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Vacuum ammonia stripping from liquid digestate:Effects of pH,alkalinity,temperature,negative pressure and process optimization

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Journal of Environmental Sciences 2025年第3期149卷 638-650页

作者： Qiuhong chen Donghai Yang Xiang chen Xiankai Wang Bin Dong Xiaohu Dai State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China YANGTZE Eco-Environment Engineering Research Center National Engineering Research Center of Eco-environment Protection for Yangtze River Economic BeltChina Three Gorges CorporationWuhan 430010China

High ammonia-nitrogen digestate has become a key bottleneck limiting the anaerobic digestion of organic solid *** ammonia stripping can simultaneously remove and recover ammonia nitrogen,which has attracted a lot of attention in recent *** investigate the parameter effects on the efficiency and mass transfer,five combination conditions(53℃ 15 kPa,60°C 20 kPa,65°C 25 kPa,72°C 35 kPa,and 81°C 50 kPa)were conducted for ammonia stripping of sludge *** results showed that 80%of ammonia nitrogen was stripped in 45 min for all experimental groups,but the ammonia transfer coefficient varied under different conditions,which increased with the rising of boiling point temperature,and reached the maximum value(39.0 mm/hr)at 81°C 50 *** ammonia nitrogen removal efficiency was more than 80%for 30 min vacuum stripping after adjusting the initial pH to above 9.5,and adjustment of the initial alkalinity also affects the pH value of liquid *** was found that pH and alkalinity are the key factors influencing the ammonia nitrogen dissociation and removal efficiency,while temperature and vacuum mainly affect the ammonia nitrogen mass transfer and removal *** terms of the mechanism of vacuum ammonia stripping,it underwent alkalinity destruction,pH enhancement,ammonia nitrogen dissociation,and free ammonia *** this study,two-stage experiments of alkalinity destruction and ammonia removal were also carried out,which showed that the two-stage configuration was beneficial for ammonia *** provides a theoretical basis and practical technology for the vacuum ammonia stripping from liquid digestate of organic solid waste.

关键词： Liquid digestate Vacuum ammonia stripping Alkalinity Mass transfer Process optimization

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Unraveling the reaction mechanism of high reversible capacity CuP_(2)/C anode with native oxidation PO_(x) component for sodium-ion batteries

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Chinese Chemical Letters 2025年第1期36卷 574-578页

作者： Huixin chen chen Zhao Hongjun Yue Guiming Zhong Xiang Han Liang Yin Ding chen State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body College of Mechanical and Vehicle EngineeringHunan UniversityChangsha 410082China CAS key Laboratory of Design and Assembly of Functional Nanostructures and Fujian Provincial Key Laboratory of NanomaterialsFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China College of Materials Science and Engineering Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesNanjing Forestry UniversityNanjing 210037China Laboratory of Advanced Spectro-electrochemistry and Li-ion Batteries Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Institute of Physics Chinese Academy of SciencesBeijing 100190China Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi institutesChinese Academy of SciencesXiamen 361021China

Phosphorus-based anode is a promising anode for sodium-ion batteries(SIBs)due to its high specific capacity,however,suffers from poor electronic conductivity and unfavorable electrochemical *** metals such as copper(Cu)into phosphorus has been demonstrated to not only improve the electronic conductivity but also accommodate the volume change during cycling,yet the underline sodiation mechanism is not ***,take a copper phosphide and reduced graphene oxide(CuP_(2)/C)composite as an example,which delivers a high reversible capacity of>900 mAh/***,it is revealed that the native oxidation PO_(x)components of the CuP_(2)/C composite show higher electrochemical reversibility than the bulk Cu P_(2),based on a quantitative analysis of high-resolution solid-state^(31)P NMR,ex-situ XPS and synchrotron X-ray diffraction characterization *** sodiation products Na_(3)PO_(4) and Na_(4)P_(2)O_(7) derived from PO_(x) could react with Na-P alloys and regenerate to PO_(x) during charge process,which probably accounts for the high reversible capacity of the Cu P_(2)/C *** findings also illustrate that the phosphorus transforms into nanocrystalline Na_(3)P and Na_(x)P alloys,which laterally shows crystallization-amorphization evolution process during cycling.

关键词： CuP_(2)/C composite POx component Reaction mechanism Solid-state NMR Sodium-ion batteries

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Anammox-based technologies:A review of recent advances,mechanism,and bottlenecks

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Journal of Environmental Sciences 2025年第2期148卷 151-173页

作者： Mabruk Adams Eliasu Issaka Chongjun chen School of Environmental Science and Engineering Suzhou University of Science and TechnologySuzhou 2155009China Civil Engineering School of EngineeringCollege of Science and EngineeringUniversity of GalwayGalway H91 TK33Ireland School of Environmental and Safety Engineering Institute of Environmental Health and Ecological SecurityJiangsu UniversityZhenjiang 212013China

The removal of nitrogen via the ANAMMOX process is a promising green wastewater treatment technology,with numerous *** incessant studies on the ANAMMOX process over the years due to its long start-up and high operational cost has positively influenced its technological advancement,even though at a rather slow *** the moment,relatively newANAMMOX technologies are being developedwith the goal of treating lowcarbon wastewater at low temperatures,tackling nitrite and nitrate accumulation and methane utilization from digestates while also recovering resources(phosphorus)in a sustainable *** review compares and contrasts the handful of ANAMMOX-based processes developed thus far with plausible solutions for addressing their respective bottlenecks hindering full-scale ***,future prospects for advancing understanding of mechanisms and engineering application of ANAMMOX process are *** a whole,technological advances in process design and patents have greatly contributed to better understanding of the ANAMMOX process,which has greatly aided in the optimization and industrialization of the ANAMMOX *** review is intended to provide researchers with an overview of the present state of research and technological development of the ANAMMOX process,thus serving as a guide for realizing energy autarkic future practical applications.

关键词： Anammox Commamox Denitrification Full-scale Partial nitrification

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Synergistic effect of silicon availability and salinity on metal adsorption in a common estuarine diatom

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Journal of Environmental Sciences 2025年第2期148卷 364-374页

作者： Fengyuan chen Jie Ma Ke Pan SZU-HKUST Joint PhD Program in Marine Environmental Science Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Marine Microbiome Engineering Institute for Advanced StudyShenzhen UniversityShenzhen 518060China Department of Ocean Science The Hong Kong University of Science and TechnologyHong Kong 999077China

Increasing nitrogen and phosphorus discharge and decreasing sediment input have made silicon(Si)a limiting element for diatoms in *** in nutrient structure and salinity fluctuation can greatly affect metal uptake by estuarine ***,the combined effects of Si and salinity on metal accumulation in these diatoms have not been *** this study,we aimed to investigate how salinity and Si availability combine to influence the adsorption of metals by a widely distributed diatom Phaeodactylum *** data indicate that replete Si and low salinity in seawater can enhance cadmium and copper adsorption onto the diatom *** the single-cell level,surface potential was a dominant factor determining metal adsorption,while surface roughness also contributed to the highermetal loading capacity at lower *** a combination of noninvasive micro-test technology,atomic force microscopy,X-ray photoelectron spectroscopy,and Fourier transform infrared spectroscopy,we demonstrate that the diversity and abundance of the functional groups embedded in diatom cell walls vary with salinity and Si *** results in a change in the cell surface potential and transient metal *** study provides novel mechanisms to explain the highly variable metal adsorption capacity of a model estuarine diatom.

关键词： Diatom Metal adsorption Silicon Salinity Functional group Surface potential

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Correlation between grain size,mechanical properties and deformed microstructure of Fe-20Mn-6Al-0.6C-0.15Si low-density steel

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Journal of Iron and Steel Research International 2025年第1期32卷 282-292页

作者： Qi Zhang Guang-hui chen Zheng-liang Xue Zheng-kun chen Guang Xu State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan430081HubeiChina Key Laboratory for Ferrous Metallurgy and Resources Utilization of Ministry of Education Wuhan University of Science and TechnologyWuhan430081HubeiChina Red Eagle Novel Refractory Materials Research Institute Zhejiang Red Eagle Group Co.Ltd.Huzhou313000ZhejiangChina

The effects of austenite grain size on the deformed microstructure and mechanical properties of an Fe-20Mn-6Al-0.6C-0.15Si(wt.%)low-density steel were *** microstructure of the experimental steel after solution treatment was single austenitic *** austenite grain size increased with solution temperature and time.A model was established to show the relationship between temperature,time and austenite grain size for the experimental *** addition,as the solution temperature increased,the strength decreased,while the elongation first increased and then *** decrease in elongation after solution treatment at 1100℃ for 90 min is contributed to the over-coarse austenite ***,after solution treatment at 900℃ for 90 min,the strength-elongation product reached the highest value of 44.4 GPa%.As the austenite grain size increased,the intensity of//tensile direction fiber *** was accompanied by a decrease in dislocation density,resulting in a lower fraction of low-angle grain boundaries and a lower work hardening ***,the austenite grain size has a critical influence on the mechanical properties of the low-density *** grains lead to a lower yield strength due to the Hall-Petch effect and a lower tensile strength because of lower dislocation strengthening.

关键词： Austenitic low-density steel Solution treatment Grain size Mechanical property Deformed microstructure

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Mining Subsidence Based on Integrated SBAS-InSAR and Unmanned Aerial Vehicles Technology

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Journal of Ocean University of China 2025年第1期24卷 113-129页

作者： chen Xuewei chen Jianping WANG Genhou ZHANG Qian ZHENG Yanwei School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China Beijing Key Laboratory of Development and Research for Land Resources Information Beijing 100083China

The Small Baseline Subset InSAR(SBAS-InSAR)and unmanned aerial vehicles(UAVs)as common ocean-land technologies,have been extensively applied in subsidence,glacial movement,surface deformation,and maritime positioning and navigation.A novel method integrating SBAS-InSAR and UAV photogrammetry is used to analyze ground subsidence deformation in the Gesar gold mine located in Maqu,Northwest *** approach uses SBAS-InSAR to calculate two-dimensional deformation data for capturing ascending and descending *** method can provide precise information on small-sized deformations within mining *** deformation data obtained from UAVs and the vertical deformation data derived from InSAR are integrated to generate comprehensive and accurate ground subsidence data from the mining *** demonstrate that using a combined InSAR(vertical)and UAV technique to analyze surface subsidence in mining districts resolves inconsistency between the line-of-sight and deformation ***,the incoherence issue of InSAR in regions with large deformation gradients is addressed,while the inherent errors of UAV monitoring of mining surface subsidence are *** genetic algorithm(GA)-backpropagation(BP)neural network algorithm is combined with InSAR data to predict subsidence in collapsed *** observed,the GA-BP algorithm has the smallest residual under the same training ***,the GA-BP neural network model can effectively predict surface subsidence in mining areas and can be used for subsequent subsidence prediction.

关键词： SBAS-InSAR two-dimensional deformation solution UAV photogrammetry data fusion subsidence prediction

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Synthesis and Photochromism of Diazocine Derivatives:Relationship Between Photoswitching Properties and Molecular Structures

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Chemical Research in Chinese Universities 2025年第1期41卷 33-39页

作者： WANG Yaxin chen Yulan Key Laboratory of Organic Integrated Circuit Ministry of Education&Tianjin Key Laboratory of Molecular Optoelectronic SciencesDepartment of ChemistrySchool of ScienceTianjin UniversityTianjin300072P.R.China State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun130012P.R.China

We design and synthesize five novel diazocine derivatives,using diazocine as the core,amide or imine bonds as the connecting units attached with different peripheral *** photoisomerization yield and thermal stability of these derivatives are tested by^(1)H NMR and UV-Vis absorption *** them,the imine-linked derivative exhibits the lowest photoisomerization efficiency,while the amide-linked ones show an elevated switching efficiency in transitioning from the cis to the trans configuration,compared to the unmodified 3,3′-***,based on experiments together with density functional theory(DFT)calculations,we find that the thermal stability of these derivatives is associated with the electron cloud density and steric hindrance of their *** to these unique photophysical properties,diazocine derivatives provide a foundation for the development and application of molecular optical switches.

关键词： Diazocine Photoisomerization Thermal stability

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Enhanced Cd^(2+)removal from aqueous solution using olivine and magnesite combination:New insights into the mechanochemical synergistic effect

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Journal of Environmental Sciences 2025年第1期147卷 714-725页

作者： Xiaofang chen Chao Wang Min chen Huimin Hu Junwei Huang Ting Jiang Qiwu Zhang School of Resources&Environmental Engineering Wuhan University of TechnologyWuhan 430070China State Environmental Protection Key Laboratory of Water Environmental Simulation and Pollution Control South China Institute of Environmental SciencesMinistry of Ecology and EnvironmentGuangzhou 510655China

In this study,an efficient stabilizer material for cadmium(Cd^(2+))treatment was successfully prepared by simply co-milling olivine with *** analyticalmethods including XRD,TEM,SEM and FTIR,combined with theoretical calculations(DFT),were used to investigate mechanochemical interfacial reaction between twominerals,and the reaction mechanism of Cd removal,with ion exchange between Cd^(2+)and Mg^(2+)as the main pathway.A fixation capacity of Cd^(2+)as high as 270.61 mg/g,much higher than that of the pristine minerals and even the individual/physical mixture of milled olivine and magnesite,has been obtained at optimized conditions,with a neutral pH value of the solution after treatment to allow its direct *** as-proposed Mg-based stabilizer with various advantages such as cost benefits,green feature etc.,will boosts the utilization efficiency of naturalminerals over the elaborately prepared adsorbents.

关键词： Olivine Magnesite Interface reaction Mechanochemical activation Cadmium removal

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Dirac-geodesics with curvature term

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Science China Mathematics 2025年第2期68卷 433-446页

作者： Qun chen Mingwei Zhang School of Mathematics and Statistics Wuhan UniversityWuhan 430072China

Dirac-geodesics with curvature term are Dirac-harmonic maps with curvature term from onedimensional domains. In this paper, we first describe the structure of Dirac-geodesics with curvature term in surfaces and give solutions on the unit 2-sphere and the hyperbolic plane, and then we give the structure of solutions in warped product spaces. Finally, we define the heat flow of Dirac-geodesics with curvature term and prove the global existence and sub-convergence of the heat flow into any closed surfaces and space forms. Our results provide the first examples and general existence theorems of Dirac-geodesics with curvature term.

关键词： Dirac-geodesic Dirac-harmonic map curvature heat flow existence

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地球同火星蒸发岩沉积的对比

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高校地质学报 2014年第2期20卷 169-176页

作者：郑绵平孔维刚陈文西孔凡晶张雪飞中国地质科学院矿产资源研究所北京100037 国土资源部盐湖资源与环境研究重点开放实验室北京100037

迄今为止,人类已经通过火星轨道探测器、火星着陆器及火星漫游车在火星上发现了碳酸盐、硫酸盐及氯化物等一系列的盐类矿物,尽管整体上火星盐类矿物组合与地球上基本一致,但在许多细节方面还是和地球上有所不同。文中首先对于火星盐类... 详细信息

迄今为止,人类已经通过火星轨道探测器、火星着陆器及火星漫游车在火星上发现了碳酸盐、硫酸盐及氯化物等一系列的盐类矿物,尽管整体上火星盐类矿物组合与地球上基本一致,但在许多细节方面还是和地球上有所不同。文中首先对于火星盐类认知的现状作了简要综述;基于地球火星蒸发盐沉积及成盐作用规律的对比,预测火星表面及次表面可能存在着广泛分布的钾盐;此外,发现火星轨道伽玛光谱仪所获的火星表面K的分布与火星表面已探测到的氯化物的分布有比较强的相关性,喻示火星表面氯化物沉积地区的卤水浓度已经接近或达到钾盐形成的条件,同时指出这些地区存在钾盐的可能性很大。

关键词：火星蒸发岩沉积比较研究钾盐

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