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PVDF/6H-SiC composite fiber films with enhanced piezoelectric performance by interfacial engineering for diversified applications

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Journal of Materials Science & Technology 2024年第3期170卷 238-245页

作者： Linlin zhou tao Yang Chunyu Guo Kang Wang Enhui Wang Laipan Zhu Hailong Wang Sheng Cao Kuo-Chih Chou Xinmei Hou Institute for Carbon Neutrality University of Science and Technology BeijingBeijing 100083China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China School of Materials Science Engineering Zhengzhou UniversityZhengzhou 450001China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi UniversityNanning 530004China

Piezoelectric silicon carbide(SiC)has been quite attractive due to its superior chemical and physical properties as well as wide potential ***,the inherent brittleness and unsatisfactory piezoelectric response of piezoelectric semiconductors remain the major obstacles to their diversified ***,flexible multifunctional PVDF/6H-SiC composite fiber films are fabricated and utilized to assemble both piezoelectric nanogenerators(PENGs)and stress/temperature/light *** open cir-cuit voltage(V_(oc))and the density of short circuit current(I_(sc))of the PENG based on the PVDF/5 wt%6H-SiC composite fiber films reach 28.94 V and 0.24μA cm^(-2),showing a significant improvement of 240%and 300%compared with that based on the pure PVDF *** effect of 6H-SiC nanoparticles(NPs)on inducing interfacial polarization and stress concentration in composite fiber films is proved by first-principles calculation and finite element *** stress/temperature/light sensors based on the composite fiber film also show high sensitivity to the corresponding *** study shows that the PVDF/6H-SiC composite fiber film is a promising candidate for assembling high-performance energy harvesters and diverse sensors.

关键词： 6H-SiC PVDF Multifunctional composite fiber film Energy harvester Stress/temperature/light sensor

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Prestoring lithium into SnO_(2)coated 3D carbon fiber cloth framework as dendrite-free lithium metal anode

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Particuology 2024年第1期84卷 89-97页

作者： tao Wei Yanyan zhou Cheng Sun Lesheng Liu Sijia Wang Mengting Wang Ye Liu Qing Huang Quanchao Zhuang Yongfu Tang School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang212003China College of Materials Science and Engineering Nanjing Forestry UniversityNanjing210037China Li-ion Batteries Lab School of Materials Science and EngineeringChina University of Mining and TechnologyXuzhouChina Hebei Key Laboratory of Applied Chemistry School of Environmental and Chemical EngineeringYanshan UniversityQinhuangdao066004China

For several decades,the promise of implementing of lithium(Li)metal anodes has been regarded as the"holy grail"for Li-based ***,we have proposed a facile design of a carbon fiber cloth(CFC)framework coated with SnO_(2)nanoparticles through a hydrothermal process,which served as a reliable host for prestoring molten Li to produce a CFC@SnO_(2)@Li composite ***,TEM,HRTEM,XPS and different electrochemical characterizations were carried *** to the synergetic effects of the 3D conductive CFC and the coated lithiophilic SnO_(2)nanoparticles,the designed CFC@SnO_(2)@Li electrodes can buffer the volume changes and reduce the local current density,thus suppress the Li dendrites during ***,the CFC@SnO_(2)electrodes showed a high and stable CE of 98.6%for 1000 cycles at a current density of 1 mA cm^(-2)(1 mAh cm^(-2)).What is more,at a high current density of 5 mA cm^(-2)and a high areal capacity of 5 mAh cm^(-2),the symmetric cell displayed relatively low overpotential and long cycling lifetime of 1600 *** results confirm its great potential as lithium metal anodes in practical battery applications.

关键词： Lithiophilic Lithium metal anodes SnO_(2) 3D anode Dendrite-free

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A Global Optimality Principle for Fully Coupled Mean-field Control Systems

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 379-413页

作者： tao HAO School of Statistics and Mathematics Shandong University of Finance and EconomicsJinan 250014China

This paper concerns a global optimality principle for fully coupled mean-field control *** the first-order and the second-order variational equations are fully coupled mean-field linear FBSDEs. A new linear relation is introduced, with which we successfully decouple the fully coupled first-order variational equations. We give a new second-order expansion of Y^(ε) that can work well in mean-field framework. Based on this result, the stochastic maximum principle is proved. The comparison with the stochastic maximum principle for controlled mean-field stochastic differential equations is supplied.

关键词： optimal control global maximum principle fully coupled general mean-field FBSDE adjoint equation recursive utility

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Regulating the key performance parameters for Hg-based IR NLO chalcogenides via bandgap engineering strategy

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Chinese Chemical Letters 2024年第10期35卷 490-494页

作者： A-Yang Wang Sheng-Hua zhou Mao-Yin Ran Xin-tao Wu Hua Lin Qi-Long Zhu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of Sciences(CAS)Fuzhou 350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China College of Chemistry Fuzhou UniversityFuzhou 350108China University of Chinese Academy of Sciences Bejing 100049China

Recently,non-centrosymmetric(NCS)Hg-based chalcogenides have garnered significant interest due to their strong second-harmonic-generation intensities(deff),making them attractive candidates for infrared nonlinear optical(IR-NLO)***,achieving both wide band gaps(Eg)and large phasematched deffsimultaneously in these materials remains a challenge due to their inherent constraints on each *** this research,we have successfully obtained two quaternary NCS Hg-based chalcogenides,Rb2HgGe_(3)S_(8)and Cs_(2)HgGe_(3)S_(8),by implementing a bandgap engineering strategy that involves alkali metal introduction and Hg/Ge ratio *** compounds consist of 2D[Hg Ge_(3)S_(8)]_(2)–anionic layers made of 1D[HgGeS_(6)]^(6–)chains and dimeric[Ge_(2)S_(6)]_(4–)polyhedra arranged alternately,and the charge-balanced Rb+/Cs+cations located between these ***,Rb_(2)HgGe_(3)S_(8)and Cs_(2)HgGe_(3)S_(8)exhibit overall properties required for promising IR-NLO materials,including sufficient PM deff(0.55–0.70×AgGaS_(2)@20_(5)0 nm),large Eg(3.27–3.41 e V),giant laser-induced damage thresholds(17.4–19.7×AgGaS_(2)@1064 nm),broad optical transmission intervals(0.32–17.5μm),and suitable theoretical birefringence(0.069–0.086@2050 nm).Furthermore,in-depth theoretical analysis reveals that the exceptional IRNLO performance is attributed to the synergy effects of distorted[HgS_(4)]and[GeS_(4)]*** study provides a useful strategy for enhancing the Eg and advancing Hg-based IR-NLO materials,which is expected to extended and implemented in other chalcogenide systems.

关键词： Hg-based chalcogenides IR nonlinear material Structure-activity relationship Wide energy gap Bandgap engineering strategy

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Monomorphic epitheliotropic intestinal T-cell lymphoma with bone marrow involved: A case report

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World Journal of Clinical Cases 2024年第4期12卷 814-819页

作者： Fen-Juan Zhang Wen-Juan Fang cang-Jian Zhang Department of Hematology Lishui Municipal Central HospitalLishui 323000Zhejiang ProvinceChina

BACKGROUND Monomorphic epithelial intestinal T-cell lymphoma(MEITL)is a rare type of peripheral T-cell *** clinical manifestations are diarrhea,abdominal pain,perforation and an abdominal *** SUMMARY We present a 52-year-old female patient who was diagnosed with *** disease progression was observed after multiline ***,the patient died of a severe *** MEITL is a rare intestinal primary T-cell lymphoma with aggressive behavior,a high risk of severe life-threatening complications,and a poor prognosis.

关键词： Monomorphic epithelial intestinal T-cell lymphoma Autologous stem cell transplantation Chemotherapeutics Case report

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Exploring geometry of genome space via Grassmann manifolds

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The Innovation 2024年第5期5卷 92-99,91页

作者： Xiaoguang Li tao zhou Xingdong Feng Shing-Tung Yau Stephen S.-T.Yau School of Statistics and Management Shanghai University of Finance and EconomicsShanghai 200433China Department of Mathematical Sciences Tsinghua UniversityBeijing 100084China Yanqi Lake Beijing Institute of Mathematical Sciences and Applications Beijing 101408China

It is important to understand the geometry of genome space in *** transforming genome sequences into frequency matrices of the chaos game representation(FCGR),we regard a genome sequence as a point in a suitable Grassmann manifold by analyzing the column space of the corresponding *** assess the sequence similarity,we employ the generalized Grassmannian distance,an intrinsic geometric distance that differs from the traditional Euclidean distance used in the classical k-mer frequency-based *** this method,we constructed phylogenetic trees for various genome datasets,including influenza A virus hemagglutinin gene,Orthocoronavirinae genome,and SARS-CoV-2 complete genome *** comparative analysis with multiple sequence alignment and alignment-free methods for large-scale sequences revealed that our method,which employs the subspace distance between the column spaces of different FCGRs(FCGR-SD),outperformed its competitors in terms of both speed and *** addition,we used low-dimensional visualization of the SARS-CoV-2 genome sequences and spike protein nucleotide sequences with our methods,resulting in some intriguing *** not only propose a novel and efficient algorithm for comparing genome sequences but also demonstrate that genome data have some intrinsic manifold structures,providing a new geometric perspective for molecular biology studies.

关键词： methods. manifold geometry

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Decreased Nrf2 protein level and low sperm quality in intractable spermatocystitis

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Asian Journal of Andrology 2024年第2期26卷 189-194页

作者： Shi-Ze Wang Jian-Nan Liu Fen-Fang zhou Ye-Jin-Peng Wang Peng Zhang Song-tao Cheng Department of Urology Sichuan Provincial People's HospitalUniversity of Electronic Science and Technology of ChinaChengdu 610072China Department of Urology Zhongnan Hospital of Wuhan UniversityWuhan 430071China Department of Health Management and Clinical Medicine School of Medicine and HealthWuhan PolytechnicUniversityWuhan 430071China

To investigate the molecular etiology of low sperm quality in patients with intractable spermatocystitis,spermatozoa samples from patients with persistent hematospermia undergoing transurethral seminal vesiculoscopy and healthy volunteers were *** samples were collected from the seminal vesicles through transurethral seminal vesiculoscopy or by masturbation *** quality was analyzed by a WLJY-9000 color semen analysis *** of tumor necrosis factor alpha(TNFa)and interleukin-6(IL-6)in the seminal plasma was performed using enzyme-linked immunosorbent assay(ELISA).Measurement of H_(2)O_(2)in the seminal plasma was performed with a hydrogen peroxide *** protein levels of nuclear factor erythroid 2-related factor 2(Nrf2)and phosphorylated-Nrf2(p-Nrf2)were measured by western blot analysis and immunofluorescence *** sperm quality parameters and increased levels of inflammatory cytokines(TNFa,IL-6,and H_(2)O_(2))in the seminal plasma were detected among the semen samples from the patients with persistent ***2 and p-Nrf2 were strongly expressed in the nucleus and periphery of human sperm cells,according to the results of the immunofluorescence *** protein levels of Nrf2 and p-Nrf2 were significantly lower in the spermatozoa samples from patients with persistent hematospermia than in those from healthy volunteers with normal sperm *** results suggested that Nrf2 signaling might play a role in the low sperm quality of patients with intractable spermatocystitis.

关键词： H_(2)O_(2) Nrf2 sperm quality spermatocystitis

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Optical multipath self-interference cancellation for a wideband in-band full-duplex system using a silicon photonic modulator chip

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Chinese Optics Letters 2024年第7期22卷 126-131页

作者： Xiao Yu Jia Ye Lianshan Yan tao zhou Yue Zhu Peng Li Xihua Zou Wei Pan Center for Information Photonics and Communications School of Information Science and TechnologySouthwest Jiaotong UniversityChengdu 611756China Key Laboratory of Electronic Information Control Southwest China Research Institute of Electronic EquipmentChengdu 610029China Microwave Photonics Research Laboratory School of Electrical Engineering and Computer ScienceUniversity of OttawaOttawaONK1N6N5Canada

We propose and experimentally demonstrate a photonic method for wideband multipath self-interference cancellation using a silicon photonic modulator *** chip generates phase-inverted reference signals by leveraging the opposite phase between optical *** managing amplitude and phase imbalances between self-interference and reference signals,the approach rectifies discrepancies through consistent chip manufacturing and packaging *** photonic multi-dimensional multiplexing,including wavelength and polarization,enables the acquisition of multiple reference *** results show multipath cancellation depths of 25.53 dB and 23.81 dB for bandwidths of 500 MHz and 1 GHz,achieved by superimposing 2-path reference signals.

关键词： microwave photonics multipath self-interference silicon photonics

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Prediction of soil organic carbon stock combining Sentinel-1 and Sentinel-2 images in the Zoige Plateau, the northeastern Qinghai-Tibet Plateau

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Ecological Processes 2024年第2期13卷 165-176页

作者： Junjie Lei Changli Zeng Lv Zhang Xiaogang Wang Chanhua Ma tao zhou Benjamin Laffitte Ke Luo Zhihan Yang Xiaolu Tang State Key Laboratory of Geohazard Prevention and Geoenvironment Protection Chengdu University of Technology Sichuan Academy of Geological Survey Sichuan Institute of Nuclear Geological Survey College of Earth Sciences Chengdu University of Technology Tianfu Yongxing Laboratory

Background Soil organic carbon（SOC） is a critical component of the global carbon cycle, and an accurate estimate of regional SOC stock（SOCS） would significantly improve our understanding of SOC sequestration and cycles. Zoige Plateau, locating in the northeastern Qinghai-Tibet Plateau, has the largest alpine marsh wetland worldwide and exhibits a high sensitivity to climate fluctuations. Despite an increasing use of optical remote sensing in predicting regional SOCS, optical remote sensing has obvious limitations in the Zoige Plateau due to highly cloudy weather, and knowledge of on the spatial patterns of SOCS is limited. Therefore, in the current study, the spatial distributions of SOCS within 100 cm were predicted using an XGBoost model—a machine learning approach, by integrating Sentinel-1, Sentinel-2 and field observations in the Zoige *** The results showed that SOC content exhibited vertical distribution patterns within 100 cm, with the highest SOC content in topsoil. The tenfold cross-validation approach showed that XGBoost model satisfactorily predicted the spatial patterns of SOCS with a model efficiency of 0.59 and a root mean standard error of 95.2 Mg ha-1. Predicted SOCS showed a distinct spatial heterogeneity in the Zoige Plateau, with an average of 355.7 ± 123.1 Mg ha-1within 100 cm and totaled 0.27 × 10～9 Mg *** High SOC content in topsoil highlights the high risks of significant carbon loss from topsoil due to human activities in the Zoige Plateau. Combining Sentinel-1 and Sentinel-2 satisfactorily predicted SOCS using the XGBoost model, which demonstrates the importance of selecting modeling approaches and satellite images to improve efficiency in predicting SOCS distribution at a fine spatial resolution of 10 m. Furthermore, the study emphasizes the potential of radar（Sentinel-1） in developing SOCS mapping, with the newly developed fine-resolution mapping having important applications in land management, ecological resto

关键词： SOC Vegetation index Texture XGBoost Sentinel-1 Sentinel-2

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High-entropy rare earth stannate ceramics:Acid corrosion resistant radiative cooling materials with high atmospheric transparency window emissivity and high near-infrared solar reflectivity

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Journal of Advanced Ceramics 2024年第5期13卷 630-640页

作者： tao Chen Yanyan He Yanyu Pan Kaixian Wang Minzhong Huang Liyan Xue Yazhu Li Fan Yang Yanchun zhou Heng Chen Fujian Institute of Research on the Structure of Matter Chinese Academy of SciencesFuzhou 350002China College of Chemistry and Materials Science Fujian Normal UniversityFuzhou 350117China Xiamen Institute of Rare Earth Materials Haixi InstitutesChinese Academy of SciencesXiamen 361021China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi InstitutesChinese Academy of SciencesXiamen 361021China Key Laboratory of Rare Earths Ganjiang Innovation AcademyChinese Academy of SciencesGanzhou 341000China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China

In response to the development of the concepts of“carbon neutrality”and“carbon peak”,it is critical to developing materials with high near-infrared(NIR)solar reflectivity and high emissivity in the atmospheric transparency window(ATW;8–13μm)to advance zero energy consumption radiative cooling *** regulate emission and reflection properties,a series of high-entropy rare earth stannate ceramics(HE-RE_(2)Sn_(2)O_(7):(Y_(0.2)La_(0.2)Nd_(0.2)Eu_(0.2)Gd_(0.2))_(2)Sn_(2)O_(7),(Y_(0.2)La_(0.2)Sm_(0.2)Eu_(0.2)Lu_(0.2))_(2)Sn_(2)O_(7),and(Y_(0.2)La_(0.2)Gd_(0.2)Yb_(0.2)Lu_(0.2))_(2)Sn_(2)O_(7))with severe lattice distortion were prepared using a solid phase reaction followed by a pressureless sintering method for the first *** distortion is accomplished by introducing rare earth elements with different cation radii and *** as-synthesized HE-RE_(2)Sn_(2)O_(7)ceramics possess high ATW emissivity(91.38%–95.41%),high NIR solar reflectivity(92.74%–97.62%),low thermal conductivity(1.080–1.619 W·m^(−1)·K^(−1)),and excellent chemical *** the one hand,the lattice distortion intensifies the asymmetry of the structural unit to cause a notable alteration in the electric dipole moment,ultimately enlarging the ATW *** the other hand,by selecting difficult excitation elements,HE-RE_(2)Sn_(2)O_(7),which has a wide band gap(Eg),exhibits high NIR solar ***,the multi-component design can effectively enhance radiative cooling ability of HE-RE_(2)Sn_(2)O_(7)and provide a novel strategy for developing radiative cooling materials.

关键词： radiative cooling materials high-entropy ceramics(HECs) rare earth stannate(RE_(2)Sn_(2)O_(7)) high atmospheric transparency window emissivity high near-infrared(NIR)solar reflectivity

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