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Changes in global land surface frozen ground and freeze-thaw processes during 1950-2020 based on ERA5-Land data

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Advances in Climate Change Research 2024年第2期15卷 265-274页

作者： yong YANG Ren-Sheng chen yong-Jian {3. Hong-Yuan LI Zhang-Wen LIU Qilian Alpine Ecology and Hydrology Research Station Key Laboratory of Ecological Safety and Sustainable Development in Arid LandsNorthwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 73000China State Key Laboratory of Cryospheric sciences Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 73000China Shandong Provincial Key Laboratory of Water and Soil Conservation and Environmental Protection College of Resources and EnvironmentLinyi UniversityLinyi 276000China

Frozen ground(FG)plays an important role in global and regional climates and environments through changes in land freeze-thaw processes,which have been conducted mainly in different ***,the changes in land surface freeze-thaw processes under climate change on a global scale are still *** on ERA5-Land hourly land skin temperature data,this study evaluated changes in the global FG area,global land surface first freeze date(FFD),last freeze date(LFD)and frost-free period(FFP)from 1950 to *** results show that the current FG areas(1991-2020 mean)in the Northern Hemisphere(NH),Southern Hemisphere(SH),and globe are 68.50×10^(6),9.03.10^(6),and 77.53.10^(6)km^(2),which account for 72.4%,26.8%,and 60.4%of the exposed land(excluding glaciers,ice sheets,and water bodies)in the NH,SH and the globe,respectively;further,relative to 1951-1980,the FG area decreased by 1.9%,8.8%,and 2.8%,*** FG at lower latitudes degrades to intermittently FG,and intermittently FG degrades to non-frozen ground,which caused the global FG boundary to retreat to higher latitudes from 1950 to *** annual FG areas in the NH,SH,and globe all show significant decreasing trends(p1950 to 2020 at-0.3.×10^(6),-0.22×10^(6),and-0.54×10^(6)km^(2)per decade,*** FFP prolongation in the NH is mainly influenced by LFD advance,while in the SH it is mainly controlled by FFD *** prolongation trend of FFP in the NH(1.3. d per decade)is larger than that in the SH(1.15 d per decade).

关键词： Frozen ground Freeze-thaw processes Frost-free period First freeze date Global warming

GA-LSTM speed prediction-based DDQN energy management for extended-range vehicles

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Energy and AI

Energy and AI 2024年第3期17卷 11-28页

作者： Laiwei Lu Hong Zhao Fuliang Xv yong Luo Junjie chen Xiaoyun ding College of Mechanical and Electrical Engineering Qingdao UniversityQingdao266071Shandong ProvinceChina

In this paper,a dual deep Q-network(DDQN)energy management model based on long-short memory neural network(LSTM)speed prediction is proposed under the model predictive control(MPC)*** initial learning rate and neuron dropout probability of the LSTM speed prediction model are optimized by the genetic algorithm(GA).The prediction results show that the root-mean-square error of the GA-LSTM speed prediction method is smaller than the SVR method in different speed prediction *** predicted demand power,the state of charge(SOC),and the demand power at the current moment are used as the state input of the agent,and the real-time control of the control strategy is realized by the MPC *** simulation results show that the proposed control strategy reduces the equivalent fuel consumption by 0.03.4 kg compared with DDQN,0.843. kg compared with ECMS,and 0.742 kg compared with the power-following control *** difference between the proposed control strategy and the dynamic planning control strategy is only 0.0048 kg,0.193.,while the SOC of the power battery remains ***,the hardware-in-the-loop simulation verifies that the proposed control strategy has good real-time performance.

关键词： Extended-range vehicle LSTM speed prediction Genetic algorithm Model predictive control(MPC) Deep reinforcement learning Double deep Q-network(DDQN)

Preparation of calcium carbonate with microstructure and nanostructure from carbide slag for CO_(2) sequestration by using recyclable ammonium chloride

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Particuology 2024年第7期90卷 1-9页

作者： Jin Yao Qiuju chen Li Zeng Wenjin ding Key Laboratory of Ministry of Education for Solid Waste Treatment and Resource Recycle Southwest University of Science and TechnologyMianyang621010China Sichuan Engineering Lab of Non-metallic Mineral Powder Modification and High-value Utilization Mianyang621010China School of Architecture and Civil Engineering Chengdu UniversityChengdu610106China

Based on the composition characteristics of carbide slag and the application of polyvinyl chloride,a method of preparing calcium carbonate with microstructure and nanostructure by using carbide slag as a raw material and ammonium chloride as a leaching agent was *** factors for the preparation of calcium carbonate and the effects of different conditions on the crystal phase,grain size,and morphology of calcium carbonate were systematically *** results showed that the nanosized calcium carbonate was prepared at 60 mL/min,25°C,no additional ammonia,and 60 *** product of spherical vaterite was in accordance with the relevant standards for the industrial precipitation of calcium ***,the reuse of carbonation filtrate was *** crystal phase,grain size,and morphology of the carbonation product could be controlled by adjusting the reaction *** manuscript provided a new idea for resource utilization of carbide slag and preparing nanocalcium carbonate.

关键词： Carbide slag Ammonium chloride Cyclic utilization Micro and nano structure Product control

Modification of BCC phase and the enhanced reversible hydrogen storage properties of Ti-V-Fe-Mn alloys with varied V/Fe ratios

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china Foundry 2024年第5期21卷 546-554页

作者： Xiang-feng Ma Xin ding En-lai Liu Rui-run chen Xin-xiu Wang yong Zhang and Jing-jie Guo National Key Laboratory for Precision Hot Processing of Metals Harbin Institute of TechnologyHarbin 150001China School of Materials science and Engineering Shandong University of Science and TechnologyQingdao 266500ShandongChina AECC Harbin Dongan Engine Co.Ltd.Harbin 150001China

Ti-V-based alloys are proved of huge potential in storing hydrogen,but the incomplete reversible hydrogen storage capacity caused by overstability of V hydride has limited the large-scale *** this study,Ti_(3.)V_(40+x)Fe_(23.x)Mn_(5)(x=0,4,8,12,at.%)alloys were designed,and the effects of V/Fe ratio on phase constitution and hydrogen storage properties were *** main phase of the alloys is body-centered cubic(BCC)phase,and the lattice constants of the BCC phase decrease with the decrease of V/Fe ***,C14 Laves phase exists in alloys with a Fe content of 19at.%to 23.t.%.For hydrogenation,the C14 Laves phase can accelerate the hydrogen absorption rate,but the hydrogen absorption capacity is *** the decrease of V/Fe ratio,the hydride gradually *** to its large lattice constant and high hydrogen absorption phase content,the Ti_(3.)V_(52)Fe_(11)Mn_(5)alloy shows the most enhanced hydrogen storage properties with hydrogenation and dehydrogenation capacities of 3.588wt.%at 298 K and 1.688wt.%at 3.3.K,*** hydrogen absorption capacity of this alloy can be reserved to 3.574wt.%after 20 cycles of hydrogen absorption and desorption.

关键词： hydrogen storage Ti-based alloy lattice constant BCC phase

Diversification of interfaces triggered hydrogen storage properties enhancement

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Rare Metals 2024年第5期43卷 2324-2330页

作者： Jia-Xin Zhang Xin ding Rui-Run chen Xiang-Feng Ma Wen-Chao Cao yong Zhang Jing-Jie Guo National Key Laboratory for Precision Hot Processing of Metals Harbin Institute of TechnologyHarbin 150001China

Dual effects of grain refinement and alloying are achieved and the mechanism of"diverse interfaces reinforcement"for hydrogen storage Mg alloys is first *** interface reinforced Mg-Y-Zn-Al alloy for hydrogen storage is *** work figures out that the adventurous Al-rich phase exhibits an ordered face-centered cubic(FCC)structure with composition of(3.±2)at%Y-(28±1)at%Zn-(41±3.at%Al,i.e.,Y_(3.Zn_(3.Al_(4),and an incoherent interface between Y3.n3.l4phase and Mg substrate is observed.

关键词： hydrogen alloying alloy

Unveiling strain-enhanced moiréexciton localization in twisted van der Waals homostructures

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Nano Research 2024年第4期17卷 3245-3252页

作者： Henry Rui He Haihong Zheng Biao Wu Shaofei Li Junnan ding Zongwen Liu Jian-Tao Wang Anlian Pan yanping Liu Institute of Quantum Physics School of PhysicsCentral South UniversityChangsha 410083China State Key Laboratory of Precision Manufacturing for Extreme Service Performance Central South UniversityChangsha 410083China School of Chemical and Biomolecular Engineering The University of SydneyNSW 2006Australia Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China College of Materials science and Engineering Hunan UniversityChangsha 410082China State Key Laboratory of High-Performance Complex Manufacturing Central South UniversityChangsha 410083China Shenzhen Research Institute of Central South university Shenzhen 51800China

Moirésuperlattices,arising from the controlled twisting of van der Waals homostructures at specific angles,have emerged as a promising platform for quantum emission ***,the manipulation of strain provides a versatile strategy to finely adjust electronic band structures,enhance exciton luminescence efficiency,and establish a robust foundation for two-dimensional quantum light ***,the intricate interplay between strain and moirépotential remains partially ***,we introduce a meticulously designed fusion of strain engineering and the twisted 2L-WSe_(2)/2L-WSe_(2) homobilayers,resulting in the precise localization of moiré*** low-temperature photoluminescence spectroscopy,we unveil the emergence of highly localized moiré-enhanced emission,characterized by the presence of multiple distinct emission ***,our investigation demonstrates the effective regulation of moirépotential depths through strain engineering,with the potential depths of strained and unstrained regions differing by 91%.By combining both experimental and theoretical approaches,our study elucidates the complex relationship between strain and moirépotential,thereby opening avenues for generating strain-induced moiréexciton single-photon sources.

关键词： moirésuperlattices strain engineering moiréexcitons moirépotential

Genomic profiling of colorectal cancer in large-scale Chinese patients:amplification and somatic mutations in ERBB2

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Oncology Research 2024年第9期32卷 1429-1438页

作者： YUZHI LIU EVELYNE BISCHOF ZHIQIN chen JIAHUAN ZHOU BEI ZHANG ding ZHANG yong GAO MING QUAN department of Oncology Shanghai East HospitalTongji University School of MedicineShanghaiChina State Key Laboratory of Oncogenes and Related Genes Shanghai Cancer InstituteDepartment of OncologyRenji HospitalSchool of MedicineShanghai Jiao Tong UniversityShanghaiChina Jiangsu Hengrui Pharmaceuticals Co. Ltd.ShanghaiChina D Medicines Inc. ShanghaiChina

Objectives:Human epidermal growth factor receptor 2(HER2)-targeted therapies have demonstrated potential benefits for metastatic colorectal cancer(mCRC)patients with HER2 amplification,but are not satisfactory in cases of HER2 mutant ***:Consequently,further elucidation of amplifications and somatic mutations in erythroblastic oncogene B-2(ERBB2)is *** genomic profiling was conducted on 2454 Chinese CRC cases to evaluate genomic alterations in 73. cancer-related genes,tumor mutational burden,microsatellite instability,and programmed death ligand 1(PD-L1)***:Among 2454 CRC patients,85 cases(3.46%)exhibited ERBB2 amplification,and 55 cases(2.24%)carried ERBB2 mutation.p.R678Q(28%),p.V8421(24%),and p.S3.0F/Y(12%)were the most prevalent of the 16 detected mutation *** comparison to the ERBB2 altered(alt)group,KRAS/BRAF mutations were more prevalent in ERBB2 wild-type(wt)samples(ERBB2wt ***2alt,KRAS:50.9%vs.25.6%,p3.,p3..7%(18/55)of CRCs with ERBB2 mutation exhibited microsatellite instability high(MSI-H),while no cases with HER2 amplification displayed *** genes varied between ERBB2 copy number variation(CNV)and ERBB2 single nucleotide variant(SNV);TP53.alterations tended to co-occur with ERBB2 amplification(92.3.)as opposed to ERBB2 mutation(58.3.).KRAS and PIK3.A alterations were more prevalent in ERBB2 SNV cases(KRAS/PIK3.A:45.8%/3..2%)compared to ERBB2 amplification cases(KRAS/PIK3.A:14.1%/7.7%).Conclusion:Our study delineates the landscape of HER2 alterations in a large-scale cohort of CRC patients from *** findings enhance our understanding of the molecular features of Chinese CRC patients and offer valuable implications for further investigation.

关键词： Colorectal cancer ERBB2 HER2 Human epidermal growth factor receptor 2 Genetic profiling Precision oncology

A review on g-C_(3.N_(4)decorated with silver for photocatalytic energy conversion

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Chinese Chemical Letters 2024年第2期35卷 187-196页

作者： Ziyu Pan Wufan ding Hanchun chen Haodong Ji Eco-environment and Resource Efficiency Research Laboratory School of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China

Artificial photocatalytic energy conversion is considered as the most potential strategy for solving the increasingly serious energy crisis and environmental pollution problems by directly capturing solar ***,high efficiency photocatalyst has drawn significant research attention in recent *** to the excellent electronic,optical,structural,and physicochemical performances,silver-based g-C_(3.N_(4)have become promising *** review emphasizes the recent progresses and challenges on g-C_(3.N_(4)decorated with silver for photocatalytic energy *** extensive use of g-C_(3.N_(4)decorated with silver in diverse photocatalytic reactions,including hydrogen evolution,pollutant degradation and carbon dioxide reduction,is also fully *** addition,we propose the perspectives of g-C_(3.N_(4)decorated with silver on photocatalytic *** hope that this review will shed some light on the photocatalytic energy conversion of g-C_(3.N_(4)decorated with silver.

关键词： g-C_(3.N_(4) Silver-modified g-C_(3.N_(4) Photocatalytic energy conversion H_(2)evolution Pollutant degradation CO_(2)reduction

Copper-catalyzed C(sp)-H aryl amination enables modular synthesis of quinolines and 2-quinolinones

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science china Chemistry 2024年第2期67卷 595-603页

作者： Yang Gao Haixia Li Simin Yang yanping Huo Qian chen Xianwei Li Zhe Wang Xiao-Qiang Hu School of Chemical Engineering and Light Industry Guangdong University of TechnologyGuangzhou510006China Jieyang Branch of Chemistry and Chemical Engineering Guangdong Laboratory Jieyang515200China Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education&Hubei Key Laboratory of Catalysis and Materials science School of Chemistry and Materials ScienceSouth-Central University for NationalitiesWuhan430074China

Herein,we disclose a novel copper-catalyzed C(sp)-H aryl amination of terminal alkynes with anthranils,enabling the rapid generation of highly reactive secondary N-aryl ynamines for the modular synthesis of structurally diverse C2-substituted quinolines and *** in-situ formed carbonyl-ynamines are prone to tautomerize to carbonyl-ketenimines,which can efficiently react with a series of nucleophiles,including amines,alcohols,phenols,thiols,thiophenols,active-methylene compounds,and even water to produce various quinoline derivatives with the generation of H_(2)O as a sole and green *** method also unlocks a practical route to create various quinoline-fused heterocycles and can be successfully applied to the late-stage modification of complex molecules and the concise synthesis of bioactive *** studies reveal a coppercatalyzed inner-sphere nitrene transfer process by using anthranils as novel aryl nitrene precursors.

关键词： copper catalysis anthranils C(sp)-H aryl amination carbonyl-ketenimines quinolines