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Simultaneously optimizing exciton diffusion length and nonradiative energy loss in organic solar cells via ternary strategy

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Science China Chemistry 2024年第9期67卷 3004-3011页

作者： Huanxiang Jiang Hao lu Zezhou Liang Yonghai Li Guangliu Ran Chenyu han Yuqiang Liu Hongxiang Li Xichang Bao Zhishan bo College of Textiles and Clothing State Key Laboratory of Bio-fibers and Eco-textiles Qingdao University Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi Key Lab of Photonic Technique for InformationSchool of Electronics Science & Engineering Faculty of Electronic and Information Engineering Xi'an Jiaotong University Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Laboratory of Solar Energy Shandong Energy Institute Department of Physics and Applied Optics Beijing Area Major Laboratory Center for Advanced Quantum Studies Beijing Normal University College of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University

Significant nonradiative energy loss and short exciton diffusion length in organic solar cells(OSCs) are two major obstacles to achieving state-of-the-art efficiencies. It is crucial to conduct a study on the intensive mechanism and improvement strategies for future breakthroughs in the efficiency of OSCs. In this work, nonradiative energy loss and exciton diffusion length are optimized simultaneously by incorporating a guest acceptor(LA15) to construct ternary OSC(D18:L8-bo:LA15). Firstly, LA15 exhibits excellent compatibility with the host acceptor L8-bo, and effectively improves the fluorescence quantum efficiency(FLQY),resulting in suppressed non-radiative energy loss. Moreover, LA15 effectively prolongs the fluorescent lifetime of the acceptor phase from 0.85 to 1.12 ns, leading to larger exciton diffusion length, which is beneficial for reducing geminate ***, the addition of LA15 optimizes the crystallinity of the active layer with amplified charge transport capacity. As a result,the optimized D18:L8-bo:LA15 device achieves ultralow nonradiative energy loss of 0.18 e V and improved fill factor(FF) with high efficiency up to 19.13%. These results highlight the crucial roles of regulating FLQYand exciton lifetime in achieving highefficiency OSCs.

关键词： organic solar cells nonradiative energy loss exciton lifetime exciton diffusion length

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Mechanical Behavior and Failure Mechanism of an As-Extruded Mg-11wt%Y Alloy at Elevated Temperature

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Acta Metallurgica Sinica(English Letters) 2024年第6期37卷 969-981页

作者： Lan Zhang Dao-Kui Xu Bao-Jie Wang Cui-Lan lu Shuo Wang Xiang-bo Xu Dong-Liang Wang Xin Lv En-Hou han School of Materials Science and Engineering University of Science and Technology of ChinaShenyang110016China Key Laboratory of Nuclear Materials and Safety Assessment Institute of Metal ResearchChinese Academy of SciencesShenyang110016China School of Environmental and Chemical Engineering Shenyang Ligong UniversityShenyang110159China Key Lab of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang110819China Institute of Corrosion Science and Technology Guangdong510070China

Through carrying out the high-temperature tensile experiments on an as-extruded Mg-11wt%Y alloy at 350℃,400℃,450℃,500℃and 550℃,the mechanical behavior and fracture mechanisms at elevated temperatures are investigated and *** results show that with the increase of temperature,the yield strength and ultimate tensile strength of the alloy increase at first and then decrease,while that the elongation ratio decreases firstly and then *** the sample being tested at 350℃,the values of yield strength,ultimate tensile strength and the elongation ratio are 188 MPa,266 MPa and 11%,*** 400℃,the yield strength and ultimate tensile strength reach the maximum values of,respectively,198 MPa and 277 MPa,but the elongation ratio is the lowest and its value is only 8%.When the applied temperature is increased to 550℃,the values of yield strength and ultimate tensile strength,respectively,decrease to 140 MPa and 192 MPa and the elongation ratio increases to 38%.Failure analysis demonstrates that the fracture surfaces of different samples are mainly composed of plastic dimples and exhibit the typical characteristic of ductile *** observation to the fracture side surfaces indicates that at the temperatures of 350℃and 400℃,microcracks mainly initiate in the interior of Mg_(24)Y_(5)*** the temperatures are 450℃,500℃and 550℃,the cracks preferentially initiate at the Mg_(24)Y_(5)/α-Mg interfaces.

关键词： Mg-Y alloy High-temperature tensile properties Fracture mechanism Failure analysis

Variability of the Pacific subtropical cells under global warming in CMIP6 models

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Journal of Oceanology and Limnology 2024年第1期42卷 24-40页

作者： Xue han Junqiao FENG Yunlong lu Dunxin HU Key Laboratory of Ocean Circulation and Waves Chinese Academy of SciencesQingdao 266071China Institute of Oceanology Chinese Academy of SciencesQingdao 266071China University of Chinese Academy of Sciences Beijing 100049China Center for Ocean Mega-Science Chinese Academy of SciencesQingdao 266071China Laboratory for Ocean Dynamics and Climate Pilot National Laboratory for Marine Science and Technology(Qingdao)Qingdao 266237China

The Pacific subtropical cells(STCs)are shallow meridional overturning circulations connecting the tropics and subtropics,and are assumed to be an important driver of the tropical Pacific decadal *** variability of STCs under global warming is investigated using multimodal outputs from the latest phase of the Coupled Model Inter-comparison Project(CMIP6)and ocean reanalysis ***,the volume transport diagnostic analysis is employed to evaluate how coupled models and ocean reanalysis products reproduce interior STC *** variation of heat transport by the interior STC under the high-emissions warming scenarios is also *** results show that the multimodal-mean linear trends of the interior STC transport along 9°S and 9°N are-0.02 Sv/a and 0.04 Sv/a under global warming,respectively,which is mainly due to the combined effect of the strengthened upper oceanic stratification and the weakening of wind *** is a compensation relationship between the interior STC and the western boundary transport in the future climate,and the compensation relationship of 9°S is more significant than that of 9°*** addition,compared with ocean reanalysis products,the coupled models tend to underestimate the variability of the interior STC transport convergence,and thus may lose some sea surface temperature(SST)driving force,which may be the reason for the low STC-SST correlation simulated by the *** future scenario simulation shows that the heat transport of interior STC is weakened under global warming,with a general agreement across models.

关键词： interior subtropical cell(STC) global warming Coupled Model Inter-comparison Project(CMIP6) western boundary transport

Aggregation-regulated bioreduction process of graphene oxide by Shewanella bacteria

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Chinese Journal of Chemical Engineering 2024年第5期69卷 56-62页

作者： Kaixin han Yibo Zeng Yinghua lu Ping Zeng Liang Shen Department of Chemical and Biochemical Engineering College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Pen-Tung Sah Institute of Micro-Nano Science and Technology Xiamen UniversityXiamen 361005China Chinese Research Academy of Environmental Sciences Beijing 100012China

The bioreduction of graphene oxide(GO)using environmentally functional bacteria such as Shewanella represents a green approach to produce reduced graphene oxide(rGO).This process differs from the chemical reduction that involves instantaneous molecular *** bioreduction,the contact of bacterial cells and GO is considered the rate-limiting *** reveal how the bacteria-GO integration regulates rGO production,the comparative experiments of GO and three Shewanella strains were carried ***-transform infrared spectroscopy,X-ray photoelectron spectroscopy,Raman spectroscopy,and atomic force microscopy were used to characterize the reduction degree and the aggregation *** results showed that a spontaneous aggregation of GO and Shewanella into the condensed entity occurred within 36 h.A positive linear correlation was established,linking three indexes of the aggregation potential,the bacterial reduction ability,and the reduction degree(ID/IG)comprehensively.

关键词： Graphene oxide Reduced graphene oxide Bioreduction Aggregation Shewanella

Fixed-Time Antidisturbance Consensus Tracking for Nonlinear Multiagent Systems With Matching and Mismatching Disturbances

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IEEE/CAA Journal of Automatica Sinica 2024年第6期11卷 1410-1423页

作者： Xiangmin Tan Chunyan Hu Guanzhen Cao Qinglai Wei Wei Li bo han Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190 School of Aeronautics and Astronautics University of Chinese Academy of SciencesBeijing 100049China Institute of Automation Chinese Academy of SciencesBeijing 100190 School of Artificial Intelligence University of Chinese Academy of SciencesBeijing 100049China IEEE

In this paper,fixed-time consensus tracking for mul-tiagent systems(MASs)with dynamics in the form of strict feed-back affine nonlinearity is addressed.A fixed-time antidistur-bance consensus tracking protocol is proposed,which consists of a distributed fixed-time observer,a fixed-time disturbance observer,a nonsmooth antidisturbance backstepping controller,and the fixed-time stability analysis is conducted by using the Lyapunov theory *** paper includes three main ***,a distributed fixed-time observer is developed for each follower to obtain an estimate of the leader’s output by utilizing the topology of the communication ***,a fixed-time disturbance observer is given to estimate the lumped disturbances for feedforward ***,a nonsmooth antidisturbance backstepping tracking controller with feedforward compensation for lumped disturbances is *** order to mitigate the“explosion of complexity”in the tradi-tional backstepping approach,we have implemented a modified nonsmooth command filter to enhance the performance of the closed-loop *** simulation results show that the pro-posed method is effective.

关键词： Antidisturbance backstepping consensus tracking fixed-time stability multiagent system(MASs) strict feedback affine nonlinear systems.

Reducing Subspaces of Toeplitz Operators Induced by a Class of Non-analytic Monomials over the Unit Ball

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Acta Mathematica Sinica,English Series 2024年第7期40卷 1767-1777页

作者： Yan Yue SHI bo ZhanG Xu TANG Yu Feng lu School of Mathematical Sciences Ocean University of ChinaQingdao 266100P.R.China School of Mathematics and Information Sciences Yantai UniversityYantai 264005P.R.China School of Mathematical Sciences Space Engineering UniversityBeijing 101416P.R.China School of Mathematical Sciences Dalian University of TechnologyDalian 116024P.R.China

In this paper,we describe the minimal reducing subspaces of Toeplitz operators induced by non-analytic monomials on the weighted Bergman spaces and Dirichlet spaces over the unit ball B_(2).It is proved that each minimal reducing subspace M is finite dimensional,and if dim M≥3,then M is induced by a ***,the structure of commutant algebra v(T_(w)N_(z)N):={M^(*)_(w)NM_(z)N,M^(*)_(z)NM_(w)N}′is determined by N and the two dimensional minimal reducing subspaces of(T_(w)N_(z)*** also give some interesting examples.

关键词： Reducing subspace operator-weighted shifts Toeplitz operator von Neumann algebra

On the electric behaviour of conductive grease inside the contact zone

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Friction 2024年第4期12卷 683-697页

作者： Yuxin ZHOU Jinjie LIU Xinming LI He CHONG bo han Qinghua BAI SKF(Shanghai)Automotive Technologies Co. Ltd.Shanghai 201814China School of Mechanical and Automotive Engineering Qingdao University of TechnologyQingdao 266250China

Conductive grease has been considered as a potential solution in addressing electric erosion issue inside motor *** the conductive grease performance,especially the electric and tribological behaviour is crucial for its *** paper combines bulk grease characterization and contact film study considering both electrical and tribological loading *** results show that the electric performance for the selected conductive grease sample is electric field dependent,including both frequency and voltage *** film impedance inside the contact area is closely related to the external electric field,running condition,and lubrication *** following film impedance calculation tells that not only bulk grease electric parameters,but the contact parameter,lubricant film contour and lubrication condition should be considered when performing the overall bearing electrical modelling.

关键词： Electric erosion lubricant conductivity grease film impedance

Adsorptive interaction between typical VOCs and various topological zeolites:Mixture effect and mechanism

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Journal of Environmental Sciences 2024年第2期136卷 626-636页

作者： bo Yu Hua Deng Yuqin lu Tingting Pan Wenpo Shan Hong He Center for Excellence in Regional Atmospheric Environment and Key Laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of Chinese Academy of Sciences Beijing 100049China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Adsorption is one of the most feasible and effective methods to alleviate the volatile organic compounds(VOCs)***,the mixture effect and mechanism for competitive adsorption of VOCs on zeolites are barely *** this study,toluene,acetone,and ethyl acetate as prevalent VOCs species were removed by four potential zeolites(13X,USY,Beta,ZSM-5)in both single-and multi-component *** structure-property relationship between adsorbate-adsorbent pairs was revealed by X-ray diffraction,scanning electron microscopy,energy dispersive spectrometer,X-ray fluorescence,N_(2) adsorption and density function theory *** molecular polarity and volatility of VOCs species played key roles in adsorption and the dynamic uptakes were generally listed as follows:ethyl acetate>toluene>*** for the above VOCs mixtures,13X zeolite selectively adsorbed oxygenated VOCs rather than *** contrast,USY exhibited a preference to trap *** acetate could be readily enriched by ZSM-5 and Beta *** possible explanations and implications are discussed based on the subtle change in electron *** results obtained are vital for understanding the mixture effect of VOCs adsorption and may guide the selection of proper adsorbent for real applications.

关键词： Adsorption Zeolites VOCs Mixture effect DFT

Type Synthesis of Self-Alignment Parallel Ankle Rehabilitation Robot with Suitable Passive Degrees of Freedom

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Chinese Journal of Mechanical Engineering 2024年第1期37卷 160-175页

作者： Ya Liu Wenjuan lu Dabao Fan Weijian Tan bo Hu Daxing Zeng School of Mechanical Engineering Yanshan UniversityQinhuangdao 066004China School of Mechanical Engineering Dongguan University of TechnologyDongguan 523808China Dongguan Engineering Technology Research Center for Parallel Robot Dongguan 523808China The DGUT Innovation Center of Robotics and Intelligent Equipment Dongguan 523808China

The current parallel ankle rehabilitation robot(ARR)suffers from the problem of difficult real-time alignment of the human-robot joint center of rotation,which may lead to secondary injuries to the *** study investigates type synthesis of a parallel self-alignment ankle rehabilitation robot(PSAARR)based on the kinematic characteristics of ankle joint rotation center drift from the perspective of introducing"suitable passive degrees of freedom(DOF)"with a suitable number and ***,the self-alignment principle of parallel ARR was proposed by deriving conditions for transforming a human-robot closed chain(HRCC)formed by an ARR and human body into a kinematic suitable constrained system and introducing conditions of"decoupled"and"less limb".Second,the relationship between the self-alignment principle and actuation wrenches(twists)of PSAARR was analyzed with the velocity Jacobian matrix as a"bridge".Subsequently,the type synthesis conditions of PSAARR were ***,a PSAARR synthesis method was proposed based on the screw theory and type of PSAARR synthesis ***,an HRCC kinematic model was established to verify the self-alignment capability of the *** this study,93 types of PSAARR limb structures were synthesized and the self-alignment capability of a human-robot joint axis was verified through kinematic analysis,which provides a theoretical basis for the design of such an ARR.

关键词： Ankle rehabilitation robot Self-alignment Parallel mechanism Type synthesis Screw theory