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seasonal c.a.ges in Hermit Thrush (catharus guttatus) song syntax

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Avian Research 2024年第2期15卷 172-179页

作者： sean p.Roach Luke c.McLean Jeff W.MacLeod Leslie s.phillmore psychology Department University of New Brunswick Saint John100 Tucker Park RoadSaint JohnNBCanada Department of psychology and Neuroscience Dalhousie University1355 Oxford StHalifaxNSB3H 4J1Canada

In many songbird species,birdsong features phonological syntax,meaning that the units within their vocal se-quences are ordered in a non-random way that adheres to a *** such syntactical patterns have been richly described in many species,comparatively little is known about how those patterns contribute to song achieving its important *** each of song’s main functions,territorial defense and mate attraction,evidence of a role for syntax is *** species for which syntax has been thoroughly described is the Hermit Thrush(catharus guttatus),which presents song types from their repertoires in a semi-predic.a.le order and,in doing so,rapidly cycle up and down the frequency *** objective of the present study was to explore the importance of song syntax in the Hermit Thrush through a within-subject examination of how measures of syntax,such as the predic.a.ility of song type order within song sequences,shift over the breeding *** hypothesized that,if such syntactical c.a.acteristics are important to breeding behaviour,they would be most prominent at the start of the breeding season when activity assoc.a.ed with territory establishment and mate attraction is most *** revealed that,as predicted,the rigidness of song type ordering within se-quences was highest at the start of the season and declined *** song type sequences were most predic.a.le at the vitally important early part of the breeding season fit our hypothesis that this aspect of song syntax is important to song’s functions related to territory establishment and/or mate *** work will c.a.ify whether that role relates to one of song’s two main functions or serves song transmission in some broader way.

关键词： Birdsong Hermit Thrush seasonal c.a.ge stereotypy syntax

Bile acid signaling in the regulation of whole body metabolic.a.d immunological homeostasis

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science china(Life sciences) 2024年第5期67卷 865-878页

作者： Wei Jia Yitao Li Kenneth c.p.cheung Xiaojiao Zheng school of chinese Medicine Hong Kong Baptist UniversityHong KongChina center for Translational Medicine and shanghai Key Laboratory of Diabetes Mellitus Shanghai Sixth People's Hospital Affiliated to Shanghai JiaoTong University School of MedicineShanghai 200233China

Bile acids(BAs)play a cruc.a. role in nutrient absorption and act as key regulators of lipid and glucose metabolism and immune *** the enterohepatic circulation,BAs are synthesized,metabolized,and reabsorbed,with a portion entering the vascular circulation and distributing *** allows BAs to interact with receptors in all major organs,leading to organ-organ interactions that regulate both local and global metabolic processes,as well as the immune *** review focuses on the whole-body effects of BA-mediated metabolic.a.d immunological regulation,including in the brain,heart,liver,intestine,eyes,skin,adipose tissue,and *** BA synthesis and receptor signaling is a promising strategy for the development of novel therapies for various diseases throughout the body.

关键词： bile acid whole body metabolism immunity

Magnesium oxide(MgO)nanoadsorbents in wastewater treatment:A comprehensive review

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Journal of Magnesium and Alloys 2024年第5期12卷 1709-1773页

作者： H.c.s.perera V.Gurunanthanan Anoop singh M.M.M.G.p.G.Mantilaka G.Das sandeep Arya Department of physics Khalifa UniversityAbu Dhabi12788United Arab Emirates postgraduate Institute of science University of PeradeniyaPeradeniyaSri Lanka Department of Humanities and sciences Guru Nanak Institutions Technical CampusIbrahimpatnamHyderabad501506India centre for Global Health Research Saveetha Medical College and HospitalsSaveetha Institute of Medical and Technical SciencesChennai602105Tamil NaduIndia Department of physics University of JammuJammu and Kashmir180006India

Wastewater contamination by heavy metals and synthetic dyes presents a significant environmental c.a.lenge,necessitating effective and sustainable separation *** review article provides a detailed examination of magnesium oxide(MgO)nanoparticles as an innovative nanoadsorbent for wastewater treatment,with a specific focus on heavy metal and dye *** review comprehensively explores various aspects of MgO nanoparticles,including their structural c.a.acteristics and synthesis *** article delves into the morphology and crystallographic.a.rangement of MgO nanoparticles,offering insights into their structural *** the complexity of adsorption processes,the review identifies and analyzes parameters influencing the adsorption efficiency of MgO nanoparticles,such as temperature,pH,contact time,initial concentration,and co-existing *** interplay between these parameters and the adsorption capability of MgO nanoparticles emphasizes the importance of optimizing operational ***,the review assesses various synthesis methods for MgO nanoparticles,including sol-gel,hydrothermal,precipitation,green synthesis,solvothermal,and template-assisted *** discusses the advantages,limitations,and resulting nanoparticle c.a.acteristics of each method,enabling readers to grasp the implications of synthesis processes on adsorption *** comprehensive review consolidates current insights into the effectiveness of MgO nanoparticles as a potent nanoadsorbent for removing heavy metals and dyes from wastewater covering a wide spectrum of aspects related to MgO ***,there is a need to investigate the use of MgO in the treatment of actual wastewater or river water,in order to leverage its cost-effectiveness and high efficiency for practical water treatment applications in real-time.

关键词： MgO nanoparticles Nanoadsorbent Wastewater treatment Heavy metals Dye separation Adsorption synthesis methods

collisionless shock acceleration of protons in a plasma slab produced in a gas jet by the collision of two laser-driven hydrodynamic shockwaves

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Matter and Radiation at Extremes 2024年第2期9卷 12-25页

作者： J.-R.Marquès L.Lanc.a.p.Loiseau p.Forestier-colleoni M.Tarisien E.Atukpor V.Bagnoud c.Brabetz F.consoli J.Domange F.Hannachi p.Nicolaï M.salvadori B.Zielbauer LULI CNRSÉcole PolytechniqueCEASorbonne UniversitéInstitut Polytechnique de Paris91128 Palaiseau CedexFrance cEA DAMDIF91297 Arpajon CedexFrance Universitéparis-sac.a. CEALMCE91680 Bruyères-le-ChatelFrance cENBG CNRS-IN2P3Universitéde Bordeaux33175 Gradignan CedexFrance GsI Helmholtzzentrum für schwerionenforschung GmbH Planckstraße 164291 DarmstadtGermany University of Darmstadt Schloßgartenstr.764289 DarmstadtGermany ENEA Fusion and Technologies for Nuclear safety Department C.R.FrascatiVia Enrico Fermi 45FrascatiRomeItaly cELIA Universitéde Bordeaux–CNRS–CEA33405 TalenceFrance Universitéparis-sac.a. CEALIDYL91191 Gif-sur-YvetteFrance

We have recently proposed a new technique of plasma tailoring by laser-driven hydrodynamic shockwaves generated on both sides of a gas jet[Marquès et al.,*** 28,023103(2021)].In a continuation of this numerical work,we study experimentally the influence of the tailoring on proton acceleration driven by a high-intensity picosecond laser in three cases:without tailoring,by tailoring only the entrance side of the picosecond laser,and by tailoring both sides of the gas *** tailoring,the acceleration is transverse to the laser axis,with a low-energy exponential spectrum,produced by coulomb *** the front side of the gas jet is tailored,a forward acceleration appears,which is significantly enhanced when both the front and back sides of the plasma are *** forward acceleration produces higher-energy protons,with a peaked spectrum,and is in good agreement with the mec.a.ism of collisionless shock acceleration(c.a..The spatiotemporal evolution of the plasma profile is c.a.acterized by optical shadowgraphy of a probe *** refraction and absorption of this beam are simulated by post-processing 3D hydrodynamic simulations of the plasma *** with the experimental results allows estimation of the thickness and near-critical density of the plasma slab produced by tailoring both sides of the gas *** parameters are in good agreement with those required for c.a.

关键词： acceleration hydrodynamic collision

Radiative decays D*(s)→ D(s)γ in covariant confined quark model

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chinese physics c 2024年第2期48卷 45-56页

作者： c.T.Tran M.A.Ivanov p.santorelli Q.c.Vo Department of physics HCMC University of Technology and EducationVo Van Ngan 1700000 Ho Chi Minh CityVietnam Bogoliubov Laboratory of Theoretical physics Joint Institute for Nuclear Research141980 DubnaRussia Dipartimento di Fisica"E.pancini" Universitàdi Napoli Federico ⅡComplesso Universitario di Monte S.AngeloVia CintiaEdificio 680126 NapoliItaly Istituto Nazionale di Fisica Nucleare Sezione di Napoli80126 NapoliItaly University of science 700000 Ho Chi Minh CityVietnam

Radiative decays D((s))*→D((s))γare revisited in light of new experimental data from the BaBar and BEsⅢ*** radiative couplings gD*Dγencoding nonperturbative QcD effects are calculated in the framework of the covariant confined quark model developed by *** compare our results with other theoretical studies and experimental *** couplings(in GeV-1)|g(D*+D+γ)|=0.45(9)and|g(D*0D0γ)|=1.72(34)calculated in our model agree with the corresponding experimental data|g(D*+D+γ)|=0.47(7)and|g(D*0D0γ)|=1.77(16).The most interesting case is the decay Ds*→Dsγ,for which a recent prediction based on light-cone sum rules at next-to-leading order|gDs*Dsγ|=0.60(19)deviates from the first(and only to date)lattice QcD result|gDs*Dsγ|=0.11(2)at nearly3σ.Our calculation yields|gDs*Dsγ|=0.29(6),which falls somehow between the two mentioned results,although it is larger than those predicted in other studies using quark models or QcD sum rules.

关键词： covariant quark model radiative decay c.a.med meson

A functional gel polymer electrolyte based on pVDF-HFp/gelatin toward dendrite-free lithium metal batteries

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Nano Research 2024年第4期17卷 2790-2799页

作者： Xiaoyi Hu Kangli Liu shijie Zhang Guosheng shao s.Ravi p.silva peng Zhang state center for International cooperation on Designer Low-carbon and Environmental Materials(cDLcEM) School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Zhengzhou Materials Genome Institute(ZMGI) ZhongyuanzhiguXingyang 450100China Nanoelectronics center Advanced Technology InstituteUniversity of SurreyGuildfordGU27XHUK

The leakage of liquid electrolyte and the formation of lithium dendrites pose c.a.lenges to safety and stability of lithium metal batteries(LMBs).The appearance of gel polymer electrolyte(GpE)has obviously improved the safety of traditional ***,the limited inhibition of GpE on lithium dendrites is detrimental to the safety of ***,a kind of poly(vinylidene fluoride-co-hexafluoropropylene)(pVDF-HFp)/gelatin(GN)GpE with high ionic conductivity,high-temperature resistance,and flame-retardancy,was prepared by electrospinning and soaking *** the electrospinning network of pVDF-HFp,its affinity to liquid electrolytes,makes this GpE more benefic.a. to ions transport and the formation of ***,the GN with sol–gel properties,enhances the mec.a.ical property(13.5 Mpa)of HFp-GN ***,X-ray photoelectron spectroscopy(Xps)and density functional theory(DFT)suggest that the attraction of polar groups of GN to Li+can regulate the distribution of Li+and protect Li ***,the application of HFp-GN GpEs to LMBs with cathodes of LiFepO_(4) and LicoO_(2) deliver excellent electrochemical performances:after 300 cycles,the LiFepO_(4)/HFp-GN GpE/Li battery keeps a low capacity decay rate of 0.09%at 5 c.a.ter 400 cycles at 2 c,the LicoO_(2)/HFp-GN GpE/Li cell retains a high capacity retention of 74%.This GpE is demonstrated for the application prospect of safe LMBs.

关键词： poly(vinylidene fluoride-co-hexafluoropropylene)(pVDF-HFp) gelatin polar groups lithium metal battery lithium dendrite

Temperature and structure measurements of heavy-ion-heated diamond using in situ X-ray diagnostics

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Matter and Radiation at Extremes 2024年第4期9卷 80-89页

作者： J.Lutgert p.Hesselbach M.schorner V.Bagnoud R.Belikov p.Drechsel B.Heuser O.sHumphries p.Katrik B.Lindqvist c.Qu R.Redmer D.Riley G.sc.a.mann s.schumacher A.Tauschwitz D.Varentsov K.Weyrich X.Yu B.Zielbauer Zs.Major p.Neumayer D.Kraus Institut fur physik Universitat RostockAlbert-Einstein-Str.2318059 RostockGermany GsI Helmholtzzentrum fur schwerionenforschung Planckstr.164291 DarmstadtGermany Institut für Angewandte physik Goethe-Universität Frankfurt am MainMax-von-Laue-Str.160438 Frankfurt am MainGermany Institut fur Geowissensc.a.ten Goethe-Universitat Frankfurt am MainAltenhoferallee 160438 Frankfurt am MainGermany Helmholtz-Zentrum Dresden-Rossendorf Bautzner Landstr.40001328 DresdenGermany European XFEL GmbH Holzkoppel 422869 SchenefeldGermany centre for plasma physics School of Mathematics and PhysicsQueen’s University BelfastUniversity RoadBelfast BT71NNUnited Kingdom Institut für Kernphysik Technische Universität DarmstadtSchlossgartenstr.964289 DarmstadtGermany state Key Laboratory of Nuclear physics and Technology Institute of Heavy Ion PhysicsPeking UniversityBeijing 100871China Helmholtz Institut Jena Frobelstieg 307743 JenaGermany

We present in situ measurements of spectrally resolved X-ray scattering and X-ray diffraction from monocrystalline diamond samples heatedwith an intense pulse of heavy *** this way,we determine the samples’heating dynamics and their microscopic.a.d macroscopic structuralintegrity over a timespan of several *** the ratio of elastic to inelastic scattering with state-of-the-art density functionaltheory molecular dynamics simulations allows the inference of average temperatures around 1300 K,in agreement with predictions fromstopping power *** simultaneous diffraction measurements show no hints of any volumetric graphitization of the material,butdo indicate the onset of fracture in the diamond *** experiments pave the way for future studies at the Facility for Antiproton andIon Research,where a substantially increased intensity of the heavy ion beam will be available.

关键词： heated intense structure

single atom cu-N-c catalysts for the electro-reduction of cO_(2) to cO assessed by rotating ring-disc electrode

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Journal of Energy chemistry 2024年第1期88卷 169-182,I0004页

作者： s.pérez-Rodríguez M.Gutiérrez-Roa c.Giménez-Rubio D.Ríos-Ruiz p.Arévalo-cid M.V.Martínez-Huerta A.Zitolo M.J.Lázaro D.sebastián Instituto de carboquímica(csIc) Miguel Luesma Castán 450018 ZaragozaSpain Instituto de catálisis y petroleoquímica(csIc) Marie Curie 228049 MadridSpain synchrotron sOLEIL L’Orme des MerisiersDépartementale 12891190France

The electrochemical cO_(2) reduction reaction(cO_(2)RR) to controllable chemicals is considered as a promising pathway to store intermittent renewable energy. Herein, a set of catalysts based on copper-nitrogendoped carbon xerogel(cu-N-c) are successfully developed varying the copper amount and the nature of the copper precursor, for the efficient cO_(2)RR. The electrocatalytic performance of cu-N-c materials is assessed by a rotating ring-disc electrode(RRDE), technique still rarely explored for cO_(2)RR. For comparison, products are also c.a.acterized by online gas chromatography in a H-cell. The as-synthesized cu-Nc catalysts are found to be active and highly cO selective at low overpotentials(from -0.6 to -0.8 V ***) in 0.1 M KHcO_(3), while H_(2) from the competitive water reduction appears at larger overpotentials(-0.9 V vs. RHE). The optimum copper acetate-derived catalyst containing cu-N_(4) moieties exhibits a cO_(2)-to-cO turnover frequency of 997 h^(-1) at -0.9 V vs. RHE with a H_(2)/cO ratio of 1.8. These results demonstrate that RRDE configuration can be used as a feasible approach for identifying electrolysis products from cO_(2)RR.

关键词： cu-N-c carbon xerogel Rotating ring disc electrode carbon dioxide reduction reaction carbon monoxide

Design,synthesis,and Applications of Mesoporous covalent Organic Frameworks

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ccs chemistry 2024年第1期6卷 57-68页

作者： Niyati Arora cassandra flores Milinda c.senarathna christina M.Thompson Ronald A.smaldone Department of chemistry and Biochemistry University of TexasDallasRichardsonTexas 75080

covalent organic frameworks(cOFs)are highly ordered and permanently porous organic polymers that can be c.a.sified as two-dimensional or *** tunable design and crystalline order endow a range of pore sizes,shapes,functions,and applications that differentiate them from other *** cOF pore sizes and shapes rely on the geometry of the monomers and dynamic covalent chemistry,while the stacking of the sheets relies on noncovalent *** tunability allows for post-modification or the incorporation of additional functional groups for the reinforcement by various noncovalent *** limits of mesoporous cOFs are still being investigated,with the design rules continuing to *** we report a comprehensive review of mesoporous cOFs,explore strategies for large pore reinforcement,highlight structural design and features,elucidate their various functions and applications,discuss fundamental c.a.lenges faced that need to be addressed,and predict future directions.

关键词： covalent organic frameworks mesoporous supramolecular chemistry polymers pore size