competition engineering of conductive/dielectric *** migration modes within HEAs as manipulated by the electronegativity,valence electron configurations and molar proportions of constituent elements determine the steady state and efficiency of equivalent ***,enlightened by skin-like effect,a reformative carbothermal shock method using carbonized cellulose paper(CCP)as carbon supporter is used to preserve the oxygencontaining functional groups(O·)of carbonized cellulose fibers(CCF).Nucleation of HEAs and construction of emblematic shell-core CCF/HEAs heterointerfaces are inextricably linked to carbon metabolism induced by O·.Meanwhile,the electron migration mode of switchable electronrich sites promotes the orientation polarization of anisotropic equivalent *** virtue of the reinforcement strategy,CCP/HEAs composite prepared by 35%molar ratio of Mn element(CCP/HEAs-Mn_(2.15))achieves efficient electromagnetic wave(EMW)absorption of−51.35 dB at an ultra-thin thickness of 1.03 *** mechanisms of the resulting dielectric properties of HEAs-based EMW absorbing materials are elucidated by combining theoretical calculations with experimental characterizations,which provide theoretical bases and feasible strategies for the simulation and practical application of electromagnetic functional devices(e.g.,ultra-wideband bandpass filter).

关键词： High-entropy alloys Carbothermal shock Switchable electron migration modes Emblematic shell-core heterointerfaces Ultra-thin thickness

“Zero‑Strain” NiNb_(2)O_(6) Fibers for All‑Climate Lithium Storage

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Nano-Micro Letters 2025年第1期17卷 348-360页

作者： Yan Zhao Qiang Yuan Liting Yang Guisheng Liang Yifeng cheng Limin Wu Chunfu Lin Renchao che College of Physics Donghua UniversityShanghai 201620People’s Republic of China School of Materials Science and Engineering Institute of Materials for Energy and EnvironmentQingdao UniversityQingdao 266071People’s Republic of China Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Zhejiang Laboratory Hangzhou 311100People’s Republic of China Inner Mongolia University Hohhot 010021People’s Republic of China

Niobates are promising all-climate Li^(+)-storage anode material due to their fast charge transport,large specific capacities,and resistance to electrolyte ***,their moderate unit-cellvolume expansion(generally 5%–10%)during Li^(+)storage causes unsatisfactory long-term ***,“zero-strain”NiNb_(2)O_(6) fibers are explored as a new anode material with comprehensively good electrochemical *** Li^(+)storage,the expansion of electrochemical inactive NiO_(6) octahedra almost fully offsets the shrinkage of active NbO_(6) octahedra through reversible O *** superior volume-accommodation capability of the NiO_(6) layers guarantees the“zero-strain”behavior of NiNb_(2)O_(6) in a broad temperature range(0.53%//0.51%//0.74%at 25//−10//60℃),leading to the excellent cyclability of the NiNb_(2)O_(6) fibers(92.8%//99.2%//91.1%capacity retention after 1000//2000//1000 cycles at 10C and 25//−10//60℃).This NiNb_(2)O_(6) material further exhibits a large reversible capacity(300//184//318 mAh g−1 at 0.1C and 25//−10//60℃)and outstanding rate performance(10 to 0.5C capacity percentage of 64.3%//50.0%//65.4%at 25//−10//60℃).Therefore,the NiNb_(2)O_(6) fibers are especially suitable for large-capacity,fast-charging,long-life,and all-climate lithium-ion batteries.

关键词： NiNb_(2)O_(6)porous fiber “Zero-strain”mechanism Electrochemical property Harsh-temperature operation Operando characterization

Designing Electronic Structures of Multiscale Helical Converters for Tailored Ultrabroad Electromagnetic Absorption

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Nano-Micro Letters 2025年第1期17卷 439-455页

作者： Zhaobo Feng Chongbo Liu Xin Li Guangsheng Luo Naixin Zhai Ruizhe Hu Jing Lin Jinbin Peng Yuhui Peng Renchao che Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle School of Environmental and Chemical EngineeringNanchang Hangkong UniversityNanchang 330063People’s Republic of China School of Physics and Materials Nanchang UniversityNanchang 330031People’s Republic of China Key Laboratory of Nondestructive Testing Ministry of EducationNanchang Hangkong UniversityNanchang 330063People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering and TechnologyFudan UniversityShanghai 200438People’s Republic of China

Atomic-scale doping strategies and structure design play pivotal roles in tailoring the electronic structure and physicochemical property of electromagnetic wave absorption(EMWA)***,the relationship between configuration and electromagnetic(EM)loss mechanism has remained ***,drawing inspiration from the DNA transcription process,we report the successful synthesis of novel in situ Mn/N co-doped helical carbon nanotubes with ultrabroad EMWA *** calculation and EM simulation confirm that the orbital coupling and spin polarization of the Mn–N4–C configuration,along with cross polarization generated by the helical structure,endow the helical converters with enhanced EM *** a result,HMC-8 demonstrates outstanding EMWA performance,achieving a minimum reflection loss of−63.13 dB at an ultralow thickness of 1.29 *** precise tuning of the graphite domain size,HMC-7 achieves an effective absorption bandwidth(EAB)of 6.08 GHz at 2.02 mm ***,constructing macroscale gradient metamaterials enables an ultrabroadband EAB of 12.16 GHz at a thickness of only 5.00 mm,with the maximum radar cross section reduction value reaching 36.4 dB *** innovative approach not only advances the understanding of metal–nonmetal co-doping but also realizes broadband EMWA,thus contributing to the development of EMWA mechanisms and applications.

关键词： Metal-nonmetal co-doping 3d-2p orbital coupling Spin polarization Helical structure Broadband EM wave absorption

THE MORTAR ELEMENT METHOD FOR A NONLINEAR BIHARMONIC EQUATION

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Journal of Computational Mathematics 2005年第5期23卷 537-560页

作者： Shi, zc Xu, XJ CHINESE ACAD SCI

The mortar element method is a new domain decomposition method（DDM） with nonoverlapping subdomains. It can handle the situation where the mesh on different subdomains need not align across interfaces, and the matching of discretizations on adjacent subdomains is only enforced weakly. But until now there has been very little work for nonlinear PDEs. In this paper, we will present a mortar-type Morley element method for a nonlinear biharmonic equation which is related to the well-known Navier-Stokes equation. Optimal energy and H^1-norm estimates are obtained under a reasonable elliptic regularity assumption.

关键词： Mortar method Nonlinear biharmonic equation H^1-norm error Energy norm error

SUBSTRUCTURE PRECONDITIONERS FOR NONCONFORMING PLATE ELEMENTS

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Journal of Computational Mathematics 1998年第4期16卷 289-304页

作者： Shi, zc Xie, ZH Chinese Acad Sci ICMSEC State Key Lab Sci & Engn Comp Beijing 100080 Peoples R China Chinese Acad Sci Inst Atmospher Phys LASG Beijing 100080 Peoples R China

In this paper, we consider the problem of solving finite element equations of biharmonic Dirichlet problems. We divide the given domain into non-overlapping subdomains, construct a preconditioner for Morley element by substructuring on the basis of a function decomposition for discrete biharmonic functions. The function decomposition is introduced by partitioning these finite element functions into the low and high frequency components through the intergrid transfer operators between coarse mesh and fine mesh, and the conforming interpolation operators. The method leads to a preconditioned system with the condition number bounded by C(1 + log(2) H/h) in the case with interior cross points, and by C in the case without interior cross points, where H is the subdomain size and h is the mesh size. These techniques are applicable to other nonconforming elements and are well suited to a parallel computation.

关键词： substructure preconditioner biharmonic equation nonconforming plate element

MULTIGRID METHODS FOR MORLEY ELEMENT ON NONNESTED MESHES

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Journal of Computational Mathematics 1998年第5期16卷 385-394页

作者： Shi, zc Xie, ZH Chinese Acad Sci ICMSEC State Key Lab Sci & Engn Comp Beijing 100080 Peoples R China Chinese Acad Sci Inst Atmospher Phys LASG Beijing 100080 Peoples R China

In this paper, we consider some multigrid algorithms for the biharmonic problem discretized by Morley element on nonnested meshes. Through taking the averages of the nodal variables we construct an intergrid transfer operator that satisfies a certain stable approximation property. The so-called regularity-approximation assumption is then established. Optimal convergence properties of the W-cycle and a uniform condition number estimate for the variable V-cycle preconditioner are presented. This technique is applicable to other nonconforming plate elements.

关键词： multigrid method Morley element nonnested meshes

Discrete Element with Flexible Connector for Dynamic Analysis of 3-D Beam Structures

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China Ocean Engineering 1997年第1期12卷 11-20页

作者： cheng, BR Zheng, zc Hou, zc Department of Engineering Mechanics Tsinghua University Beijing 100084 China

Combined multi-body dynamics with structural dynamics, a new discrete element with flexible connector, which is applicable for 3-D beam structures, is developed in this paper. Both the generalized elastic coefficient matrix of the flexible connector and the mass matrix of discrete element may be off-diagonal in a general case. The zero-length rigid element is introduced to simulate the node at which multiple elements are jointed together. It may also be effective when the axes of adjacent elements are not in the same line. The examples for eigenvalue calculation show that the model is successful. It can be extended to the geometric nonlinear response analysis.

关键词： discrete element flexible connector zero-length rigid element 3-D beam structures dynamic analysis

Preparation　of　Homocitrate　using　a　Modified　Method

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chemical Research in Chinese Universities 1998年第1期14卷 93-95页

作者： Li, zc Xu, JQ Inner Mongolia Natl Teachers Coll Dept Chem Tongliao 028043 Peoples R China Jilin Univ Dept Chem Changchun 130023 Peoples R China

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ＰｒｅｐａｒａｔｉｏｎｏｆＨｏｍｏｃｉｔｒａｔｅｕｓｉｎｇａＭｏｄｉｆｉｅｄＭｅｔｈｏｄＬＩＺｅｎｇ－ｃｈｕｎ（ＤｅｐａｒｔｍｅｎｔｏｆＣｈｅｍｉｓｔｒｙ，ＩｎｎｅｒＭｏｎｇｏｌｉａＮａｔｉｏｎａｌＴｅａｃｈｅｒｓＣｏｌｌｅｇｅ，Ｔｏｎｇｌｉａｏ，０...

关键词： Preparation using Modified Homocitrate Method

A Monte-Carlo Approach to Cellular Pattern Evolution for Binary Alloys during Directional Solidification

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Journal of Materials Science & Technology 1995年第2期11卷 127-132页

作者： LIU, JM LIU, ZG WU, zc Nanjing Univ Nanjing China

A Monte-Carlo approach of cellular pattern evolution during directional solidification of a binary alloy has been carried out by imposing a non-uniform probability distribution of particle emission from the particle source, as an approach to the contribution of solute redistribution to the interface evolution. Both the bulk and interface diffusion have been involved in the simulation, and coarsening of the cellular patterns with time has been clearly revealed. The remarkable influence of the interface relaxation and the solute redistribution on the profile bf;solidifying interface has been presented.

关键词： Monte Carlo methods