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Exploring one material for dual applications:A red-emitting Mg2GeO4:Eu3+ nanophosphor for future generation energy efficient WLEDs and dosimetric applications

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Journal of Rare Earths 2024年第10期42卷 1835-1845页

作者： Akshay Arjun G.P.Darshan S.c.Sharma H.Nagabhushana D.V.Sunitha H.B.Premkumar Department of Physics Faculty of Mathematical and Physical SciencesM.S.Ramaiah University of Applied Sciences Jain University c.N.R.Rao centre for Advanced Materials Tumkur University School of Applied Sciences (Physics) REVA University

The envisaged design and developme nt of individual mate rials to excavate a broader spectrum of desired properties and offer multiple applications are highly *** this in mind,a series of forsterite-structured Mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors was synthesized via a solution combustion method using oxalyl dihydrazide as a *** x-ray diffraction patterns confirm the orthorhombic crystal system with a Puma space *** results clearly show irregularly shaped cluster-like structures with aggregation of the *** diffuse reflectance spectra,the optical energy band gap of the Mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors was estimated and obtained to be～4.12-4.32 *** photoluminescence emission spectra exhibit intense peaks at ～579,589,610,661,and 707 nm,which are due to characteristic5D0→7F0,5D0→7F1,5Do→7F2,5D0→7F3and5D0→7F4transitions of Eu3+ions,*** commission International de L'Eclairage color coordinates are gradually tuned from pale red（0.5980,0.4012） to a pure red（0.6385,0.3611） *** glow peaks showcase excellent super-linear response at low doses of γ-irradiations,indicating that the prepared phosphor can be used in thermoluminescent personal dosimetry which is a biological tissue *** aforementioned results demonstrate that the prepared Mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors are considered an excellent candidate for dual applications,i.e.,red component in future generation white-light-emitting diodes（WLEDs） and personal dosimetric applications.

关键词： Dosimetry Nanophosphors Photoluminescence Photometric properties Rare earths Thermoluminescence

Enhancing visible-light-driven NO oxidation through molecular‐level insights of dye-loaded sea sands

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Rare Metals 2024年第2期43卷 543-554页

作者： Yu-Han Li Bang-Fu chen Sónia A.c.carabineiro You-Yu Duan Ping Tan Wing-Kei Ho Fan Dong Engineering Research center for Waste Oil Recovery Technology and Equipment Ministry of EducationChongqing Key Laboratory of Catalysis and New Environmental MaterialsChongqing Technology and Business UniversityChongqing400067China Nanchang Institute of Technology Nanchang33044China LAQV-REQUIMTE Department of ChemistryNOVA School of Science and TechnologyUniversidade NOVA de Lisboa2829-516CaparicaPortugal college of Physics and center of Quantum Materials and Devices Chongqing UniversityChongqing401331China Department of Science and Environmental Studies The Education University of Hong KongHong Kong999077China

Natural minerals,abundant and easily obtained through simple physical processing,offer a cost-effective and environmentally friendly solution for dyeing wastewater disposal and air pollution *** study investigates the photocatalytic removal of NO using natural different types of dyes,loaded on natural sand,under visible light *** examining various coating concentrations of dyes and sand weights,we discovered that sand loaded with Rhodamine B(RhB)exhibits high activity for the photo-oxidation of NO.A combination results of x-ray diffraction(xRD),x-ray photoelectron spectroscopy(xPS),Fourier transform infrared spectroscopy(FTIR)and thermogravimetric(TG)analyses confirm the presence of SiO_(2),cacO_(3),Al_(2)O_(3)and iron oxides as the main components of the ***,studying RhB-loaded individual components reveals that cacO_(3)plays a crucial role in enhancing the NO removal *** results and theoretical calculations demonstrate the establishment of a directional charge transfer channel from cacO_(3)to RhB,facilitating the adsorption and activation of molecular NO and O_(2).This work not only promotes the utilization of natural mineral resources but also enriches the fields of environmental photochemistry and semiconductor photocatalysis.

关键词： Sand dyes Rhodamine B Photo-oxidation of NO Visible light illumination

Limit of Spectral Resolution in Terahertz Time—Domain Spectroscopy

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chinese Physics Letters 2003年第8期20卷 1266-1268页

作者： Jingzhouxu TaoYuan SamuelMickan x.-c.Zhang centerforTHzResearch RensselaerPolytechnicInstituteTroyNY12180USA

The pulsed nature of terahertz time-domain spectroscopy (THz-TDS) sets a fundamental limit on its spectral resolution. The spectral resolution of THz-TDS can be improved by increasing the duration of the temporal measurement, but is limited by the dynamic range of the system in the time domain. This paper presents calculations and experimental results relating the temporal dynamic range of a THz-TDS system to its spectral resolution. We discuss three typical terahertz sources in terms of their dynamic range and hence achievable spectral resolution.

关键词： Terahertz spectroscopy

Planning and control of cOP-Switch-Based Planar Biped Walking

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Journal of Bionic Engineering 2011年第1期8卷 33-48页

作者： x. Luo W. Li c. Zhu School of Mechanical Engineering Southeast University Nanjing 210018 P. R. China Department of Systems Life Engineering Maebashi Institute of Technology Gunma Prefecture 371-0816 Japan

Efficient walking is one of the main goals of researches on biped robots. A feasible way is to translate the understanding from human walking into robot walking, for example, an artificial control approach on a human like walking structure. In this paper, a walking pattern based on center of Pressure （cOP） switched and modeled after human walking is introduced firstly. Then, a parameterization method for the proposed walking gait is presented. In view of the complication, a multi-space planning method which divides the whole planning task into three sub-spaces, including simplified model space, work space and joint space, is proposed. Furthermore, a finite-state-based control method is also developed to implement the proposed walking pattern. The state switches of this method are driven by sensor events. For convincing verification, a 2D simulation system with a 9-1ink planar biped robot is developed. The simulation results exhibit an efficient walking gait.

关键词： biped walking bio-inspired cOP switch control multi-space planning simulation

Morphology control and Optical Absorption Properties of Ag Nanoparticles by Ion Implantation

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Journal of Materials Science & Technology 2009年第5期25卷 669-672页

作者： G.x. cai F. Ren x.H. xiao L.x. Fan x.D. Zhou c.Z. Jiang Key Laboratory of Acoustic and Photonie Materials and Devices of Ministry of Education Wuhan University Wuhan 430072 China

Ion implantation is a powerful method for fabricating nanoparticles in dielectric. For the actual application of nanoparticle composites, a careful control of nanoparticles has to be achieved. In this letter, the size, distribution and morphology of Ag nanoparticles are controlled by controlling the ion current density, ion implantation sequence and ion irradiation dose. Single layer Ag nanoparticles are formed by Ag^＋ ion implantation at current density of 2.5 μ^A/cm2. By Ag and cu ions sequential implantation, the size of single layer Ag nanoparticles increases. While, by cu and Ag ions sequential implantation, uniform Ag nanoparticles with wide distribution are formed. The morphology of Ag nanoparticles changes to hollow and sandwiched nanoparticles by cu^＋ ion irradiation to doses of 3×10^16 and 5×10^16 ions/cm^2. The optical absorption properties of Ag nanoparticles are also tailored by these ways.

关键词： Nanoparticles Ion implantation Transmission electron microscopy

Mechanical Properties and Defective Effects of 316LN Stainless Steel by First-Principles Simulations

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Journal of Materials Science & Technology 2011年第11期27卷 1029-1033页

作者： x.Q. Li J.J. Zhao J.c. xu x. Liu Key Laboratory of Materials Modification by Laser Ion and Electron Beams Ministry of Education Dalian University of Technology Dalian 116024 China college of Advanced Science and Technology Dalian University of Technology Dalian 116024 China School of chemical Engineering Dalian University of Technology Dalian 116024 China

In current International Thermonuclear Experimental Reactor （ITER） design, the 316LN austenitic stainless steel （316LN SS） is used for first-wall/blanket structures. Thus, it is necessary to study the fundamental mechanical properties and irradiation effect of 316LN SS. A random solid solution model of Fe-cr-Ni-Mn- Mo-Si alloy is used for describing 310LN S$. Using first-principles approaches, the elastic constants and ideal strength of the alloy were calculated. Such alloy exhibits good ductile behavior according to the theoretical values of cauchy pressure and ratio of bulk modulus and shear modulus. Within the 256-atom supercell, inclusion of single vacancy defect further enhances the ductility of the alloy, and the existence of interstitial （Fe, H, He） atoms enhances the Young＇s modulus.

关键词： Stainless steel Mechanical properties Vacancy Interstitial

Electrically conductive Honeycomb Monolith of Nanolaminated Ti_3Alc_2:Preparation and characterization

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Journal of Materials Science & Technology 2015年第1期31卷 125-128页

作者： x.M.Fang x.H.Wang H.Zhang Y.c.Zhou Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of Sciences University of chinese Academy of Sciences Science and Technology of Advanced Functional composite Laboratory ARIMPT

Nanolaminated Ti3Alc2honeycomb monolith with parallel and uniform holes has been prepared through a facile extrusion route by using Ti3Alc2powder as the main raw *** fabricated honeycomb monolith has high compressive strength of 133 ± 11 and 59 ± 9 MPa,along and perpendicular to the extrusion direction,*** also has good electrical conductivity,and excellent match of thermal expansion coefficient with the washcoat material of γ-*** combined properties endow the honeycomb monolith a promising candidate as catalysis substrate for cleaning vehicle exhaust.

关键词： Honeycomb ceramic Ti3Alc2 Extrusion catalysis

Recent experimental progress of fractional quantum Hall effect: 5/2 illing state and graphene

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National Science Review 2014年第4期1卷 564-579页

作者： x.Lin R.R.Du x.c.x.e International center for Quantum Materials Peking University

The phenomenon of fractional quantum Hall efect(FQHE)was irst experimentally observed 33 years *** involves strong coulomb interactions and correlations among the electrons,which leads to quasiparticles with fractional elementary *** decades later,the ield of FQHE is still active with new discoveries and new technical developments.A signiicant portion of atention in FQHE has been dedicated to illing factor 5/2 state,for its unusual even denominator and possible application in topological quantum ***,FQHE has been observed in high-mobility Ga As heterostructure,but new materials such as graphene also open up a new area for *** review focuses on recent progress of FQHE at 5/2 state and FQHE in graphene.

关键词： fractional quantum Hall efect experimental progress 5/2 state graphene

On the spray drying of uniform functional microparticles

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Particuology 2015年第5期13卷 1-12页

作者： W.Liu x.D.chen c.Selomulya Department of chemical Engineering Monash University18 Alliance LaneClayton 3800VICAustralia Department of Pharmaceutics School of Pharmaceutical SciencesCentral South University School of chemical and Environmental Engineering Soochow UniversitySuzhou Industrial Park

Spray drying is a typical method to produce particles in dry powder forms at industrial scale. Most spray-dried products often show a wide range of particle properties even within the same batch. At Monash University, we utilise a microfluidic spray drying approach to generate uniform microparticles with tightly controlled characteristics and sizes in a scalable, almost waste-flee process. The technique is useful to correlate the effects of formulation and spray drying conditions on the properties of spray-dried particles, and can be used to test new formulations for targeted applications such as encapsulation and release of active ingredients. The synthesis route can be applied to other self-assembling systems, includ- ing mesoporous, crystalline, and hierarchically structured microparticles. As spray drying is commonly used in commercial scales, the understanding of how functional particles are formed in relation to formulations and process conditions could assist in developing a cost effective, energy and material-efficient route to produce powders with better properties and ease of handling for more advanced applications such as selective adsorption and bio-separation.

关键词： Microfluidic spray drying Uniform microparticles Encapsulation controlled release