检索结果-南通市图书馆

Chinese Journal of Polymer Science 2024年第10期42卷 1610-1618,I0016页

作者： Xin-Yu chen Yu-Bing Fu xue-Ling Yan Lan Liu School of Materials Science and Engineering Key Lab of Guangdong Province for High Property and Functional Polymer MaterialsSouth China University of TechnologyGuangzhou510641China

Elastomers with high strength and toughness,excellent self-healing properties,and biocompatibility have broad application prospects in wearable electronics and other fields,but preparing it remains a *** this work,we propose a highly adaptable strategy by introducing the small molecule crosslinking agent of triethanolamine(TEA)to the poly(thioctic acid)(PTA)chains and preparing the PAx Ey elastomers using a simple synthesis *** strategy stabilizes the PTA chains by constructing multiple non-covalent cross-linked dynamic networks,endowing materials with excellent strength and toughness(tensile strength of 288 kPa,toughness of 278.2 kJ/m3),admirable self-healing properties(self-healing efficiency of 121.6%within 7 h at 70℃),and good *** PAx Ey elastomers can also be combined with MWNTs to become flexible strain sensors,which can be used to monitor human joint movements with high sensitivity,repeatable responses,and stability.

关键词： Thioctic acid Ion clusters Multiple dynamic networks Self-healing strengthening Flexible strain sensor

Frequency-dependent Electrical Capacitance and Resistance of Ultra-high Performance Concrete and Their Responses to Compressive Strain

在线全文

学校读者我要写书评

暂无评论

Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 968-978页

作者：吴瑜孙明清 ZHU Lutao song Qiulei chen Jianzhong Hubei Key Laboratory of Theory and Application of Advanced Materials Mechanics School of ScienceWuhan University of TechnologyWuhan 430070China School of Civil Engineering and Architecture Hubei University of Arts and ScienceXiangyang 441053China Suzhou Concrete and Cement Products Research Institude Co. LtdSuzhou 215026China

The frequency-dependent electrical properties and strain self-sensing behaviour of ultra-high performance concrete(UHPC)as cement-based stress/strain self-sensing(CBSS)smart materials were investigated in the frequency range from 100 Hz to 300 *** using the electrical parameters of the equivalent electric circuit model,the quantitative relations of capacitance and conductance of CBSS with the measurement frequency were *** capacitance and the conductance exhibit power-law type dependence on the measurement *** calculated capacitance values at frequencies beyond 2 kHz and conductance values are consistent with the experimental *** sweep-frequency test and the fixed-frequency test were performed to examine effects of the excitation frequencies on strain self-sensing properties of *** fractional change in capacitance(FCC)and resistance(FCR)of CBSS are frequency-dependent in the frequency range from 100 Hz to the f_(B),but frequency-independent in the frequency range from the f_(B)to 300 *** f_(A)and the f_(B)are 1.7-4.0 kHz and 11-78 kHz depending on the fiber dosages,*** and FCR reach their maximum at the f_(A)and 100 Hz,*** responses of capacitance and resistance of CBSS to strain show good repeatability during cyclic *** the fiber dosage increases,capacitance-based sensitivity to strain increases initially and then decreases at the f_(A),and resistance-based sensitivity to strain of CBSS increases with increasing fiber contents.

关键词： UHPC strain self-sensing capacitance-based frequency-dependent

Progress and prospects of Mg-based amorphous alloys in azo dye wastewater treatment

在线全文

学校读者我要写书评

暂无评论

Journal of Magnesium and Alloys 2024年第3期12卷 873-889页

作者： Yanan chen Fengchun chen Liang Li chen Su Bo song Hongju Zhang Shengfeng Guo Fusheng Pan School of Materials and Energy Southwest UniversityChongqing 400715China Analytical and Testing Center Southwest UniversityChongqing 400715China College of Materials Science and Engineering Chongqing UniversityChongqing 400044China

Mg-based amorphous alloys exhibit efficient catalytic performance and excellent biocompatibility with a promising application probability,specifically in the field of azo dye wastewater ***,the problems like difficulty in preparation and poor cycling stability need to be *** present,Mg-based amorphous alloys applied in wastewater degradation are available in powder and *** amorphous alloy powder fabricated by ball milling has a high specific surface area,and its reactivity is thousands of times better than that of gas atomized alloy *** the development is limited due to the high energy consumption,difficult and costly process of powder *** single roller melt-spinning method is a new manufacturing process of amorphous alloy *** to amorphous powder,the specific surface area of amorphous ribbon is relatively lower,therefore,it is necessary to carry out surface modification to enhance *** is a way that can form a pore structure on the surface of the amorphous alloys,increasing the specific surface area and providing more reactive sites,which all contribute to the catalytic *** the optimal conditions for Mg-based amorphous alloys in wastewater degradation by adjusting amorphous alloy composition,choosing suitable method to preparation and surface modification,reducing cost,expanding the pH range will advance the steps to put Mg-based amorphous alloys in industrial environments into practice.

关键词： Mg-based amorphous alloys Azo dyes Dealloying Surface modification Wastewater degradation.

Personal Thermal Management by Radiative Cooling and Heating

在线全文

学校读者我要写书评

暂无评论

Nano-Micro Letters 2024年第8期16卷 225-267页

作者： Shidong xue Guanghan Huang Qing chen Xungai Wang Jintu Fan Dahua Shou School of Fashion and Textiles The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China Future Intelligent Wear Centre The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China State Key Laboratory of Precision Electronic Manufacturing Technology and Equipment Guangdong University of TechnologyGuangzhou 510006People’s Republic of China Shanghai International Fashion Innovation Center Donghua UniversityShanghai 200051People’s Republic of China Research Centre of Textiles for Future Fashion The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China

Maintaining thermal comfort within the human body is crucial for optimal health and overall *** merely broadening the setpoint of indoor temperatures,we could significantly slash energy usage in building heating,ventilation,and air-conditioning *** recent years,there has been a surge in advancements in personal thermal management(PTM),aiming to regulate heat and moisture transfer within our immediate surroundings,clothing,and *** advent of PTM is driven by the rapid development in nano/micro-materials and energy science and *** emerging research area in PTM is personal radiative thermal management(PRTM),which demonstrates immense potential with its high radiative heat transfer efficiency and ease of ***,it is less taken into account in traditional textiles,and there currently lies a gap in our knowledge and understanding of *** this review,we aim to present a thorough analysis of advanced textile materials and technologies for ***,we will introduce and discuss the underlying radiation heat transfer mechanisms,fabrication methods of textiles,and various indoor/outdoor applications in light of their different regulation functionalities,including radiative cooling,radiative heating,and dual-mode ***,we will shine a light on the current hurdles,propose potential strategies,and delve into future technology trends for PRTM with an emphasis on functionalities and applications.

关键词： Personal thermal management Radiative cooling and heating Thermal comfort Dynamic thermoregulation

Synthesis of uniform two-dimensional MoS_(2) films via thermal evaporation

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第4期17卷 3217-3223页

作者： xue-Wei Lu Zhewei Li chen-Kai Yang Weijia Mou Liying Jiao Key Laboratory of Organic Optoelectronics and Molecular Engineering of the Ministry of Education Department of ChemistryTsinghua UniversityBeijing 100084China

Two-dimensional(2D)molybdenum disulfide(MoS_(2))holds great potential for various applications such as electronic devices,catalysis,lubrication,anti-corrosion and so *** evaporation is a versatile thin film deposition technique,however,the conventional thermal evaporation techniques face challenges in producing uniform thin films of MoS_(2) due to its high melting temperature of 1375℃.As a result,only thick and rough MoS_(2) films can be obtained using these *** address this issue,we have designed a vacuum thermal evaporation system specifically for large-scale preparation of MoS_(2) thin *** using K2MoS4 as the precursor,we achieved reliable deposition of uniform polycrystalline MoS_(2) thin films with a size of 50 mm×50 mm and controllable thickness ranging from 0.8 to 2.4 *** approach also allows for patterned deposition of MoS_(2) using shadow masks and sequential deposition of MoS_(2) and tungsten disulfide(WS_(2)),similar to conventional thermal evaporation ***,we have demonstrated the potential applications of the obtained MoS_(2) thin films in field effect transistors(FETs),memristors and electrocatalysts for hydrogen evolution reaction(HER).

关键词： thermal evaporation molybdenum disulfide two-dimensional memristors hydrogen evolution reaction

Experimental investigation on coal pore-fracture variation and fractal characteristics synergistically affected by solvents for improving clean gas extraction

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

International Journal of Mining Science and Technology 2024年第3期34卷 413-425页

作者： Feilin Han Sheng xue Chunshan Zheng Zhongwei chen Guofu Li Bingyou Jiang Key Laboratory of Safe and Effective Coal Mining of Ministry of Education Anhui University of Science and TechnologyHuainan 232001China School of Safety Science and Engineering Anhui University of Science and TechnologyHuainan 232001China School of Mechanical and Mining Engineering University of QueenslandQLD 4072Australia State Key Laboratory of Coal and Coalbed Methane Co-Mining Jincheng 048012China

Chemical solvents instead of pure water being as hydraulic fracturing fluid could effectively increase permeability and improve clean methane extraction ***,pore-fracture variation features of lean coal synergistically affected by solvents have not been fully *** testing,nuclear magnetic resonance analysis,liquid phase mass spectrometry was adopted to comprehensively analyze pore-fracture change characteristics of lean coal treated by combined solvent(NMP and CS_(2)).Meanwhile,quantitative characterization of above changing properties was conducted using geometric fractal *** model between permeability,fractal dimension and porosity were *** indicate that the end face fractures of coal are well developed after CS2and combined solvent treatments,of which,end face box-counting fractal dimensions range from 1.1227 to *** decreases in ultrasonic longitudinal wave velocity of coal affected by NMP,CS_(2)and combined solvent are 2.700%,20.521%,22.454%,*** treatments could lead to increasing amount of both mesopores and *** ratio of fractal dimension Dsis 0.259%–2.159%,while permeability increases ratio of NMR ranges from 0.1904 to ***,combined solvent could dissolve coal polar and non-polar small molecules and expand flow *** could provide reference for solvent selection and parameter optimization of permeability-enhancement technology.

关键词： Clean gas extraction Chemical solvent Experimental investigation Fractal characteristics Pore fracture

Insight into demand-driven preparation of single-atomic mediators for lithium–sulfur batteries

在线全文

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2024年第3期90卷 205-219,I0007页

作者： Miaoyu Lu Yifan Ding Zaikun xue Ziang chen Yuhan Zou Jingyu Sun College of Energy Soochow Institute for Energy and Materials InnovationsKey Laboratory for Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceSoochow UniversitySuzhou 215006JiangsuChina Beijing Graphene Institute Beijing 100095China

Lithium-sulfur(Li-S) batteries have attracted considerable attention as one of the most appealing energy storage *** efforts have been devoted to tackling the tremendous challenges,mainly pertaining to the severe shuttle effect,sluggish redox kinetics and lithium dendritic ***-atomic mediators as promising candidates exhibit impressive performance in addressing these intractable *** research often utilizes a trial-and-error approach,proposing solutions to fabricate single-atomic materials with diversified ***,comprehensive review articles especially targeting demand-driven preparation are still in a nascent *** by these considerations,this review summarizes the design of single-atomic mediators based on the application case-studies in LiS batteries and other metal-sulfur *** preparation routes represented by chemical vapor deposition technology are introduced in a demand-oriented ***,future research directions are proposed to foster the advancement of single-atomic mediators in Li-S realm.

关键词： Single-atom catalyst Lithium–sulfur battery Chemical vapor deposition Demand-driven preparation

Experimental observation of the significant difference between surface and bulk Kondo processes in Kondo lattice YbCu_(2)Si_(2)

在线全文

学校读者我要写书评

暂无评论

Science China(Physics,Mechanics & Astronomy) 2024年第4期67卷 154-160页

作者： Yin-Zou Zhao Jiao-Jiao song Qi-Yi Wu Hao Liu chen Zhang Bo chen Hong-Yi Zhang Zhen-Hua chen Yao-Bo Huang xue-Qing Ye Ya-Hua Yuan Yu-Xia Duan Jun He Jian-Qiao Meng School of Physics Central South UniversityChangsha 410083China Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201204China

Synchrotron-based angle-resolved photoemission spectroscopy was employed to investigate the temperature evolution of the Yb 4 f spectral for surface and bulk in the Kondo lattice YbCu_(2)Si_(2).Our study quantitatively distinguishes between the surface and bulk hybridization processes,revealing that the onset temperatures for both surface and bulk hybridization processes are significantly higher than the Kondo ***,we found that the effective surface Kondo temperature is much lower than that of the *** findings offer valuable insights into the understanding of heavy fermion physics.

关键词： Kondo lattice angle-resolved photoemission spectroscopy electronic structure hybridization surface state

New approach to measuring topological phase transitions utilizing Floquet technology

在线全文

学校读者我要写书评

暂无评论

Chinese Physics B 2024年第9期33卷 282-288页

作者： xue-Ying Yang Wei Wu Ping-Xing chen College of Sciences National University of Defense TechnologyChangsha 410073China

The Floquet technique provides a novel anomalous topological phase for non-equilibrium phase *** on the high symmetry of the quantum anomalous Hall model,the findings suggest a one-to-one correspondence between the average spin texture and the Floquet quasi-energy spectrum.A new approach is proposed to directly measure the quasienergy spectrum,replacing previous measurements of the average spin ***,we proposed a reliable experimental scheme based on ion trap *** scheme markedly reduces the measurement workload,improves the measurement fidelity,and is applicable to multiple platforms such as cold atoms and nuclear magnetic resonance.

关键词： topological phase transition Floquet technique ion trap

Legacy and emerging per-and polyfluoroalkyl substances(PFAS) in the atmosphere: A comprehensive review

在线全文

学校读者我要写书评

暂无评论

Science China Technological Sciences 2024年第10期67卷 3032-3050页

作者： QIAO BiTing song DongBao chen Hao YAO YiMing SUN HongWen MOE Key Laboratory of Pollution Processes and Environmental Criteria College of Environmental Science and EngineeringNankai University

With long-term production and widespread application, per-and polyfluoroalkyl substances(PFAS) have been detected in various media worldwide, including the atmosphere. Since the gradual restriction and phase-out of C8perfluoroalkyl acids(PFAAs), environmental contamination by emerging PFAS substitutes such as short-chain PFAA homologues, perfluoroether carboxylic, and sulfonic acids has been reported. Although there has been extensive monitoring of emerging PFAS substitutes in the aquatic environment, few studies have conducted target analysis and nontarget screening(NTS) of emerging unknown PFAS in the atmosphere over the past decade. To fill the gap, this review focused on emerging PFAS in the atmosphere in addition to legacy PFAS. The reported sampling, pretreatment, and instrumental analysis methods for target analysis and NTS of both neutral and ionic PFAS in the atmosphere are summarized, along with the advantages and current limitations of different sampling and NTS methods for PFAS in the atmosphere. The global levels, composition, and spatiotemporal distribution characteristics of legacy and emerging PFAS in the atmosphere are summarized and their transport, transformation, and dry/wet deposition are elucidated. The review highlights the importance of developing and applying the all-in-one strategy integrating target, suspect screening, and NTS to gain insights into emerging PFAS in the atmosphere and provide a reference for future research.

关键词： emerging PFAS atmosphere nontarget screening spatiotemporal distribution fate