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Towards advanced zinc anodes by interfacial modification strategies for efficient aqueous zinc metal batteries

Journal of Energy Chemistry 2024年第6期93卷 79-110,I0003页

作者： changchun Fan Weijia Meng Jiaye Ye Key Laboratory of Bio-Inspired Smart Interfacial science and Technology Ministry of EducationSchool of ChemistryBeihang UniversityBeijing 100191China Shaanxi Key Laboratory of New Transportation Energy and Automotive Energy Saving School of Energy and Electrical EngineeringChang’an UniversityXi’an 710061ShaanxiChina school of Chemistry and Physics Faculty of ScienceQueensland University of TechnologyBrisbaneQLD 4001Australia Centre for Materials science Queensland University of TechnologyBrisbaneQLD 4001Australia

Developing sustainable and clean energy sources(e.g.,solar,wind,and tide energy)is essential to achieve the goal of carbon *** to the discontinuous and inco nsistent nature of common clean energy sources,high-performance energy storage technologies are a critical part of achieving this *** zinc metal batteries(AZMBs)with inherent safety,low cost,and competitive performance are regarded as one of the promising candidates for grid-scale energy ***,zinc metal anodes(ZMAs)with irreversible problems of dendrite growth,hydrogen evolution reaction,self-corrosio n,and other side reactions have seriously hindered the development and commercialization of *** increasing number of researchers are focusing on the stability of ZMAs,so assessing the effectiveness of existing research strategies is critical to the development of *** review aims to provide a comprehensive overview of the fundamentals and challenges of *** rch strategies for interfacial modification of ZMAs are systematically *** features of artificial interfacial coating and in-situ interfacial coating of ZMAs are compared and discussed in detail,as well as the effect of modified interfacial ZMA on the full-battery ***,perspectives are provided on the problems and challenges of *** review is expected to offer a constructive reference for the further development and commercialization of AZMBs.

关键词： Aqueous zinc metal batteries Zinc metal anode Interfacial modification Artificial interfacial coating In-situ interfacial coating

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Quantifying quantum entanglement via machine learning models

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Communications in Theoretical Physics 2024年第7期76卷 52-56页

作者： changchun Feng Lin Chen LMIB(Beihang University) Ministry of EducationBeijing 100191China school of Mathematical sciences Beihang UniversityBeijing 100191China International Research Institute for Multidisciplinary science Beihang UniversityBeijing 00191China

Quantifying entanglement measures for quantum states with unknown density matrices is a challenging *** learning offers a new perspective to address this *** training machine learning models using experimentally measurable data,we can predict the target entanglement *** this study,we compare various machine learning models and find that the linear regression and stack models perform better than *** investigate the model's impact on quantum states across different dimensions and find that higher-dimensional quantum states yield better ***,we investigate which measurable data has better predictive power for target entanglement *** correlation analysis and principal component analysis,we demonstrate that quantum moments exhibit a stronger correlation with coherent information among these data features.

关键词： quantum information entanglement predict machine learning coherence

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A method of combining SE-tree to compute all minimal hitting sets

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Progress in Natural science:Materials International 2006年第2期16卷 169-174页

作者： ZHAO Xiangfu and OUYANG Dantong (school of Computer science and Technology, Jilin University, {2. 130012, china Key Laboratory of Symbolic Computation and Knowledge Engineering of Ministry of Education, {2. 130012, china) [a]school of Computer science and Technology Jilin University Changchun China

In model-based diagnosis, the candidate diagnostic results are generally characterized by all minimal hitting sets for the collection of all conflict sets. In this paper, a new method is proposed to judge a hitting set by the number of conflict sets corresponding to components, and the computing procedure is formalized by combining revised SE-tree (set enumeration tree) with closed nodes to generate all minimal hitting sets. Results show that because closed nodes are added into SE-tree, the search efficiency is highly improved. Furthermore, the proposed method is easy to be understood and implemented. Compared with other effective algorithms with completeness in some experimental tests, the diagnosis efficiency of our proposed method is higher, particularly for single- and double-fault diagnosis.

关键词： model-based diagnosis conflict set minimal hitting set set enumeration tree.

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Wet-chemical synthesis and characteristics of Au nanoshell

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science china Chemistry 2005年第5期48卷 431-435页

作者： LIU Zhongxin1,2. SONG Hongwei1, YU Lixin1,2. YANG Linmei1,2.& PAN Guohui1,2.1. Key Laboratory of Excited State Physics, changchun Institute of Optics, Fine Mechanics and Physics, Chinese academy of {2.s, changchun 130033, china 2. Graduate school of the Chinese academy of {2.s, Beijing 100039, china 1. Key Laboratory of Excited State Physics Changchun Institute of Optics Fine Mechanics and Physics Chinese Academy of Sciences 130033 Changchun China 2. Graduate school of the Chinese academy of {2.s 100039 Beijing China

Gold nanoshells were prepared by an easy wet-chemical method, with Ag nanoparticles used as the templates. Transmission electron microscopy (TEM) indicated that the shells were sphere in shape, the size was homogenous, being about 2. nm, and no hard ag-glomerates were observed. The plasma resonance absorption of gold was tuned from visible to near-infrared (NIR) with the increased volume of HAuCl4. The temperature grads (?T) of the gold nanoshell hydrosol under the exposure of an 808-nm optical fiber laser with different power den-sities were measured. The highest ?T was 30℃ (5 W/cm2. irradiation area was 2.cm2.. This kind of gold nanoshell hydrosol is a promising material to be used in biomedicine such as photo-thermal cancer therapy, and its special photothermal convert property will photothermally trigger drug release.

关键词： wet-chemical synthesis, Au, nanoshell, NIR absorption, photothermal conversion.

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Effects of MoO_3 Amounts on Sintering and Electrical Properties of Ce_(0.8)Nd_(0.2.O_(1.9)

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Chemical Research in Chinese Universities 2012年第1期28卷 9-13页

作者： ZHOU De-feng1, ZHAO Gui-chun1, YANG Mei1, XIA Yan-jie2.and MENG Jian2.1. school of Chemistry and Life science, {2. University of Technology, {2. 130012, P. R. china 2. State Key Laboratory of Rare Earth Resources Utilization, {2. Institute of Applied Chemistry, Chinese academy of sciences, {2. 13002., P. R. china school of Chemistry and Life science Changchun University of Technology Changchun 130012 changchun Institute of Applied Chemistry Chinese Academy of Sciences State Key Laboratory of Rare Earth Resources Utilization Changchun 130022

The high purity （Ce0.8Nd0.2.1.9）1-x（MoO3）x（x=0, 0.005, 0.010, 0.02.; Ce0.8Nd0.2.1.9=NDC） solid solutions were prepared by modified sol-gel method. The structures and electric conductivities were characterized by X-ray diffraction（XRD）, field-emission scanning electron microscopy（FESEM） and electrochemical impedance spectros copy（EIS）. The XRD results show that the materials were pure phase with a cubic fluorite structure. Compared to the undoped-NDC samples, MoO3 doped-NDC showed higher sintered density（over 96%） at reduced sintering tempera ture. The electric conductivity（σt） of （Ce0.8Nd0.2.1.9）1-x（MoO3）x at 400 °C was 9.58×10-4 S/cm when x=0.010, which was higher than that of undoped-NDC samples（σt=3.2.×10-4 S/cm）. The obtained optimal amount of the MoO3 was x=0.010 in this system.

关键词： Neodymium-doped ceria Molybdenum oxide Sol-gel method Grain boundary conductivity

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A hybrid method for inverse cavity scattering problem for shape

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Applied Mathematics(A Journal of Chinese Universities) 2010年第2期25卷 127-136页

作者： LIU Juan MA Fu-ming school of Mathematics, Jilin University, changchun {2., china. school of Mathematics Jilin University Changchun China

In this paper, we give a hybrid method to numerically solve the inverse open cavity scattering problem for cavity shape, given the scattered solution on the opening of the cavity. This method is a hybrid between an iterative method and an integral equations method for solving the Cauchy problem. The idea of this hybrid method is simple, the operation is easy, and the computation cost is small. Numerical experiments show the feasibility of this method, even for cases with noise.

关键词： Open cavity Cauchy problem Helmholtz equation integral equations system method iterativehybrid method.

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The rate of convergence of the Lax-Oleinik semigroup-degenerate fixed point case

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science china Mathematics 2011年第3期54卷 545-554页

作者： WANG KaiZhi1,2.& YAN Jun1 1school of Mathematical sciences and Key Lab of Mathematics for Nonlinear science, Fudan University, Shanghai 2.0433, china 2.0} of Mathematics, Jilin University, changchun 130012, china 1. school of Mathematical sciences and Key Lab of Mathematics for Nonlinear science Fudan University Shanghai 200433 China2. School of Mathematics Jilin University Changchun 130012 China

For the standard Lagrangian in classical mechanics, which is defined as the kinetic energy of the system minus its potential energy, we study the rate of convergence of the corresponding Lax-Oleinik semigroup. Under the assumption that the unique global minimum point of the Lagrangian is a degenerate fixed point, we provide an upper bound estimate of the rate of convergence of the semigroup.

关键词： Hamiltonian system weak KAM theorem Lax-Oleinik semigroup

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Portable fluorescence instrument for detecting membrane integrity in membrane bioreactor (MBR)

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Frontiers of Environmental science & Engineering 2024年第2期18卷 121-131页

作者： Yang Yu changchun Xin Yuxiang Liu Fei Gao Lei Zhang Hui Jia Jie Wang State Key Laboratory of Separation Membranes and Membrane Processes Tiangong UniversityTianjin 300387China school of Environmental science and Engineering Tiangong UniversityTianjin 300387China school of Environmental science and Engineering Tianjin UniversityTianjin 300072China Shenyang academy of Environmental sciences Shenyang 110167China Cangzhou Institute of Tiangong University Tiangong UniversityCangzhou 061000China

This study proposed the design, fabrication, and assembly of membrane integrity detection instruments in membrane bioreactors (MBR) based on fluorescence spectroscopy. Based on the PARAFAC model, we found that the peak at 2.0/335 nm strengthened after membrane breakage. The peak at 340/430 nm reflected the sludge concentration in the MBR and reduced the influence of internal filtration effects on detection. Therefore, we determined that the dual-LED light source excitation detection system can detect tryptophan-like substances at 2.0 nm (T-peak) and humic acid at 340 nm (C-peak). T-peak was identified as the core index indicating membrane integrity. Moreover, the C-peak is the reference indicator factor for a sensitive response to changes in the sludge concentration. The portable fluorescence instrument exhibited high sensitivity and good feedback accuracy compared to particle counting and turbidity detection, where the log reduction value was greater than 3.5. This overcomes the disadvantage of false alarms in particle counters and is not affected by the position of the pump system. This portable instrument provides a flexible and highly sensitive method for the assessment of industrial membrane integrity.

关键词： Membrane integrity Fluorescence spectrum Portable instrument Membrane bioreactor

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The restricted EM algorithm under linear inequalities in a linear model with missing data

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science china Mathematics 2005年第6期48卷 819-828页

作者： ZHENG Shurong, SHI Ningzhong & GUO Jianhua school of Mathematics and Statistics, Northeast Normal University, changchun 13002., {2. Institute of Mathematics, Jilin University, changchun 130012, {2. 1. school of Mathematics and Statistics Northeast Normal University 130024 Changchun China 2. Institute of Mathematics Jilin University 130012 Changchun China

This paper discusses the maximum likelihood estimate of β under linear inequalities A0β≥ a in a linear model with missing data, proposes the restricted EM algo rithm and proves the convergence.

关键词： EM algorithm, linear model, maximum likelihood estimate, missing data.

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Deriving all minimal consistency-based diagnosis sets using SAT solvers

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Progress in Natural science:Materials International 2009年第4期19卷 489-494页

作者： Xiangfu Zhao a,b, Liming Zhang a,b, Dantong Ouyang a,b, Yu Jiao a,b a Key Laboratory of Symbolic Computation and Knowledge Engineering of Ministry of Education, Jilin University, changchun 130012, {2. b school of Computer science and Technology, Jilin University, changchun 130012, {2. [a]Key Laboratory of Symbolic Computation and Knowledge Engineering of Ministry of Education Jilin University Changchun 130012 China [b]School of Computer Science and Technology Jilin University Changchun 130012 China

In this paper, a novel method is proposed for judging whether a component set is a consistency-based diagnostic set, using SAT solv- ers. Firstly, the model of the system to be diagnosed and all the observations are described with conjunctive normal forms (CNF). Then, all the related clauses in the CNF files to the components other than the considered ones are extracted, to be used for satisfiability checking by SAT solvers. Next, all the minimal consistency-based diagnostic sets are derived by the CSSE-tree or by other similar algorithms. We have implemented four related algorithms, by calling the gold medal SAT solver in SAT07 competition – RSAT. Experimental results show that all the minimal consistency-based diagnostic sets can be quickly computed. Especially our CSSE-tree has the best effciency for the singleor double-fault diagnosis.

关键词： Conjunctive normal form Consistency-based diagnosis Model-based diagnosis SAT solver

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