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Activation of peroxymonosulfate by sustainable biomass-based carbon nanotubes for controlling the spread of plant viruses in water environments

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Journal of Environmental Sciences 2025年第3期149卷 99-112页

作者： Jian Tang Yujie Wang JunMa Yujie chen Ming chen College of Resources and Environment Yangtze UniversityWuhan 430100China Key Laboratory of Reservoir Aquatic Environment Chongqing Institute of Green and Intelligent TechnologyChinese Academy of SciencesChongqing 400714China Chongqing School University of Chinese Academy of SciencesChongqing 400714China School of Geography and Tourism Chongqing Normal UniversityChongqing 400714China

With the increasing demand for water in hydroponic systems and agricultural irrigation,viral diseases have seriously affected the yield and quality of *** removing plant viruses in water environments,virus transmission can be prevented and agricultural production and ecosystems can be *** so far,there have been few reports on the removal of plant viruses in water ***,in this study,easily recyclable biomass-based carbon nanotubes catalysts were synthesized with varying metal activities to activate peroxymonosulfate(PMS).Among them,the magnetic 0.125Fe@NCNTs-1/PMS system showed the best overall removal performance against pepper mild mottle virus,with a 5.9 log_(10)removal within 1 ***,the key reactive species in the 0.125Fe@NCNTs-1/PMS system is^(1)O_(2),which can maintain good removal effect in real water matrices(river water and tap water).Through RNA fragment analyses and label free analysis,it was found that this system could effectively cleave virus particles,destroy viral proteins and expose their *** capsid protein of pepper mild mottle virus was effectively decomposed where serine may be the main attacking sites by^(1)O_(2).Long viral RNA fragments(3349 and 1642 nt)were cut into smaller fragments(∼160 nt)and caused their *** summary,this study contributes to controlling the spread of plant viruses in real water environment,which will potentially help protect agricultural production and food safety,and improve the health and sustainability of ecosystems.

关键词： Pepper mild mottle virus Removal Plant virus spread Biomass-based carbon nanotubes Water environments

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Green disposal of waste smartphone protective film:Efficiency,mechanism,bench-scale test and secondary waste reutilization

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Journal of Environmental Sciences 2025年第5期151卷 692-702页

作者： Jiangyao chen Shunyu Ding chenxu Gao Canhui chen Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

The manufacture and obsolescence of smartphones produce numerous waste plastic accessories(e.g.,waste smartphone protective film(WSPF)),possessing immense potential for ***,available recycling technologies have limitations such as substrate damage and secondary pollutant *** present study aimed to develop a green disposal method that not only recycled polyethylene terephthalate(PET)from WSPF,but also reused the stripped polyacrylate(PAA)adhesive as an adsorbent to reduce solid waste *** the WSPF was treated in 1 mol/L NaOH solution at 90°C,the PAA hydrolyzed to two main by-products of 1-butanol and 2-ethylhexanol,weakening the binding strength between PAA and PET and then efficient separation of *** bench-scale test revealed that over 97.2%of detachment efficiency toward PAA was achieved during continuous treatment of 17 batches of WSPF(200 g for each)without supplement of NaOH and generation of ***,the economic evaluation indicated that the recycling method would generate a net profit margin of 647%for the second year without considering the incurrence of new cost and ***,the pyrolysis of waste PAA enabled its conversion into potential adsorbent,which showed 2 to 4 times enhanced adsorption capacity toward styrene and ethyl acetate after modification with NaOH *** study provides a green method for recycling waste plastics and inspires a referable solution for solid waste treatment in the smartphone industry.

关键词： Smartphone accessory Waste protective film Green recycle Polyethylene terephthalate Polyacrylate Adsorbent

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冀蒙交界裕民文化锛状器的制作技术

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人类学学报 2023年第3期42卷 317-330页

作者：叶灿阳陈胜前赵潮胡晓农郭明建包青川中国人民大学历史学院考古文博系北京100872 陕西师范大学历史文化学院西安710119 乌兰察布博物馆乌兰察布012000 暨南大学文学院历史学系广州510632 内蒙古自治区文物考古研究院呼和浩特010010

锛状器是旧石器时代晚期开始出现的一类特殊的打制石器类型,进入新石器时代以后,在北方森林草原交错带延续并有技术改进。十多年来,在裕民文化多个考古遗址的调查和发掘中发现了大量的锛状器,是该文化代表性的石器。本研究通过形态观察... 详细信息

锛状器是旧石器时代晚期开始出现的一类特殊的打制石器类型,进入新石器时代以后,在北方森林草原交错带延续并有技术改进。十多年来,在裕民文化多个考古遗址的调查和发掘中发现了大量的锛状器,是该文化代表性的石器。本研究通过形态观察与特征测量、加工痕迹与制作技术分析、操作链重建与复制实验等手段,对裕民文化出土的锛状器进行技术观察和实验分析,还原了裕民文化锛状器的生产工艺,并结合文化背景阐释了这类石器工具在裕民文化中的技术适应意义。锛状器可分为以平直刃为特征的单面加工类型和以弧凸刃为特征的两面加工类型,这种类型划分同时具有形态和技术上的意义。结合裕民文化的石器组合来看,锛状器在形态上具有一定规范性,操作链上具有高度灵活性,与其他工具一起反映了裕民文化人群对北方森林-草原交错地带风险环境的弹性技术适应。

关键词：考古石制品锛状器技术复制实验

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Utilizing BP neural networks to accurately reconstruct the tritium depth profile in materials for BIXS

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Nuclear Science and Techniques 2025年第1期36卷 103-114页

作者： chen Zhao Wei Jin Yan Shi Chang-An chen Yi-Ying Zhao Institute of Materials China Academy of Engineering PhysicsJiangyou 621908China

β-ray-induced X-ray spectroscopy(BIXS)is a promising method for tritium detection in solid materials because of its unique advantages,such as large detection depth,nondestructive testing capabilities,and low requirements for sample ***,high-accuracy reconstruction of the tritium depth profile remains a significant challenge for this *** this study,a novel reconstruction method based on a backpropagation(BP)neural network algorithm that demonstrates high accuracy,broad applicability,and robust noise resistance is *** average reconstruction error calculated using the BP network(8.0%)was much lower than that obtained using traditional numerical methods(26.5%).In addition,the BP method can accurately reconstruct BIX spectra of samples with an unknown range of tritium and exhibits wide applicability to spectra with various tritium ***,the BP network demonstrates superior accuracy and stability compared to numerical methods when reconstructing the spectra,with a relative uncertainty ranging from 0 to 10%.This study highlights the advantages of BP networks in accurately reconstructing the tritium depth profile from BIXS and promotes their further application in tritium detection.

关键词： β-ray-induced X-ray spectroscopy Tritium detection BP network Ridge regression Reconstruction problem

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高校学生创新创业参赛满意度提升路径探析

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创新创业理论研究与实践 2023年第5期6卷 188-192页

作者：姜永波陈胜乾李莉空军指挥学院北京100097 青岛理工大学商学院山东青岛266520

创新创业大赛是高校人才培养的重要平台,在大赛中获得满意成绩将有效激发高校学生的创新创业热情、极大提升其创新创业自信心及主观能动性。该文以911份参加过“双创”大赛的高校学生问卷为基础,基于SEM分析参赛结果满意度的影响因素:... 详细信息

创新创业大赛是高校人才培养的重要平台,在大赛中获得满意成绩将有效激发高校学生的创新创业热情、极大提升其创新创业自信心及主观能动性。该文以911份参加过“双创”大赛的高校学生问卷为基础,基于SEM分析参赛结果满意度的影响因素:学校参赛氛围、大赛性质、参赛动机是重要的外源变量,对资源整合、团队协作、教师指导具有显著正影响;而教师指导、资源整合、团队协作对满意度具有显著正影响;并由此提出“一个中心、二个基点、三条路径”的高校学生创新创业参赛满意度提升策略。

关键词：创新创业大赛参赛效果满意度影响因素提升路径 SEM分析

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The advanced development of innovative photocatalytic coupling strategies for hydrogen production

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Chinese Chemical Letters 2025年第1期36卷 80-91页

作者： Yuehai Zhi chen Gu Huachao Ji Kang chen Wenqi Gao Jianmei chen Dafeng Yan College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology) Nanjing 210023China Hubei Key Laboratory for Precision Synthesis of Small Molecule Pharmaceuticals&Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules&College of Chemistry and Chemical Engineering Hubei UniversityWuhan 430062China

Photocatalytic technology harnesses solar energy to facilitate chemical transformations,presenting significant potential in energy generation and environmental ***,the conventional O_(2)evolution process is hindered by high reaction barriers and inefficiencies,which limit its widespread ***,exploring novel photocatalytic coupling strategies to replace water oxidation has become a key route to enhance the efficiency of H_(2)*** this review,organic pollutants removal and the valorization of organics as substitutes for water oxidation coupling strategies for photocatalytic H_(2)production are comprehensively *** strategies not only circumvent the high reaction barriers associated with O_(2)evolution to enhance the H_(2)production but also aid in the removing of organic pollutants or synthesis of value-added *** also present future research directions and underscore the significance of advanced catalyst design,in-depth analysis of reaction mechanisms,and systematic optimization strategies in realizing an efficient and sustainable photocatalytic *** guidance is anticipated to provide theoretical and practical new insights for the future development of photocatalytic coupling reactions,fostering further explorations in the realm of renewable energy and environmental governance.

关键词： Photocatalysis Pollutants removal Valorization of organics Catalyst design

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Phase changes and electromagnetic wave absorption performance of XZnC(X=Fe/Co/Cu)loaded on melamine sponge hollow carbon composites

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International Journal of Minerals,Metallurgy and Materials 2025年第3期32卷 566-577页

作者： Xiubo Xie Ruilin Liu chen chen Di Lan Zhelin chen Wei Du Guanglei Wu School of Environmental and Material Engineering Yantai UniversityYantai 264005China School of Materials Science and Engineering Hubei University of Automotive TechnologyShiyan 442002China Shandong Key Laboratory of Eco-Environmental Science for the Yellow River Delta Shandong University of AeronauticsBinzhou 256603China Institute of Materials for Energy and Environment State Key Laboratory of Bio-fibers and Eco-textilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China

Non-stoichiometric carbides have been proven to be effective electromagnetic wave(EMW)absorbing *** this study,phase and morphology of XZnC(X=Fe/Co/Cu)loaded on a three dimensional(3D)network structure melamine sponge(MS)carbon composites were investigated through vacuum filtration followed by *** FeZnC/CoZnC/CuZnC with carbon nanotubes(CNTs)were uniformly dispersed on the surface of melamine sponge carbon skeleton and Co-containing sample exhibits the highest CNTs *** minimum reflection loss(RL_(min))of the CoZnC/MS composite(m_(composite):m_(paraffin)=1:1,m represents mass)reached-33.60 dB,and the effective absorption bandwidth(EAB)reached 9.60 *** outstanding electromagnetic wave absorption(EMWA)properties of the CoZnC/MS composite can be attributed to its unique hollow structure,which leads to multiple reflections and *** formed conductive network improves dielectric and conductive *** incorporation of Co enhances the magnetic loss capability and optimizes interfacial polarization and dipole *** simultaneously improving dielectric and magnetic losses,ex-cellent impedance matching performance is *** clarification of element replacement in XZnC/MS composites provides an effi-cient design perspective for high-performance non-stoichiometric carbide EMW absorbers.

关键词： electromagnetic wave absorption three dimensional network structure melamine sponge derived carbon non-stoichiometric carbide

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Characteristics of catalytic destruction of dichloromethane and ethyl acetate mixture over HxPO4-RuOx/CeO2 catalyst

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Journal of Environmental Sciences 2025年第2期148卷 336-349页

作者： Jiawen chen Qingjie Meng Feng Bi Jingkun chen Xiaole Weng Zhongbiao Wu Key Laboratory of Environment Remediation and Ecological Health Ministry of EducationCollege of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China School of Civil&Environmental Engineering and Geography Science Ningbo UniversityNingbo 315211China ZJU-Hangzhou Global Scientific and Technological Innovation Center Hangzhou 311200China Zhejiang Provincial Engineering Research Centre of Industrial Boiler&Furnace Flue Gas Pollution Control Hangzhou 310058China

Catalytic destruction is an ascendant technology for the abatement of volatile organic compounds(VOCs)originating fromsolvent-based industrial *** varied composition tends to influence each VOC’s catalytic behavior in the reaction *** investigated the catalytic destruction of multi-component VOCs including dichloromethane(DCM)and ethyl acetate(EA),as representatives from pharmaceutical waste gases,over co-supported HxPO_(4)-RuOx/CeO_(2) catalyst.A mutual inhibitory effect relating to concentrations because of competitive adsorption was verified in the binary VOCs oxidation and EA posed a more negative effect on DCM oxidation owing to EA’s superior adsorption *** adsorption of EA on acidic sites(HxPO_(4)/CeO_(2))promoted DCM activation on basic sites(O^(2−))and the dominating EA oxidation blocked DCM’s access to oxidation centers(RuOx/CeO_(2)),resulting in boosted monochloromethane yield and increased chlorine deposition for DCM *** impaired redox ability of Ru species owing to chlorine deposition in turn jeopardized deep oxidation of EA and its by-products,leading to increased gaseous by-products such as acetic acid originating fromEA ***,DCM at low concentration slightly promoted EA conversion at low temperatures with or without water,consistent with the enhanced EA adsorption in co-adsorption *** was mainly due to that DCM impeded the shielding effect of hydrolysate deposition from rapid EA hydrolysis depending on the decreased ***,water benefited EA hydrolysis but decreased CO_(2) selectivity while the generated water derived from EA was likely to affect DCM *** work may provide theoretical guidance for the promotion of applied catalysts toward industrial applications.

关键词： Catalytic destruction Multi-component VOCs Mixture effect Interaction mechanism

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Effects of surface fluoride modification on TiO_(2)for the photocatalytic oxidation of toluene

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Journal of Environmental Sciences 2025年第1期147卷 561-570页

作者： Shaoyu Yuan Min chen Xiaoxiao Qin Xueyan chen Jianghao Zhang Changbin Zhang State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

In the present study,we investigated the influence of surface fluorine(F)on TiO_(2)for the photocatalytic oxidation(PCO)of ***_(2)modified with different F content was prepared and *** was found that with the increasing of F content,the toluene conversion rate first increased and then ***,CO_(2)mineralization efficiency showed the opposite *** on the characterizations,we revealed that F substitutes the surface hydroxyl of TiO_(2)to form the structure of≡*** presence of the appropriate amount of surface≡Ti-F on TiO_(2)greatly enhanced the separation of photogenerated carriers,which facilitated the generation of·OH and promoted the activity for the PCO of *** was further revealed that the increase of only·OH promoted the conversion of toluene to ring-containing intermediates,causing the accumulation of intermediates and then conversely inhibited the·OH generation,which led to the decrease of the CO_(2)mineralization *** above results could provide guidance for the rational design of photocatalysts for toluene oxidation.

关键词： Photocatalysis TiO_(2) Toluene Fluorine

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Target Search and Navigation in Heterogeneous Robot Systems with Deep Reinforcement Learning

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Machine Intelligence Research 2025年第1期22卷 79-90页

作者： Yun chen Jiaping Xiao Department of Mechanical Engineering University of AlabamaTuscaloosa35487USA School of Mechanical and Aerospace Engineering Nanyang Technological UniversitySingapore639798Singapore

Collaborative heterogeneous robot systems can greatly enhance the efficiency of target search and navigation *** this paper,we design a heterogeneous robot system consisting of an unmanned aerial vehicle(UAV)and an unmanned ground vehicle(UGV)for search and rescue missions in unknown *** system is able to search for targets and navigate to them in a maze-like mine environment with the policies learned through deep reinforcement learning *** the training process,if two robots are trained simultaneously,the rewards related to their collaboration may not be properly ***,we introduce a multi-stage reinforcement learning framework and a curiosity module to encourage agents to explore unvisited *** in simulation environments show that our framework can train the heterogeneous robot system to achieve the search and navigation with unknown target locations while existing baselines may *** UGV achieves a success rate of 89.1%in the mission within the original environment,and maintains a 67.6%success rate in untrained complex environments.

关键词： Heterogeneous intelligent systems deep reinforcement learning multiagent systems robot learning target search

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