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Study of the reaction mechanism for preparing powdered activated coke with SO_(2)adsorption capability via one-step rapid activation method under flue gas atmosphere

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Chinese Journal of Chemical Engineering 2024年第1期65卷 158-168页

作者： Binxuan Zhou Jingcai chang Jun Li Jinglan Hong Tao Wang Liqiang zhang Ping Zhou Chunyuan Ma School of Environmental Science and Engineering Shandong UniversityQingdao 266237China School of Energy and Power Engineering Shandong UniversityJinan 250061China Weihai Research Institute of Industrial Technology of Shandong University Weihai 264209China

In this study,the impact of different reaction times on the preparation of powdered activated carbon(PAC)using a one-step rapid activation method under flue gas atmosphere is investigated,and the underlying reaction mechanism is *** indicate that the reaction process of this method can be divided into three stages:stage I is the rapid release of volatiles and the rapid consumption of O_(2),primarily occurring within a reaction time range of 0-0.5 s;stage II is mainly the continuous release and diffusion of volatiles,which is the carbonization and activation coupling reaction stage,and the carbonization process is the main in this *** stage mainly occurs at the reaction time range of 0.5 -2.0 s when SL-coal is used as material,and that is 0.5-3.0 s when JJ-coal is used as material;stage III is mainly the activation stage,during which activated components diffuse to both the surface and interior of *** stage mainly involves the reaction stage of CO_(2)and H2O(g)activation,and it mainly occurs at the reaction time range of 2.0-4.0 s when SL-coal is used as material,and that is 3.0-4.0 s when JJ-coal is used as ***,the main function of the first two stages is to provide more diffusion channels and contact surfaces/activation sites for the diffusion and activation of the activated components in the third *** the reaction mechanism would serve as a crucial reference and foundation for designing the structure,size of the reactor,and optimal positioning of the activator nozzle in PAC preparation.

关键词： Reaction mechanism Powdered activated coke preparation SO_(2)adsorption One-step rapid activation Flue gas atmosphere

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Pyridine-regulated Sb@InSbS_(3)ultrafine nanoplates as high-capacity and long-cycle anodes for sodium-ion batteries

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Rare Metals 2024年第5期43卷 2080-2092页

作者： Jia-Ying Ren Xiang-Lin Yu chang-Miao Chen Xin-Yu Hu Ting Yang Ming zhang College of Materials Science and Engineering and College of Science Central South University of Forestry and TechnologyChangsha 410004China College of Semiconductors(College of Integrated Circuits) Changsha Semiconductor Technology and Application Innovation Research InstituteHunan UniversityChangsha 410082China

Sb-based materials exhibit considerable potential for sodium-ion storage owing to their high theoretica ***,the bulk properties of Sb-based materials always result in poor cycling and rate *** overcome these issues,pyridine-regulated Sb@InSbS_(3)ultrafine nanoplates loaded on reduced graphene oxides(Sb@InSbS_(3)@rGO)were designed and *** the synthesis process,pyridine was initially adopted to coordinate with In^(3+),and uniformly dispersed In_(2)S_(3)ultrafine nanoplates on reduced graphene oxide were generated after ***,partial In^(3+)was exchanged with Sb^(3+),and Sb@InSbS_(3)@rGO was obtained by using the subsequent annealing *** unique structure of Sb@InSbS_(3)@rGO effectively shortened the transfer path of sodium ions and electrons and provided a high *** the anode in sodium-ion batteries,the Sb@InSbS_(3)@rGO electrode demonstrated a significantly higher reversible capacity better stability(445 m Ah·g^(-1)at 0.1 A·g^(-1)after 200 cycles and 212 mAh·g^(-1)at 2 A·g^(-1)after 1200 cycles),and superior rate(210 mAh·g^(-1)at 6.4 A·g^(-1))than the electrode without pyridine(355 mAh·g-1at 0.1 A·g-1after 55 cycles and 109 mAh·g^(-1)at 2 A·g^(-1)after 770 cycles)Furthermore,full cells were assembled by using the Sb@InSbS_(3)@rGO as anode and Na_(3)V_(2)(PO_(4))_(3)as cathode which demonstrated good cycling and rate performances and exhibited promising application *** results indicate that adjusting the microstructure of electrode materials through coordination balance is A·good strategy for obtaining high-capacity,high-rate,and longcycle sodium storage performances.

关键词： Sodium-ion battery Sb-based anode material Pyridine coordination Reduced size nanostructure Half/full cell

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Atomically Dispersed Ruthenium Catalysts with Open Hollow Structure for Lithium-Oxygen Batteries

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Nano-Micro Letters 2024年第2期16卷 154-164页

作者： Xin Chen Yu zhang chang Chen Huinan Li Yuran Lin Ke Yu Caiyun Nan Chen Chen Beijing Advanced Innovation Center for Materials Genome Engineering Institute of Solid State ChemistryUniversity of Science and Technology BeijingBeijing 100083People’s Republic of China Engineering Research Center of Advanced Rare Earth Materials Department of ChemistryTsinghua UniversityBeijing 100084People’s Republic of China Beijing Key Laboratory of Energy Conversion and Storage Materials Institution College of ChemistryBeijing Normal UniversityBeijing 100875People’s Republic of China

Lithium–oxygen battery with ultrahigh theoretical energy density is considered a highly competitive next-generation energy storage device,but its practical application is severely hindered by issues such as difficult decomposition of discharge products at ***,we have developed N-doped carbon anchored atomically dispersed Ru sites cathode catalyst with open hollow structure(h-RuNC)for Lithium–oxygen *** one hand,the abundance of atomically dispersed Ru sites can effectively catalyze the formation and decomposition of discharge products,thereby greatly enhancing the redox *** the other hand,the open hollow structure not only enhances the mass activity of atomically dispersed Ru sites but also improves the diffusion efficiency of catalytic ***,the excellent activity from atomically dispersed Ru sites and the enhanced diffusion from open hollow structure respectively improve the redox kinetics and cycling stability,ultimately achieving a high-performance lithium–oxygen battery.

关键词： Atomically dispersed Open hollow structure Discharge product Lithium Oxygen battery

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Self-Driven Photo-Polarized Water Molecule-Triggered Graphene-Based Photodetector

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Research 2024年第2期2023卷 273-283页

作者： Shisheng Lin chang Liu Xin Chen Yi zhang Hongtao Lin Xutao Yu Yujiao Bo Yanghua Lu College of Information Science and Electronic Engineering Zhejiang UniversityHangzhou 310027P.R.China Hangzhou Gelanfeng Technology Co.Ltd Hangzhou 310051P.R.China State Key Laboratory of Modern Optical Instrumentation Zhejang UniversityHangzhou 310027P.R.China Key Laboratory of Wide Bandgap Semiconductor Materials and Devices HCSemitek CorporationYiwu 322009P.R.China Smart Materials for Architecture Research Lab Innovation Center of Yangtze River DeltaZhejiang UniversityJiaxing 314100P.R.China

Flowing water can be used as an energy source for generators,providing a major part of the energy for daily ***,water is rarely used for information or electronic ***,we present the feasibility of a polarized liquid-triggered photodetector in which polarized water is sandwiched between graphene and a *** to the polarization and depolarization processes of water molecules driven by photogenerated carriers,a photo-sensitive current can be repeatedly produced,resulting in a high-performance *** response wavelength of the photodetector can be fine-tuned as a result of the free choice of semiconductors as there is no requirement of lattice match between graphene and the *** zero voltage bias,the responsivity and specific detectivity of Gr/NaCl(0.5 M)W/N-GaN reach values of 130.7 mA/W and 2.3×10^(9)Jones under 350 nm illumination,***,using a polar liquid photodetector can successfully read the photoplethysmography signals to produce accurate oxygen blood saturation and heart *** with the commercial pulse oximetry sensor,the average errors of oxygen saturation and heart rate in the designed photoplethysmography sensor are~1.9%and~2.1%,*** study reveals that water can be used as a high-performance photodetector in informative industries.

关键词： polarization polarized saturation

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Comparison of the capacity of biological desulfurization of Thiobacillus ferrooxidans from different sulfur-containing substrates with or without additional ferrous iron

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International Journal of Agricultural and Biological Engineering 2024年第3期17卷 140-143页

作者： Yanjin Wang Xiaopeng chang Hongge Tao Zhenfeng Wang Quanguo zhang College of Environment Economics Henan Finance UniversityZhengzhou 450046China College of Mechanical and Electrical Engineering Henan Agricultural UniversityZhengzhou 450002China

Thiobacillus ferrooxidans,abbreviated as *** is one of the important microorganisms in the field of biological *** of ferrous iron and sulfur-containing substrates on biological desulfurization of *** were *** show that in the absence of Fe^(2+),*** can utilize three kinds of sulfur-containing substrates of Na_(2)S_(2)O_(3),elemental S and Na_(2)SO_(3) for growth and *** utilization complexity,Na_(2)S_(2)O_(3) was easiest to use,next was elemental S,and Na_(2)SO_(3) was the worst for *** the utilization of ferrous iron and sulfur-containing substrates by ***,the iron oxidation system was first *** the decrease of the Fe^(2+)concentration,the sulfur oxidation system was started,and then the two systems synergistically *** presence of three sulfur-containing substrates had different effects on Fe^(2+)oxidation,and elemental S did not inhibit the oxidation of Fe^(2+),while Na_(2)S_(2)O_(3) and Na_(2)SO_(3) had some inhibition on the oxidation of Fe^(2+),especially the inhibition of Na_(2)SO_(3) was significant,and complete oxidation of ferrous iron needed more *** isolated *** is applied to the removal of H2S gas,aiming to provide a new technological approach for biological removal of H2S.

关键词： Thiobacillus ferrooxidans ferrous iron sulfur-containing substrate biological desulfurization

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Ribonucleotide reductase M2 (RRM2): Regulation, function and targeting strategy in human cancer

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Genes & Diseases 2024年第1期11卷 218-233页

作者： Zanwen Zuo Zerong Zhou Yuzhou chang Yan Liu Yuping Shen Qizhang Li Lei zhang Innovative Drug R&D Center College of Life SciencesHuaibei Normal UniversityHuaibeiAnhui 235000China National"111"Center for Cellular Regulation and Molecular Pharmaceutics Key Laboratory of Fermentation Engineering(Ministry of Education)Hubei Key Laboratory of Industrial MicrobiologyCooperative Innovation Center of Industrial Fermentation(Ministry of Education&Hubei Province)and School of Food and Biological EngineeringHubei University of TechnologyWuhanHubei 430068China Department of Biomedical Informatics The Ohio State UniversityColumbusOH 43210USA School of Agriculture and Biology and Engineering Research Center of Cell&Therapeutic AntibodyMinistry of EducationShanghai Jiao Tong UniversityShanghai 200240China College of Chemistry and Bioengineering Hunan University of Science and EngineeringYongzhouHunan425199China Department of Pharmaceutical Botany School of PharmacyNaval Medical UniversityShanghai 200433China

Ribonucleotide reductase M2(RRM2)is a small subunit in ribonucleotide reduc-tases,which participate in nucleotide metabolism and catalyze the conversion of nucleotides to deoxynucleotides,maintaining the dNTP pools for DNA biosynthesis,repair,and ***2 performs a critical role in the malignant biological behaviors of *** structure,regulation,and function of RRM2 and its inhibitors were ***2 gene can produce two transcripts encoding the same ***2 expression is regulated at multiple levels during the processes from transcription to ***,this gene is associated with resistance,regulated cell death,and tumor *** order to develop and design inhibitors of RRM2,appropriate strategies can be adopted based on different ***,a greater appreciation of the characteristics of RRM2 is a benefit for understanding tumorigenesis,resistance in cancer,and tumor ***,RRM2-targeted therapy will be more attention in future therapeutic approaches for enhancement of treatment effects and amelioration of the dismal prognosis.

关键词： Function Inhibition Regulation Resistance RRM2

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Experimental study on the variation of optical remote sensing imaging characteristics of internal solitary waves with wind speed

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Journal of Oceanology and Limnology 2024年第2期42卷 408-420页

作者： Zhe chang Lina SUN Tengfei LIU Meng zhang Keda LIANG Junmin MENG Jing WANG School of Physics and Optoelectronic Engineering Ocean University of ChinaQingdao 266100China First Institute of Oceanography Ministry of Natural ResourcesQingdao 266061China Technology Innovation Center for Ocean Telemetry Ministry of Natural ResourcesQingdao 266061China

Optical remote sensing has been widely used to study internal solitary waves(ISWs).Wind speed has an important effect on ISW imaging of optical remote *** light and dark bands of ISWs cannot be observed by optical remote sensing when the wind is too *** relationship between the characteristics of ISWs bands in optical remote sensing images and the wind speed is still *** influence of wind speeds on the characteristics of the ISWs bands is investigated based on the physical simulation experiments with the wind speeds of 1.6,3.1,3.5,3.8,and 3.9 m/*** experimental results show that when the wind speed is 3.9 m/s,the ISWs bands cannot be observed in optical remote sensing images with the stratification of h_(1)∶h_(2)=7∶58,ρ_(1)∶ρ_(2)=1∶*** the wind speeds are 3.1,3.5,and 3.8 m/s,which is lower than 3.9 m/s,the ISWs bands can be obtained in the simulated optical remote sensing *** location of the band’s dark and light extremum and the band’s peak-to-peak spacing are almost not affected by wind ***-significant wind speeds can cause a greater gray difference of the light-dark *** provided a scientific basis for further understanding of ISW optical remote sensing imaging.

关键词： internal solitary wave(ISW) optical remote sensing wind speed characteristics of ISWs bands

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Thermal History of Cambrian Burgess Shale-Type Deposits:New Insights from the Early Cambrian Chengjiang and Qingjiang Fossils of South China

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Journal of Earth Science 2024年第4期35卷 1215-1223页

作者： Yuheng Qiao Linhao Cui Guangyuan Xing Dongjing Fu Chao chang Robert Gaines Xingliang zhang State Key Laboratory of Continental Dynamics Shaanxi Key laboratory of Early Life and EnvironmentsDepartment of GeologyNorthwest UniversityXi’an710069China Department of Geology Pomona CollegeClaremontCA91711USA

Burgess Shale-type deposits provide a wealth of information on the early evolution of *** that are central to understanding the exceptional preservation of these biotas and the paleoenvironments they inhabited may be obscured by the post-depositional alteration due to metamorphism at depth and weathering near the Earth’s *** over 50 Cambrian BST biotas,the Chengjiang and Qingjiang deposits are well known for their richness of soft-bodied taxa,fidelity of preservation,and Early Cambrian *** alteration via weathering has been well-investigated,the thermal maturity of the units bearing the two biotas has not yet been *** we investigate peak metamorphic temperatures of the two deposits using two independent *** gradient analyses demonstrate that the most fossiliferous sections of the Chengjiang were buried at a maximum depth of∼8500 m in the Early Triassic,corresponding to∼300°C,while the type area of the Qingjiang biota was buried at a maximum depth of∼8700 m in the Early Jurassic,corresponding to∼240°*** geothermometer analyses of fossil carbonaceous material demonstrate that peak temperatures varied across localities with different burial *** two productive sections of the Chengjiang biota were thermally altered at a peak temperature of approximately 300°C,and the main locality of the Qingjiang biota experienced a peak temperature of 238±22°*** results from two independent methods are *** BST deposits for which thermal maturity has been documented,the Qingjiang biota is the least thermally mature,and therefore holds promise for enriching our understanding of BST deposits.

关键词： the Chengjiang Biota the Qingjiang Biota burial history Raman geothermometer thermal history Burgess Shale-type Lagerstätte

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Experimental Study on the Variation of Optical Imaging Characteristics with Zenith Angle due to Internal Solitary Waves in Sunglint

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Journal of Ocean University of China 2024年第4期23卷 943-952页

作者： LIU Tengfei SUN Lina chang Zhe zhang Meng LIANG Keda MENG Junmin WANG Jing School of Physics and Optoelectronic Engineering Ocean University of ChinaQingdao 266100China First Institute of Oceanography Ministry of Natural ResourcesQingdao 266061China Technology Innovation Center for Ocean Telemetry Ministry of Natural ResourcesQingdao 266061China

Internal solitary waves(ISWs)change the roughness of the sea surface,thus producing dark and bright bands in optical ***,reasons for changes in imaging characteristics with the solar zenith angle remain *** this paper,the optical imaging pattern of ISWs in sunglint under different zenith angles of the light source is investigated by collecting optical images of ISWs through physical *** experiment involves setting 10 zenith angles of the light source,which are divided into area a the optical images of ISWs in the three areas show dark-bright mode,single bright band,and bright-dark mode,which are consistent with those observed by optical remote *** addition,this study analyzed the percentage of the dark and bright areas of the bands and the change in the relative gray difference and found changes in both areas under different zenith angles of the light *** MODIS and ASAR images display a similar brightness-darkness distance of the same ***,the relationship between the brightness-darkness distance and the characteristic half-width of ISWs is determined in accordance with the eKdV theory and the imaging mechanism of ISWs of the SAR ***,the relationship between them in the experiment is almost consistent with the theoretical result.

关键词： internal solitary waves optical imaging characteristic laboratory simulation zenith angle sunglint

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Research on Reservoir Landslide Thrust Based on Improved Morgenstern-Price Method

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Journal of Earth Science 2024年第4期35卷 1263-1272页

作者： Xuan Wang Xinli Hu chang Liu Lifei Niu Peng Xia Jian Wang Jiehao zhang Faculty of Engineering China University of GeosciencesWuhan430074China

The curve of landslide thrust plays a key role in landslide *** commonly used transfer coefficient method(TCM)and Morgenstern-Price method(MPM)are *** does not take into account the moment balance between *** MPM considers the moment balance,the calculation is complex,and it does not consider that the force between slices may be less than zero at the back edge of the *** rationality and feasibility of the improved MPM are verified by calculating the landslide stability coefficient and landslide thrust at different reservoir water *** paper studies the law of landslide thrust when the reservoir water level changes,and discusses the determination of design thrust,to provide a certain theoretical basis for the design of reservoir landslides.

关键词： reservoir transfer coefficient method Morgenstern-Price landslide thrust design thrust landslides

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