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The evolution and morphological stability of a spherical crystal

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Science china(Technological sciences) 2008年第3期51卷 225-243页

作者： chen mingwen1,2, wang zidong2 & xu jianjun3.4 1 school of applied sciences, university of Science and {3. beijing, beijing 100083. china 2 school of Materials Science and Engineering, university of Science and {3. beijing, beijing 100083. china 3.school of Mathematical sciences, Nankai university, Tianjin 3.0071, china 4 Department of Mathematics and Statistics, McGill university, Montreal H3. 2K6, Canada 1. school of applied sciences University of Science and Technology Beijing Beijing 100083 China 2. school of Materials Science and Engineering University of Science and Technology Beijing Beijing 100083 China 3. school of Mathematical sciences Nankai University Tianjin 300071 China 4. Department of Mathematics and Statistics McGill University Montreal H3A 2K6 Canada

The growth model of a spherical crystal in the undercooled melt including the surface energy, interfacial kinetics and convective flow is established. The effect of the convective flow induced by a small far field flow on the evolution and morphological stability of the interface of the spherical crystal is studied. The interface shape of the spherical crystal, which is affected by the far field flow, and the dispersion relation of the growth rate of amplitude of the perturbed interface are derived. It is shown that the convection induced by the far field flow makes the interface of the growing spherical crystal further grow in the upstream direction of the far field flow and inhibit growth in the downstream direction; the interface of the decaying spherical crystal further decays in the upstream direction and inhibits decay in the downstream direction. The theoretical result suggests that both the growth of the sphere in the upstream direction and the decay of the sphere in the downstream direction make the spherical crystal tend to evolve into an oval; the morphological stability of the interface depends on a certain radius R c such that the spherical crystal is unstable when its radius is greater than R c and stable when its radius is less than R c . The surface energy and interfacial kinetics have strong stabilizing effects on the growth of the spherical crystal. In the meantime interfacial kinetics is a table factor of the interface when the interface of the sphere is growing; it is an unstable factor of the interface when the interface is decaying.

关键词： solid-liquid interface spherical crystal convective flow crystal growth morphological stability

Boosting the catalytic performance of Cu-SAPO-3.in NO_(x) removal via hydrothermal treatment

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Journal of Environmental sciences 2024年第1期135卷 640-655页

作者： Xiaoyan Tian Huimin wang Siyuan xu Lianyun Gao Jinyan Cao jianjun {3. Qiulin Zhang Ping Ning Jiming Hao Faculty of Environmental Science and Engineering Kunming University of Science and TechnologyKunming 650500China National-Regional Engineering Center for Recovery of Waste Gases from Metallurgical and Chemical Industries Kunming University of Science and TechnologyKunming 650500China school of Environment State Key Joint Laboratory of Environment Simulation and Pollution ControlTsinghua UniversityBeijing 100084China

Phosphate ions promoted Cu-SAPO-3.(P-Cu-SAPO-3.)were prepared using bulk CuO particles as Cu^(2+)precursor by a solid-state ion exchange technique for the selective catalytic reduction of NO_(x) with NH_3.NH_3.SCR).The effects of high temperature(H-T)hydrothermal aging on the NO_(x) removal(de-NO_(x))performance of Cu-SAPO-3. with and without phosphate ions were systematically investigated at atomic *** results displayed that both Cu-SAPO-3. and P-Cu-SAPO-3. presented relatively poor NO_(x) removal activity with a low conversion(3.%)at 250-500℃.However,after H-T hydrothermal treatment(800℃ for 10 hr at 10%H_2O),these two samples showed significantly satisfied NO_(x) elimination performance with a quite high conversion(70%-90%)at 250-500℃.Additionally,phosphate ions decoration can further enhance the catalytic performance of Cu-SAPO-3. after hydrothermal treatment(Cu-SAPO-3.H).The textural properties,morphologies,structural feature,acidity,redox characteristic,and surface-active species of the fresh and hydrothermally aged samples were analyzed using various characterization *** systematical characterization results revealed that increases of 28%of the isolated Cu^(2+)active species(Cu^(2+)-2Z,Cu(OH)^(+)-Z)mainly from bulk CuO and 50%of the Bronsted acid sites,the high dispersion of isolated Cu^(2+)active component as well as the Bronsted acid sites were mainly responsible for the accepted catalytic activity of these two hydrothermally aged samples,especially for P-Cu-SAPO-3.H.

关键词： NH_(3.-SCR Cu-SAPO-3. Hydrothermal induced Phosphate ions

Study of proton resonances in ^(18)Ne via resonant elastic scattering of ^(17)F+p and its astrophysical implication

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Science china(Physics,Mechanics & Astronomy) 2011年第S1期54卷 32-36页

作者： HE jianjun1, HU Jun1,2, xu ShiWei1, chen ZhiQiang1, ZHANG xueYing1, wang JianSong1, YU XiangQing1, ZHANG LiYong1,2, LI Long1,2, YANG YanYun1,2, MA Peng1,2, ZHANG xueHeng1, HU ZhengGuo1, GUO ZhongYan1, xu Xing1,2, YUAN XiaoHua1, LU Wan1,2, YU YuHong1, ZANG YongDong1,2, TANG ShuWen1,2, YE RuiPing1,2, chen JinDa1,2, JIN ShiLun1,2, DU chengMing1,2, wang ShiTao1,2, MA JunBing1,2, LIU LongXiang1,2, BAI Zhen1,2, LEI XiangGuo1, SUN ZhiYu1, ZHANG YuHu1, ZHOU XiaoHong1, xu HuShan1, SU Jun3. LI ErTao3. wang HongWei4, TIAN WenDong4 & LI XiangQing5 1 Institute of Modern Physics (IMP), Chinese Academy of sciences, Lanzhou 73.000, {13. 2 Graduate university of Chinese Academy of sciences, beijing 100049, {13. 3.{13. Institute of Atomic Energy (CIAE), beijing 102413. {13. 4 Shanghai Institute of applied Physics (SINAP), Chinese Academy of sciences, Shanghai 201800, {13. 5 school of Physics and State Key Laboratory of Nuclear Physics and technology, Peking university, beijing 100871, {13. 1. Institute of Modern Physics (IMP) Chinese Academy of Sciences Lanzhou 730000 China2. Graduate University of Chinese Academy of Sciences Beijing 100049 China3. China Institute of Atomic Energy (CIAE) Beijing 102413 China4. Shanghai Institute of Applied Physics (SINAP) Chinese Academy of Sciences Shanghai 201800 China5. School of Physics and State Key Laboratory of Nuclear Physics and Technology Peking University Beijing 100871 China

The proton resonant properties in 18Ne, which determine the reaction rate of the key stellar 14O(α,p)17F reaction, have been studied by using a technique of proton resonant elastic scattering of 17F+p. A 4.22 MeV/nucleon 17F radioactive ion (RI) beam was produced via a projectile-fragmentation reaction, and separated by a Radioactive Ion Beam Line in Lanzhou (RIBLL). By bombarding a thick (CH2)n target, the energy spectra of the recoiled protons were measured by two ΔE-E silicon telescopes at the center-of-mass scattering angles of θc.m.≈175°±5°, θc.m.≈152°±8°, respectively. Several proton resonances in 18Ne were ob served clearly. A further R-matrix analysis of the experimental data is under way to determine the resonant parameters. The present work reports the preliminary results briefly.

关键词： resonant reaction reaction rate explosive burning accreting binary systems

A Soft Sensor with Light and Efficient Multi-scale Feature Method for Multiple Sampling Rates in Industrial Processing

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Machine Intelligence Research 2024年第2期21卷 400-410页

作者： Dezheng wang Yinglong wang Fan Yang Liyang xu Yinong Zhang Yiran {3. Ning Liao school of Automation Southeast UniversityNanjing 210096China Software and Artificial Intelligence College Chongqing Institute of EngineeringChongqing 400056China beijing National Research Center for Information Science and technology(BNRist) Department of AutomationTsinghua UniversityBeijing 100084China Liangjiang International College Chongqing University of TechnologyChongqing 401135China Smart City College Beijing Union UniversityBeijing 100101China

In industrial process control systems,there is overwhelming evidence corroborating the notion that economic or technical limitations result in some key variables that are very difficult to measure *** data-driven soft sensor is an effective solution because it provides a reliable and stable online estimation of such *** paper employs a deep neural network with multiscale feature extraction layers to build soft sensors,which are applied to the benchmarked Tennessee-Eastman process(TEP)and a real wind farm *** comparison of modelling results demonstrates that the multiscale feature extraction layers have the following advantages over other ***,the multiscale feature extraction layers significantly reduce the number of parameters compared to the other deep neural ***,the multiscale feature extraction layers can powerfully extract dataset ***,the multiscale feature extraction layers with fully considered historical measurements can contain richer useful information and improved representation compared to traditional data-driven models.

关键词： Multi-scale feature extractor deep neural network(DNN) multirate sampled industrial processes prediction

High-order Autler–Townes splitting in electrically tunable photonic molecules

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Photonics Research 2024年第8期12卷 1794-1801页

作者： YIHAO chen JUNTAO DUAN JIN LI YAN chen JIEWEN LI JIANAN DUAN XIAOCHUAN xu JIAWEI {3. school of Integrated Circuit Harbin Institute of Technology(Shenzhen)Shenzhen 518055China College of Advanced Interdisciplinary Studies National University of Defense TechnologyChangsha 410073China National Key Laboratory of Laser Spatial Information Harbin Institute of Technology(Shenzhen)Shenzhen 518055China

Whispering gallery mode optical microresonators represent a promising avenue for realizing optical analogs of coherent light–atom interactions,circumventing experimental ***-optical analogs of Autler–Townes splitting have been widely demonstrated,harnessing coupled optical microresonators,also known as photonic molecules,wherein the strong coupling between resonant fields enables energy level ***,we report the characterizations of Autler–Townes splitting in waveguide-coupled microring dimers featuring mismatched *** exploiting backscattering-induced coupling via Rayleigh and Mie scatterers in individual rings,high-order Autler–Townes splitting has been realized,yielding supermode hybridization in a multi-level *** resonance detuning using an integrated phase shifter,intra-cavity coupling-induced splitting becomes almost indistinguishable at the zero-detuning point where the strong inter-cavity coupling counteracts the imbalance of backscattering strengths in individual *** demonstrations on the maturing silicon photonics platform,our findings establish a framework of electrically tunable photonic molecules for coupling-mediated Autler–Townes splitting,offering promising prospects for on-chip signal generation and processing across classical and quantum regimes.

关键词： tunable tuning waveguide

A core-satellite self-assembled SERS aptasensor containing a“biological-silent region”Raman tag for the accurate and ultrasensitive detection of histamine

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Food Science and Human Wellness 2024年第2期13卷 1029-1039页

作者： chen chen Yingfang Zhang Ximo wang {3.guang Qiao Geoffrey I.N.Waterhouse Zhixiang {3. Key Laboratory of Food Processing technology and Quality Control in Shandong Province College of Food Science and EngineeringShandong Agricultural UniversityTai’an 271018China school of Chemical sciences The University of AucklandAuckland 1142New Zealand

Herein,a novel interference-free surface-enhanced Raman spectroscopy(SERS)strategy based on magnetic nanoparticles(MNPs)and aptamer-driven assemblies was proposed for the ultrasensitive detection of histamine.A core-satellite SERS aptasensor was constructed by combining aptamer-decorated Fe_(3.O_(4)@Au MNPs(as the recognize probe for histamine)and complementary DNA-modified silver nanoparticles carrying 4-mercaptobenzonitrile(4-MBN)(Ag@4-MBN@Ag-c-DNA)as the SERS signal probe for the indirect detection of *** an applied magnetic field in the absence of histamine,the assembly gave an intense Raman signal at“Raman biological-silent”region due to *** the presence of histamine,the Ag@4-MBN@Ag-c-DNA SERS-tag was released from the Fe_(3.O_(4)@Au MNPs,thus decreasing the SERS *** optimal conditions,an ultra-low limit of detection of 0.65×10^(-3.ng/mL and a linear range 10^(-2)-10^5 ng/mL on the SERS aptasensor were *** histamine content in four food samples were analyzed using the SERS aptasensor,with the results consistent with those determined by high performance liquid *** present work highlights the merits of indirect strategies for the ultrasensitive and highly selective SERS detection of small biological molecules in complex matrices.

关键词： Surface-enhanced Raman spectroscopy Raman biological-silent region Aptamer Histamine detection Universal SERS-tag

Introducing urea into tirapazamine derivatives to enhance anticancer therapy

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National Science Review 2024年第4期11卷 245-253页

作者： Yajun xu Jianlin Lv Chaoying Kong Ya Liu Kun wang Zhaohui Tang xuesi {3. Key Laboratory of Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of Sciences school of applied Chemistry and Engineering University of Science and Technology of China

Tirapazamine（TPZ） has been approved for multiple clinical trials relying on its excellent anticancer ***,as a typical hypoxia-activated prodrug（HAP）,TPZ did not exhibit survival advantages in Phase Ⅲ clinical trials when used in combination therapy due to the insufficient hypoxia levels in patients' *** this study,to improve the therapeutic effects of TPZ,we first introduced urea to synthesize a series of urea-containing derivatives of *** urea-containing TPZ derivatives showed increased hypoxic cytotoxicity（9.51-3..85-fold） compared with TPZ,while maintaining hypoxic ***,one of these derivatives,showed 20-fold higher cytotoxicity than TPZ while maintaining a similar hypoxic cytotoxicity *** highly efficiently deliver TPZP to the tumors and reduce its side effects on healthy tissues,we further prepared TPZP into a nanodrug with fibrin-targeting ability:***4-NPs,a vascular disrupting agent,was used to increase the fibrin level within tumors and exacerbate tumor *** being combined with CA4-NPs,FT11-TPZP-NPs can accumulate in the hypoxia-aggravated tumors and activate sufficiently to kill tumor *** a single-dose treatment,FT11-TPZP-NPs+CA4-NPs showed a high inhibition rate of 98.1% against CT26 tumor models with an initial volume of ～480 mm3.nd four out of six tumors were completely eliminated;it thereby exerted a significant antitumor *** study provides a new strategy for improving the therapeutic effect of TPZ and other HAPs in anticancer therapy.

关键词： tirapazamine vascular disrupting agent hypoxia-activated prodrug combretastatin A4 urea

Utilization of 3. printing technology in hepatopancreatobiliary surgery

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Journal of Zhejiang university-Science B(Biomedicine & Biotechnology) 2024年第2期25卷 123-134页

作者： Wujiang SHI Jiangang wang jianjun GAO Xinlei ZOU Qingfu DONG Ziyue HUANG Jialin SHENG Canghai GUAN Yi xu Yunfu CUI Xiangyu ZHONG Department of Hepatopancreatobiliary Surgery the Second Affiliated Hospital of Harbin Medical UniversityHarbin150086China Department of General Surgery Tangdu HospitalAir Force Medical UniversityXi’an710032China Key Laboratory of Basic Pharmacology of Ministry of Education Zunyi Medical UniversityZunyi563006China Key Laboratory of Functional and Clinical Translational Medicine Fujian Province UniversityXiamen Medical CollegeXiamen361000China Department of Pathology Li Ka Shing Faculty of MedicineThe University of Hong KongHong KongChina Jiangsu Province Engineering Research Center of Tumor Targeted Nano Diagnostic and Therapeutic Materials Yancheng Teachers UniversityYancheng224007China Key Laboratory of Biomarkers and In Vitro Diagnosis Translation of Zhejiang Province Hangzhou310053China Key Laboratory of Gastrointestinal Cancer(Fujian Medical university) Ministry of EducationSchool of Basic Medical SciencesFujian Medical UniversityFuzhou350122China Key Laboratory of Myocardial Ischemia Harbin Medical UniversityMinistry of EducationHarbin150086China

The technology of three-dimensional(3.)printing emerged in the late 1970s and has since undergone considerable development to find numerous applications in mechanical engineering,industrial design,and *** biomedical science,several studies have initially found that 3. printing technology can play an important role in the treatment of diseases in hepatopancreatobiliary *** example,3. printing technology has been {3. to create detailed anatomical models of disease organs for preoperative personalized surgical strategies,surgical simulation,intraoperative navigation,medical training,and patient ***,cancer models have been created using 3. printing technology for the research and selection of chemotherapy *** the aim to clarify the development and application of 3. printing technology in hepatopancreatobiliary surgery,we introduce seven common types of 3. printing technology and review the status of research and application of 3. printing technology in the field of hepatopancreatobiliary surgery.

关键词： 3. printing Hepatopancreatobiliary surgery Organ model Cancer model

Flexible,high-density,laminated ECoG electrode array for high spatiotemporal resolution foci diagnostic localization of refractory epilepsy

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Bio-Design and Manufacturing 2024年第4期7卷 388-398页

作者： Yafeng Liu Zhouheng wang Yang Jiao Ying chen Guangyuan xu Yinji Ma xue Feng applied Mechanics Laboratory Department of Engineering MechanicsTsinghua UniversityBeijing 100084China Laboratory of Flexible Electronics technology Tsinghua UniversityBeijing 100084China College of Artificial Intelligence Southwest UniversityChongqing 400715China Institute of Flexible Electronics technology of THU Jiaxing 314000China Qiantang Science and technology Innovation Center Hangzhou 310016China school of Artificial Intelligence Beijing University of Posts and TelecommunicationsBeijing 100876China

High spatiotemporal resolution brain electrical signals are critical for basic neuroscience research and high-precision focus diagnostic localization,as the spatial scale of some pathologic signals is at the submillimeter or micrometer *** entails connecting hundreds or thousands of electrode wires on a limited *** study reported a class of flexible,ultrathin,highdensity electrocorticogram(ECoG)electrode *** challenge of a large number of wiring arrangements was overcome by a laminated structure design and processing technology *** flexible,ultrathin,high-density ECoG electrode array was conformably attached to the cortex for reliable,high spatial resolution electrophysiologic *** minimum spacing between electrodes was 15μm,comparable to the diameter of a single *** hundred electrodes were prepared with an electrode density of 4444 mm^(-2).In focal epilepsy surgery,the flexible,high-density,laminated ECoG electrode array with 3. electrodes was applied to collect epileptic spike waves inrabbits,improving the positioning accuracy of epilepsy lesions from the centimeter to the submillimeter *** flexible,high-density,laminated ECoG electrode array has potential clinical applications in intractable epilepsy and other neurologic diseases requiring high-precision electroencephalogram acquisition.

关键词： Electrocorticogram(ECoG)electrode Epilepsy High density High resolution Laminated structure