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Defence Technology（防务技术） 2024年第1期31卷 387-399页

作者： Binghui Duan Hongchang Mo bojun Tan Xianming Lu Bozhou wang Ning Liu Xi'an Modern Chemistry Research Institute Xi'an710065People's Republic of China State Key Laboratory of Fluorine&Nitrogen Chemicals Xi'an710065People's Republic of China

The weak interface interaction and solid-solid phase transition have long been a conundrum for 1,3,5,7-tetranitro-1,3,5,7-tetraazacyclooctane(HMX)-based polymer-bonded explosives(PBX).A two-step strategy that involves the pretreatment of HMX to endow—OH groups on the surface via polyalcohol bonding agent modification and in situ coating with nitrate ester-containing polymer,was proposed to address the problem.Two types of energetic polyether—glycidyl azide polymer(GAP)and nitrate modified GAP(GNP)were grafted onto HMX crystal based on isocyanate addition reaction bridged through neutral polymeric bonding agent(NPBA)layer.The morphology and structure of the HMX-based composites were characterized in detail and the core-shell structure was validated.The grafted polymers obviously enhanced the adhesion force between HMX crystals and fluoropolymer(F2314)binder.Due to the interfacial reinforcement among the components,the two HMX-based composites exhibited a remarkable increment of phase transition peak temperature by 10.2°C and 19.6°C with no more than 1.5%shell content,respectively.Furthermore,the impact and friction sensitivity of the composites decreased significantly as a result of the barrier produced by the grafted polymers.These findings will enhance the future prospects for the interface design of energetic composites aiming to solve the weak interface and safety concerns.

关键词： HMX crystals Polyalcohol bonding agent Energetic polymer Core-shell structure Interfacial reinforcement

A Secure and Cost-Effective Training Framework Atop Serverless Computing for Object Detection in Blasting

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Computer Modeling in Engineering & Sciences 2024年第5期139卷 2139-2154页

作者： Tianming Zhang Zebin Chen Haonan Guo bojun Ren Quanmin Xie Mengke Tian Yong wang Department of Computer and Science Shanghai Jiaotong UniversityShanghai200240China Aerospace System Engineering Shanghai Shanghai200240China State Key Laboratory of Precision Blasting Jianghan UniversityWuhan430056China Beijing Microelectronics Technology Institute Beijing100076China

The data analysis of blasting sites has always been the research goal of relevant researchers.The rise of mobile blasting robots has aroused many researchers’interest in machine learning methods for target detection in the field of blasting.Serverless Computing can provide a variety of computing services for people without hardware foundations and rich software development experience,which has aroused people’s interest in how to use it in the field ofmachine learning.In this paper,we design a distributedmachine learning training application based on the AWS Lambda platform.Based on data parallelism,the data aggregation and training synchronization in Function as a Service(FaaS)are effectively realized.It also encrypts the data set,effectively reducing the risk of data leakage.We rent a cloud server and a Lambda,and then we conduct experiments to evaluate our applications.Our results indicate the effectiveness,rapidity,and economy of distributed training on FaaS.

关键词： Serverless computing object detection blasting

Ratiometric fluorescence probe for accurate detection of Concanavalin A by coupling fluorescent microsphere with boric acid functionalized carbon dots

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Chinese Chemical Letters 2024年第2期35卷 460-463页

作者： Mingyue Xie Juan Chen Yufei wang bojun Liu Rong-Bin Song Hong-Min Meng Zhaohui Li College of Chemistry Institute of Analytical Chemistry for Life ScienceHenan Joint International Research Laboratory of Green Construction of Functional Molecules and their Bioanalytical ApplicationsZhengzhou UniversityZhengzhou 450001China Zhengzhou Key Laboratory of Forensic Science and Technology Railway Police CollegeZhengzhou 450053China School of Ecology and Environment Zhengzhou UniversityZhengzhou 450001China

Accurate and sensitive strategies for Concanavalin A(Con A)sensing are conducive to the better cognition of various important biological and physiological processes.Here,by designing dextran-functionalized fluorescent microspheres(DxFMs)and boric acid-modified carbon dots(BCDs)as recognition unit and built-in signal reference respectively,a ratiometric fluorescent detection platform was proposed for Con A detection with high reliability.In this protocol,the BCDs/DxFMs precipitation was formed due to the covalent interactions between cis-diol of DxFMs and boronic acid groups of BCDs,thus only fluorescence of BCDs could be detected in the supernatant.When Con A was presented,it could bind to DxFMs through its carbohydrate recognition ability and suppress the subsequent assembly between DxFMs and BCDs,leading to the simultaneous capture of DxFMs and BCDs fluorescence in the supernatant.Since the BCDs content was superfluous,their fluorescence intensities were basically constant in all cases.Based on the unchanged BCDs fluorescence signal and target-dependent DxFMs fluorescence signal in supernatant,the ratiometric detection of Con A was realized.Under optimized conditions,this ratiometric fluorescent platform displayed a linear detection range from 0.125μg/mL to 12.5μg/mL with a detection limit of 0.089μg/mL.Moreover,satisfied analytical outcomes for Con A detection in serum samples were obtained,manifesting huge application potential of this ratiometric fluorescent platform in clinical diagnosis.

关键词： Concanavalin A Fluorescent microspheres Carbon dots Ratiometric fluorescent assay Reliability

Fluorinated soft carbon as an ultra-high energy density potassium-ion battery cathode enabled by a ternary phase K_(x)FC

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Journal of Energy Chemistry 2023年第2期77卷 38-44,I0002页

作者： Pengyu Chen bojun wang Zhenrui Wu Xiaobin Niu Chuying Ouyang Hong Li Liping wang School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731SichuanChina School of Engineering The University of British ColumbiaKelowna V1V 1V7Canada C Innovation Laboratory Contemporary Amperex Technology Ltd.(21C LAB)Ningde 352100FujianChina Key Laboratory for Renewable Energy Institute of PhysicsChinese Academy of SciencesBeijing 100190China

Fluorinated carbons(CFx)have been widely applied as lithium primary batteries due to their ultra-high energy density.It will be a great promise if CFx can be rechargeable.In this study,we rationally tune the C-F bond strength for the alkaline intercalated CFx via importing an electronegative weaker element K instead of Li.It forms a ternary phase K_(x)FC instead of two phases(LiF+C)in lithium-ion batteries.Meanwhile,we choose a large layer distance and more defects CFx,namely fluorinated soft carbon,to accommodate K.Thus,we enable CFx rechargeable as a potassium-ion battery cathode.In detail fluorinated soft carbon CF_(1.01) presents a reversible specific capacity of 339 mA h g^(-1)(797 Wh kg^(-1))in the 2nd cycle and maintains 330 mA h g^(-1)(726 Wh kg^(-1))in the 15th cycle.This study reveals the importance of tuning chemical bond stability using different alkaline ions to endow batteries with rechargeability.This work provides good references for focusing on developing reversible electrode materials from popular primary cell configurations.

关键词： Fluorinated carbon High energy density battery Potassium-ion battery Conversion reaction K-free cathode

Kinetic network models to elucidate aggregation dynamics of aggregation-induced emission systems

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Aggregate

Aggregate 2024年第1期5卷 1-8页

作者： Zige Liu Michae L.Kalin bojun Liu Siqin Cao Xuhui Huang Theoretical Chemistry Institute Department of ChemistryUniversity of Wisconsin-MadisonMadisonWisconsinUSA Biophysics University of Wisconsin-MadisonMadisonWisconsinUSA

Aggregation-induced emission(AIE)is a phenomenon where a molecule that is weakly or non-luminescent in a diluted solution becomes highly emissive when aggregated.AIE luminogens(AIEgens)hold promise in diverse applications like bioimaging,chemical sensing,and optoelectronics.Investigation in AIE luminescence is also critical for understanding aggregation kinetics as the aggregation process is an essential component of AIE emission.Experimental investigation of AIEgen aggregation is challenging due to the fast timescale of the aggregation and the amorphous aggregate structures.Computer simulations such as molecular dynamics(MD)simulation provide a valuable approach to complement experiments with atomic-level knowledge to study the fast dynamics of aggregation processes.However,individual simulations still struggle to systematically elucidate heterogeneous kinetics of the formation of amorphous AIEgen aggregates.Kinetic network models(KNMs),constructed from an ensemble of MD simulations,hold great potential in addressing this challenge.In these models,dynamic processes are modeled as a series ofMarkovian transitions occurring among metastable conformational states at discrete time intervals.In this perspective article,we first review previous studies to characterize the AIEgen aggregation kinetics and their limitations.We then introduce KNMs as a promising approach to elucidate the complex kinetics of aggregations to address these limitations.More importantly,we discuss our perspective on linking the output of KNMs to experimental observations of time-resolved AIE luminescence.We expect that this approach can validate the computational predictions and provide great insights into the aggregation kinetics for AIEgen aggregates.These insights will facilitate the rational design of improved AIEgens in their applications in biology and materials sciences.

关键词： hydrophobic aggregation kinetic network models molecular dynamics simulations

In situ photoelectric biosensing based on ultranarrowband near-infrared plasmonic hot electron photodetection

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Advanced Photonics 2024年第2期6卷 81-89页

作者： Xianghong Nan Wenduo Lai Jie Peng Haiquan wang bojun Chen Huifan He Zekang Mo Zikun Xia Ning Tan Zhong Liu Long Wen Dan Gao Qin Chen Jinan University College of Physics&Optoelectronic EngineeringInstitute of NanophotonicsGuangdong Provincial Key Laboratory of Nanophotonic ManipulationGuangzhouChina Tsinghua University Shenzhen International Graduate SchoolState Key Laboratory of Chemical OncogenomicsShenzhenChina Jinan University College of Life Science and TechnologyGuangzhouChina

Narrowband photodetection is an important measurement technique for material analysis and sensing,for example,nondispersive infrared sensing technique.Both photoactive material engineering and nanophotonic filtering schemes have been explored to realize wavelength-selective photodetection,while most devices have a responsive bandwidth larger than 2%of the operating wavelength,limiting sensing performance.Near-infrared photodetection with a bandwidth of less than 0.2%of the operating wavelength was demonstrated experimentally in Au/Si Schottky nanojunctions.A minimum linewidth of photoelectric response down to 2.6 nm was obtained at a wavelength of 1550 nm by carefully tailing the absorptive and radiative loss in the nanostructures.Multiple functions were achieved on chip with the corrugated Au film,including narrowband resonance,light harvesting for sensing and photodetection,and electrodes for hot electron emission.Benefiting from such a unity integration with in situ photoelectric conversion of the optical sensing signal and the ultranarrowband resonance,self-contained on-chip biosensing via simple intensity interrogation was demonstrated with a limit of detection down to 0.0047%in concentration for glucose solution and 150 ng∕m L for rabbit IgG.Promising potential of this technique is expected for the applications in on-site sensing,spectroscopy,spectral imaging,etc.

关键词： plasmonics hot electron sensor photodetector spectroscopy

Comparative Study of 3D-Printed Porous Titanium Alloy with Rod Designs of Three Different Geometric Structures for Orthopaedic Implantation

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Acta Metallurgica Sinica(English Letters) 2024年第1期37卷 54-66页

作者： Jiaxin Li Haozhang Zhong bojun Cao Zhaoyang Ran Jia Tan Liang Deng Yongqiang Hao Jinglong Yan Department of Orthopedics The Second Affiliated Hospital of Harbin Medical UniversityHarbin150001China Shanghai Engineering Research Center of Innovative Orthopaedic Instruments and Personalized Medicine Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai200011China Institute of Materials Modification and Modeling Shanghai Jiao Tong UniversityShanghai200240China

Porous titanium alloy is currently widely used in clinical treatment of orthopaedic diseases for its lower elastic modulus and ability to integrate with bone tissue.At the micro-level,cells can respond to different geometries,and at the macro-level,the geometric design of implants will also affect the biological function of cells.In this study,three kinds of porous scaffolds with square,triangular and circle rod shapes were designed and 3D printed.This study observed the proliferation and differentiation of MC3T3-E1 cells during surface culture of the three types of scaffolds.It also evaluated the characteristics of the three scaffolds by means of compression tests and scanning electron microscopy to provide a reference for the design of porous titanium alloy implants for clinical applications.The trends of cell proliferation and gene expression between the three types of scaffolds were observed after treatment with two inhibitors.The results show that the square rod porous scaffolds have the best proliferative and osteogenic activities,and these findings may be due to differences in piezo-type mechanosensitive ion channel component 1(Piezo1)and Yes-associated protein(YAP)expression caused by the macro-geometric topography.

关键词： Porous titanium scaffolds Geometric morphology Cell proliferation Structural design

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契丹字拟音的再检讨

中国语文 2024年第1期 100-110,128页

作者：孙伯君中国社会科学院民族学与人类学研究所北京

鉴于此前学界基于汉字拟定契丹文的读音时,对古代汉语与阿尔泰语语音系统的总体差异,汉语在契丹人口语中的“番式”变读的认识还不够系统,本文特结合女真文文献、汉语在蒙古语中的“番式”变读规律,以及契丹小字对汉字的注音等,梳理了... 详细信息

鉴于此前学界基于汉字拟定契丹文的读音时,对古代汉语与阿尔泰语语音系统的总体差异,汉语在契丹人口语中的“番式”变读的认识还不够系统,本文特结合女真文文献、汉语在蒙古语中的“番式”变读规律,以及契丹小字对汉字的注音等,梳理了契丹人口语中汉语的声韵规律,进一步探讨了契丹文的拟音问题。契丹“番式”汉语的语音特征包括:汉语疑母字-和来母字1-在契丹人口语中发生了增音变读,分别读作*■-、*■-;汉语匣、喻、影母字在契丹人口语中发生了变读,匣母字变读作h-/g-/k-,部分影、喻母字发生了增音变读,作*-■(i);汉语非、敷两母f-在契丹人口语中读作p-;契丹人把汉语齿头音ts-ts^(h)-、s-变读为一个s-音位;汉语日母字在契丹人口语中往往读作■-或s-;汉语人声字韵尾-t、-k、p在契丹人口语中变成阴声韵;汉语部分鼻音-m、-■韵尾字在契丹人口语中有变读人-n的情况;契丹语中只有一套塞音声母,不区分汉语的送气塞音和不送气塞音。这种带有“番式”变读的辽代汉语,在金代又进一步得到强化。

关键词：契丹小字语音构拟 “番式”汉语

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基于深度元学习的小样本图像分类研究综述

计算机工程与应用 2024年第8期60卷 1-15页

作者：周伯俊陈峙宇南通大学工程训练中心江苏南通226019 河海大学计算机与信息学院南京211100

深度元学习是解决小样本分类问题的流行范式。对近年来基于深度元学习的小样本图像分类算法进行了详细综述。从问题的描述出发对基于深度元学习的小样本图像分类算法进行概括,并介绍了常用小样本图像分类数据集及评价准则;分别从基于模... 详细信息

深度元学习是解决小样本分类问题的流行范式。对近年来基于深度元学习的小样本图像分类算法进行了详细综述。从问题的描述出发对基于深度元学习的小样本图像分类算法进行概括,并介绍了常用小样本图像分类数据集及评价准则;分别从基于模型的深度元学习方法、基于优化的深度元学习方法以及基于度量的深度元学习方法三个方面对其中的典型模型以及最新研究进展进行详细阐述。最后,给出了现有算法在常用公开数据集上的性能表现,总结了该课题中的研究热点,并讨论了未来的研究方向。

关键词：深度学习元学习小样本学习图像分类

浅析智能建筑能耗管理系统设计及运维管理平台应用--以工人体育场改造复建项目为例

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智能建筑电气技术 2024年第3期18卷 58-63,69页

作者：王博筠北京市建筑设计研究院股份有限公司北京100045

本文采用文献研究、案例分析法,以工人体育场改造复建项目为案例对智慧能耗管理系统的设计思路以及运维管理平台的实现路径进行分析,以典型高能耗公共建筑为代表,为今后类似大型公共建筑能耗管理系统的设计和运维管理平台建设提供借鉴,... 详细信息

本文采用文献研究、案例分析法,以工人体育场改造复建项目为案例对智慧能耗管理系统的设计思路以及运维管理平台的实现路径进行分析,以典型高能耗公共建筑为代表,为今后类似大型公共建筑能耗管理系统的设计和运维管理平台建设提供借鉴,助力我国建筑设计行业高质量、低碳、绿色可持续发展。

关键词：建筑智能化设计能耗监管系统运维管理平台体育场馆节能