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Monothetic and conductive network and mechanical stress releasing layer on micron-silicon anode enabling high-energy solid-state battery

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Rare Metals 2024年第3期43卷 1017-1029页

作者： Xiang Han Min Xu Lan-Hui Gu Chao-Fei Lan Min-Feng chen Jun-jie Lu Bi-Fu {2. Peng Wang Song-Yan chen ji-Zhang chen College of Materials Science and Engineering Co-Innovation Center of Efficient Processing and Utilization of Forestry ResourcesNanjing Forestry UniversityNanjing210037China department of physics Xiamen UniversityXiamen361005China Western Digital Corporation MilpitasCA95035USA

Silicon has ultrahigh capacity,dendrite-free alloy lithiation mechanism and low cost and has been regarded as a promising anode candidate for solid-state *** to the low infiltration of solid-state electrolyte(SSE),not the unstable solid-electrolyte interphase(SEI),but the huge stress during lithiation-and delithiation-induced particle fracture and conductivity lost tend to be the main *** this study,starting with micron-Si,a novel monothetic carbon conductive framework and a MgO coating layer are designed,which serve as electron pathway across the whole electrode and stress releasing layer,*** addition,the in situ reaction between Si and SSE helps to form a LiF-rich and mechanically stable SEI *** a result,the mechanical stability and charge transfer kinetics of the uniquely designed Si anode are significantly ***,high initial Coulombic efficiency,high capacity and durable cycling stability can be achieved by applying the Si@MgO@C anode in *** example,high specific capacity of 3.1}4.6 mAh·g^(-1)and long cycling durability of 2.0 cycles are *** work provides a new concept for designing alloy-type anode that combines surface coating on particle and electrode structure design.

关键词： Lithium-ion battery(LIB) Solid-state electrolyte(SSE) Silicon anode Stress relief Coating

Nondestructive Nonlinear Optical Microscopy Revealed the Blackening Mechanism of Ancient Chinese Jades

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Research 2024年第3期2023卷 391-399页

作者： Yaxin chen Rong Wang Minbiao ji State Key Laboratory of Surface physics and department of physics Human Phenome InstituteAcademy for Engineering and TechnologyKey Laboratory of Micro and Nano Photonic Structures(Ministry of Education)Yiwu Research Institute of Fudan UniversityFudan UniversityShanghai 200433China department of Cultural Heritage and Museology Fudan UniversityShanghaiChina

Jade is most valued in Chinese culture since ancient times. For unearthed jade artifacts, the alteration color resulting from weathering effects and human activities provides information for cultural heritage conservation, archaeology, and history. Currently, the noninvasive 3.dimensional characterization of jade artifacts with high chemical and spatial resolution remains challenging. In this work, we applied femtosecond pump–probe microscopy and second harmonic generation microscopy techniques to study the black alteration of an ancient jade artifact of the late Spring and Autumn period (546 to 476 BC). The direct cause of the “mercury alteration” phenomena was discovered to be the conversion of metacinnabar from buried cinnabar in the tomb. Furthermore, a 3.dimensional optical reconstruction of the black alteration was achieved, providing a high-resolution method for analyzing the blackening mechanism without the need of sample damage. Our approach opens up new opportunities to extract microscopic spatiochemical information for a broad range of alteration colors in jade artifacts.

关键词： pump Nonlinear buried

Regulating Anderson localization with structural defect disorder

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Chinese physics B 2024年第10期33卷 102-107页

作者： Mouyang cheng Haoxiang chen {2. chen School of physics Peking UniversityBeijing 100871China Interdisciplinary institute of Light-Element Quantum Materials and Research Center for Light-Element Advanced Materials Peking UniversityBeijing 100871China Frontiers Science Center for Nano-Optoelectronics Peking UniversityBeijing 100871China Collaborative Innovation Center of Quantum Matter Beijing 100871China

Localization due to disorder has been one of the most intriguing theoretical concepts that evolved in condensed matter ***,we expand the theory of localization by considering two types of disorders at the same time,namely,the original Anderson’s disorder and the structural defect disorder,which has been suggested to be a key component in recently discovered two-dimensional amorphous *** increasing the degree of both disorders could induce localization of wavefunction in real space,we find that a small degree of structural defect disorder can significantly enhance the *** the degree of structural defect disorder increases,localized states quickly appear within the extended phase to enter a broad crossover region with mixed *** establish two-dimensional diagrams for the wavefunction localization and conductivity to highlight the interplay between the two types of *** theoretical model provides a comprehensive understanding of localization in two-dimensional amorphous materials and highlights the promising tunability of their transport properties.

关键词： Anderson localization structural defect disorder electronic transport properties

In-situ powder mixing for laser-based directed energy deposition of functionally graded materials

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Advances in Manufacturing 2024年第1期12卷 150-166页

作者： ji-Peng chen Shou-Chun Xie He Huang School of Mechanical and Electronic Engineering Nanjing Forestry UniversityNanjing210037People’s Republic of China Nanjing Huirui Photoelectric Technology Co. LtdNanjing211121People’s Republic of China

The mixing of powders is a highly relevant field under additive manufacturing,however,it has attracted limited interest to *** in-situ mixing of various powders remains a significant *** paper proposes a new method utilizing a static mixer for the in-situ mixing of multiple powders through the laser-based directed energy deposition(DED)of functionally graded ***,a powder-mixing experimental platform was established;WC and 3.6L powders were selected for the mixing ***,scanning electron microscopy,energy dispersive spectroscopy,and image processing were used to visually evaluate the homogeneity and proportion of the in-situ mixed ***,powder-mixing simulations were conducted to determine the powder-mixing *** the simulations,a powder carrier gas flow field and particle mixing were ***,a WC/3.6L metal matrix composite sample was produced using laser-based DED to verify the application potential of the static *** was found that the static mixer could adjust the powder ratio online,and a response time of 1–2.s should be considered when adjusting the ratio of the mixed powder.A feasible approach for in-situ powder mixing for laser-based DED was demonstrated and investigated,creating the basis for functionally graded materials.

关键词： Laser Deposition Static mixer Powder mixing Functionally graded materials

Narrow line Seyfert 1 galaxies: where are the broad line regions?

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Science china(physics,Mechanics & Astronomy) 2010年第12期53卷 2307-2311,2339-2343页

作者： MAO WeiMing 1,2.3., HU chen 2., WANG {3.anMin 2., BIAN WeiHao 4 , ZHANG Shu 2.& ZHAO Gang 1 1 Key Laboratory of Optical Astronomy, National Astronomical Observatories, Chinese Academy of Sciences, Bei{3.ng 100012. china 2.Key Laboratory for particle Astrophysics, institute of High Energy physics, Chinese Academy of Sciences, Bei{3.ng 100049, china 3.Graduate University of the Chinese Academy of Sciences, Bei{3.ng 100049, china 4 {12. of physics, Nan{3.ng Normal University, Nan{3.ng 2.0011, china Key Laboratory of Optical Astronomy National Astronomical Observatories Chinese Academy of Sciences Beijing China Key Laboratory for particle Astrophysics Institute of High Energy Physics Chinese Academy of Sciences Beijing China Graduate University of the Chinese Academy of Sciences Beijing China department of physics Nanjing Normal University Nanjing China

A sample consisting of 2.1 narrow line Seyfert 1 galaxies (NLS1s) with high quality spectra from the Sloan Digital Sky Survey (SDSS) is selected to explore where broad line regions are in these objects. We find that the Hβ profile can be fitted well by three (narrow, intermediate and broad) Gaussian components, and the FWHM ratios of the broad to the intermediate components hold a constant of 3.0 roughly for the entire sample. If the broad components originate from the region scaled by the well-determined Hβ reverberation mapping relation, we find that the intermediate components originate from the inner edge of the torus, which is scaled by dust K-band reverberation. We find that the IC and the BC are strongly linked dynamically, but the relation of their covering factors is much more relaxed, implying that both regions are clumpy.

关键词： black hole physics galaxies: evolution quasars: general

Polyoxometalates for continuous power generation by atmospheric humidity

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Nano Research 2024年第3期17卷 1875-1885页

作者： Tuo ji Weilin chen Zhenhui Kang Liming Zhang Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Northeast Normal UniversityChangchun 130024China institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices DepartmentSoochow UniversitySuzhou 215123China Macao institute of Materials Science and Engineering Macao University of Science and TechnologyTaipaMacao 999078China institute of Functional State Key Laboratory of Luminescence and Applications Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China

Atmospheric humidity is a sustainable low-value energy widely existing in natural environment,which is a promising candidate to solve the noncontinuous and low efficiency of low-value energy power *** the mono-substituted Dawson-type polyoxometalates are constructed to be highly dispersed organic ammonium-polyoxoanion clusters and are assembled into thin films power generators with micropores,working in atmospheric *** optimal polyoxometalates generator with the thickness of 7.2.m and the area of 0.3. cm^(2. produces a voltage of 0.68 V and a current density of 19.5μA·cm^(-2. under simulated natural environment,and works continuously and stably under almost all-natural environments(humidity 10%–90%).The highly dispersed polyoxometalate nanoclusters can form microporous in polyoxometalate films to effectively absorb atmospheric humidity and spontaneously form distribution gradient of water,which is the structural basis of power *** continuous power generation may be maintained by the effective adsorption and utilization of H_(2.O,the huge electrostatic field of organic ammonium-polyoxoanion clusters,and the reasonably designed polyoxometalates containing inorganic small ions with high *** is the first humidity generator designed with polyoxometalates,which may provide a new research direction for polyoxometalates in sustainable utilization of low-value energy.

关键词： atmospheric humidity continuous power generations nanomaterials polyoxoanions polyoxometalates

Absorption Cross Section of Einstein-Maxwell Dilation Axion Black Hole for Dirac particles

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Communications in Theoretical physics 2007年第12期48卷 1051-1054页

作者： LIU Chang-Qing jiNG ji-Liang {2. of {3. and department of {3.,Hunan Normal University,Changsha 410081,china institute of physics and {2. of physics Hunan Normal University Changsha 410081 China

The absorption cross section of the Einstein-Maxwell Dilaton Axion (EMDA) black hole for Dirac particlesis *** is shown that the absorption cross section decreases as both the v and the absolute value of the dilatonincrease,but it increases as the mass of the particle *** is also shown that the absorption cross section for themassless Dirac particles is 1/8 of the area of the horizon,which may be an universal property for minimally coupledmassless Dirac particles.

关键词： black hole absorption cross section Dirac particle

Properties of the 3.2.-[52.] band in the odd-N rare-earth nuclei

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Science china(physics,Mechanics & Astronomy) 2011年第S1期54卷 37-43页

作者： chen Liang1,2. ZHOU XiaoHong1,2. ZHANG YuHu1, ZHANG ShuangQuan3.& ZHU LiHua4 1{3. of Modern {2., Chinese Academy of Sciences, Lanzhou 73.000, china 2.raduate University of Chinese Academy of Sciences, Beijing 100049, china 3.tate Key Laboratory of Nuclear {2. and Technology, School of {2., Peking University, Beijing 100871, china 4china {3. of Atomic Energy, Beijing 102.13. china institute of Modern physics Chinese Academy of Sciences Lanzhou China Graduate University of Chinese Academy of Sciences Beijing China State Key Laboratory of Nuclear physics and Technology School of Physics Peking University Beijing China china institute of Atomic Energy Beijing China

High-spin states in 161Er have been studied experimentally via the 150Nd(16O, 5n) reaction at a beam energy of 86 MeV. Three rotational bands built on the 5/2.[642., 3.2.[52.], and 11/2.[505] configurations have been extended up to high-spin states, and particularly, the α = -1/2.branch of the ground state 3.2.[52.] band has been revised significantly. It is found that signature inversion occurs in the 3.2.[52.] band after the band crossing in 161Er. The systematics of the signature inversion associated with the 3.2.[52.] configuration in the rare-earth region is discussed. The band properties are analyzed within the framework of a triaxial particle-rotor model, and a triaxial deformation is proposed to the 3.2.[52.] band.

关键词： high-spin states signature inversion triaxial particle-rotor model

Solvothermal synthesis of nanocrystalline FeS_2

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Science china(physics,Mechanics & Astronomy) 2005年第2期48卷 188-200页

作者： chen Yanhua1, ZHENG Yufeng1, ZHANG Xiaogang2. SUN Yanfei1 & DONG Youzhong11. physics {2. of Xinjiang University, Urumqi 83.046, china 2. institute of Applied Chemistry of Xinjiang University, Urumqi 83.046, china physics department of Xin{2.ang University Urumqi China institute of Applied Chemistry of Xinjiang University Urumqi China

This paper reports on the synthesis of the nanocrystalline FeS2.via a solvent-thermal process. Using FeSO4 and NH2.SNH2.as precursors and polyvinyl- pyrrolidone (PVP) as a protective agent (dispersant), we have successfully synthesized nanocrystalline FeS2.both under acidic conditions (pH = 5) and under alkali conditions (pH = 10) at various temperatures and for different time in alcohol-water solution. X-ray diffraction (XRD), Transmission electron microscopy (TEM) and Ultraviolet Visible (UV-VIS) spectroscopy were used to characterize the morphology, structure, particle size and optical characterization of sample synthesized under acidic condition, and the XRD pattern was refined by Rietveld method. The experimental result shows that nanocrystalline FeS2.with uniform size, highly crystallized quality and excellent dispersivity has been synthesized at 2.0℃for 3. h.

关键词： FeS2 (Pyrite), solvothermal, PVP, the Rietveld method.