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Fabrication of lithium silicates from zeolite for CO2 capture at high temperatures

Journal of Energy Chemistry 2019年第6期28卷 81-89页

作者： Yu Zhang Yanshan Gao benoit louis Qiang Wang Weiran Lin College of Environmental Science and Engineering Beijing Forestry UniversityBeijing 100083China ICPEES - Institut de Chimie et Procedes pour l’energie l’Environnement et la SanteUMR 7515 CNRS - Universite de Strasbourg67087 StrasbourgFrance Beijing Research Institute of Chemical Industry SINOPECBeijing 100013China

Li4Si O4 has been regarded as one of the most promising high-temperature CO2 ***,for practical applications,its CO2sorption kinetics,cycling stability and sorption properties at lower temperatures or lower CO2 concentrations have to be *** this contribution,four Li4Si O4 sorbents were synthesized from zeolite precursors MCM-41,MCM-48,TS-1,and *** CO2 uptake,cycling stability and the optimal CO2 sorption conditions were *** the samples,MCM-41-Li4Si O4 showed the best cycling stability at 650°C,with a stable reversible CO2 uptake of 29.1 wt%under 100 vol%CO2 during 20 *** its sorption kinetics and CO2 uptakes at lower temperatures and lower CO2 concentrations need to be *** then demonstrated that the sorption kinetics can be improved by modifying the MCM-41 precursor with metals such as Al,Ti,Ca,and *** Na-MCM-41-Li4Si O4 sample exhibited the highest sorption rate,and reached the equilibrium sorption capacity close to the theoretical value of 36.7 wt%within 20 *** addition,we proved that coating the MCM-41-Li4Si O4with Na2CO3and K2CO3can significantly increase the CO2uptakes at lower temperatures(e.g.550℃)and lower CO2concentrations(10–20 vol%).At 550℃ and under 20 vol%CO2,15 wt%K2CO3-MCM-41-Li4Si O4 and 10 wt%Na2CO3-MCM-41-Li4Si O4 sorbents resulted in a CO2 uptake of 32.2 wt%and 34.7 wt%,respectively,which are much higher than that of MCM-41-Li4Si O4(11.8 wt%).These two sorbents also showed good cycling *** promoiting mechasnim by alkali carbonate coating was discussed by a doubleshell model.

关键词： Li4SiO4 Zeolite Lithium silicate-based CO2 sorbents Global warming

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Molten salts-modified MgO-based adsorbents for intermediate-temperature CO_2 capture: A review

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Journal of Energy Chemistry 2017年第5期26卷 830-838页

作者： Wanlin Gao Tuantuan Zhou Yanshan Gao benoit louis Dermot O'Hare Qiang Wang College of Environmental Science and Engineering Beijing Forestry University Beijing 100083 China Laboratoire de Synthese Reactivite Organiques et Catalyse Institut de Chimie UMR 7177 Universite de Strasbourg1 rue Blaise Pascal 67000 StrasbourgFrance Chemistry Research Laboratory Department of Chemistry University of Oxford Mansﬁeld Road Oxford OX1 3TA United Kingdom

Carbon dioxide（CO2） capture using magnesium oxide（MgO）-based adsorbents at intermediate temperatures has been regarded as a very prospective technology for their relatively high adsorption capacity,low cost, and wide availability. During the past few years, great effort has been devoted to the fabrication of molten salts-modified MgO-based adsorbents. The extraordinary progress achieved by coating with molten salts greatly promotes the COcapture capacity of MgO-based adsorbents. Therefore, we feel it necessary to deliver a timely review on this type of COcapturing materials, which will benefit the researchers working in both academic and industrial areas. In this work, we classified the molten saltsmodified MgO adsorbents into four categories:（1） homogenous molten salt-modified MgO adsorbents,（2） molten salt-modified double salts-based MgO adsorbents,（3） mixed molten salts-modified MgO adsorbents, and（4） molten salts-modified MgO-based mixed oxides adsorbents. This contribution critically reviews the recent developments in the synthetic method, adsorption capacity, reaction kinetics, promotion mechanism, operational conditions and regenerability of the molten salts-modified MgO COadsorbents. The challenges and prospects in this promising field of molten salts-modified MgO COadsorbents in real applications are also briefly mentioned.

关键词： Global warming Magnesium oxide CO2 adsorption Molten salts Intermediate temperatures

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Impact of organic interlayer anions on the CO2 adsorption performance of Mg-Al layered double hydroxides derived mixed oxides

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Journal of Energy Chemistry 2017年第3期26卷 346-353页

作者： Qingqing Qin Junya Wang Tuantuan Zhou Qianwen Zheng Liang Huang Yu Zhang Peng Lu Ahmad Umar benoit louis Qiang Wang College of Environmental Science and Engineering Beijing Forestry University Faculty of Environmental Science and Engineering Kunming University of Science and Technology Department of Chemistry College of Science and ArtsNajran University Promising Centre for Sensors and Electronic Devices(PCSED) Najran University Universitéde Strasbourg CNRSCHIMIE

Herein we report a systematical investigation on the promoting effect of the carbon chain length of the intercalated carboxylic anions on the COcapture performance of Mg-Al layer double hydroxides（LDHs）.A series of organo-LDHs were successfully synthesized via co-precipitation and calcination-rehydration methods. All as-prepared samples were characterized by many techniques including XRD, ATR-FTIR, BET,and TGA. The XRD and ATR-FTIR studies indicated that organic anions were successfully intercalated into LDHs. The influence of some important parameters such as calcination temperature, adsorption temperature, and coating with（Li-Na-K）NOmolten salt was investigated. The results exhibited that when the number of carbon is greater than 10, the COcapture capacity steadily increased with the increase in carbon number. After coating with 55 mol%（Li-Na-K）NOmolten salt, the COuptake of LDH-C16 sample with high Mg/Al ratios can be increased up to 3.25 mmol/g. The COadsorption/desorption cycling stability was also studied using temperature swing adsorption, which showed a stable COcapture performance even after 22 cycles. Considering its high COcapture capacity and good cycling stability, this novel COadsorbent is very promising in the sorption-enhanced water gas shift（SEWGS） processes.

关键词： Pre-combustion CO2 capture capacity Organo-LDHs Carboxylates Cycling stability Molten salts coating

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Supervised Learning Method: Critical Analysis and Updating of Cubing Rate Formulas for Determining Bark Masses of Prunus africana (Hook. f.) Kalkman (Rosaceae) in Cameroon

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Open Journal of Forestry 2024年第3期14卷 346-368页

作者： Armand Ndedy Bile Alain Mpouam benoit Fouadjio Lorette Guedeu Kambale Muhesi Steve Tassiamba Paulette Kouam Eric Wete Marius Ela Michèle Yimga Joseph Ambara louis Aimé Fono Jean Lagarde Betti Department of Plant Biology Faculty of Science The University of Douala Douala Cameroon Department of Wood and Forest Sciences ISABEE University of Bertoua Bertoua Cameroon Department of Water and Forests Higher Institute of Agronomic Veterinary and Forestry Studies of Butembo Butembo Democratic Republic of Congo Department of Forestry Faculty of Agronomy and Agricultural Sciences University of Dschang Dschang Cameroon Department of Biology and Plant Faculty of Sciences University of Maroua Maroua Cameroon Deutsche Gresellschaft fur Internationale Zusammenarbeit GmbH (GIZ) Bertoua Cameroon Department of Mathematics and Computer Science Faculty of Science The University of Douala Douala Cameroon

The stem barks of Prunus africana are used in the treatment of the benign prostate. Cameroon is one of the important exporters of the barks. Despite the important measures adopted in Cameroon for sustaining its harvesting, some many chalenges still remain. The objective of this work is to refine the forest management parameters in relation to P. africana in the regions of Adamaoua and the South-West by developing a volume rate which makes it possible to estimate the production for a new stem. The work took place in two phases: in the South-West in 2010 and in Adamaoua in 2011. Data collection used the semi-direct method, while the cubing equation was deduced by the multiple linear regression method. Two models for volume estimation and three models for mass prediction were developed. The predictive parameters retained are diameter, height of the bole and thickness of the bark. Results show that the average mass of the dry bark for a given P. africana tree species is 27.55 ± 14.44 kg and this varies according to the site. The strong adjusted coefficient of determination (adjusted R2) observed illustrates the reliability of the proposed models. These models provide a reliable tool that can be adopted as a standard in Cameroon for P. africana.

关键词： Prunus africana Prostate Quota Mass Model Sustainable Management

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A Numerical Model of a U-Tube Vertical Ground Heat Exchanger Used as an Evaporator

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Journal of Energy and Power Engineering 2013年第2期7卷 237-249页

作者： benoit Beauchamp louis Lamarche Stanislaw Kajl Ecole de Techonologie Superieure Mechanical Engineering Montreal H3C 1K3 QC Canada

The paper presents a general distributed model of a vertical U-tube direct expansion heat exchanger coupled with the ground. This model is developed for studying the dynamic thermal behavior of a buried heat exchanger which is an integral part of a so-called direct expansion heat pump. The transient conservative equations of mass, momentum and energy considering single and two-phase flow of refrigerant are derived and presented. The diffusive heat exchange with the ground is treated using an analytical approach to treat short-time scale response of vertical boreholes based on an imposed temperature. The thermal interference between the two pipes of the heat exchanger is also considered. The mathematical equations of the model are numerically presented using a control volume formulation and the solution of the system of equations is obtained by successive iterations. The dynamic behavior of the evaporator is simulated and the numerical results are analyzed regarding spatial parameters distribution and thermal interference influence.

关键词：埋管换热器数值模型垂直钻孔蒸发器 U型管能量守恒方程热交换器分布式模型

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Transversal Instability for the Thermodiffusive Reaction-Diffusion System

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Chinese Annals of Mathematics,Series B 2015年第5期36卷 871-882页

作者： Michal KOWALCZYK benoit PERTHAME Nicolas VAUCHELET Departamento de Ingenieria Matematica and Centro de Modelamiento Matem'atico(UMI CNRS 2807) Universidad de Chile Sorbonne Universités UPMC Univ Paris 06UMR 7598Laboratoire Jacques-Louis LionsF-75005ParisFrance CNRS UMR 7598Laboratoire Jacques-Louis LionsF-75005ParisFrance INRIA-Paris-Rocquencourt EPC MAMBADomaine de VoluceauBP10578153 Le Chesnay CedexFrance

The propagation of unstable interfaces is at the origin of remarkable patterns that are observed in various areas of science as chemical reactions, phase transitions, and growth of bacterial colonies. Since a scalar equation generates usually stable waves, the simplest mathematical description relies on two-by-two reaction-diffusion systems. The authors' interest is the extension of the Fisher/KPP equation to a two-species reaction which represents reactant concentration and temperature when used for flame propagation,and bacterial population and nutrient concentration when used in *** authors study circumstances in which instabilities can occur and in particular the effect of dimension. It is observed numerically that spherical waves can be unstable depending on the coefficients. A simpler mathematical framework is to study transversal instability, which means a one-dimensional wave propagating in two space ***, explicit analytical formulas give explicitely the range of paramaters for instability.

关键词： Traveling waves Stability analysis Reaction-diffusion equation Thermodiffusive system

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Analysis of a System Describing Proliferative-Quiescent Cell Dynamics

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Chinese Annals of Mathematics,Series B 2018年第2期39卷 345-356页

作者： Jean CLAIRAMBAULT benoit PERTHAME Andrada Quillas MARAN Inria de Paris Team MambaF75005 Paris France Sorbonne Univ. UPMC Univ. Paris 06 Laboratoire Jacques-Louis Lions UMR CNRS 7598 Univ. Paris-DiderotF75005 Paris France

Systems describing the dynamics of proliferative and quiescent cells are commonly used as computational models, for instance for tumor growth and *** on the very earliest stages of hematopoiesis, stem cells and early progenitors, the authors introduce a new method, based on an energy/Lyapunov functional to analyze the long time behavior of solutions. Compared to existing works, the method in this paper has the advantage that it can be extended to more complex situations. The authors treat a system with space variable and diffusion, and then adapt the energy functional to models with three equations.

关键词：动力学系统房间静止计算模型长时间行为肿瘤生长干细胞

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Dirac Concentrations in a Chemostat Model of Adaptive Evolution(In honor of the immense scientific influence of Ham Brezis)

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Chinese Annals of Mathematics,Series B 2017年第2期38卷 513-538页

作者： Alexander LORZ benoit PERTHAME Cécile TAING Sorbonne Universits UPMC Univ Paris 06InriaLaboratoire Jacques-Louis Lions UM R CNRS 7598F75005 ParisFrance

This paper deals with a non-local parabolic equation of Lotka-Volterra type that describes the evolution of phenotypically structured populations. Nonlinearities appear in these systems to model interactions and competition phenomena leading to selection. In this paper, the equation on the structured population is coupled with a differential equation on the nutrient concentration that changes as the total population *** methods aimed at showing the convergence of the solutions to a moving Dirac mass are reviewed. Using either weak or strong regularity assumptions, the authors study the concentration of the solution. To this end, BV estimates in time on appropriate quantities are stated, and a constrained Hamilton-Jacobi equation to identify where the solutions concentrates as Dirac masses is derived.

关键词： Adaptive evolution, Asymptotic behaviour, Chemostat, Dirac concentrations,Hamilton-Jacobi equations, Lotka-Volterra equations, Viscosity solutions

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Composite Waves for a Cell Population System Modeling Tumor Growth and Invasion

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Chinese Annals of Mathematics,Series B 2013年第2期34卷 295-318页

作者： Min TANG Nicolas VAUCHELET Ibrahim CHEDDAD Irene VIGNON-CLEMENTEL Dirk DRASDO benoit PERTHAME Department of mathematics Institute of Natural Sciences and MOE-LSCShanghai Jiao Tong University INRIA Paris Rocquencourt ParisFrance Laboratoire Jacques-louis Lions UPMC Univ Paris 06 and CNRS UMR 7598F-75005ParisFrance

In the recent biomechanical theory of cancer growth,solid tumors are considered as liquid-like materials comprising elastic *** this fluid mechanical view,the expansion ability of a solid tumor into a host tissue is mainly driven by either the cell diffusion constant or the cell division rate,with the latter depending on the local cell density(contact inhibition) or/and on the mechanical stress in the *** the two by two degenerate parabolic/elliptic reaction-diffusion system that results from this modeling,the authors prove that there are always traveling waves above a minimal speed,and analyse their *** appear to be complex with composite shapes and *** small parameters allow for analytical solutions,and in particular,the incompressible cells limit is very singular and related to the Hele-Shaw *** singular traveling waves are recovered numerically.

关键词：反应扩散系统肿瘤生长细胞群合成波侵袭建模力学理论弹性元件

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Design of Fe(3–x)O4 raspberry decorated graphene nanocomposites with high performances in lithium-ion battery

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Journal of Energy Chemistry 2016年第2期25卷 270-275页

作者： Olivier Gerber Sylvie Bégin-Colin benoit P.Pichon Elodie Barraud Sébastien Lemonnier Cuong Pham-Huu Barbara Daffos Patrice Simon Jeremy Come Dominique Bégin Institut de Physique et Chimie des Materiaux de Strasbourg UMR 7504 - CNRS Universite de Strasbourg 23 rue du Loess 67034 Strasbourg Cedex 08France RS2E - FR CNRS n 3459 Universite Paul Sabatier Toulouse III CIRIMAT 118 route de Narbonne 31062 Toulouse Cedex 9 France French-German Research Institute of Saint-louis 5 rue du General Cassagnou 68300 Saint-Louis France Institut de Chimie et Procedes pour l'Energie l'Environnement et la Sante UMR 7515-CNRS Universite de Strasbourg 25 rue Becquerel 67087 Strasbourg Cedex 02 France

Fe（3–x）O4 raspberry shaped nanostructures/graphene nanocomposites were synthesized by a one-step polyol-solvothermal method to be tested as electrode materials for Li-ion battery（LIB）. Indeed, Fe（3–x）O4 raspberry shaped nanostructures consist of original oriented aggregates of Fe（3–x）O4 magnetite nanocrystals, ensuring a low oxidation state of magnetite and a hollow and porous structure, which has been easily combined with graphene sheets. The resulting nanocomposite powder displays a very homogeneous spatial distribution of Fe（3–x）O4 nanostructures at the surface of the graphene sheets. These original nanostructures and their strong interaction with the graphene sheets resulted in very small capacity fading upon Li＋ion intercalation. Reversible capacity, as high as 660 m Ah/g, makes this material promising for anode in Li-ion batteries application.

关键词： Graphene Fe3–xO4 raspberry shaped nanostructures Fe3–xO4/graphene nanocomposites Lithium-ion battery Reversible capacity

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