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Roadmap for rechargeable batteries:present and beyond

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Science china Chemistry 2024年第1期67卷 13-42页

作者： Sen Xin xu zhang Lin Wang Haijun Yu Xin Chang Yu-Ming Zhao Qinghai Meng Pan xu chen-Zi Zhao Jiahang chen Huichao Lu Xirui Kong Jiulin Wang Kai chen Gang Huang Xinbo zhang Yu Su Yao Xiao Shu-Lei Chou Shilin zhang Zaiping Guo Aobing Du Guanglei Cui Gaojing Yang Qing Zhao Liubing Dong Dong Zhou Feiyu Kang Hu Hong Chunyi Zhi Zhizhang Yuan Xianfeng Li Yifei Mo Yizhou Zhu Dongfang Yu Xincheng Lei Jianxiong Zhao Jiayi Wang Dong Su Yu-Guo Guo Qiang zhang jun chen Li-jun Wan CAS Key laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of Sciences.beijing 100049 China institute of Advanced Battery Materials and Devices Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China Key laboratory of Advanced Functional Materials Ministry of EducationBeijing University of TechnologyBeijing 100124China beijing Key laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China State Key laboratory of Chemistry and Utilization of Carbon-Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China Department of Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China State Key laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChangchun 130022China institute for Carbon Neutralization College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaide 5000Australia Qingdao Industrial Energy Storage Research institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China Frontiers Science Center for New Organic Matter Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China College of Chemistry and Materials Science Jinan UniversityGuangzhou 511443China Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China Department of Materials Science and Engineering City University of Hong KongHong Kong 999077China Division of Energy Storage Dalian National Laboratory for Clean Energy(DNL)Dalian Institute of Chem

Rechargeable batteries currently hold the largest share of the electrochemical energy storage market,and they play a major role in the sustainable energy transition and industrial decarbonization to respond to global climate *** to the increased popularity of consumer electronics and electric vehicles,lithium-ion batteries have quickly become the most successful rechargeable batteries in the past three decades,yet growing demands in diversified application scenarios call for new types of rechargeable *** efforts are made to developing the next-generation post-Li-ion rechargeable batteries,which include,but are not limited to solid-state batteries,lithium–sulfur batteries,sodium-/potassium-ion batteries,organic batteries,magnesium-/zinc-ion batteries,aqueous batteries and flow *** the great achievements,challenges persist in precise understandings about the electrochemical reaction and charge transfer process,and optimal design of key materials and interfaces in a *** roadmap tends to provide an overview about the current research progress,key challenges and future prospects of various types of rechargeable *** computational methods for materials development,and characterization techniques will also be discussed as they play an important role in battery research.

关键词： energy storage rechargeable batteries battery materials electrochemistry

Churning loss characteristics of a wet three-phase high-speed reluctance motor

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Journal of Zhejiang University-Science A(applied physics & Engineering) 2024年第3期25卷 251-267页

作者： Zhenzhou zhang Mingzhu DAI chenchen zhang Yi chen Bin MENG College of Mechanical Engineering Zhejiang University of TechnologyHangzhou 310023China

With the increasing requirements of electro-hydrostatic actuators(EHAs)for power,volume,and pressure,there is a growing tendency in the industry to combine the motor and pump to form a so-called'motor pump'to improve the *** this paper,a novel structure for a wet three-phase high-speed reluctance motor pump is proposed,which can further improve integration by removing the dynamic seal on the pump shaft,thereby avoiding the problems of dynamic seal wear and oil leakage and improving heat dissipation under high-speed working ***,after the motor is wetted,the churning loss caused by immersion of the rotor in the oil causes additional fluid resistance *** on fundamental fluid mechanics,an analytical model of the churning torque of a wet motor was *** verify the accuracy of the analytical model,a simulation model of churning loss was established based on computational fluid dynamics(CFD),and the churning torque and flow field state were ***,an experimental prototype was designed and manufactured,and a test bench for churning loss was *** oil churning torque was measured at different speeds and *** results from the analytical,simulation,and experimental models agreed *** experimental results validated the analytical model and CFD *** research provides a practical method for calculating the churning loss and serves as guidance for future optimization of churning loss reduction.

关键词： Motor pump Wet motor Churning loss Analytical model computational fluid dynamics(CFD)

Reflection behavior of insensitive explosive detonation propagating around a cylinder

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Acta Mechanica Sinica 2024年第7期40卷 55-65页

作者： Zixuan zhang Yuan Wang Xiaomian Hu Haitao chen institute of applied physics and computational mathematics Beijing 100094China Graduate School of china Academy of Engineering physics Beijing 100088China

Insensitive explosive detonation has wide applications in compressing and driving inert materials,and thereby the interaction between detonation and inert materials has received more *** this paper,a two-dimensional numerical simulation based on the Euler multiphase flow framework is used to investigate the reflection behavior of the insensitive explosive detonation propagating around a *** results show that there is a critical incident angle,defined as transition angle for detonation propagating around the cylinder,below which the regular reflection(RR)on the cylinder surface is *** the incident angle is greater than the transition angle,RR changes to Mach *** transition angle is larger than that obtained by polar curve theory and the change of incident angle is used to interpret above *** addition,the influence of cylindrical radius and detonation reaction zone width on the reflection behavior is *** the cylindrical radius increases,the height of Mach stem increases while the transition angle decreases and gradually approaches the value in pole curve *** Neumann reflection is observed when the reaction zone width is relatively *** is because the energy release rate in the reaction zone is high for small reaction zone width,resulting in the formation of a series of compression waves near the cylindrical interface.

关键词： Insensitive explosive detonation Cylindrical inert material Reflection behavior

Elaborating strengthen mechanism of Pt-Ir solid solution superalloy at finite temperature

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Rare Metals 2024年第3期43卷 1243-1256页

作者： Wei Yu Xiao-Yu Chong yun-xuan Zhou Meng-Di Gan Ying-xue Liang Yan Wei Ai-Min zhang Chang-Yi Hu Xing-Yu Gao Li chen Hai-Feng Song Jing Feng Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming650093China yunnan Precious Metals laboratory Co.LTD Kunming650106China laboratory of computational physics Institute of Applied Physics and Computational MathematicsBeijing100088China

Pt-Ir alloy is potential superalloys used above 1300℃because of their high strength and creep ***,the ductility of Pt-Ir alloy has rapidly deteriorated with the increase of Ir,resulting in poor *** work quantitatively evaluated the solid solution strengthening(SSS)and grain refinement strengthening(GRS)of Pt-Ir alloy using first-principles calculations combined with experimental ***,the stretching force constants in the second nearest neighbor region(SFC^(2nd))of pure Ir(193.7 eV·nm^(-2))are 3.40 times that of pure Pt(57.0 eV·nm^(-2)),i.e.,the interatomic interaction is greatly enhanced with the increase of Ir content,which leads to the decrease of ductility,and modulus misfit plays a dominant role in ***,the physical mechanisms responsible for the hardness(H_(V))of Pt-Ir alloy,using the power-law-scaled function of electron work function coupled SSS and GRS,are attributed to the electron redistribution caused by different Ir ***,a thorough assessment of the thermodynamic characteristics of Pt-Ir binary alloy was conducted,culminating in development of a mapping model that effectively relates enmposition,temperature and *** results revealed that the compressive strength incrcases with the Ir content,and the highest strength was observed in Pt_(0.25)Ir_(0.75).This study provides valuable insights into the Pt-Ir alloy system.

关键词： Elastic properties Phonon Solid solution strengthen Force constants CALPHAD

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Delaunay三角网格的一种快速生成法

数值计算与计算机应用 2001年第4期22卷 267-275页

作者：邬吉明沈隆钧张景琳北京应用物理与计算数学研究所计算物理实验室

Delaunay triangulation has been widely used in many fields such as compu- tational fluid dynamics, statistics, meteorology solid state physics, computational geometry and so on. Bowyer-Watson algorithm is a very popular one for generating Delaunay triangulation. In generating the Delaunay triangulation of a preassigned set of n points, the complexity of Bowyer-Watson algorithm can at most be reduced to O(n log n) for the simple reason that the complexity of its tree search process is O(nlog n). In this paper we suggest a tree search technique whose complexity is O(n). Noting that the order of point insertion can affect the efficiency of Bowyer- Watson algorithm, we propose a technique to optimize the point insertion process. Based on these two techniques, we obtain a fast algorithm for generating Delaunay triangulation.

关键词：流体力学 Delaunay三角网格 Bowyer-Watson算法树搜索方法加点过程优化

Radiation Spectral Analysis of 3D Dust Molecular Clusters(PAHs)and Peptoids under Ionization and Electric Field in ISM

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Research in Astronomy and Astrophysics 2024年第1期24卷 70-77页

作者： Ruiqing Wu Chunhua Zhu Guoliang Lü Xiaojiao zhang Xizhen Lu Jinlong Yu Wujin chen Mengqiu Long School of physics and Electronics Central South UniversityChangsha 410083China School of Physical Science and Technology Xinjiang UniversityUrumqi 830046China School of Microelectronics and physics Hunan University of Technology and BusinessChangsha 410205China College of Mechanical and Electronic Engineering Tarim UniversityAlar 843300China School of Medicine Xinjiang Medical UniversityUrumqi 830011China

Polycyclic aromatic hydrocarbons(PAHs),PANHs,and peptoids dust spectral calculations from the interstellar medium(ISM)are important for dust observations and *** goal is to calculate the radiation spectrum of spherical PAHs dust clusters in a vacuum containing ionized and applied in the presence of an electric *** propose a new simple computational model to calculate the size of three-dimensional spherical dust clusters formed by different initial dust *** the Vienna Ab-initio Simulation Package code,the density functional theory with the generalized approximation was used to calculate the electron density gradient and obtain the radiation spectrum of *** the radius of spherical dust clusters is~[0.009-0.042]μm,the dust radiation spectrum agrees well with the Z=0.02 mMMP stellar spectra,and the PAHs radiation spectrum of NGC 4676 at wavelengths of(0-5]μm and(5-10]μm,*** the ionized state,the N-PAH,C_(10)H_(9)N,2(C_(4)H_(4))^(1+),and peptoids 4(CHON),(C_(8)H_(10)N_(2)O_(5))^(1+)dust clusters at 3.3μm,while the 2(C_(22)H_(21)N_(3)O_(2))^(1+),4(CHON)dust clusters at 5.2μm have obvious *** is a characteristic of part of PAHs and peptoids clusters radiation at the nearinfrared wavelength of 2μ***,especially after applying an electric field to the dust,the emission spectrum of the dust increases significantly in the radiation wavelength range[3-10]μ***,the dust clusters of PAHs,PANHs,and peptoids of the radius size~[0.009-0.042]μm are likely to exist in the ISM.

关键词： ISM:structure ISM:molecules radiation mechanisms:general (ISM:)dust extinction

Scintillation Arc from FRB 20220912A

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Science china(physics,Mechanics & Astronomy) 2024年第1期67卷 134-142页

作者： Zi-Wei Wu Robert AMain Wei-Wei Zhu Bing zhang Peng Jiang Jia-Rui Niu Jin-Lin Han Di Li Ke-Jia Lee Dong-Zi Li Yuan-Pei Yang Fa-Yin Wang Rui Luo Pei Wang chen-Hui Niu Heng xu Bo-jun Wang Wei-Yang Wang Yong-Kun zhang Yi Feng De-Jiang Zhou Yong-Hua xu Can-Min Deng Yu-Hao Zhu National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China Max-Planck-Institut für Radioastronomie Bonn 53121Germany institute for Frontier in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China Nevada Center for Astrophysics and Department of physics and Astronomy University of NevadaLas VegasNV 89154USA CAS Key laboratory of FAST National Astronomical ObservatoriesChinese Academy of SciencesBeijing 100101China School of Astronomy University of Chinese Academy of SciencesBeijing 100049China NAOC-UKZN computational Astrophysics Centre University of KwaZulu-NatalDurban 4000South Africa Department of Astronomy Peking UniversityBeijing 100871China Kavli institute for Astronomy and Astrophysics Peking UniversityBeijing 100871China Cahill Center for Astronomy and Astrophysics California Institute of TechnologyPasadena 91125USA South-Western institute For Astronomy Research Yunnan UniversityKunming 650504China School of Astronomy and Space Science Nanjing UniversityNanjing 210093China Key laboratory of Modern Astronomy and Astrophysics(Nanjing University) Ministry of EducationNanjing 210023China CSIRO Space and Astronomy Epping 1710Australia Department of Astronomy School of Physics and Materials ScienceGuangzhou UniversityGuangzhou 510006China Research Center for Intelligent Computing Platforms Zhejiang LaboratoryHangzhou 311100China yunnan Observatories Chinese Academy of SciencesKunming 650011China Guangxi Key laboratory for Relativistic Astrophysics Department of PhysicsGuangxi UniversityNanning 530004China

We present the interstellar scintillation analysis of fast radio burst(FRB)20220912A during its extremely active episode in 2022using data from the Five-hundred-meter Aperture Spherical Radio Telescope(FAST).We detect a scintillation arc in the FRB’s secondary spectrum,which describes the power in terms of the scattered FRB signals’time delay and Doppler *** arc indicates that the scintillation is caused by a highly localized *** analysis favors a Milky Way origin of the ionized interstellar medium(IISM)for the localized scattering medium but cannot rule out a host galaxy *** present our method for detecting the scintillation arc,which can be applied generally to sources with irregularly spaced bursts or *** methods could help shed light on the complex interstellar environment surrounding the FRBs and in our Galaxy.

关键词： fast radio burst scintillation FRB 20220912A

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共享存储并行机的算法设计

数值计算与计算机应用 1997年第3期18卷 187-198页

作者：刘兴平张景琳北京应用物理与计算数学研究所计算物理实验室

In this paper we discuss algorithm design and programing of iterative methods of large sparse linear system on a vector computer and a shared memory parallel *** examples indicate that the efficiency of the methods is... 详细信息

关键词：算法共享存储并行计算机设计

Accurate prediction of interference minima in linear molecular harmonic spectra by a modified two-center model

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Chinese physics B 2016年第3期25卷 163-168页

作者：崔鑫张頔玉陈高陈基根曾思良郭福明杨玉军 institute of Atomic and Molecular physics Jilin UniversityChangchun 130012China Jilin Provincial Key laboratory of applied Atomic and Molecular Spectroscopy Jilin UniversityChangchun 130012China School of Science Changchun University of Science and TechnologyChangchun 130022China Department of physics and Materials Engineering Taizhou UniversityTaizhou 318000China institute of applied physics and computational mathematics Beijing 100088China

We demonstrate that the interference minima in the linear molecular harmonic spectra can be accurately predicted by a modified two-center model. Based on systematically investigating the interference minima in the linear molecular harmonic spectra by the strong-field approximation （SFA）, it is found that the locations of the harmonic minima are related not only to the nuclear distance between the two main atoms contributing to the harmonic generation, but also to the symmetry of the molecular orbital. Therefore, we modify the initial phase difference between the double wave sources in the two-center model, and predict the harmonic minimum positions consistent with those simulated by SFA.

关键词： high-order harmonic generation molecular harmonics