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Displacement Current in Domain Walls of Bismuth Ferrite

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npj Computational Materials 2018年第1期4卷 597-605页

作者： Sergey Prosandeev Yurong Yang charles paillard L.Bellaiche Physics Department and Institute for Nanoscience and Engineering University of ArkansasFayettevilleAR 72701USA Institute of Physics and Physics Department of Southern Federal UniversityRostov-na-Donu 344090Russia

In 1861,Maxwell conceived the idea of the displacement current,which then made laws of electrodynamics more complete and also resulted in the realization of devices exploiting such displacement ***,it is presently unknown if such displacement current can result in large intrinsic ac current in ferroic systems possessing domains,despite the flurry of recent activities that have been devoted to domains and their corresponding conductivity in these ***,we report firstprinciples-based atomistic simulations that predict that the transverse(polarization-related)displacement currents of 71°and 109°domains in the prototypical BiFeO_(3) multiferroic material are significant at the walls of such domains and in the GHz regime,and,in fact,result in currents that are at least of the same order of magnitude than previously reported dc currents(that are likely extrinsic in nature and due to electrons).Such large,localized and intrinsic ac currents are found to originate from low-frequency vibrations at the domain walls,and may open the door to the design of novel devices functioning in the GHz or THz range and in which currents would be confined within the domain wall.

关键词： currents regime magnitude

Strain control of layer-resolved negative capacitance in superlattices

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npj Computational Materials 2020年第1期6卷 127-130页

作者： Raymond Walter Sergey Prosandeev charles paillard L.Bellaiche Department of Physics and Institute for Nanoscience and Engineering University of ArkansasFayettevilleAR 72701USA Department of Mathematical Sciences University of ArkansasFayettevilleAR 72701USA Identity Engineering Kinesso LLCConwayAR 72032USA Institute of Physics and Physics Department of Southern Federal University Rostov-na-Donu 344090Russia Laboratoire Structures Propriétés et Modélisation des SolidesCentraleSupélecUMR CNRS 8580UniversitéParis-Saclay91190 Gif-sur-YvetteFrance

Negative capacitance in BaTiO_(3)/SrTiO_(3) superlattices is investigated by Monte Carlo simulations in an atomistic effective Hamiltonian model,using fluctuation formulas for responses to the local macroscopic field that incorporates depolarizing *** show that epitaxial strain can tune the negative capacitance of the BaTiO_(3) ferroelectric layer and the overall capacitance of the *** addition,we predict and explain an original switching of the negative capacitance from the BaTiO3 layer to the SrTiO_(3) layer at low temperatures for intermediate strains.

关键词： capacitance layer resolved

Strain-induced resonances in the dynamical quadratic magnetoelectric response of multiferroics

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npj Computational Materials 2020年第1期6卷 1156-1161页

作者： S.Omid Sayedaghaee charles paillard Sergey Prosandeev Bin Xu Laurent Bellaiche Physics Department and Institute for Nanoscience and Engineering University of ArkansasFayettevilleArkansas 72701USA Microelectronics-Photonics Program University of ArkansasFayettevilleArkansas 72701USA Laboratoire Structures Propriétés et Modélisation des SolidesCentraleSupélecCNRS UMR 8580UniversitéParis-Saclay91190 Gifsur-YvetteFrance Institute of Physics and Physics Department of Southern Federal University Rostov-na-Donu 344090Russia School of Physical Science and Technology Soochow UniversitySuzhouJiangsu 215006China

For the last few years,the research interest in magnetoelectric(ME)effect,which is the cross-coupling between ferroelectric and magnetic ordering in multiferroic materials,has experienced a significant *** extensive recent studies are not only conducted towards the design of sensors,actuators,transducers,and memory devices by taking advantage of the cross-control of polarization(or magnetization)by magnetic(or electric)fields,but also aim to create a clearer picture in understanding the sources of ME responses and the novel effects associated with *** we derive analytical models allowing to understand the striking and novel dynamics of ME effects in multiferroics and further confirm it with atomistic ***,the role of strain is revealed to lead to the existence of electroacoustic magnons,a new quasiparticle that mixes acoustic and optical phonons with magnons,which results in resonances and thus a dramatic enhancement of magnetoelectric ***,a unique aspect of the dynamical quadratic ME response under a magnetic field with varying frequencies,which is the second harmonic generation(SHG),has not been discussed prior to the present *** SHGs put emphasis on the fact that nonlinearities should be considered while dealing with such systems.

关键词： quadratic dynamical resonance

Tailoring properties of hybrid perovskites by domain-width engineering with charged walls

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npj Computational Materials 2018年第1期4卷 26-31页

作者： Lan Chen charles paillard Hong Jian Zhao JorgeÍñiguez Yurong Yang Laurent Bellaiche Physics Department and Institute for Nanoscience and Engineering University of ArkansasFayettevilleArkansas 72701USA Materials Research and Technology Department Luxembourg Institute of Science and Technology(LIST)5 Avenue des Hauts-FourneauxL-4362 Esch/AlzetteLuxembourg National Laboratory of Solid State Microstructures Jiangsu Key Laboratory of Artificial Functional Materials and Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China

Charged ferroelectric domain walls are fascinating electrical topological defects that can exhibit unusual ***,in the search for novel phenomena,we perform and analyze first-principles calculations to investigate the effect of domain width on properties of domains with charged walls in the photovoltaic material consisting of methylammonium lead iodide hybrid *** report that such domains are stable and have rather low domain wall energy for any investigated width(that is,up to 13 lattice constants).Increasing the domain width first linearly decreases the electronic band gap from≃1.4 eV to about zero(which therefore provides an efficient band-gap engineering),before the system undergoes an insulator-to-metal transition and then remains metallic(with both the tail-to-tail and head-to-head domain walls being conductive)for the largest *** these results can be understood in terms of:(i)components of polarization along the normal of the domain walls being small in magnitude;(ii)an internal electric field that is basically independent of the domain width;and(iii)rather negligible charge transfer between *** findings deepen the knowledge of charged ferroelectric domain walls and can further broaden their potential for applications,particularly in the context of halide perovskites for photovoltaics.

关键词： properties walls perovskite

Author Correction:Strain engineering of electro-optic constants in ferroelectric materials

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npj Computational Materials 2019年第1期5卷 254-255页

作者： charles paillard Sergei Prokhorenko Laurent Bellaiche Department of Physics and Institute for Nanoscience and Engineering University of ArkansasFayettevilleAR 72701USA

After publishing this article,we realized that the calculation of the piezoelectric constants dij by Density Functional Perturbation Theory(DFPT),as explained in the methods described in the original version of the Supplementary Information,are incorrect in the case of a partially clamped *** correct methodology is to inverse the subspace matrix of elastic constants.

关键词： constants ferroelectric piezoelectric

Design and current progress of the Apollon 10 PW project

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High Power Laser Science and Engineering 2015年第1期3卷 32-35页

作者： J.P.Zou C.Le Blanc D.N.Papadopoulos G.Chériaux P.Georges G.Mennerat F.Druon L.Lecherbourg A.Pellegrina P.Ramirez F.Giambruno A.Fréneaux F.Leconte D.Badarau J.M.Boudenne *** T.Valloton J.L.paillard J.L.Veray M.Pina P.Monot J.P.Chambaret P.Martin F.Mathieu P.Audebert F.Amiranoff Laboratoire pour l’Utilisation des Lasers Intenses CNRSEcole Polytechnique Laboratoire d’Optique Appliquée ENSTA Paris TechCNRS Laboratoire charles Fabry UMR 8501Institut d’OptiqueCNRSUniversité Paris Sud CEA IramisSPAM

The objective of the Apollon project is the generation of 10 PW peak power pulses of 15 fs at 1 shot/minute. In this paper the Apollon facility design, the technological challenges and the current progress of the proj... 详细信息

关键词： titanium lasers PW class facilities

Characterization and performance of the Apollon short-focal-area facility following its commissioning at 1 PW level

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Matter and Radiation at Extremes 2021年第6期6卷 12-25页

作者： K.Burdonov A.Fazzini V.Lelasseux J.Albrecht P.Antici Y.Ayoul A.Beluze D.Cavanna T.Ceccotti M.Chabanis A.Chaleil S.N.Chen Z.Chen F.Consoli M.Cuciuc X.Davoine J.P.Delaneau E.d’Humieres J.-L.Dubois C.Evrard E.Filippov A.Freneaux P.Forestier-Colleoni L.Gremillet V.Horny L.Lancia L.Lecherbourg N.Lebas A.Leblanc W.Ma L.Martin F.Negoita J.-L.paillard D.Papadopoulos F.Perez S.Pikuz G.Qi F.Quere L.Ranc P.-A.Soderstrom M.Sciscio S.Sun S.Vallieres P.Wang W.Yao F.Mathieu P.Audebert J.Fuchs LULI–CNRS CEASorbonne UniversiteEcole PolytechniqueInstitut Polytechnique de ParisF-91128 Palaiseau CedexFrance Sorbonne Universite Observatoire de ParisUniversite PSLCNRSLERMAF-75005 ParisFrance IAP Russian Academy of Sciences603155 Nizhny NovgorodRussia INRS-EMT 1650Boulevard Lionel-BouletVarennesQuebec J3X 1S2Canada Universite Paris-Saclay CEACNRSLIDYL91191Gif-sur-YvetteFrance Universite Paris-Saclay CEALMCE91680 Bruy`eres-le-ChˆatelFrance “Horia Hulubei”National Institute for Physics and Nuclear Engineering 30 Reactorului StreetRO-077125 Bucharest-MagureleRomania ENEA Fusion and Technologies for Nuclear Safety DepartmentC.R.FrascatiVia E.Fermi 4500044 FrascatiItaly University of Bordeaux Centre Lasers Intenses et ApplicationsCNRSCEAUMR 5107F-33405 TalenceFrance Joint Institute for High Temperatures RAS125412 MoscowRussia Laboratoire d’Optique Appliquee Ecole Polytechnique–ENSTA–CNRS–Institut Polytechnique de ParisPalaiseauFrance State Key Laboratory of Nuclear Physics and Technology School of PhysicsCAPTPeking UniversityBeijing 100871China Laboratoire charles Fabry Institut d’Optique Graduate SchoolCNRSUniversite Paris-Saclay91127 Palaiseau CedexFrance

We present the results of the first commissioning phase of the short-focal-length area of the Apollon laser facility(located in Saclay,France),which was performed with the first available laser beam(F2),scaled to a nominal power of 1 *** the conditions that were tested,this beam delivered on-target pulses of 10 J average energy and 24 fs *** diagnostics were fielded to assess the performance of the *** on-target focal spot and its spatial stability,the temporal intensity profile prior to the main pulse,and the resulting density gradient formed at the irradiated side of solid targets have been thoroughly characterized,with the goal of helping users design future *** of energetic electrons,ions,and electromagnetic radiation were recorded,showing good laser-to-target coupling efficiency and an overall performance comparable to that of similar international *** will be followed in 2022 by a further commissioning stage at the multipetawatt level.

关键词： performance beam nominal