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Fabrication of heteroatom-doped cobalt oxide yolk-shell microsphere using recycled solution from waste materials and their excellent electrochemical properties as an anode material for lithium-ion batteries

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Rare Metals 2024年第10期43卷 4934-4947页

作者： Yeong Beom kim chanho kim Seung-Hyun kim Yun Chan Kang Dongju Lee Gi Dae Park Department of Advanced Materials Engineering Chungbuk National UniversityChungbuk 28644Korea Department of Materials Science and Engineering Korea UniversitySeoul 136-713Korea Research Institute YKSintering Co.Ltd.Chungbuk 28581Korea

Heteroatom-doped transition metal oxides have attracted great attention as advanced anode materials for lithium-ion batteries due to their high theoretical capacity and superior ***,the limited resource availability has led to a substantial rise in prices for valuable metals such as Ni and Co,posing a significant challenge for their *** address this issue,recycling of these metals from waste materials have gained prominence,and particularly the recovery of Co has been mostly focused on its economic ***,we introduced a novel recycling strategy for fabrication of heteroatomdoped CoO_(x)(comprising mainly Co_(3)O_(4)with a minor CoO phase)anode with a yolk–shell structure for lithium-ion batteries,by separating Co from cemented tungsten carbide *** employing a simple leaching process and subsequent spray pyrolysis,the yolk–shell structured microsphere comprising CoO_(x)was successfully ***,the presence of other waste metals in the leachate facilitated multi-heteroatom doping during ***,the introduction of various dopants into CoO_(x)induced oxygen vacancy formation,thereby enhancing the electrochemical properties of the CoO_(x)*** a result,compared with the phase-pure(undoped)CoO_(x)yolk–shell,the heteroatom-doped CoO_(x)yolk–shell exhibited robust cycling stability(602 mAh·g^(-1)for 200 cycles at 1 A·g^(-1))and excellent rate capability(210 mAh·g^(-1)at 10 A·g^(-1)).

关键词： Recycling Heteroatom doping Cobalt oxide Anode Lithium-ion batteries

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Electrolyte accessibility of non-precious-metal catalysts with different spherical particle sizes under alkaline conditions for oxygen reduction reaction

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Journal of Energy Chemistry 2021年第1期30卷 326-331,I0011页

作者： Jiyeon Lee Jong Gyeong kim chanho Pak Graduate Program of Energy Technology School of Integrated TechnologyInstitute of Integrated TechnologyGwangju Institute of Science and TechnologyGwangju 61005Republic of Korea

Fuel cells are one of the most competitive alternative energy sources because their theoretical efficiency is~15%higher than that of internal combustion engines (ICEs) and they are considered cleaner and *** fuel cells are used to replace ICEs in cars and energy conversion systems,the system efficiency increases;furthermore,the process becomes more environmentally-friendly because fuel cells produce electricity by using only hydrogen and oxygen,obtained by purifying atmospheric air by filtering out dust and ***,their final product is only water,instead of pollutants like carboFuel cells are one of the most competitive alternative energy sources because their theoretical efficiency is~15%higher than that of internal combustion engines (ICEs) and they are considered cleaner and *** fuel cells are used to replace ICEs in cars and energy conversion systems,the system efficiency increases;furthermore,the process becomes more environmentally-friendly because fuel cells produce electricity by using only hydrogen and oxygen,obtained by purifying atmospheric air by filtering out dust and ***,their final product is only water,instead of pollutants like carbon dioxide.n dioxide.

关键词： Non-precious-metal catalyst Oxygen reduction reaction Size effect Electrolyte accessibility Alkaline fuel cell

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Progress of Materials and Devices for Neuromorphic Vision Sensors

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Nano-Micro Letters 2022年第12期14卷 239-271页

作者： Sung Woon Cho chanho Jo Yong-Hoon kim Sung Kyu Park Department of Electrical and Electronics Engineering Chung-Ang UniversitySeoul 06974Republic of Korea Department of Advanced Components and Materials Engineering Sunchon National UniversitySunchŏnJeonnam 57922Republic of Korea School of Advanced Materials Science and Engineering Sungkyunkwan UniversitySuwon 16419Republic of Korea SKKU Advanced Institute of Nanotechnology(SAINT) Sungkyunkwan UniversitySuwon 16419Republic of Korea

The latest developments in bio-inspired neuromorphic vision sensors can be summarized in 3 keywords:smaller,faster,and smarter.(1)Smaller:Devices are becoming more compact by integrating previously separated components such as sensors,memory,and processing *** a prime example,the transition from traditional sensory vision computing to in-sensor vision computing has shown clear benefits,such as simpler circuitry,lower power consumption,and less data redundancy.(2)Swifter:Owing to the nature of physics,smaller and more integrated devices can detect,process,and react to input more *** addition,the methods for sensing and processing optical information using various materials(such as oxide semiconductors)are evolving.(3)Smarter:Owing to these two main research directions,we can expect advanced applications such as adaptive vision sensors,collision sensors,and nociceptive *** review mainly focuses on the recent progress,working mechanisms,image pre-processing techniques,and advanced features of two types of neuromorphic vision sensors based on near-sensor and in-sensor vision computing methodologies.

关键词： In-sensor computing Near-sensor computing Neuromorphic vision sensor Optoelectronic synaptic circuit Optoelectronic synapse

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Multifunctional Ir–Ru alloy catalysts for reversal-tolerant anodes of polymer electrolyte membrane fuel cells

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Journal of Materials Science & Technology 2021年第1期60卷 105-112页

作者： Seung Woo Lee Bongho Lee Chaekyung Baik Tae-Yang kim chanho Pak Graduate Program of Energy Technology School of Integrated TechnologyInstitute of Integrated TechnologyGwangju Institute of Science and TechnologyGwangju 61005Republic of Korea Research Institute for Solar and Sustainable Energies Gwangju Institute of Science and TechnologyGwangju 61005Republic of Korea

To address the problem of fuel starvation in fuel-cell electric vehicles,which causes cell voltage reversal and results in cell failure when repeated continuously,we developed a reversal-tolerant anode(RTA) to promote water oxidation in preference to carbon *** carbon-supported Ir-Ru alloys with different compositions are employed as RTA catalysts in an acidic polyol solution and are shown to exhibit composition-dependent average crystallite sizes of <5.33 *** adopted approach allows the generation of relatively well-dispersed Ir-Ru alloy nanoparticles on the carbon support without severe *** activity of IrRu_(2)/C for the hydrogen oxidation reaction is 1.10 times that of the stateof-the-art Pt/C *** reversal testing by simulation of fuel starvation reveals that the durability of IrRu_(2)/C(~7 h) significantly exceeds that of the conventional Pt/C catalyst(~10 min) and is the highest value reported so ***,the developed Ir-Ru alloy catalyst can be used to fabricate practical RTAs and replace Pt catalysts in the anodes of polymer electrolyte membrane fuel cells.

关键词： Polymer electrolyte membrane fuel cell Polyol process Reversal-tolerant anode Oxygen evolution reaction Hydrogen oxidation reaction

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Avoiding heating interference and guided thermal conduction in stretchable devices using thermal conductive composite islands

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Nano Research 2021年第9期14卷 3253-3259页

作者： Seung Ji Kang Haeleen Hong chanho Jeong Ju Seung Lee Hyewon Ryu Jae-hun Yang Jong Uk kim Yiel Jae Shin Tae-il kim School of Chemical Engineering Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea Department of Biomedical Engineering Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea Biomedical Institute for Convergence(BICS) Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea

The miniaturization and high integration of devices demand significant thermal management *** technologies for the thermal management of electronics show some limitations in the case of multiple chip arrays.A device in multiple chip array is affected by heat from adjacent devices,along with thermal conductive *** address this problem,we present a nano composite of aligned boron nitride(BN)nanosheet islands with porous polydimethylsiloxane(PDMS)foam to have mechanical stability and non-thermal *** islands of tetrahedrally-structured BN in the composite have a high thermal conductivity of 1.219 W·m^(-1)·K^(-1) in the through-plane direction(11.234W·m^(-1)·K^(-1)in the in-plane direction)with 16 wt.%loading of *** the other hand,porous PDMS foam has a low thermal conductivity of 0.0328W·m^(-1)·K^(-1) in the through-plane direction at 70%*** pathways are then formed only in the structured BN islands of the *** porous PDMS foam can be applied as a thermal barrier between structured BN islands to inhibit thermal interference in multiple device ***,this composite can maintain selective thermal dissipation performance with 70%tensile *** beauty of the work is that it could have guided heat dissipation by assembling of multiple layers which have high vertical thermal conductive islands,while inhibiting thermal *** selective heat dissipating composite can be applied as a heatsink for multiple chip arrays electronics.

关键词： selective thermal conduction non-thermal interference thermal conductive composite island stretchable electronics structured boron nitride nanosheet(s-BN) porous polydimethylsiloxane(p-PDMS)

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Enhanced delivery of a low dose of aducanumab via FUS in 5×FAD mice,an AD model

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Translational Neurodegeneration 2022年第1期11卷 31-45页

作者： chanho Kong Eun-Jeong Yang Jaewoo Shin Junwon Park Si-Hyun kim Seong-Wook Park Won Seok Chang Chang-Han Lee Hyunju kim Hye-Sun kim Jin Woo Chang Department of Neurosurgery Yonsei University College of Medicine50 Yonsei-RoSeodaemun-GuSeoulRepublic of Korea Department of Pharmacology College of MedicineSeoul National University103 DaehakroJongro-GuSeoulRepublic of Korea Neuroscience Research Center College of MedicineSeoul National University103 DaehakroJongro-GuSeoulRepublic of Korea Department of Biomedical Sciences College of MedicineSeoul National University103 DaehakroJongro-GuSeoulRepublic of Korea Bundang Hospital Seoul National University College of MedicineBundang-GuSungnamRepublic of Korea.

Background:Aducanumab(Adu),which is a human IgG1 monoclonal antibody that targets oligomer and fibril forms of beta-amyloid,has been reported to reduce amyloid pathology and improve impaired cognition after administration of a high dose(10 mg/kg)of the drug in Alzheimer’s disease(AD)clinical *** purpose of this study was to investigate the effects of a lower dose of Adu(3 mg/kg)with enhanced delivery via focused ultrasound(FUS)in an AD mouse ***:The FUS with microbubbles opened the blood-brain barrier(BBB)of the hippocampus for the delivery of *** combined therapy of FUS and Adu was performed three times in total and each treatment was performed biweekly.Y-maze test,Brdu labeling,and immunohistochemical experimental methods were employed in this *** addition,RNA sequencing and ingenuity pathway analysis were employed to investigate gene expression profiles in the hippocampi of experimental ***:The FUS-mediated BBB opening markedly increased the delivery of Adu into the brain by approximately 8.1 times in the *** combined treatment induced significantly less cognitive decline and decreased the level of amyloid plaques in the hippocampi of the 5×FAD mice compared with Adu or FUS *** treatment with FUS and Adu activated phagocytic microglia and increased the number of astrocytes associated with amyloid plaques in the hippocampi of 5×FAD ***,RNA sequencing identified that 4 enriched canonical pathways including phagosome formation,neuroinflammation signaling,CREB signaling and reelin signaling were altered in the hippocami of 5×FAD mice receiving the combined ***:In conclusion,the enhanced delivery of a low dose of Adu(3 mg/kg)via FUS decreases amyloid deposits and attenuates cognitive function ***-mediated BBB opening increases adult hippocampal neurogenesis as well as drug *** present an AD treatment strategy through the synergistic effect of the combined therapy of

关键词： Aducanumab Alzheimer’s disease Focused ultrasound Transcriptome profiling

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Phase stability and mechanical properties of wire+arc additively manufactured H13 tool steel at elevated temperatures

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Journal of Materials Science & Technology 2021年第8期67卷 80-94页

作者： A.N.M.Tanvir Md.R.U.A hsan Gijeong Seo Brian Bates chanho Lee Peter K.Liaw Mark Noakese Andrzej Nycz Changwook Ji Duck Bong kim Department of Mechanical Engineering Tennessee Technological UniversityCookevilleTN 38505USA Department of Manufacturing and Engineering Technology Tennessee Technological UniversityCookevilleTN 38505USA Center for Manufacturing Research Tennessee Technological UniversityCookevilleTN 38505USA Department of Materials Science and Engineering University of TennesseeKnoxvilleTN 37996USA Manufacturing Demonstration Facility Oak Ridge National LaboratoryOak RidgeTN 37830USA Advanced Forming Process R&D Group Korea Institute of Industrial TechnologyUlsan 44413Republic of Korea

Wire+arc additive manufacturing(WAAM)is considered an innovative technology that can change the manufacturing landscape in the near *** offers the benefits of inexpensive initial system setup and a high deposition rate for fabricating medium-and large-sized parts such as die-casting *** this study,AISI H13 tool steel,a popular die-casting tool metal,is manufactured by cold metal transfer(CMT)-based WAAM and is then comprehensively analyzed for its microstructural and mechanical ***-dependent phase combinations are observed,which could be explained by nonequilibrium thermal cycles that resulted from the layer-by-layer stacking mechanism used in *** addition,remelting and reheating of the layers reduces welding anomalies(e.g.,pores and voids).The metallurgical characteristics of the H13 strongly correlate with the mechanical *** combinations of phases at different locations of the additively manufactured part exhibit a periodic microhardness ***,Retained Austenite,Ferrite,and Carbide phases are found in combination at different locations of the part based on the part’s temperature distribution during additive ***,the tensile properties at elevated temperatures(23℃,300℃,and 600℃)are comparable to those from other WAAM and additive manufacturing(AM)*** X-ray diffraction results verify that the microstructural stability of the fabricated parts at high temperatures would allow them to be used in high temperatures.

关键词： Tool steel Martensitic steel Wire+arc additive manufacturing(WAAM) High temperature tensile test High temperature XRD

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利用远震接收函数研究黄海周边地区的地壳上地幔结构

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地球物理学报 2010年第6期53卷 1336-1343页

作者： chanho YU Kwang-Hee kim Mancheol Suh Bongchool Suk Paul Rydelek Suyoung Kang Yongcheol Park 刘劲松韩国海洋与发展研究所韩国公州大学韩国极地研究所中国科学院地质与地球物理研究所北京100029

利用宽频带流动台站(YSBSN)记录的远震波形数据和远震接收函数方法,反演了黄海东、西两侧地壳上地幔的S波速度结构.结果表明,莫霍面深度在30～38 km之间变化,位于中方一侧的JNN台下方地壳厚度最大,可以归因于华北板块和扬子板块的碰撞;... 详细信息

利用宽频带流动台站(YSBSN)记录的远震波形数据和远震接收函数方法,反演了黄海东、西两侧地壳上地幔的S波速度结构.结果表明,莫霍面深度在30～38 km之间变化,位于中方一侧的JNN台下方地壳厚度最大,可以归因于华北板块和扬子板块的碰撞;韩方一侧的地壳厚度自北向南逐渐变厚,但仍然难以厘定朝鲜半岛南部潜在碰撞带的位置,这些问题的解决需要更大范围的流动台站观测.由于部分台站位于巨厚的沉积层和多孔的火山岩之上,与浅部构造的相关性使得接收函数表现出较大振幅的混响,从而影响了来自深部结构的转换震相.

关键词：黄海宽频带流动地震台阵 S波速度结构远震接收函数

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