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High-rate lithium-ion battery performance of a ternary sea urchin-shaped CoNiO_(2)@NiP_(6)Mo_(18)/CNTs composites

Journal of Energy Chemistry 2024年第9期96卷 516-525页

作者： Li-ping Cui shuang sun Kai Yu shu Zhang Mei-lin Wang Jia-jia Chen Bai-bin Zhou Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of EducationSchool of Chemistry and Chemical EngineeringHarbin Normal UniversityHarbin 150025HeilongjiangChina state Key Laboratory of Physical Chemistry of solid surfaces Department of ChemistryCollege of Chemistry and Chemical EngineeringCollaborative Innovation Centre of Chemistry for Energy MaterialsXiamen UniversityXiamen 361005FujianChina

Bimetallic oxides are attractive anode materials for lithium-ion batteries(LIBs)due to their large theoretical ***,the low conductivity,short cycle life,and poor rate capability are the bottlenecks for their further *** overcome above issues,the basket-like polymolybdate(NiP_(6)Mo_(18))and carbon nanotubes(CNTs)were uniformly embedded on the urchin-shaped CoNiO_(2)nanospheres to yield a ternary composites CoNiO_(2)@NiP_(6)Mo_(18)/CNTs via electrostatic *** multi-level morphology of urchin spinules accelerates the diffusion rate of Li^(+);CNT improves the conductivity and enhances cycle stability of the material;and heteropoly acid contributes more redox activity ***,CoNiO_(2)@NiP_(6)Mo_(18)/CNTs as an anode of LIBs exhibits a high initial capacity(1396.7 mA h g^(−1)at 0.1 A g^(−1)),long-term cycling stability(750.2 mA h g^(−1)after 300 cycles),and rate performance(450.3 mA h g^(−1)at 2 A g^(−1)),which are superior to reported metallic oxides anode of *** density functional theory(DFT)and kinetic mechanism suggest that CoNiO_(2)@NiP_(6)Mo_(18)/CNTs delivers an outstanding pseudocapacitance and rapid Li^(+)diffusion behaviors,which is due to the rich surface area of the urchin-like CoNiO_(2)with the uniform embeddedness of NiP_(6)Mo_(18)and *** study provides a new idea for optimizing the performance of bimetallic oxides and developing high-rate lithium-ion battery composites.

关键词： Bi-metal oxides Transition metal oxides Polyoxometalates Nanocomposite LIBs

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Direct recycling of Li-ion batteries from cell to pack level:Challenges and prospects on technology,scalability,sustainability,and economics

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Carbon Energy 2024年第6期6卷 1-39页

作者： Joseph Jegan Roy Do Minh Phuong Vivek Verma Richa Chaudhary Michael Carboni Daniel Meyer bin Cao Madhavi srinivasan Energy Research Institute@NTU(ERI@N) SCARCE LaboratoryNanyang Technological UniversitySingaporeSingapore school of Materials science and engineering Nanyang Technological UniversitySingaporeSingapore CEA CNRSENSCMUniversity of MontpellierUMR 5257(ICSM)Bagnols-sur-Cèze CedexFrance school of Civil and Environmental engineering Nanyang Technological UniversitySingaporeSingapore

Direct recycling is a novel approach to overcoming the drawbacks of conventional lithium-ion battery(LIB)recycling processes and has gained considerable attention from the academic and industrial sectors in recent *** primary objective of directly recycling LIBs is to efficiently recover and restore the active electrode materials and other components in the solid phase while retaining electrochemical *** technology's advantages over traditional pyrometallurgy and hydrometallurgy are costeffectiveness,energy efficiency,and sustainability,and it preserves the material structure and morphology and can shorten the overall recycling *** review extensively discusses the advancements in the direct recycling of LIBs,including battery sorting,pretreatment processes,separation of cathode and anode materials,and regeneration and quality enhancement of electrode *** encompasses various approaches to successfully regenerate high-value electrode materials and streamlining the recovery process without compromising their electrochemical ***,we highlight key challenges in direct recycling when scaled from lab to industries in four perspectives:(1)battery design,(2)disassembling,(3)electrode delamination,and(4)commercialization and *** on these challenges and changing market trends,a few strategies are discussed to aid direct recycling efforts,such as binders,electrolyte selection,and alternative battery designs;and recent transitions and technological advancements in the battery industry are presented.

关键词： battery design cathode regeneration direct recycling graphite recycling lithium-ion battery,scaling-up

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{1012}twin–twin intersection-induced lattice rotation and dynamic recrystallization in Mg–6Al–3sn–2Zn alloy

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Journal of Magnesium and Alloys 2024年第4期12卷 1529-1539页

作者： bin-Jiang Lv sen Wang Fu-Hao Gao Ning Cui Yi-Nan Li Tie-Wei Xu Feng Guo school of Mechanical and Automotive engineering Qingdao University of Technology266520China Key Lab of industrial Fluid Energy Conservation and Pollution Control Qingdao University of Technology266520China

This study investigated the formation mechanism of new grains due to twin–twin intersections in a coarse-grained Mg–6Al–3sn–2Zn alloy during different strain rates of an isothermal *** results of electron backscattered diffraction investigations showed that the activated twins were primarily{1012}tension twins,and 60°boundaries formed due to twin–twin intersections under different strain *** twin variants with 60°boundaries transformed into new grains through lattice rotations at a low strain rate(0.01 s^(−1)).At a high strain rate(10 s^(−1)),the regions surrounded by subgrain boundaries through high-density dislocation arrangement and the 60°boundaries transformed into new grains via dynamic recrystallization.

关键词： Mg alloy Twin-twin intersection Lattice rotation Dynamic recrystallization

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spatial-temporal Patterns of Urban Parks’Effects on the sentiments and Their Associated Factors Based on social Media Data——a Case study in Beijing

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Journal of Geodesy and Geoinformation science 2024年第2期7卷 95-110页

作者： YUAN Yuting WANG Juan WEI Yali ZHU Yanrong sHI Changs.eng Meng bin College of Applied Arts and science Beijing Union UniversityBeijing 100191China Laboratory of Urban Cultural sensing&Computing Beijing Union UniversityBeijing 100191China Beijing Guohuan Environmental Technology Co. Ltd.Tangshan 063020China

As the pivotal green space,urban parks play an important role in urban residents’daily *** can not only bring people physical health,but also can be more likely to elicit positive sentiment to those who visit ***,social media big data has provided new data sources for sentiment ***,there was limited researches that explored the connection between urban parks and individual’s ***,this study firstly employed a pre-trained language model(BERT,Bidirectional Encoder Representations from Transformers)to calculate sentiment scores based on social media ***,this study analysed the relationship between urban parks and individual’s sentiment from both spatial and temporal ***,by utilizing structural equation model(sEM),we identified 13 factors and analyzed its degree of the *** research findings are listed as below:①It confirmed that individuals generally experienced positive sentiment with high sentiment scores in the majority of urban parks;②The urban park type showed an influence on sentiment *** this study,higher sentiment scores observed in Eco-parks,comprehensive parks,and historical parks;③The urban parks level showed low impact on sentiment *** distinctions observed mainly at level-3 and level-4;④Compared to internal factors in parks,the external infrastructure surround them exerted more significant impact on sentiment *** instance,number of bus and subway stations around urban parks led to higher sentiment scores,while scenic spots and restaurants had inverse *** study provided a novel method to quantify the services of various urban parks,which can be served as inspiration for similar studies in other cities and countries,enhancing their park planning and management strategies.

关键词： urban parks sentiment analysis social media data sEM Beijing

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In-situ sludge reduction based on Mn^(2+)-catalytic ozonation conditioning:Feasibility study and microbial mechanisms

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Journal of Environmental sciences 2024年第1期135卷 185-197页

作者： Haozhe Huang Tingting Wei Hui Wang bing Xue sisi Chen Xiankai Wang Haibin Wu bin Dong Zuxin Xu College of Environmental science and engineering Tongji UniversityShanghai 200092China YANGTZE Eco-Environment engineering Research Center China Three Gorges CorporationBeijing 100038China

To improve the sludge conditioning efficiency without increasing the ozone dose,an in-situ sludge reduction process based on Mn^(2+)-catalytic ozonation conditioning was *** ozone conditioning alone as a control,a lab-scale sequencing batch reactor coupled with ozonated sludge recycle was evaluated for its operating performance at an ozone dose of 75 mg O_(3)/g Vss and 1.5 mmol/L Mn^(2+)*** results showed a 39.4%reduction in MLss and an observed sludge yield of 0.236 kg MLss/kg COD for the O_(3)+Mn^(2+)group compared to the O_(3)group (15.3%and 0.292 kg MLss/kg COD),accompanied by better COD,NH_(4)^(+)-N,TN and TP removal,improved effluent ss and limited impact on excess sludge ***,activity tests,BIOLOG ECO microplates and 16s rRNA sequencing were applied to elucidate the changing mechanisms of Mn^(2+)-catalytic ozonation related to microbial action:(1) Dehydrogenase activity reached a higher peak.(2) Microbial utilization of total carbon sources had an elevated effect,up to approximately 18%,and metabolic levels of six carbon sources were also increased,especially for sugars and amino acids most pronounced.(3) The abundance of Defluviicoccus under the phylum Proteobacteria was enhanced to 12.0%and dominated in the sludge,they had strong hydrolytic activity and metabolic *** bacteria of the genus Ferruginibacter also showed an abundance of 7.6%,they contributed to the solubilization and reduction of sludge *** results could guide researchers to further reduce ozonation conditioning costs,improve sludge management and provide theoretical support.

关键词： Activated sludge In-situ reduction Catalytic ozonation conditioning Dehydrogenase activity Carbon source utilization Microbial community

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Assessing donor-recipient arterial pressure dynamics in sTA-MCA bypass for moyamoya disease

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中华神经外科杂志(英文) 2024年第3期10卷 1-10页

作者： Helmy Mohamed Liao Yujun Zhao Zehao Li Zhiqi He Kangmin Xu bin Neurosurgery Department Fudan University Huashan Hospital Shanghai People’s Republic of China National Center for Neurological Disorders Shanghai People’s Republic of China

Background In bypass surgery for moyamoya disease (MMD), the superficial temporal artery’s (sTA) pressure needs to surpass that of the cortical M4 recipient of the middle cerebral artery (MCA), boosting cerebral blood flow into the MCA and enhancing cerebral circulation. This study investigates the sTA-MCA arterial pressure parameters and gradients during bypass surgery, aiming to deepen our understanding of hemodynamic shifts pre- and *** DsA imaging data were prospectively collected from patients diagnosed with bilateral MMD who underwent sTA-MCA bypass surgery between 2022 and 2023 and stratified according to the suzuki stage. The mean arterial pressure (MAP) of the donor and recipient arteries was directly measured during the sTA-MCA bypass procedure, and these data were statistically analyzed and *** Among 48 MMD patients, suzuki grading revealed that 43.8% were in early stages (II and III), while 56.2% were in advanced stages (IV, V, and VI). Predominantly, 77.1% presented with ischemic-type MMD and 22.9% with hemorrhagic type. Pre-bypass assessments showed that 62.5% exhibited antegrade blood flow direction, and 37.5% had retrograde. The mean recipient artery pressure was 35.0 ± 2.3 mmHg, with a mean donor-recipient pressure gradient (δP) of 46.4 ± 2.5 mmHg between donor and recipient arteries. Post-bypass, mean recipient artery pressure increased to 73.3 ± 1.6 mmHg. No significant correlation (r= 0.18,P= 0.21) was noted between δP and suzuki *** Our study elucidated that cerebral blood pressure significantly decreases beyond the moyamoya network at the distal M4 segment. Furthermore, we observed bidirectional flow in MCA territories and a significant positive pressure gradient between the sTA and M4 segments. The lack of correlation between suzuki stages and M4 pressures indicates that angiographic severity may not reflect hemodynamic conditions before surgery, highlighting the need for customized surgical appr

关键词： Moyamoya disease Pressure gradient Cerebral hemodynamic suzuki stage

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Characterizing the complete mitochondrial genome of Psephenothrips eriobotryae Dang&Qiao(Thysanoptera:Phlaeothripidae)with massive gene arrangement in Phlaeothripidae

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Zoological systematics 2024年第2期49卷 116-128页

作者： Lihong Dang Chengwen Li Dongxue Wang Yuxin Gao Linpeng Zhao bin Zhang school of Biological science&engineering Shaanxi University of TechnologyHanzhong 723000China engineering Research Center of Quality Improvement and safety Control of Qinba special Meat Products Universities of Shaanxi ProvinceHanzhong 723000China shaanxi Changqing National Nature Reserve Changqing JiayuanNo.176Hanzhong 723000China College of Life sciences&Technology Inner Mongolia Normal UniversityHohhot 010022China

Each species within the order Thysanoptera has a distinct mitochondrial gene order displaying a high level of gene rearrangement,particularly massive in *** understand the evolutionary patterns of rearrangement in this family,we sequenced the complete mitochondrial genome of Psephenothrips eriobotryae,a notable potential pest of loquat *** mitogenome is a circular DNA molecule(15,413 bp in size)composed of 37 genes:13 PCGs,22 tRNAs,two rRNAs,and two putative control regions(CRs).By comparing with the ancestral mitogenome of arthropods,*** exhibits notable gene rearrangement ***,it shares four conserved gene blocks with three closely related species in *** the phylogenetic tree,*** was clustered with these three leaffeeding Phlaeothripinae *** presence of more similar conserved gene blocks probably indicates a strong correlation between gene rearrangements and the phylogeny within ***,the mitogenome of *** shows some characteristics:(a)two putative CRs in which CR2 is the copy of partial CR1 with 99.62%sequence similarity,and CR1 consists of two 237 bp repeat unites;(b)high A+T content of 82.6%in overall base composition;(c)trn s1 lacking a complete dihydrouridine(DHU)arm;(d)the protein coding gene,atp8 started with TTG instead of the more common ATN,while nad3 terminated by TAG rather than TAA;(e)translocations and inversions observed in fifteen of the 37 genes.

关键词： Mitogenome structure phylogenetic relationships Liothrips-lineage repeat regions

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Novel sandwich structured glass fiber Cloth/Poly(ethylene oxide)-MXene composite electrolyte

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Nano Materials science 2024年第1期6卷 60-67页

作者： Yu-Qin Mao Guang-He Dong Wei-bin Zhu Yuan-Qing Li Pei Huang shao-Yun Fu College of Aerospace engineering Chongqing UniversityChongqing400044China state Key Laboratory of Power Transmission Equipment and system security and New Technology Chongqing UniversityChongqing400044China

Recently,poly(ethylene oxide)(PEO)-based solid polymer electrolytes have been attracting great attention,and efforts are currently underway to develop PEO-based composite electrolytes for next generation high performance all-solid-state lithium metal *** this article,a novel sandwich structured solid-state PEO composite electrolyte is developed for high performance all-solid-state lithium metal *** PEO-based composite electrolyte is fabricated by hot-pressing PEO,LiTFsI and Ti_(3)C_(2)T_(x) MXene nanosheets into glass fiber cloth(GFC).The as-prepared GFC@PEO-MXene electrolyte shows high mechanical properties,good electrochemical stability,and high lithium-ion migration number,which indicates an obvious synergistic effect from the microscale GFC and the nanoscale *** as,the GFC@PEO-1 wt%MXene electrolyte shows a high tensile strength of 43.43 MPa and an impressive Young's modulus of 496 MPa,which are increased by 1205%and 6048%over those of ***,the ionic conductivity of GFC@PEO-1 wt%MXene at 60℃ reaches 5.01×10^(-2) s m^(-1),which is increased by around 200%compared with that of GFC@PEO *** addition,the Li/Li symmetric battery based on GFC@PEO-1 wt%MXene electrolyte shows an excellent cycling stability over 800 h(0.3 mA cm^(-2),0.3 mAh cm^(-2)),which is obviously longer than that based on PEO and GFC@PEO electrolytes due to the better compatibility of GFC@PEO-1 wt%MXene electrolyte with Li ***,the solid-state Li/LiFePO_(4) battery with GFC@PEO-1 wt%MXene as electrolyte demonstrates a high capacity of 110.2–166.1 mAh g^(-1) in a wide temperature range of 25–60C,and an excellent capacity retention *** developed sandwich structured GFC@PEO-1 wt%MXene electrolyte with the excellent overall performance is promising for next generation high performance all-solid-state lithium metal batteries.

关键词： solid polymer electrolyte Ti_(3)C_(2)T_(x)MXene Poly(ethylene oxide) Glass fiber cloth All-solid-state Li metal Battery

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支持批量证明的sM2适配器签名及其分布式扩展

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软件学报 2024年第5期35卷 2566-2582页

作者：涂彬彬陈宇山东大学网络空间安全学院山东青岛266237 密码科学技术全国重点实验室北京100878 密码技术与信息安全教育部重点实验室(山东大学) 山东青岛266237 山东区块链研究院山东济南250001 泉城实验室山东济南250014

适配器签名,又称无脚本脚本,是解决区块链应用(如密码货币)中扩展性差、吞吐量低等问题的重要密码技术.适配器签名可看作数字签名关于困难关系的扩展,同时具有签名授权和证据提取两种功能,在区块链应用中具有以下优点:(1)降低链上成本;... 详细信息

适配器签名,又称无脚本脚本,是解决区块链应用(如密码货币)中扩展性差、吞吐量低等问题的重要密码技术.适配器签名可看作数字签名关于困难关系的扩展,同时具有签名授权和证据提取两种功能,在区块链应用中具有以下优点:(1)降低链上成本;(2)提高交易的可替代性;(3)突破区块链脚本语言限制.sM2签名是我国自主设计的国家标准签名算法,在各种重要信息系统中有着广泛应用.基于sM2签名构造出高效的适配器签名方案,并在随机谕言机模型下给出安全性证明.所提方案结合sM2签名结构,可避免在预签名阶段生成额外的零知识证明,与现有ECDsA/sM2适配器签名相比更加高效,其中,预签名生成效率提升4倍,预签名验证效率提升3倍.随后,基于sM2协同签名,构造分布式sM2适配器签名,可避免单点故障问题,提升签名私钥安全.最后,在实际应用方面,基于sM2适配器签名构造适用于一对多场景下安全高效的批量原子交换协议.

关键词： sM2算法适配器签名分布式适配器签名区块链原子交换

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Effect of the mixing of s-wave and chiral p-wave pairings on electrical shot noise properties of normal metal/superconductor tunnel junctions

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Chinese Physics B 2024年第7期33卷 538-545页

作者：胡雨辰胡梁宾 Guangdong Provincial Key Laboratory of Quantum engineering and Quantum Materials School of PhysicsSouth China Normal UniversityGuangzhou 510631China

We study theoretically the electrical shot noise properties of tunnel junctions between a normal metal and a superconductor with the mixture of singlet s-wave and chiral triplet p-wave pairing due to broken inversion symmetry. We investigate how the shot noise properties vary as the relative amplitude between the two parity components in the pairing potential is changed. It is demonstrated that some characteristics of the electrical shot noise properties of such tunnel junctions may depend sensitively on the relative amplitude between the two parity components in the pairing potential, and some significant changes may occur in the electrical shot noise properties when the relative amplitude between the two parity components is varied from the singlet s-wave pairing dominated regime to the chiral triplet p-wave pairing dominated regime. In the chiral triplet p-wave pairing dominated regime, the ratio of noise power to electric current is close to 2e both in the in-gap and in the out-gap region. In the singlet s-wave pairing dominated regime, the value of this ratio is close to 4e in the inner gap region but may reduce to about 2e in the outer gap region as the relative amplitude of the chiral triplet pairing component is increased. The variations of the differential shot noise with the bias voltage also exhibit some significantly different features in different regimes. such different features can serve as useful diagnostic tools for the determination of the relative magnitude of the two parity components in the pairing potential.

关键词： normal metal/superconductor tunnel junctions shot noise mixing of s-wave and chiral p-wave pairing spin–orbit coupling

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