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Optimizing theπ-Bridge of Non-fullerene Acceptors to Suppress Dark Current in NIR Organic Photodetectors

Chemical Research in Chinese Universities 2024年第4期40卷 712-721页

作者： SHAO Lin HUANG Yijun hong Ling XU Zishuo YANG Xiye LIU Chunchen HUANG Fei cao Yong State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesSchool of Materials Science and EngineeringSouth China University of TechnologyGuangzhou510640P.R.China Lumidar Technology Co. Ltd.Guangzhou510530P.R.China

Recently,the rapid development of non-fullerene acceptors(NFAs)has laid the foundation for performance improvements in near-infrared(NIR)organic photodetectors(OPDs).However,reducing the bandgap of NFAs to achieve strong absorption in the shorter-wave region usually leads to increased dark current density(J_(d))and decreased responsivity(R),severely limiting the detectivity(D*)of *** date,it remains challenging to manipulate the J_(d) of NIR-OPDs through rational structure engineering of ***,three NIR-NFAs,namely bis(2-decyltetradecyl)4,4′-(2′,7′-di-tert-butylspiro[cyclopenta[2,1-b:3,4-b′]dithiophene-4,9′-fluorene]-2,6-diyl)bis(6-(((Z)-1-(dicyanomethylene)-5,6-difluoro-3-oxo-1,3-dihydro-2H-inden-2-ylidene)methyl)thieno[3,4-b]thiophene-2-carboxylate)(TSIC-4F),bis(2-decyltetradecyl)6,6′-(2′,7′-di-tert-butylspiro[cyclopenta[2,1-b:3,4-b′]dithiophene-4,9′-fluorene]-2,6-diyl)bis(4-(((Z)-1-(dicyanomethylene)-5,6-difluoro-3-oxo-1,3-dihydro-2H-inden-2-ylidene)methyl)thieno[3,4-b]thiophene-2-carboxylate)(STIC-4F),and 2,2′-((2Z,2′Z)-(((2′,7′-di-tert-butylspiro[cyclopenta[2,1-b:3,4-b′]dithiophene-4,9′-fluorene]-2,6-diyl)bis(2,3-bis(5-(2-butyloctyl)thiophen-2-yl)thieno[3,4-b]pyrazine-7,5-diyl))bis(metha-neylylidene))bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene))dimalononitrile(TPIC-4F),were designed using the thieno[3,4-b]thiophene(TT)and thieno[3,4-b]pyrazine(TPy)derivatives as theπ-*** to the intramolecular S-S and S-N interactions,STIC-4F and TPIC-4F exhibited smaller backbone distortions than TSIC-4F.A significantly red-shifted absorption with a peak at 1015 nm was observed in TPIC-4F film,larger than that(ca.960 nm)for TSIC-4F and STIC-4F ***,OPDs operating in a photovoltaic mode were successfully fabricated,and TPIC-4F-based OPDs achieved the lowest J_(d) of 3.18×10^(-8) A/cm^(2) at-0.1 ***,although TPIC-4F-based OPDs exhibited the lowest R,higher shot-noise-limited specific detectivity(D_(sh)*)in 1000-1200 nm co

关键词： π-Bridge Near-infrared Non-fullerene acceptor Dark current Organic photodetector

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基于概率论原理的特大桥梁船舶撞击力确定方法

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桥梁建设 2005年第6期35卷 48-51页

作者：曹映泓周颖罗林阁广东省路桥建设发展有限公司广东广州510635 华南理工大学交通学院广东广州510640

现行的桥梁设计规范关于船舶撞击力及防撞设计的内容少,而且不适应大型船舶通行的航道情况。针对这一现象,借鉴抗风抗震的概率论原理提出了一套用于确定船舶撞击力的概率论原理,该原理如果成功应用可以为大桥防撞设计提供一个合理的普... 详细信息

现行的桥梁设计规范关于船舶撞击力及防撞设计的内容少,而且不适应大型船舶通行的航道情况。针对这一现象,借鉴抗风抗震的概率论原理提出了一套用于确定船舶撞击力的概率论原理,该原理如果成功应用可以为大桥防撞设计提供一个合理的普遍实用的方法。

关键词：桥梁船舶撞击设计概率论

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Development of a Decision Aid for Family Surrogate Decision Makers of Critically Ill Patients Requiring Renal Replacement Therapy in ICU:A User-Centered Design for Rapid Prototyping

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Chinese Medical Sciences Journal 2024年第2期39卷 91-101页

作者： Miao Zheng Yong-Hui Zhang ying cao Chang-Lin Yin Li-Hua Wang Department of Outpatient First Affiliated Hospital of Army Medical UniversityChongqing 400038China Department of Critical Care Medicine First Affiliated Hospital of Army Medical UniversityChongqing 400038China Administration Office First Affiliated Hospital of Army Medical UniversityChongqing 400038China

Objectives Renal replacement therapy(RRT)is increasingly adopted for critically ill patients diagnosed with acute kidney injury,but the optimal time for initiation remains unclear and prognosis is uncertain,leading to medical complexity,ethical conflicts,and decision dilemmas in intensive care unit(ICU)*** study aimed to develop a decision aid(DA)for the family surrogate of critically ill patients to support their engagement in shared decision-making process with *** Development of DA employed a systematic process with user-centered design(UCD)principle,which included:(i)competitive analysis:searched,screened,and assessed the existing DAs to gather insights for design strategies,developmental techniques,and functionalities;(ii)user needs assessment:interviewed family surrogates in our hospital to explore target user group's decision-making experience and identify their unmet needs;(iii)evidence syntheses:integrate latest clinical evidence and pertinent information to inform the content development of *** The competitive analysis included 16 relevant DAs,from which we derived valuable insights using existing *** decision needs were explored among a cohort of 15 family surrogates,revealing four thematic issues in decision-making,including stuck into dilemmas,sense of uncertainty,limited capacity,and delayed decision confirmation.A total of 27 articles were included for evidence *** decision making knowledge on disease and treatment,as delineated in the literature sourced from decision support system or clinical guidelines,were formatted as the foundational knowledge ***-one items of evidence were extracted and integrated into the content panels of benefits and risks of RRT,possible outcomes,and reasons to *** DA was drafted into a web-based phototype using the elements of *** platform could guide users in their preparation of decision-making through a sequential four-step process:identifying

关键词： decision aids renal replacement therapy intensive care units shared decision-making user-centered design surrogate

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Unique polysulfide reaction on VO_(2) for restraining shuttle effect in soft-packaged Li-S pouch cells

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Rare Metals 2024年第6期43卷 2842-2850页

作者： Ruo-Xuan Yang Qing-Chun Zhang Jing-Sheng Cai Xuan cao Qin Yang ying-Ze Song Wei Zhang State Key Laboratory of Environment-Friendly Energy Materials Tianfu Institute of Research and InnovationSchool of Materials and ChemistrySouthwest University of Science and TechnologyMianyang 621010China School of Materials Engineering Changshu Institute of TechnologyChangshu 215500China Chongqing Institute of Green and Intelligent Technology Chinese Academy of SciencesChongqing 400714China

The shuttle phenomenon and retarded conversion kinetics of lithium poly sulfides(LiPSs)are relatively severe in lithium-sulfur(Li-S)pouch *** to their redox potential in the sulfur working window,VO_(2)nanobelts show ... 详细信息

关键词： mechanism sulfide lithium

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Tuning the electronic conductance of REH_(x)(RE=Nd,Ce,Pr)by structural deformation

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Journal of Energy Chemistry 2024年第8期95卷 440-445,I0010页

作者： Shangshang Wang Weijin Zhang Jirong Cui Shukun Liu hong Wen Jianping Guo Teng He Hujun cao Ping Chen Dalian Institute of Chemical Physics Chinese Academy of SciencesDalian 116023LiaoningChina Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Catalysis Chinese Academy of SciencesDalian 116023LiaoningChina

Hydride ion(H-)conductors have drawn much attention due to their potential applications in hydrideion-based *** earth metal hydrides(REH_(x))have fast H-conduction which,unfortunately,is accompanied by detrimental electron conduction preventing their application as ion ***,REH_(x)(RE=Nd,Ce,and Pr)with varied grain sizes,rich grain boundaries,and defects have been prepared by ball milling and subsequent *** electronic conductivity of the ball-milled REH_(x)samples can be reduced by 2-4 orders of magnitude compared with the non-ball-milled *** relationship of electron conduction and miscrostructures in REH_(x)is studied and discussed based on experimental data and previously-proposed classical and quantum *** H-conductivity of all REH_(x)is about 10^(-4)to 10^(-3)S cm^(-1)at room temperature,showing promise for the development of H-conductors and their applications in clean energy storage and conversion.

关键词： Hydride ion conduction Electron conduction Nanosized grain Crystal defect Electron scattering

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Effect of lens surgery on health-related quality of life in preschool children with congenital ectopia lentis

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International Journal of Ophthalmology(English edition) 2024年第1期17卷 66-72页

作者： Yan-Qiao Huang Qian-Zhong cao Yi-Yao Wang Yi-Jing Zhou Dan-ying Zheng State Key Laboratory of Ophthalmology Zhongshan Ophthalmic CenterSun Yat-sen UniversityGuangdong Provincial Key Laboratory of Ophthalmology and Visual ScienceGuangdong Provincial Clinical Research Center for Ocular DiseasesGuangzhou 510060Guangdong ProvinceChina

AIM:To evaluate the effect of lens surgery on health-related quality of life(HRQoL)of preschool children with congenital ectopia lentis(CEL).METHODS:A prospective self-controlled study was conducted in Zhongshan Ophthalmic *** aged from 5 to 7y whom were diagnosed with CEL and underwent phacoemulsification with scleral-fixated posterior chamber intraocular lens implantation and their parents were enrolled in this *** of them completed the child and proxy(parental)PedsQL™4.0 before and after the *** preoperative scores were compared to their postoperative *** analyses were performed based on gender and preoperative bilateral presenting visual acuity of the ***:Thirty-two children with CEL successfully underwent surgery without any complications,among whom 8 had monocular surgery and 24 had binocular *** and postoperative questionnaires were completed by 32 child-parent *** intervention could significantly improve the vision of affected children(P<0.001).The medians of physical,psychosocial and total health scores self-reported by the children were 68.75(62.50,81.25),65.00(60.00,80.00)and 67.39(60.87,78.26)preoperatively and were 93.75(87.50,100.00),90.00(83.33,96.67)and 89.13(85.32,95.65)*** preoperative scores of the affected children were significantly lower in all scales than age-matched healthy children(P<0.001).All the postoperative scores were significantly higher than the preoperative scores in affected children and their parents(P<0.001).In the physical functioning evaluation,the preoperative score reported by parents of girls was higher than parents of boys(P=0.041),and the postoperative score of girls was higher than that of boys(P=0.036).CONCLUSION:CEL is associated with significantly worse quality of life in preschool *** intervention can significantly improve the HRQoL in affected children from both personal and family perspective.

关键词： congenital ectopia lentis surgical intervention health-related quality of life preschool children

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大气颗粒物及降尘中重金属的分布特征与人体健康风险评价

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环境科学 2017年第9期38卷 3575-3584页

作者：王永晓曹红英邓雅佳张倩中国科学院地理科学与资源研究所北京100101 中国科学院陆地表层格局与模拟重点实验室北京100101 中国科学院大学资源与环境学院北京100049

为了解PM_(2.5)、PM_(10)和降尘中Cu、Mn、Pb、Ti、V、Cd、Cr、Co、Mo、Ni等10种重金属元素的分布特征及人体健康风险,利用大流量颗粒物采样器采集了北京城区某地四季大气中PM_(2.5)、PM_(10)及降尘样品,用ICP-MS测定了上述10种金属元... 详细信息

为了解PM_(2.5)、PM_(10)和降尘中Cu、Mn、Pb、Ti、V、Cd、Cr、Co、Mo、Ni等10种重金属元素的分布特征及人体健康风险,利用大流量颗粒物采样器采集了北京城区某地四季大气中PM_(2.5)、PM_(10)及降尘样品,用ICP-MS测定了上述10种金属元素的质量浓度.结果表明,PM_(2.5)和PM_(10)的年均质量浓度分别为153.40μg·m^(-3)和232.93μg·m^(-3),超出GB 3095-2012中二类环境功能区标准限值的5倍和3倍;PM_(2.5)/PM_(10)的均值为0.74,表明大气颗粒物中以粒径小于2.5μm的颗粒为主;后向轨迹分析结果表明外源颗粒物的来向随季节变化而改变,冬、春、夏、秋季主要来向为西北、北-东北、东南、东南-西北.PM_(2.5)和PM_(10)中10种元素的年均质量浓度从高到低依次为Ti>Mn>Pb>Cu>Cr>Ni>V>Cd>Mo>Co,其中Ti、Mn、Pb、Cu和Cr这5种元素占10种目标元素总质量浓度的91.93%和92.49%.除PM_(10)中Cd年均质量浓度(6.53 ng·m^(-3))高于GB 3095-2012限定值(5.00 ng·m^(-3))外,其他元素的质量浓度均不超标.降尘中各元素的含量由高到低依次为Ti>Mn>Pb>Cu>Ni>Cr>V>Co>Mo>Cd,Ti(2561.48μg·g^(-1))占所有元素的质量分数为72.57%,地累积指数(Igeo)结果表明,Cd(4.03)属重度污染,Pb(2.49)介于中度污染和重度污染之间,Cu(1.33)属中度污染,Ni(0.43)属轻微污染.重金属的致癌健康风险(<10-4)和非致癌健康风险(<1),均处于较低水平,短期内不会对人体健康造成威胁,但不能忽视长期处于此环境所带来的健康危害.

关键词：大气颗粒物降尘重金属分布特征健康风险

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健康监测系统数据的信息提取——利用挠度和应变监测值估算通行荷载重量

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桥梁建设 2009年第3期39卷 77-80页

作者：曹映泓李健梁勇周颖广东省路桥建设发展有限公司广东广州510635 广东省建筑科学研究院广东广州510500 湛江海湾大桥有限公司广东湛江524057 华南理工大学交通学院广东广州510400

结构健康监测系统是利用先进技术保障结构运营安全的新兴技术。目前已被学术界和工程界广泛接受和使用。然而,如何充分挖掘监测数据中包含的重要信息,充分发挥健康监测系统的功能并未受到足够重视。以湛江海湾大桥健康监测系统为工程背... 详细信息

结构健康监测系统是利用先进技术保障结构运营安全的新兴技术。目前已被学术界和工程界广泛接受和使用。然而,如何充分挖掘监测数据中包含的重要信息,充分发挥健康监测系统的功能并未受到足够重视。以湛江海湾大桥健康监测系统为工程背景,利用挠度和应变监测值估算通行荷载的重量。除方法本身之外,该研究能够体现监测数据的重要性,激发更多的充分利用健康监测系统监测数据、拓展健康监测系统功能的新思路、新方法。

关键词：结构健康监测超重车辆 GPS系统

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Preparation of Environmentally Friendly Urea-Hexanediamine-Glyoxal(HUG)Resin Wood Adhesive

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Journal of Renewable Materials 2024年第2期12卷 235-244页

作者： Qianyu Zhang Shi Chen Long cao hong Lei Antonio Pizzi Xuedong Xi Guanben Du Yunnan Key Laboratory of Wood Adhesives and Glue Products College of Material Science and EngineeringSouthwest Forestry UniversityKunming650224China International Joint Research Center for Biomass Materials Southwest Forestry UniversityKunming650224China College of Chemical and Materials Engineering Zhejiang A&F UniversityHangzhou311300China LERMAB University of LorraineEpinal88000France

Using non-toxic,low-volatile glyoxal to completely replace formaldehyde for preparing urea-glyoxal(UG)resin adhesive is a hot research topic that could be of great interest for the wood ***,urea-glyoxal(UG)resins prepared by just using glyoxal instead of formaldehyde usually yields a lower degree of *** results in a poorer bonding performance and water resistance of UG resins.A good solution is to pre-react urea to preform polyurea molecules presenting already a certain degree of polymerization,and then to condense these with glyoxal to obtain a novel UG ***,in this present work,the urea was reacted with hexamethylene diamine to form a polyurea named HU,and then this was used to react it with different amounts of glyoxal to synthesize hexamethylenediamine-urea-glyoxal(HUG)polycondensation resins,and to use this for bonding *** results show that the glyoxal can well react with HU polyuria via addition and schiff base reaction,and also the HUG resin exhibits excellent bonding strength and water *** shear strength of the plywood bonded with this HUG at 160°C hot press temperature as high as 1.93 MPa,2.16 MPa and 1.61 MPa,respectively,which meets the requirement of the China national standard GB/T 9846-2015(≥0.7 MPa),and can be a good choice as a wood adhesive for industrial application.

关键词： Urea-glyoxal resin hexamethylene diamine wood adhesives water resistance

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Performance Characterization of CR/PU Asphalt for Potential Application in Assembled Fast-Repairing Engineering

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Fluid Dynamics & Materials Processing 2024年第5期20卷 1063-1074页

作者： hong Pang Ao Lu Ming Xiong Chen Chen Xian cao Xiong Xu Jing Wang Hubei Regional Management Headquarters CCCC Asset Management Co.Ltd.Beijing101399China School of Civil Engineering and Architecture Wuhan Institute of TechnologyWuhan430073China Hubei Provincial Engineering Research Center for Green Civil Engineering Materials and Structures Wuhan Institute of TechnologyWuhan430073China

Conventional repairing methods for asphalt pavement have some inconveniences,such as insufficient strength,and are typically *** address these issues,this study proposes a new technological method to design and prepare a high-performance assembled asphalt concrete block for fast repair of the potholes.A series of composite modified asphalt binders with 10%crumb rubber(CR)and different dosages(0%,1%,3%,5%)of polyurethane(PU)are examined to determine the optimized ***,the corresponding asphalt mixtures are prepared for further comparison and assessment of engineering properties,such as moistureinduced damage,high-temperature deformation,and low-temperature cracking *** test results show that PU can significantly improve the high-temperature performance and hardness of(crumb rubber modified asphalt)CRMA binder;3%PU contributes allowing the resistance of CRMA mixture to moisture-induced damage at higher levels,particularly under water whole immersion;as 3%PU is added,the high-temperature rutting deformation resistance of the CRMA mixture increases significantly,and the low-temperature anti-cracking properties are also improved ***,the innovatively designed high-quality assembled fast-repairing asphalt concrete block is recommended as an appropriate option for highway maintenance.

关键词： Composite modified asphalt crumb rubber polyurethane assembled fast-repairing asphalt concrete maintenance engineering

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