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Energy & Environmental Materials 2023年第2期6卷 45-53页

作者： bo niu Jiefeng Xiao Zhenming Xu School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China

The ever-increasing quantity of spent lithium-ion batteries(LIBs)is both a potential environmental pollutant and a valuable *** spent LIBs recycling mainly aimed at the separation of valuable *** issues still exist in these processes such as high energy consumption and complex separation *** study avoided element separation and proposed a facile approach to transform spent LiCoO_(2) electrode into a lithium(Li)-doped graphitic carbon nitride(g-C_(3)N_(4))/Co_(3)O_(4) composite photocatalyst through one-pot in situ thermal *** the thermal process,melamine served as the reductant for LiCoO_(2) decomposition and the raw material for g-C_(3)N_(4) *** was in situ doped in g-C_(3)N_(4) and the generated Co_(3)O_(4) was in situ integrated,forming a Li-doped g-C_(3)N_(4)/Co_(3)O_(4) composite *** special composite exhibited an enhanced photocatalytic performance,and its photocatalytic H2 production and RhB degradation rates were 8.7 and 6.8 times higher than those of g-C_(3)N_(4).The experiments combined with DFT calculation revealed that such enhanced photocatalytic efficiency was ascribed to the synergy effect of Li doping and Co_(3)O_(4) integrating,which extended the visible light absorption(450-900 nm)and facilitated the charge transfer and *** study transforms waste into a high-efficient catalyst,realizing high-valued utilization of waste and environmental protection.

关键词： composite photocatalyst environmental protection spent LIBs synergy mechanism waste utilization

Quantitative characterization of deep fault-karst carbonate reservoirs: A case study of the Yuejin block in the Tahe oilfield

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Energy Geoscience 2023年第3期4卷 63-70页

作者： Xiangyang Hu Wenbo Zheng Xiangyuan Zhao bo niu Petroleum Exploration and Production Research Institute of SINOPEC Beijing100083China

The Ordovician reservoirs in the Tahe oilfield are dominated by fractured-vuggy carbonate reservoirs, of which fault-karst reservoirs are a hot topic in recent years. Fault-karst reservoirs feature high production, large burial depth, and strong heterogeneity under the control of faulting and karstification. Based on geological, logging, and seismic data, this study classified the Ordovician fault-karst reservoirs in the Yuejin block of the Tahe oilfield into three types, namely karst-cave, dissolved-vug, and fractured types, and established the integrated identification criteria of the three types of reservoirs. This study characterized karst caves, dissolved vugs, and multi-scale faults through seismic wave impedance inversion and frequency-domain detection of multi-scale faults. 3D geological models of different types of reservoirs were built using the combined deterministic and stochastic methods and characterized the spatial distribution of multi-scale faults, karst caves, dissolved vugs, and physical property parameters of reservoir. This study established the method for the geological modeling of fault-karst reservoirs, achieved the quantitative characterization and revealed the heterogeneity of fault-karst reservoirs. The karst-cave and dissolved-vug types are high in porosity and act as reservoirs, while the fractured type is high in permeability and act as flow pathway. This study lays the foundation for the development index prediction, well emplacement, and efficient development of the fault-karst carbonate reservoirs.

关键词： Carbonate Fault-karst reservoir Quantitative reservoir characterizati on Yuejin block Tahe oilfield

An extract from the earthworm Eisenia fetida non-specifically inhibits the activity of influenza and adenoviruses

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Journal of Traditional Chinese Medicine 2012年第4期32卷 657-663页

作者： Zhizhen Liu Jianhua Wang Jianlin Zhang Baofeng Yu bo niu Biochemistry and Molecular Biology Shanxi Medical University Department of Biology technology Capital Institute of Pediatrics

OBJECTIVE： To test the in vitro antiviral activity of a crude tissue extract （CTE/from the earthworm Eisenia fetida, determine any effective components in the CTE, andelucidate possiblemechanismsofaction. METHODS： A CTE was made by homogenizing earthworms, followed by treatment with ammoni- um sulfate, then thermal denaturation. Inhibition of virus-induced cytopathic effect （CPE） was used to assess antiviral activity. Chromatographic analy- sis was used to identify effective components in the CTE. RESULTS： The CTE inhibited viral CPE at non-cyto- toxic concentrations. Chromatography indicated that antiviral components corresponded to three active peaks indicative of proteases, nucleases and lysozymes. For adenoviruses, reduction in viral ac- tivity occurred for 100 lag/mL CTE. The reduction in adenoviral activity for four fractions was 100%, 91.8%, 86.9%, and 94.7%. For influenza viruses, re- duction in viral activity of 100%, 86.6%, 69.1% and 88.3% was observed for 37 pg/mL CTE. In addition, three active fractions mixture had stronger antiviral activity （98.7% and 96.7%） than three fractions *** electrophoresis results indicated that nu- cleases from E. fetida could degrade the genome of influenza viruses and adenoviruses. CONCLUSION： The earthworm CTE displayed non-specific antiviral properties, possibly mediated by a combination of proteases, nucleases and lyso- zymes. Nucleases likely participate in the antiviral process, and degrade the genome of the virus thereby preventing further replication.

关键词： Oligochaeta Complex mixtures Influ-enza a virus, HI NI subtype Adenoviruses

Performance analysis of ARQ schemes with code combining over Nakagami-m fading channel

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The Journal of China Universities of Posts and Telecommunications 2009年第5期16卷 14-19页

作者： XU Wen-bo niu Kai LIN Jia-ru HE Zhi-qiang School of Information and Telecommunication Engineering Beijing University of Posts and Telecommunications Beijing 100876 China

This article investigates the performance of hybrid automatic repeat request （HARQ） with code combining over the ideally interleaved Nakagami-m fading channel. Two retransmission protocols with coherent equal gain code combining are adopted, where the entire frame and several selected portions of the frame are repeated in protocols I and II, respectively. Protocol II could be viewed as a generalization of the recently proposed reliability-based HARQ. To facilitate performance analysis, an approximation of the product of two independent Nakagami-m distributed random variables is first developed. Then the approximate analysis is utilized to obtain exact frame error probability （FEP） for protocol I, and the upper bound of the FEP for protocol II. Furthermore, the throughput performance of both two protocols is presented. Simulation results show the reliability of the theoretical analysis, where protocol II outperforms protocol I in the throughput performance due to the reduced amount of transmitted information.

关键词： code combining HARQ Nakagami-m fading performance analysis

An ion-released MgI_(2)-doped separator inducing a LiI-containing solid electrolyte interphase for dendrite-free Li metal anodes

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Journal of Energy Chemistry 2022年第12期75卷 83-94,I0003页

作者： Shan Yi Zhe Su Wanyu Zhang Hongli Chen Yayun Zhang bo niu Donghui Long State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory for Specially Functional Materials and Related Technology of the Ministry of Education East China University of Science and TechnologyShanghai 200237China

Lithium metal batteries are among the strong contenders to satisfy the ever-increasing needs of energy storage systems,which however suffer from poor composition of the solid electrolyte interphase(SEI)layer and uncontrolled Li dendrites *** this regard,we report on the design of an ionreleased MgI_(2)-doped polyacrylonitrile(PAN)based nanofiber(MPANF)separator,which can lead to conducive SEI layer and dendrite-free Li *** combination of the lithophilic MgI_(2)nanoparticles with polarized PAN matrix comprehensively functions as a high-compatible interpenetrating network to homogenize ionic transportation and confront dendrite *** released I ions introduce the highion-conductivity LiI into SEI layer,which could induce the formation of favorable and protective interface layer in the early stage,as embodied in the enrichment of advantageous components such as LiN_(x)O_(y),Li_(2)O,LiF,and Li_(3)*** from the high-affinity MPANF separator,the Li||Li symmetric cell achieves an ultralow voltage hysteresis of 46 mV with an extended lifespan of 580 *** a prolonged lifetime of 590cycles with an enhanced specific capacity of 140.1 m Ah g^(-1)and the Coulombic efficiency of 96.2%at 1C can be obtained in full *** work may offer a facile and high-affinity alternative to traditional polymeric separators for high-performance and dendrite-free Li metal batteries.

关键词： Lithium metal anode LiI-containing layer Dendrite-free anode Electrospun nanofiber separator

Excellent Structure-Based Multifunction of Morpho Butterfly Wings： A Review

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Journal of Bionic Engineering 2015年第2期12卷 170-189页

作者： Shichao niu bo Li Zhengzhi Mu Meng Yang Junqiu Zhang Zhiwu Han Luquan Ren Key Laboratory of Bionic Engineering (Ministry of Education China) Jilin University Changchun 130022 China

Morpho butterfly, famous for its iridescence wing scales, has gradually evolved a diversity of functions and has attracted much attention recently. On the other hand, it is known that the wing surface of Morpho butterfly has some complex and so- phisticated structures. In fact, they are composed of an alternating multilayer film system of chitin and air layers, which have different refractive indexes. More importantly, these structures can interact strongly with visible light because the feature size of the structures is in the same order of magnitude with light wavelength. It is noteworthy that it is these optical architectures that cause the excellent multifunction including structural color, antireflection, thermal response, selective vapour response, direc- tional adhesion, superhydrophobicity and so on. This review mainly covers the excellent multifunctional features of Morpho butterfly wings with representative functional structures of multilayer film system, photonic crystal and ridges. Then, the mechanism of the structure-based optical multifunction of Morpho butterfly is analyzed. In order to facilitate mechanism analysis, the models of bionic functional structures are reported, as well as the interaction process between the multiscale structures and the external media It is concluded that these functions of Morpho butterfly wings have inevitable and corre- sponding regularity connection with the structural parameters and the dielectric coefficient of the filled medium. At last, the future direction and prospects of this field are briefly addressed. It is hoped that this review could be beneficial to provide some innovative insoirations and new ideas to the researchers in the fields of engineering, biomedicine, and materials science.

关键词： Morpho butterfly wing scales microstructure structure-based functions bionics

Experimental study on hypersonic crossflow instability over a swept flat plate by flow visualization

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Acta Mechanica Sinica 2021年第9期37卷 1395-1403,I0002页

作者： Hai-bo niu Shi-He Yi Jun-Jie Huo Wen-Peng Zheng Xiao-Lin Liu College of Aerospace Science and Engineering National University of Defense TechnologyChangsha410073China

An experimental study on the traveling crossflow instability over a 60∘swept flat plate was *** Mach number is 6,the angle of attack of the model is 5∘.The traveling crossflow waves and the secondary instability of the traveling crossflow waves were visualized by nano-tracer-based planar laser scattering(NPLS)*** the spanwise NPLS images,the traveling crossflow waves appeared as regular strikes,and the secondary instability appeared as small eddies attached to *** wavelet transform was used to study the wavelength contents of the traveling crossflow *** most amplified wavelength is stable before the secondary instability happening,which is around 12 mm at Re_(∞)=3.45×10^(6)m^(−1).Besides,the Reynolds number effects on the boundary layer transition and traveling crossflow instability were discussed.

关键词： Crossflow instability Swept flat plate Flow visualization Wavelet analysis boundary layer transition

Ultrafine Vacancy-Rich Nb_(2)O_(5)Semiconductors Confined in Carbon Nanosheets boost Dielectric Polarization for High-Attenuation Microwave Absorption

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Nano-Micro Letters 2023年第10期15卷 478-493页

作者： Zhe Su Shan Yi Wanyu Zhang Xiaxi Xu Yayun Zhang Shenghu Zhou bo niu Donghui Long Shanghai Key Laboratory of Multiphase Materials Chemical Engineering School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237People’s Republic of China Key Laboratory for Specially Functional Materials and Related Technology of the Ministry of Education East China University of Science and TechnologyShanghai 200237People’s Republic of China

The integration of nano-semiconductors into electromagnetic wave absorption materials is a highly desirable strategy for intensifying dielectric polarization loss;achieving high-attenuation microwave absorption and realizing in-depth comprehension of dielectric loss mechanisms remain ***,ultrafine oxygen vacancy-rich Nb_(2)O_(5)semiconductors are confined in carbon nanosheets(ov-Nb_(2)O_(5)/CNS)to boost dielectric polarization and achieve high *** polarization relaxation,electromagnetic response,and impedance matching of the ov-Nb_(2)O_(5)/CNS are significantly facilitated by the Nb_(2)O_(5)semiconductors with rich oxygen vacancies,which consequently realizes an extremely high attenuation performance of-80.8 dB(>99.999999%wave absorption)at 2.76 *** a dielectric polarization center,abundant Nb_(2)O_(5)–carbon heterointerfaces can intensify interfacial polarization loss to strengthen dielectric polarization,and the presence of oxygen vacancies endows Nb_(2)O_(5)semiconductors with abundant charge separation sites to reinforce electric dipole ***,the three-dimensional reconstruction of the absorber using microcomputer tomography technology provides insight into the intensification of the unique lamellar morphology regarding multiple reflection and scattering dissipation ***,ov-Nb_(2)O_(5)/CNS demonstrates excellent application potential by curing into a microwave-absorbing,machinable,and heat-dissipating *** work provides insight into the dielectric polarization loss mechanisms of nano-semiconductor/carbon composites and inspires the design of high-performance microwave absorption materials.

关键词： Electromagnetic wave absorption Nb_(2)O_(5)semiconductor Dielectric polarization loss Oxygen vacancy Nb_(2)O_(5)-carbon hetero-interface

Urchin-like Nb_(2)O_(5)hollow microspheres enabling efficient and selective photocatalytic C–C bond cleavage in lignin models under ambient conditions

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Chinese Chemical Letters 2022年第9期33卷 4357-4362页

作者： Huan Chen Donghui Hong Kun Wan Junjie Wang bo niu Yayun Zhang Donghui Long State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China Shanghai Key Laboratory of Multiphase Materials Chemical Engineering East China University of Science and TechnologyShanghai 200237China

Selective cleavage of robust C−C bonds to harvest value-added aromatic oxygenates is an intriguing but challenging task in lignin *** is a promising technology with the advantages of mild reaction conditions and strong ***,we show a novel urchin-like Nb_(2)O_(5)hollow microsphere(U-Nb_(2)O_(5)HM),prepared by one-pot hydrothermal method,are highly active and selective for C_(α)−C_(β)bond cleavage of ligninβ-O-4 model compounds under mild conditions,achieving 94%substrate conversion and 96%C−C bond cleavage *** experimental studies and density functional theory(DFT)calculations revealed that the superior performance of U-Nb_(2)O_(5)HMs arises from more exposed active sites,more efficient free charge separation and the active(001)facet,which facilitates the activation of Cβ−H bond of lignin models and generate key Cβradical intermediates by photogenerated holes,further inducing the C_(α)−C_(β)bond cleavage to produce aromatic *** work could provide some suggestions for the fabrication of hierarchical photocatalysts in the lignin depolymerization system.

关键词： Niobium oxide Urchin-like hierarchical structure Photocatalysis β-O-4 Lignin model C_(β)radical

Evaluating two stages of silicone-containing arylene resin oxidation via experiment and molecular simulation

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Chinese Journal of Chemical Engineering 2024年第2期66卷 189-202页

作者： Jiangtao Cai Qingfu Huang Huan Chen Tao Zhang bo niu Yayun Zhang Donghui Long Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory of Special Functional Polymeric Materials and Related Technology(Ministry of Education) School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237China

Silicon-containing aryl acetylene resin(PSA)is a new type of high-temperature resistant resin with excellent oxidation resistance,whereas antioxidant reaction mechanism of PSA resin under ultra-high temperatures still remains ***,the oxidation behavior and mechanisms of PSA resin are systematically investigated combining kinetic analysis and Reax FF molecular dynamics(MD)*** analysis indicates that the oxidation process of PSA resin undergoes two main steps:oxidative mass gain and oxidative *** distributed activation energy model(DAEM)is employed for describing oxidation processes and the best-fit one is obtained using genetic algorithms and differential *** model demonstrates that the oxidative weight gain stage is dominated by two virtual reactants and the oxidative degradation stage consists of three virtual ***,the observation of MD reaction pathways indicates that oxygen oxidation of unsaturated structures occurs in the initial stage,which results in the formation of PSA resin ***,cracked pieces react with O_(2)to generate CO and other chemicals in the second *** resin matrix's great antioxidation resilience is illustrated by the formation of SiO_(2).The analysis based on MD simulations exhibits an efficient computational proof with the experiments and DAEM *** on the results,a two-stage reaction mechanism is proposed,which provides important theoretical support for the subsequent study of the oxidation behavior of silica-based resins.

关键词： PSA resin Oxidative degradation Thermogravimetric analysis DAEM reaction kinetics ReaxFF simulation