检索结果-南通市图书馆

Enhancing capacitive deionization performance and cyclic stability of nitrogen-doped activated carbon by the electro-oxidation of anode materials

引用

Chinese Journal of Chemical Engineering 2024年第5期69卷 23-33页

作者： Xiaona Liu baohua zhao Yanyun Hu Luyue Huang Jingxiang Ma Shuqiao Xu Zhonglin Xia Xiaoying Ma Shuangchen Ma School of Environmental Science and Engineering North China Electric Power UniversityBaoding 071003China Huadian Zhengzhou Machinery Design and Research Institute Co. LtdZhengzhou 450002China Huadian Inner Mongolia Energy Co. Ltd.Baotou Power Generation BranchBaotou 014013China

Electrode materials with high desalination capacity and long-term cyclic stability are the focus of capacitive deionization(CDI) community. Understanding the causes of performance decay in traditional carbons is crucial to design a high-performance material. Based on this, here, nitrogen-doped activated carbon(NAC) was prepared by pyrolyzing the blend of activated carbon powder(ACP) and melamine for the positive electrode of asymmetric CDI. By comparing the indicators changes such as conductivity, salt adsorption capacity, pH, and charge efficiency of the symmetrical ACP-ACP device to the asymmetric ACP-NAC device under different CDI cycles, as well as the changes of the electrochemical properties of anode and cathode materials after long-term operation, the reasons for the decline of the stability of the CDI performance were revealed. It was found that the carboxyl functional groups generated by the electro-oxidation of anode carbon materials make the anode zero-charge potential(E_(pzc)) shift positively,which results in the uneven distribution of potential windows of CDI units and affects the adsorption capacity. Furthermore, by understanding the electron density on C atoms surrounding the N atoms, we attribute the increased cyclic stability to the enhanced negativity of the charge of carbon atoms adjacent to quaternary-N and pyridinic-oxide-N.

关键词： Anodic oxidation Capacitive deionization Cyclic stability N-doping

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Call for knowledge systematization:An example from lithium ion batteries recycling

引用

Journal of Energy Chemistry 2024年第7期94卷 169-170页

作者： Yun zhao baohua Li Institute of Materials Research Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055GuangdongChina

Scientific research is one of the primary ways to drive human civilization forward.Countless research institutions and researchers worldwide are dedicated to exploring the unknown,resulting in a flood of research findings[1].For instance,Web of Science alone collects over 10,000 academic papers on a daily basis.While each research field typically has around 10%of review articles,these mainly focus on a limited portion of the subject,failing to provide a comprehensive and real-time updated overview.As a result,researchers or students in a particular field may spend several months,or even longer,comprehending the state of research that has developed over just a few years.The lack of systematic background often leads to redundant or similar studies,which is highly detrimental to the progress of science and technology.

关键词： lithium typically spend

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Considerations of advanced aqueous batteries recycling:A perspective

引用

Journal of Energy Chemistry 2024年第6期93卷 46-54,I0002页

作者： Yun zhao Yuqiong Kang Hao Du Feiyu Kang baohua Li Institute of Materials Research Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055GuangdongChina

1.Introduction Battery technology,serving as a basis for a rechargeable society,has developed rapidly over a century[1].The progress can be roughly divided into three stages,with the initial two mainly focusing on aqueous battery systems.Prior to 1859,research primarily focused on the conceptualization of batteries and the development of primary(non-rechargeable)cells[2].In the subsequent150 years,rechargeable battery technology emerged。

关键词： battery Battery primarily

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Residual alkali-evoked cross-linked polymer layer for anti-air-sensitivity LiNi_(0.89)Co_(0.06)Mn_(0.05)O_(2)cathode

引用

Journal of Energy Chemistry 2024年第5期92卷 450-458页

作者： Chao zhao Xuebao Li Yun zhao Jingjing He Yuanpeng Cao Wei Luo Ding Wang Jianguo Duan Xianshu Wang baohua Li National and Local Joint Engineering Research Center of Lithium-ion Batteries and Materials Preparation Technology Key Laboratory of Advanced Battery Materials of Yunnan ProvinceFaculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming 650093YunnanChina School of Materials Science and Engineering Central South UniversityChangsha 410083HunanChina Institute of Materials Research Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055Guangdong China City College Kunming University of Science and TechnologyKunming 650051YunnanChina

High-energy density lithium-ion batteries(LIBs)with layered high-nickel oxide cathodes(LiNi_(x)Co_(y)Mn_(1-x-y)O_(2),x≥0.8)show great promise in consumer electronics and vehicular applications.However,LiNi_(x)Co_(y)Mn_(1-x-y)O_(2)faces challenges related to capacity decay caused by residual alkalis owing to high sensitivity to air.To address this issue,we propose a hazardous substances upcycling method that fundamentally mitigates alkali content and concurrently induces the emergence of an anti-air-sensitive layer on the cathode surface.Through the neutralization of polyacrylic acid(PAA)with residual alkalis and then coupling it with 3-aminopropyl triethoxysilane(KH550),a stable and ion-conductive cross-linked polymer layer is in situ integrated into the LiNi_(0.89)Co_(0.06)Mn_(0.05)O_(2)(NCM)cathode.Our characterization and measurements demonstrate its effectiveness.The NCM material exhibits impressive cycling performance,retaining 88.4%of its capacity after 200 cycles at 5 C and achieving an extraordinary specific capacity of 170.0 mA h g^(-1) at 10 C.Importantly,this layer on the NCM efficiently suppresses unfavorable phase transitions,severe electrolyte degradation,and CO_(2)gas evolution,while maintaining commendable resistance to air exposure.This surface modification strategy shows widespread potential for creating air-stable LiNi_(x)Co_(y)Mn_(1-x-y)O_(2)cathodes,thereby advancing high-performance LIBs.

关键词： Lithium-ion batteries Nickel-rich layered cathode Residual alkalis Cross-linked polyme rmodification Airsensitivity

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Regulating the inner Helmholtz plane structure at the electrolyte-electrode interface for highly reversible aqueous Zn batteries

引用

Journal of Energy Chemistry 2024年第8期95卷 57-67页

作者： Jianghe Liu Sanlue Hu Hexin Guo Guobin Zhang Wen Liu Jianwei zhao Shenhua Song Cuiping Han baohua Li Shenzhen Key Laboratory on Power Battery Safety and Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen Key Laboratory of Advanced Materials School of Materials Science and Engineering Harbin Institute of Technology Faculty of Materials Science and Energy Engineering/Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced Technology Chinese Academy of Sciences Shenzhen HUASUAN Technology Co. Ltd.

The development of aqueous Zn batteries is limited by parasitic water reactions,corrosion,and dendrite growth.To address these challenges,an inner Helmholtz plane（IHP） regulation method is proposed by employing low-cost,non-toxic maltitol as the electrolyte additive.The preferential adsorption behavior of maltitol can expel the water from the inner Helmholtz plane,and thus hinder the immediate contact between Zn metal and H2O.Meanwhile,strong interaction between maltitol and H2O molecules can restrain the activity of H2O.Besides,the "IHP adsorption effect" along with the low LUMO energy level of maltitol-CF3SO3-can promote the in-situ formation of an organic-inorganic complex solid electrolyte interface（SEI） layer.As a result,the hydrogen/oxygen evolution side reaction,corrosion,and dendrites issues are effectively suppressed,thereby leading to highly reversible and dendrite-free Zn plating/stripping.The Zn‖I2battery with hybrid electrolytes also demonstrates high electrochemical performance and ultralong cycling stability,showing a capacity retention of 75% over 20000 charge-discharge cycles at a large current density of 5 A g-1.In addition,the capacity of the device has almost no obvious decay over20000 cycles even at-30℃.This work offers a successful electrolyte regulation strategy via the IHP adsorption effect to design electrolytes for high-performance rechargeable Zn-ion batteries.

关键词： Adsorption effect Dendrite suppression Inner Helmholtz plane SEI layer Zn||I2 battery

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Fast Cycle Structure Detection for Power Grids Based on Graph Computing

引用

CSEE Journal of Power and Energy Systems 2023年第6期9卷 2204-2213页

作者： Xinqiao Wang Kewen Liu Weijiang Lu Ting zhao baohua zhao Xiaoming Liu the Computing&Application Technology Research Division Global Energy Interconnection Research InstituteBeijing 102209China

The cycle structure in a power grid may lower the stability of the network;thus,it is of great significance to accu-rately and timely detect cycles in power grid networks.However,detecting possible cycles in a large-scale network can be highly time consuming and computationally intensive.In addition,since the power grid's topology changes over time,cycles can appear and disappear,and it can be difficult to monitor them in real time.In traditional computing systems,cycle detection requires considerable computational resources,making real-time cycle detection in large-scale power grids an impossible task.Graph computing has shown excellent performance in many areas and has solved many practical graph-related problems,such as power flow calculation and state estimation.In this article,a cycle detection method,the Paton method,is implemented and optimized on a graph computing platform.Two cases are used to test its performance in an actual power grid topology scenario.The results show that the graph computing-based Paton method reduces the time consumption by at least 60%compared to that of other methods.

关键词： Cycle detection graph computing power grid distribution grid

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Prediction of specific spoilage organisms in smoked chicken legs with modified atmosphere packaging at 4 ℃ using multivariate statistical analysis

引用

Food Science and Human Wellness 2024年

作者： Qiang Wang Yubo zhao Yumeng Sui Qian Chen Zhiming Dong Qian Liu baohua Kong Ligang Qin College of Animal Science and Technology Northeast Agricultural University College of Food Science Northeast Agricultural University

The present study monitored bacterial succession， physicochemical properties， and volatile organic compounds (VOCs) changes in smoked chicken legs with modified atmosphere packaging (MAP， 60% CO2and 40% N2) during a 25-day storage period at 4 ℃. After 15 days of storage， Serratia proteamaculans and Pseudomonas fragi became the predominant bacteria. Furthermore， physicochemical properties changed significantly， as evidenced by an increase in thiobarbituric acid reactive substances and b* (yellowness) value， and a decrease in hardness. A total of 65 VOCs were identified during storage. Correlation between bacterial succession and quality indicators (including VOCs and physicochemical properties) allowed the identification of 26 core dominant bacteria， including S. proteamaculans， Psychrobacter alimentarius， Pseudomonas putide， and Pseudomonas poae， which were positively related to spoilage VOCs (e.g.， 1-octen-3-ol， 1-pentanol， and 3-methyl-1-butanol) and could be defined as specific spoilage organisms (SSOs). The results of this study provide a systematic approach to predict SSOs in smoked chicken legs during storage， which can also provide a basis for product safety.

关键词：

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Genetic analysis and candidate gene identification of salt tolerancerelated traits in maize

引用

Journal of Integrative Agriculture 2024年第7期23卷 2196-2210页

作者： Hui Fang Xiuyi Fu Hanqiu Ge Mengxue Jia Jie Ji Yizhou zhao Zijian Qu Ziqian Cui Aixia Zhang Yuandong Wang Ping Li baohua Wang Scientific Observing and Experimental Station of Maize in Plain Area of Southern Region Ministry of Agriculture and Rural Affairs/School of Life SciencesNantong UniversityNantong 226019China Maize Research Institute Beijing Academy of Agriculture and Forestry Sciences(BAAFS)Beijing 100097China

Soil salinization poses a threat to maize production worldwide,but the genetic mechanism of salt tolerance in maize is not well understood.Therefore,identifying the genetic components underlying salt tolerance in maize is of great importance.In the current study,a teosinte-maize BC2F7 population was used to investigate the genetic basis of 21 salt tolerance-related traits.In total,125 QTLs were detected using a high-density genetic bin map,with one to five QTLs explaining 6.05–32.02%of the phenotypic variation for each trait.The total phenotypic variation explained(PVE)by all detected QTLs ranged from 6.84 to 63.88%for each trait.Of all 125 QTLs,only three were major QTLs distributed in two genomic regions on chromosome 6,which were involved in three salt tolerance-related traits.In addition,10 pairs of epistatic QTLs with additive effects were detected for eight traits,explaining 0.9 to 4.44%of the phenotypic variation.Furthermore,18 QTL hotspots affecting 3–7 traits were identified.In one hotspot(L5),a gene cluster consisting of four genes(ZmNSA1,SAG6,ZmCLCg,and ZmHKT1;2)was found,suggesting the involvement of multiple pleiotropic genes.Finally,two important candidate genes,Zm00001d002090 and Zm00001d002391,were found to be associated with salt tolerance-related traits by a combination of linkage and marker-trait association analyses.Zm00001d002090 encodes a calcium-dependent lipid-binding(CaLB domain)family protein,which may function as a Ca^(2+)sensor for transmitting the salt stress signal downstream,while Zm00001d002391 encodes a ubiquitin-specific protease belonging to the C19-related subfamily.Our findings provide valuable insights into the genetic basis of salt tolerance-related traits in maize and a theoretical foundation for breeders to develop enhanced salt-tolerant maize varieties.

关键词： maize salt tolerance-related traits QTL mapping region-based association analysis

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

我国石化产业碳中和路径展望

引用

石油炼制与化工 2024年第1期55卷 62-67页

作者：戴宝华赵祺中国石化集团经济技术研究院有限公司北京100029

我国石化产业碳排放比例高,产业仍处于增长期,有增碳需求,实现“双碳”目标面临重大挑战,必须明确发展思路,积极稳妥推动产业低碳转型和高质量发展。当前,石化产业面临交通领域替代能源快速发展、化工品需求仍将增长、氢能载体作用凸显... 详细信息

我国石化产业碳排放比例高,产业仍处于增长期,有增碳需求,实现“双碳”目标面临重大挑战,必须明确发展思路,积极稳妥推动产业低碳转型和高质量发展。当前,石化产业面临交通领域替代能源快速发展、化工品需求仍将增长、氢能载体作用凸显、“双碳”政策持续发力等形势,需要在推动产业升级、开展节能降碳、推进清洁替代、突出创新引领、加强保障措施等方面持续发力。通过对产业结构调整、实施绿氢炼化、与CCUS融合发展等关键路径的分析和研判,在碳中和目标下提出一种可能的路径组合和趋势展望,分析不同阶段的发展特征并提出建议。

关键词：石化产业碳中和低碳转型路径展望

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Physiological and transcriptome analyses of Chinese cabbage in response to drought stress

引用

Journal of Integrative Agriculture 2024年第7期23卷 2255-2269页

作者： Lin Chen Chao Li Jiahao Zhang Zongrui Li Qi Zeng Qingguo Sun Xiaowu Wang Limin zhao Lugang Zhang baohua Li State Key Laboratory for Crop Stress Resistance and High-Efficiency Production College of HorticultureNorthwest A&F UniversityYangling 712100China Institute of Vegetables and Flowers Chinese Academy of Agricultural SciencesBeijing 100081China

Chinese cabbage is an important leafy vegetable crop with high water demand and susceptibility to drought stress.To explore the molecular mechanisms underlying the response to drought,we performed a transcriptome analysis of drought-tolerant and-sensitive Chinese cabbage genotypes under drought stress,and uncovered core droughtresponsive genes and key signaling pathways.A co-expression network was constructed by a weighted gene coexpression network analysis(WGCNA)and candidate hub genes involved in drought tolerance were identified.Furthermore,abscisic acid(ABA)biosynthesis and signaling pathways and their drought responses in Chinese cabbage leaves were systemically explored.We also found that drought treatment increased the antioxidant enzyme activities and glucosinolate contents significantly.These results substantially enhance our understanding of the molecular mechanisms underlying drought responses in Chinese cabbage.

关键词： Chinese cabbage drought stress abscisic acid weighted gene co-expression network analysis glucosinolate

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：