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Theoretical study on the synergistic mechanism of Fe–Mn in sodium-ion batteries

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Particuology 2024年第10期93卷 284-290页

作者： yang You Mingliang yuan School of Mineral Processing and Bioengineering Central South UniversityChangsha410083China

This article conducts first-principles calculations to initially explore the construction of two configurations,NaFeO_(2)(NFO)and NaMnO_(2)(NMO),and studies the mixing enthalpies under different Fe–Mn *** results indicate that NaFe3/8Mn5/8O_(2)(NFMO)exhibits the most thermodynamically stable *** calculations on the mixing enthalpies and volume changes during the sodium extraction process for NFO,NMO,and NFMO configurations are presented,along with the partial density of states(PDOS)and Bader charges of transition metals(TM)and *** calculations reveal the synergistic mechanism of Fe and *** and Mn can engage in more complex electron exchanges during sodium extraction,optimizing the internal electron density distribution and overall charge balance,thereby stabilizing the crystal structure and reducing the migration of Fe^(3+)to the sodium layers during deep sodium *** interaction between Fe’s 3d electrons and Mn’s 3d electrons through the shared oxygen atoms’2p orbitals occurs in the Fe–Mn–O *** interaction can lead to a rebalancing of the electron density around Mn³⁺atoms,mitigating the asymmetric electron density distribution caused by the d4 configuration of the lone Mn³⁺and suppressing the Jahn-Teller effect of Mn^(3+).Moreover,the synergistic effects between Fe and Mn can provide a more balanced charge distribution,reducing extreme changes to the charge state of oxygen atoms and decreasing the irreversible oxygen release caused by anionic redox reactions during deep sodium extraction,thereby enhancing the material’s *** in-depth study of the interaction mechanism at the microscopic level when co-doping Fe and Mn offers valuable insights for the rational design and development of high-performance cathode materials.

关键词： First-principles calculations Sodium-ionbatteries Layered oxides NaFe_(3/8)Mn_(3/8)O_(2)

MOF glass foam: a blueprint to porous membrane scaling-up

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Science China Chemistry 2024年第3期67卷 746-748页

作者： yuan Peng Weishen yang State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesBeijing 100049China University of Chinese Academy of Sciences Beijing 100049China

In comparison with conventional energy-intensive separation technologies, such as distillation and crystallization,membrane separation is labelled as an advanced technology with low energy consumption, a small carbon footprint,continuous operation, etc. Metal-organic frameworks(MOFs) are a burgeoning category of crystalline materials consisting of metal ions/clusters coordinated with organic ligands.

关键词： separation porous distillation

Remote sensing image encryption algorithm utilizing 2D Logistic memristive hyperchaotic map and SHA-512

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Science China(Technological Sciences) 2024年第5期67卷 1553-1566页

作者： LAI Qiang LIU yuan yang Liang School of Electrical and Automation Engineering East China Jiaotong UniversityNanchang330013China

The two-dimensional Logistic memristive hyperchaotic map(2D-LMHM)and the secure hash SHA-512 are the foundations of the unique remote sensing image encryption algorithm(RS-IEA)suggested in this *** proposed map is formed from the improved Logistic map and the memristor,which has wide phase space and hyperchaotic range and is exceptionally excellent to be utilized in specific *** proposed image algorithm uses the permutation-assignment-diffusion *** generates two position matrices in a progressive manner to achieve an efficient random exchange of pixel positions,assignment is carried through on the image pixels of the permutated image to entirely remove the original image information,strengthening the relationship between permutation and diffusion,and loop diffusion in two different directions can use subtle changes of pixels to affect the whole *** random key and plain-image SHA-512 hash values are used to produce an additional key,which is then utilized to figure out the permutation parameters and the initial value of a chaotic *** experimental results with the average NPCR=99.6094%(NPCR:number of pixels change rate),average UACI=33.4638%(UACI:unified average changing intensity),100%pass rate of the targets in the test set,the average correlation coefficient is 0.00075,and the local information entropy is 7.9025,which shows that the algorithm is able to defend against a variety of illegal attacks and provide more trustworthy protection than some of the existing state-of-the-art algorithms.

关键词： chaos memristive hyperchaotic map remote sensing SHA-512 image encryption RS-IEA

Prescribed Performance Evolution Control for Quadrotor Autonomous Shipboard Landing

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IEEE/CAA Journal of Automatica Sinica 2024年第5期11卷 1151-1162页

作者： yang yuan Haibin Duan Zhigang Zeng State Key Laboratory of Virtual Reality Technology and Systems the School of Automation Science and Electrical EngineeringBeihang UniversityBeijing 100083China State Key Laboratory of Virtual Reality Technology and Systems the School of Automation Science and Electrical EngineeringBeihang UniversityBeijing 100083 Virtual Reality Fundamental Research Laboratory Department of Mathematics and TheoriesPeng Cheng LaboratoryShenzhen 518000China School of Artificial Intelligence and Automation Huazhong University of Science and TechnologyWuhan 430074China

The shipboard landing problem for a quadrotor is addressed in this paper,where the ship trajectory tracking control issue is transformed into a stabilization control issue by building a relative position *** guarantee both transient performance and steady-state landing error,a prescribed performance evolution control(PPEC)method is developed for the relative position *** addition,a novel compensation system is proposed to expand the performance boundaries when the input saturation occurs and the error exceeds the predefined *** the wind and wave on the relative position model,an adaptive sliding mode observer(ASMO)is designed for the disturbance with unknown upper *** on the dynamic surface control framework,a shipboard landing controller integrating PPEC and ASMO is established for the quadrotor,and the relative position control error is guaranteed to be uniformly ultimately *** results have verified the feasibility and effectiveness of the proposed shipboard landing control scheme.

关键词： error integrating stabilization

Cell-free biocatalysis coupled with photo-catalysis and electro-catalysis: Efficient CO2-to-chemical conversion

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Green Energy & Environment 2024年第9期9卷 1366-1383页

作者： Junzhu yang Chi-Kit Sou yuan Lu Key Laboratory of Industrial Biocatalysis Ministry of Education Tsinghua University Department of Chemical Engineering Tsinghua University

The increasing atmospheric carbon dioxide （CO2） concentration has exposed a series of crises in the earth's ecological *** to effectively fix and convert carbon dioxide into products with added value has attracted the attention of many ***-free enzyme catalytic system coupled with electrical and light have been a promising attempt in the field of biological carbon fixation in recent *** this review,the research progresses of photoenzyme catalysis,electroenzyme catalysis and photo-electroenzyme catalysis for converting carbon dioxide into chemical products in cell-free systems are systematically *** focus on reviewing and comparing various coupling methods and principles of photoenzyme catalysis and electroenzyme catalysis in cell-free systems,especially the materials used in the construction of the coupling system,and analyze and point out the characteristics and possible problems of different coupling ***,we discuss the major challenges and prospects of coupling physical signals and cell-free enzymatic catalytic systems in the field of CO2fixation,suggesting possible strategies to improve the carbon sequestration capacity of such systems.

关键词： CO 2 fixation Cell-free system Enzyme Photoenzyme catalysis Electroenzyme catalysis

Nonlinear robust adaptive control for bidirectional stabilization system of all-electric tank with unknown actuator backlash compensation and disturbance estimation

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Defence Technology（防务技术） 2024年第2期32卷 144-158页

作者： Shusen yuan Wenxiang Deng Jianyong Yao Guolai yang School of Mechanical Engineering Nanjing University of Science and TechnologyNanjing210094China

Since backlash nonlinearity is inevitably existing in actuators for bidirectional stabilization system of allelectric tank,it behaves more drastically in high maneuvering *** this work,the accurate tracking control for bidirectional stabilization system of moving all-electric tank with actuator backlash and unmodeled disturbance is *** utilizing the smooth adaptive backlash inverse model,a nonlinear robust adaptive feedback control scheme is *** unknown parameters and unmodelled disturbance are addressed separately through the derived parametric adaptive function and the continuous nonlinear robust *** the unknown backlash parameters are updated via adaptive function and the backlash effect can be suppressed successfully by inverse operation,which ensures the system ***,the system disturbance in the high maneuverable environment can be estimated with the constructed adaptive law online improving the engineering ***,Lyapunov-based analysis proves that the developed controller can ensure the tracking error asymptotically converges to zero even with unmodeled disturbance and unknown actuator *** co-simulations and experiments illustrate the advantages of the proposed approach.

关键词： Bidirectional stabilization system Robust control Adaptive control Backlash inverse Disturbance estimation

Climatic implications in earlywood and latewood width indices of Chinese pine in north central China

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Journal of Forestry Research 2024年第3期35卷 143-153页

作者： Kaixuan yang Junzhou Zhang Haowen Fan yuan Yan College of Geographic Sciences Qinghai Normal UniversityXining 810016People's Republic of China Key Laboratory of Tibetan Plateau Land Surface Processes and Ecological Conservation(Ministry of Education) Xining 810016People's Republic of China Key Laboratory of Western China's Environmental Systems(Ministry of Education) College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730030People's Republic of China Gansu Liancheng Forest Ecosystem Field Observation and Research Station Lanzhou UniversityLanzhou 730333People's Republic of China School of Geography and Information Engineering University of GeoscienceWuhan 430074People's Republic of China

Latewood width(LWW)indices of trees are considered a reliable proxy of summer precipitation in the Northern ***,the strong coupling and high correlation between earlywood width(EWW)and LWW indices often prevent registration of climate signals of the LWW *** this study,328-year-long earlywood width and latewood width chronologies were developed from Chinese pine at two sites in the Hasi Mountains,north central *** climate responses of these chronologies were analyzed and the LWW index used to derive sum-mer precipitation *** analyses showed that LWW was particularly influenced by earlywood growth and recorded stronger climate signals of the previous year as EWW,rather than those of the current year with infrequent summer climate ***,after removing the effect of earlywood growth using a simple regression model,the adjusted LWW chronology(LWW_(adj))showed a strong relationship with July precipitation in dry *** suggests that the LWW_(adj) chronology has the potential to be used to investigate long-term variability in summer precipitation in drought-limited regions.

关键词： Dendroclimatology Latewood width Climate response Summer precipitation Earlywood effect

Extraction method of typical IEQ spatial distributions based on low-rank sparse representation and multi-step clustering

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Building Simulation 2024年第6期17卷 983-1006页

作者： Yuren yang yang Geng Hao Tang Mufeng yuan Juan Yu Borong Lin School of Architecture Tsinghua UniversityBeijingChina Key Laboratory of Eco Planning&Green Building Ministry of EducationTsinghua UniversityBeijingChina

Indoor environment quality(IEQ)is one of the most concerned building performances during the operation *** non-uniform spatial distribution of various IEQ parameters in large-scale public buildings has been demonstrated to be an essential factor affecting occupant comfort and building energy ***,IEQ sensors have been widely employed in buildings to monitor thermal,visual,acoustic and air ***,there is a lack of effective methods for exploring the typical spatial distribution of indoor environmental quality parameters,which is crucial for assessing and controlling non-uniform indoor *** this study,a novel clustering method for extracting IEQ spatial distribution patterns is ***,representation vectors reflecting IEQ distributions in the concerned space are generated based on the low-rank sparse ***,a multi-step clustering method,which addressed the problems of the“curse of dimensionality”,is designed to obtain typical IEQ distribution patterns of the entire indoor *** proposed method was applied to the analysis of indoor thermal environment in Beijing Daxing international airport *** a result,four typical temperature spatial distribution patterns of the terminal were extracted from a four-month monitoring,which had been validated for their good *** typical patterns revealed typical environmental issues in the terminal,such as long-term localized overheating and temperature increases due to a sudden influx of *** extracted typical IEQ spatial distribution patterns could assist building operators in effectively assessing the uneven distribution of IEQ space under current environmental conditions,facilitating targeted environmental improvements,optimization of thermal comfort levels,and application of energy-saving measures.

关键词： indoor environment quality(IEQ) thermal environment spatial distribution temperature field low-rank sparse representation(LRSR) clustering

Distributed active vibration control for helicopter based on diffusion collaboration

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Chinese Journal of Aeronautics 2024年第8期37卷 208-232页

作者： yang yuan yang LU Xunjun MA Jingliang LI Huiyu YUE National Key Laboratory of Helicopter Aeromechanics Nanjing University of Aeronautics and AstronauticsNanjing 210016China Wuhan Second Ship Design and Research Institute Wuhan 430205China

The active vibration control technology has been successfully applied to several helicopter ***,with the increasing of control scale,traditional centralized control algorithms are experiencing significant increase of computational complexity and physical implementation *** address this issue,a diffusion collaboration-based distributed Filtered-x Least Mean Square algorithm applied to active vibration control is proposed,drawing inspiration from the concept of data fusion in wireless sensor *** algorithm distributes the computation load to each node,and constructs the active vibration control network topology of large-scale system by discarding the weak coupling secondary paths between nodes,achieving distributed active vibration *** order to thoroughly validate the effectiveness and superiority of this algorithm,a helicopter fuselage model is designed as the research ***,the excellent vibration reduction performance of the proposed algorithm is confirmed through ***,specialized node control units are developed,which utilize STM32 microcontroller as the processing ***,a distributed control system is constructed based on multi-processor *** on this foundation,a large-scale active vibration control experimental platform is *** on the platform,experiments are carried out,involving the 4-input 4-output system and the 8-input 8-output *** experimental results demonstrate that under steady-state harmonic excitation,the proposed algorithm not only ensures control effectiveness but also reduces computational complexity by 50%,exhibiting faster convergence speed compared with traditional centralized *** time-varying external excitation,the proposed algorithm demonstrates rapid tracking of vibration changes,with vibration amplitudes at all controlled points declining by over 94%,proving the strong robustness and adaptive capability of the algorithm

关键词： Helicopter Active vibration control Diffusion collaboration Distributed control Experiment