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Monolayer Graphitic carbon Nitride as Metal-Free catalyst with Enhanced Performance in Photo- and Electro-catalysis

Nano-Micro letters 2022年第3期14卷 308-321页

作者： Huiyan Piao Goeun choi Xiaoyan Jin Seong‑Ju Hwang Young Jae Song Sung‑Pyo cho Jin‑Ho choy Intelligent Nanohybrid Materials laboratory(INMl) Institute of Tissue Regeneration Engineering(ITREN)Dankook UniversityCheonan 31116Republic of Korea college of Science and Technology Dankook UniversityCheonan 31116Republic of Korea Department of Nanobiomedical Science and BK21 PlUS NBM Global Research center for Regenerative Medicine Dankook UniversityCheonan 31116Republic of Korea Department of Materials Science and Engineering College of EngineeringYonsei UniversitySeoul 03722Republic of Korea SKKU Advanced Institute of Nanotechnology(SAINT) Sungkyunkwan University(SKKU)Suwon 440‑746Republic of Korea Department of Nano Engineering Sungkyunkwan University(SKKU)Suwon 440‑746Republic of Korea National center for Inter‑University Research Facilities(NcIRF) Seoul National UniversitySeoul 08826Republic of Korea Graphene Research center Advanced Institute of Convergence TechnologySuwon 16229Republic of Korea Department of Pre‑Medical course College of MedicineDankook UniversityCheonan 31116Republic of Korea Tokyo Tech World Research Hub Initiative(WRHI) Institute of Innovative ResearchTokyo Institute of TechnologyYokohama 226‑8503Japan

The exfoliation of bulk graphitic carbon nitride(g-c_(3)N_(4))into monolayer has been intensively studied to induce maximum sur-face area for fundamental studies,but ended in failure to realize chemi-cally and physically well-defined monolayer of g-c_(3)N_(4)mostly due to the difficulty in reducing the layer thickness down to an atomic *** has,therefore,remained as a challenging issue in two-dimensional(2D)chemistry and physics *** this study,an“atomic monolayer of g-c_(3)N_(4)with perfect two-dimensional limit”was successfully prepared by the chemically well-defined two-step *** atomically resolved monolayer of g-c_(3)N_(4)was also confirmed by spectroscopic and micro-scopic *** addition,the experimental cs-HRTEM image was collected,for the first time,which was in excellent agreement with the theoretically simulated;the evidence of monolayer of g-c_(3)N_(4)in the perfect 2D limit becomes now clear from the HRTEM image of orderly hexagonal symmetry with a cavity formed by encirclement of three adjacent heptazine *** to bulk g-c_(3)N_(4),the present g-c_(3)N_(4)monolayer showed significantly higher photocatalytic gen-eration of H2O2 and H2,and electrocatalytic oxygen reduction *** addition,its photocatalytic efficiency for H2O2 production was found to be the best for any known g-c_(3)N_(4)nanomaterials,underscoring the remarkable advantage of monolayer formation in optimizing the catalyst performance of g-c_(3)N_(4).

关键词： Graphitic carbon nitride Monolayer Atomic image Electro-and photo-catalysis

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Plausible cloth animation using dynamic bending model

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Progress in Natural Science:Materials International 2008年第7期18卷 879-885页

作者： charlie c.l. Wang Department of Mechanical and Automation Engineering The chinese University of Hong Kong Hong Kong china

Simulating the mechanical behavior of a cloth is a very challenging and important problem in computer animation. The models of bending in most existing cloth simulation approaches are taking the assumption that the cloth is little deformed from a plate shape. Therefore, based on the thin-plate theory, these bending models do not consider the condition that the current shape of the cloth under large deformations cannot be regarded as the approximation to that before deformation, which leads to an unreal static bending. [This paper introduces a dynamic bending model which is appropriate to describe large out-plane deformations such as cloth buckling and bending, and develops a compact implementation of the new model on spring-mass systems. Experimental results show that wrinkles and folds generated using this technique in cloth simulation, can appear and vanish in a more natural way than other approaches.]

关键词： cloth animation Physically based animation Bending

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Effect of radiative loss mechanisms on FIR thermometric parameters of Nd^(3+)-doped lithium tellurite glasses

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Journal of Rare Earths 2024年第7期42卷 1250-1257,I0002页

作者： c.Y.Morassuti A.P.l Silva l.A.O.Nunes S.M.lima l.H.c.Andrade Optical and Photothermal Spectroscopy Group(GEOF) Center for Studies in Natural Resources(CERNA)State University of Mato Grosso do Sul(UEMS)C.P.351DouradosMSBrazil Renato Archer Information Technology center Dom Pedro I Highway(SP-65)Km 1436-Chácaras Campos dos AmaraisCampinasSPBrazil Institute of Physics of São carlos University of São PauloSão CarlosSPBrazil

Nd^(3+)-doped tellurite glasses are promising materials for thermometers based on the fluorescence intensity ratio(FIR)***,at high Nd^(3+)concentrations,energy transfer(ET)processes such as optical reabsorption and cross-relaxation can affect the Nd^(3+)emission,which has been little explored in the ***,the present work investigated the use of Nd^(3+)-doped tellurite glass(samples doped with Nd^(3+)at 0.2 mol%,0.5 mol%,2.0 mol%,and 4.0 mol%)in fluorescence thermometers,in the temperature range from 299 to 371 *** results indicate a strong dependence of the FIR parameters on the Nd^(3+)concentration,due to changes in the emission band profiles caused by optical reabsorption of the Nd^(3+)emissions and cross-relaxation processes.A decrease of the relative sensitivity of the ratio^(4)F_(5/2)→^(4)I_(9/2)/^(4)F_(3/2)→^(4)I_(9/2)is observed for samples doped with higher amounts of Nd^(3+).The maximum relative sensitivity at 299 K is 3.00%/K,which is the highest value among the reported Nd^(3+)ions.

关键词： Nd^(3+)-doped tellurite glass Fluorescence intensity ratio Optical thermometry Judd-Ofelt Rare earths

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Study on International Standard Multilingual Nomenclature of chinese Medicine

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chinese Journal of Integrative Medicine 2010年第2期16卷 176-179页

作者：王奎刘路李蔚史大卓曾文颖朱勉生 Angles Michel Attali Jean-Raymond Pedro choy Joao choy WU chi-haur 翟扶汉 Ramon Maria calduch 钟清 Translation Department World Federation of Chinese Medicine Societies Xiyuan Hospital of china Academy of chinese Medical Sciences ISN French Editorial Board(Paris) ISN Portuguese Editorial Board(lisbon) ISN Spanish Editorial Board(Madrid)

The International Standard chinese-English Basic Nomenclature of chinese medicine（ISN） was released in 2007,a nomenclature list consisting of 6 500 chinese medical *** was the culmination of several years of collaborative diligent work of over 200 specialists who represent chinese medicine in 68 *** overall goal for devising standard English nomenclature for chinese medicine is to develop a practical international standard nomenclature for chinese medical basic terms,to make it compatible with contemporary research and educational standards in the globalized health care *** this article,provided is an overview of principles and methods for the multilingual translations,the processes behind the particular content of the chinese-English ISN and an introduction to the ongoing new projects,*** multilingual versions of ISN（International Standards of chinese-Spanish,chinese-French and chinese-Portuguese Basic Nomenclature of chinese Medicine）.

关键词： international standard nomenclature (ISN) chinese medicine translating principles translating methods multilingual standards

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3D FINITE ElEMENT ANAlYSIS OF THE DAMAGE EFFEcTS ON THE DENTAl cOMPOSITE SUBJEcT TO WATER SORPTION

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Acta Mechanica Solida Sinica 2006年第3期19卷 212-222页

作者： Tsui c.P. chow c.l. Department of Industrial and Systems Engineering The Hong Kong Polytechnic University Hong Kong ChinaDepartment of Mechanical EngineeringThe University of Michigan-DearbornDearbornMichiganUSA

The damage effects of water sorption on the mechanical properties of the hydroxyapatite particle reinforced Bis-GMA/TEGDMA copolymer （HA/Bis-GMA/TEGDMA） h-ave been predicted using 3D finite cell models. The plasticizer effect on the polymer matrix was considered as a variation of its Young＇s modulus. Three different cell models were used to determine the influence of varying particle contents, interphase strength and moisture concentration on the debonding damage. The stress distribution pattern has been examined and the stress transfer mode clarified. The Young＇s modulus and fracture strength of the Bis-GMA/TEGDMA composite were also predicted using the model with and without consideration of the damage. ine Iormer results with consideration of the debonding damage are in good agreement with existing literature experimental data. The shielding effect of our proposed model and an alternative approach were discussed. The Fcc cell model has also been extended to predict the critical load for the damaged and the undamaged composite subject to the 3-point flexural test.

关键词： water sorption dental composite interphase debonding finite element method (FEM) unit cell model

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Activation characteristics of candidate structural materials for a near-term Indian fusion reactor and the impact of their impurities on design considerations

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Plasma Science and Technology 2018年第6期20卷 186-193页

作者： H l SWAMI c DANANI A K SHAW Institute for Plasma Research Gandhinagar Gujarat 382428 India Homi Bhabha National Institute (HBNI) Anushaktinagar Mumbai 400094 India

Activation analyses play a vital role in nuclear reactor *** analyses,along with nuclear analyses,provide important information for nuclear safety and maintenance *** analyses also help in the selection of materials for a nuclear reactor,by providing the radioactivity and dose rate levels after *** information is important to help define maintenance activity for different parts of the reactor,and to plan decommissioning and radioactive waste disposal *** study of activation analyses of candidate structural materials for near-term fusion reactors or ITER is equally essential,due to the presence of a highenergy neutron environment which makes decisive demands on material *** study comprises two parts; in the first part the activation characteristics,in a fusion radiation environment,of several elements which are widely present in structural materials,are *** reveals that the presence of a few specific elements in a material can diminish its feasibility for use in the nuclear *** second part of the study concentrates on activation analyses of candidate structural materials for near-term fusion reactors and their comparison in fusion radiation *** structural materials selected for this study,***-specific Reduced Activation Ferritic-Martensitic steel（IN-RAFMS）,P91-grade steel,stainless steel 316 lN ITER-grade（SS-316 lN-IG）,stainless steel 316 l and stainless steel 304,are candidates for use in ITER either in vessel components or test blanket *** is also included in this study because of its use for ITER plasma-facing *** study is carried out using the reference parameters of the ITER fusion *** activation characteristics of the materials are assessed considering the irradiation at an ITER equatorial *** presence of elements like Nb,Mo,co and Ta in a structural material enhance the activity level as well as the dose level,which has an

关键词： activation EASY nuclear safety fusion reactor structural materials

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A functional tacrolimus-releasing nerve wrap for enhancing nerve regeneration following surgical nerve repair

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Neural Regeneration Research 2025年第1期20卷 291-304页

作者： Simeon c.Daeschler Katelyn J.W.So Konstantin Feinberg Marina Manoraj Jenny cheung Jennifer Zhang Kaveh Mirmoeini JPaul Santerre Tessa Gordon Gregory HBorschel SickKids Research Institute Neuroscience and Mental Health ProgramTorontoONCanada Institute of Biomaterials and Biomedical Engineering University of TorontoTorontoONCanada Indiana University School of Medicine IndianapolisINUSA Division of Plastic and Reconstructive Surgery the Hospital for Sick ChildrenTorontoONCanada Translational Biology and Engineering Program Ted Rogers Centre for Heart ResearchInstitute of Biomedical EngineeringFaculty of DentistryUniversity of TorontoTorontoONCanada

Axonal regeneration following surgical nerve repair is slow and often incomplete,resulting in poor functional recovery which sometimes contributes to lifelong ***,there are no FDA-approved therapies available to promote nerve *** accelerates axonal regeneration,but systemic side effects presently outweigh its potential benefits for peripheral nerve *** authors describe herein a biodegradable polyurethane-based drug delivery system for the sustained local release of tacrolimus at the nerve repair site,with suitable properties for scalable production and clinical application,aiming to promote nerve regeneration and functional recovery with minimal systemic drug *** is encapsulated into co-axially electrospun polycarbonate-urethane nanofibers to generate an implantable nerve wrap that releases therapeutic doses of bioactive tacrolimus over 31 *** and drug loading are adjustable for applications in small and large caliber nerves,and the wrap degrades within 120 days into biocompatible *** released from the nerve wrap promotes axon elongation in vitro and accelerates nerve regeneration and functional recovery in preclinical nerve repair models while off-target systemic drug exposure is reduced by 80%compared with systemic *** its surgical suitability and preclinical efficacy and safety,this system may provide a readily translatable approach to support axonal regeneration and recovery in patients undergoing nerve surgery.

关键词： biodegradable local drug delivery nerve injury nerve regeneration nerve wrap tacrolimus

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Synergistic Multilayer Adsorption for low concentration Dyestuffs by Biomass

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chinese Journal of chemical Engineering 2012年第3期20卷 560-566页

作者： Keith Kim Hung choy Gordon Mckay Department of chemical and Biomolecular Engineering the Hong Kong University of Science and TechnologyHong KongChina

Due to the high cost of adsorbents and their thermal regeneration in recent years, much research has fo- cused on the search for cheaper adsorbents for treating wastewater from textile industry. The single component ad-sorption of an acidic dye, Acid Yellow 117, and a basic dye, Methylene Blue, onto several adsoroents-bamooo, waste wood, bamboo char, waste wood char, bamboo activated carbon, wood activated carbon and active carbon F400 were conducted. Based on a langmuir analysis, the monolayer adsorption capacities were determined. Three of the adsorbents were selected for binary layer adsorption to check the multilayer concept and the potential application for better adsorbent usage. The two cheapest adsorbents, bamboo and wood are compared with the commer-cial activated carbon F400, and all three systems were successful.

关键词： multilayer adsorption biomass dyestuffs

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Experimental investigation of hypersonic flight-duplicated shock tunnel characteristics

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Acta Mechanica Sinica 2021年第3期37卷 422-433,I0002页

作者： c K.Yuan Z.l.Jiang Institute of Mechanics Chinese Academy of SciencesBeijing 100190China University of chinese Academy of Sciences Beijing 100190China

Hypersonic air-breathing propulsion is one of the key techniques for future aviation and the ground aerodynamic testing for full scale test models with sufficient test time at flight conditions is of fundamental importance for verifying hypersonic air-breathing *** on the backward detonation-driven concept,the hypersonic flight-duplicated shock tunnel(or JF-12 shock tunnel)has been successfully constructed and *** facility is capable of reproducing airflow for Mach numbers ranging from 5 to 9 at an altitude of 25-50 km,with a test duration of more than 100 *** quantify the performance of the shock tunnel,experiments were conducted to investigate the aerodynamic characteristics of the test flows and the effects of several critical techniques that play important roles in the operation of the shock *** stagnation pressure was constant within士5%and the average stagnation pressure varied by less than 0.048%/*** variation of the stagnation pressure in repeated experiments is less than 2.0%,indicating the good repeatability of the wind *** non-uniformity of the Mach number in the core flow field at the nozzle exit was within士2.5%.Additional,a uniform flow field is established upstream of the nozzle *** axial gradients of the flow field are small since the Mach number varies less than 1.7%/*** regarding the ignition technology,diaphragm ruptures,detonation driver capacity,incident shock-wave decay,and tunnel operation mode are also *** findings of this study are not only helpful for operating the shock tunnel,but can also assist the future development of hypersonic wind tunnels.

关键词： Hypersonics Shock tunnels Flow characteristics

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Nonaqueous potassium-ion full-cells:Mapping the progress and identifying missing puzzle pieces

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Journal of Energy chemistry 2024年第6期93卷 384-399,I0010页

作者： Badre larhrib louiza larbi lénaïc Madec Universite de Pau et des Pays de l’Adour E2S UPPACNRSIPREMPauFrance Universitéde Haute-Alsace Institut de Science des Matériaux de Mulhouse(IS2M)CNRS UMR 7361F-68100 MulhouseFrance Universitéde Strasbourg F-67081 StrasbourgFrance Réseau sur le Stockage Electrochimique de l’Energie CNRS FR3459AmiensFrance Institut des Matériaux Jean Rouxel(IMN) CNRS UMR 6502Univ.Nantes44322 Cedex 3 NantesFrance

This review addresses the growing interest for potassium-ion full-cells(KIFcs)in view of the transition from potassium-ion half-cells(KIHcs)toward commercial K-ion batteries(KIBs).It focuses on the key parameters of KIFcs such as the electrode/electrolyte interfaces challenge,major barriers,and recent advancements in *** strategies for enhancing KIFc performance,including interfaces co ntrol,electrolyte optimization,electrodes capacity ratio,electrode material screening and electrode design,are *** review highlights the need to evaluate KIBs in full-cell configurations as half-cell results are strongly impacted by the K metal *** also emphasizes the importance of understanding solid electrolyte interphase(SEI)formation in KIFcs and explores promising nonaqueous as well as quasiand all-solid-state electrolytes *** review thus paves the way for practical,cost-effective,and scalable KIBs as energy storage systems by offering insights and guidance for future research.

关键词： K-ion full-cells Potassium-ion batteries cross-talk Solid-state batteries Potassium reactivity Electrolyte design Electrode design

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