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Loading capacity and emulsification phenomena of HREE extraction by dialkylphosphinic acids with different β,γ,δ-substituents

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Journal of Rare Earths 2024年第1期42卷 191-199,I0007页

作者： Junlian Wang Guodong Xu Wen Xu Jianguo Cui yufu Chen Ziyong Chang School of Civil and Resource Engineering University of Science and Technology BeijingBeijing100083China Key Laboratory of Ministry of Education for Efficient Mining and Safety of Metal Mines Beijing100083China State Key Laboratory of Baiyunobo Rare Earth Resource Researches and Comprehensive Utilization Baotou Research Institute of Rare EarthsBaotou014030China

The relationship between dialkylphosphinic acid structure and their loading capacity for HREEs and emulsification phenomena has rarely been *** this paper,we took Lu extraction as an example to study the effect of β,γ,δ-substituents of dialkylphosphinic acids on their loading capacity and anti-emulsification performance for *** discuss conveniently,the dialkylphosphinic acids were classified into two groups:β-substituent group(P208,INET-1,P218,USTB-1 and P227)and γ,δ-substituent group(P218,P2132 and Cyanex 272).For β-substituent group extractants,their loading capacities are in the order P208(299.7 mg/L)≈INET-1(299.5 mg/L)>P218(270.8 mg/L)>>USTB-1(163.1 mg/L)>P227(151.4 mg/L),while their anti-emulsification/gelation performances are just in the opposite order P227>USTB-1>P218>P208≈INET-1 under the studied *** γ,δ-substituent group extractants,their loading capacities are in the order P218(270.8 mg/L)>P2132(192.3 mg/L)>Cyanex272(131.7 mg/L),while the anti-emulsification performance of P218 is better than those of P2132 and Cyanex *** loading capacity data given in the parentheses are obtained through repeatedly extracting Lu from ~4×10^(-4)mol/L of Lu aqueous feed solution with initial pH of 2.40 by 0.01 mol/L extractant at phase ratio A/O of 1:1.

关键词： Heavy rare earth element Dialkylphosphinic acid Extraction Loading capacity Emulsification

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New steelmaking process based on clean deoxidation technology

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International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1249-1262页

作者： Zhongliang Wang Yanping bao State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

After the converter steelmaking process,a considerable number of ferroalloys are needed to remove dissolved oxygen from the molten steel,but it also forms a lot of oxide inclusions that cannot be completely *** the same time,it increases the carbon emis-sions in the steel production *** years of research,our team have developed a series of clean deoxidation technologies,includ-ing carbon deoxidation,hydrogen deoxidation,and waste plastic deoxidation of molten steel to address the aforementioned *** this study,thermodynamic calculations and laboratory experiments were employed to verify that carbon and hydrogen can reduce the total oxygen content in the molten steel melt to below 5×10^(-6) and 10×10^(-6),*** analysis of the deoxidation mechanisms and ef-fects of polyethylene and polypropylene was also *** addition,the applications of carbon deoxidation technology in different steels with the hot-state experiment and industrial production were discussed *** carbon deoxidation experimental results of different steels were as follows:(1)the oxygen content of bearing steel was effectively controlled at 6.3×10^(-6) and the inclusion number density was lowered by 74.73%compared to aluminum deoxidized bearing steel;(2)the oxygen content in gear steel was reduced to 7.7×10^(-6) and a 54.49%reduction of inclusion number density was achieved with almost no inclusions larger than 5μm from the average level of industry gear steels;(3)a total oxygen content of M2 high-speed steel was as low as 3.7×10^(-6).In industrial production practice,car-bon deoxidation technique was applied in the final deoxidation stage for non-aluminum deoxidized bearing steel,and it yielded excellent results that the oxygen content was reduced to below 8×10^(-6) and the oxide inclusions in the steel mainly consist of silicates,along with small amounts of spinel and calcium aluminate.

关键词： clean deoxidation carbon deoxidation hydrogen deoxidation waste plastics deoxidation

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Development and prospects of molten steel deoxidation in steelmaking process

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International Journal of Minerals,Metallurgy and Materials 2024年第1期31卷 18-32页

作者： Zhongliang Wang Yanping bao State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

In the long traditional process of steelmaking,excess oxygen is blown into the converter,and alloying elements are used for *** inevitably results in excessive deoxidation of products remaining within the steel liquid,affecting the cleanliness of the *** the increasing requirements for steel performance,reducing the oxygen content in the steel liquid and ensuring its high cleanliness is *** more than a hundred years of development,the total oxygen content in steel has been reduced from approximately 100×10^(-6)to approximately 10×10^(-6),and it can be controlled below 5×10^(-6)in some steel grades.A relatively stable and mature deoxidation technology has been formed,but further reducing the oxygen content in steel is no longer significant for improving steel *** research team developed a deoxidation technology for bearing steel by optimizing the entire conventional *** technology combines silicon–manganese predeoxidation,ladle furnace diffusion deoxidation,and vacuum final *** successfully conducted industrial experiments and produced interstitial-free steel with natural decarbonization ***-aluminum deoxidation was found to control the oxygen content in bearing steel to between 4×10^(-6) and 8×10^(-6),altering the type of inclusions,eliminating large particle Ds-type inclusions,improving the flowability of the steel liquid,and deriving a higher fatigue *** natural decarbonization predeoxidation of interstitial-free steel reduced aluminum consumption and production costs and significantly improved the quality of cast billets.

关键词： steel deoxidation deoxidizer metallurgical equipment bearing steel IF steel

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Protein acetylation sites with complex-valued polynomial model

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Frontiers of Computer Science 2024年第3期18卷 217-226页

作者： Wenzheng bao Bin YANG School of Information Engineering Xuzhou University of TechnologyXuzhou 221018China School of Information Science and Engineering Zaozhuang UniversityZaozhuang 277160China

Protein acetylation refers to a process of adding acetyl groups(CH3CO-)to lysine residues on protein *** one of the most commonly used protein post-translational modifications,lysine acetylation plays an important role in different *** our study,we developed a humanspecific method which uses a cascade classifier of complexvalued polynomial model(CVPM),combined with sequence and structural feature descriptors to solve the problem of imbalance between positive and negative *** gene expression programming and differential evolution are utilized to search the optimal CVPM *** also made a systematic and comprehensive analysis of the acetylation data and the prediction *** performances of our proposed method are 79.15%in Sp,78.17%in Sn,78.66%in ACC 78.76%in F1,and 0.5733 in MCC,which performs better than other state-of-the-art methods.

关键词： protein acetylation complex-valued polynomial model machine learning

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Global warming strengthens the association between ENSO and the Asian-Australian summer monsoon

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Science China Earth Sciences 2024年第1期67卷 309-312页

作者： bao YANG Minhui HE School of Geography and Ocean Science Nanjing UniversityNanjing 210093China Key Laboratory of Desert and Desertification Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China

Previous studies have widely reported the linkages between Asian-Australian monsoon and the ENSO(Wu,2008;Azad and Rajeevan,2016;Chen et al.,2020;Shekhar et al.,2022;Zhang J et al.,2022;Chen et al.,2023;Hau et al.,2023;Heidemann et al.,2023).It is well accepted that the monsoon is weaker during the El Niño phase and stronger during the La Niña *** example,an anomalously strong western Pacific subtropical high in 2020,related to the La Niña event.

关键词： event monsoon Asian

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Hybrid tri-memristor hyperchaotic map and application in Wasserstein Generative Adversarial Nets

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Science China(Technological Sciences) 2024年第6期67卷 1855-1865页

作者： GU Yang bao Han YU XiHong HUA ZhongYun bao BoCheng XU Quan School of Microelectronics and Control Engineering Changzhou UniversityChangzhou213159China School of Computer Science and Technology Harbin Institute of TechnologyShenzhen518055China

Inspired by basic circuit connection methods,memristors can also be utilized in the construction of complex discrete chaotic *** investigate the dynamical effects of hybrid memristors,we propose two hybrid tri-memristor hyperchaotic(HTMH)mapping structures based on the hybrid parallel/cascade and cascade/parallel operations,*** the HTMH mapping structure with hybrid parallel/cascade operation as an example,this map possesses a spatial invariant set whose stability is closely related to the initial states of the *** distributions and bifurcation behaviours dependent on the control parameters are explored with numerical ***,the memristor initial offset-boosting mechanism is theoretically demonstrated,and memristor initial offset-boosting behaviours are numerically *** results clarify that the HTMH map can exhibit hyperchaotic behaviours and extreme multistability with homogeneous coexisting infinite *** addition,an FPGA hardware platform is fabricated to implement the HTMH map and generate pseudorandom numbers(PRNs)with high ***,the generated PRNs can be applied in Wasserstein generative adversarial nets(WGANs)to enhance training stability and generation capability.

关键词： memristor hybrid tri-memristor map spatial invariant set hyperchaos extreme multistability generative adversarial nets

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Loss of heterozygosity on 10q23.3 and mutation of tumor suppressor gene PTEN in gastric cancer and precancerous lesions

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World Journal of Gastroenterology 2005年第2期11卷 285-288页

作者： Yi-LingLi ZhongTian Dong-YingWu bao-yufu YahXin DepartmentofGastroenterology FirstHospitalofChinaMedicalUniversitySh_enyang110001LiaoningProvinceofChina DepartmentofSurgery SecondHospitalofChinaMedicalUniversityShenyang110003LiaoningProvinceChina TheFourthLaboratory CancerInstituteFirstHospitalofChinaMedicalUniversityShenyang110001LiaoningProvinceChina

AIM: To investigate the loss of heterozygosity (LOH) and mutation of tumor suppressor gene PTEN in gastric cancer and precancerous ***: Thirty cases of normal gastric mucosa, advanced and early stage gastric cancer, intestinal metaplasia, atrophic gastritis, and atypical hyperplasia were analyzed for PTEN LOH and mutations within the entire coding region of PTEN gene by PCR-SSCP denaturing PAGE gel electrophoresis,and PTEN mutation was detected by PCR-SSCP sequencing followed by silver ***: LOH rate found in respectively atrophic gastritis was 10% (3/30), intestinal metaplasia 10% (3/30), atypical hyperpiasia 13.3% (4/30), early stage gastric cancer 20%(6/30), and advanced stage gastric cancer 33.3% (9/30),None of the precancerous lesions and early stage gastric cancer showed PTEN mutations, but 10% (3/30) of the advanced stage gastric cancers, which were all positive for LOH, showed PTEN ***: LOH of PTEN gene appears in precancerous lesions, and PTEN mutations are restricted to advanced gastric cancer, LOH and mutation of PTEN gene are closely related to the infiltration and metastasis of gastric cancer.

关键词：异型结合性 10q23.3 基因突变肿瘤抑制基因 PTEN 胃癌癌症前期损害消化系统 LOH

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Quantitative estimation of global mean precipitation throughout the Phanerozoic era

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Science China Earth Sciences 2024年第5期67卷 1616-1624页

作者： Xiujuan bao Yongyun HU Laboratory for Climate and Ocean-Atmospheric Studies Department of Atmospheric and Oceanic SciencesSchool of PhysicsPeking UniversityBeijing 100871China

Quantitatively estimating the global mean precipitation(GMP)throughout Earth's history is crucial for enhancing our understanding of long-term climate evolution and the hydrological ***,currently there is no established methodology for estimating global mean ***,we present the first study that estimates GMP in the Phanerozoic *** relationship between GMP and global mean surface temperature(GMST)is investigated by analyzing data from 23 models in the Coupled Model Intercomparison Project phase 6(CMIP6).The result reveals consistent and significant impact of temperature on precipitation,with a sensitivity range of 2–3%K^(-1).Additionally,we propose a method for accessing latitudinal variations in precipitation caused by land area distributions and paleo-Koppen climatic *** climatic belts are determined based on geological indicators such as coals,evaporites,and glacial *** GMP is thus quantitatively estimated by combining variations in GMST,land area distributions,and paleo-koppen climatic belts,spanning from 540 Ma to the present *** quantitative GMP curve demonstrates fluctuations in GMP about 500 mm yr^(-1),with values ranging from 948 to1442 mm yr-1over the Phanerozoic *** curve aligns closely with findings derived from numerical *** presented paleoprecipitation variations facilitate a more comprehensive understanding of the interconnected geological and paleoclimatic developments.

关键词： Paleoprecipitation Paleoclimate K?ppen climatic belts Global mean precipitation Hydrological cycle

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Interfacial tribochemical kinetics: A new perspective on superlubricity of diamond-like carbon films

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Science China(Technological Sciences) 2024年第7期67卷 2050-2052页

作者： CHEN WeiQi MA Tian-bao State Key Laboratory of Tribology in Advanced Equipment Tsinghua UniversityBeijing 100084China

Friction is considered one of the primary challenges affecting the performance of machine operations and is a significant source of energy loss in industrial applications. About 30%of disposable energy is consumed by ... 详细信息

关键词： kinetics friction operations

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Spatiotemporal changes of gross primary productivity and its response to drought in the Mongolian Plateau under climate change

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Journal of Arid Land 2024年第1期16卷 46-70页

作者： ZHAO Xuqin LUO Min MENG Fanhao SA Chula bao Shanhu bao Yuhai College of Geographical Science Inner Mongolia Normal UniversityHohhot 010022China Inner Mongolia Key Laboratory of Remote Sensing and Geographic Information Systems Hohhot 010022China

Gross primary productivity(GPP)of vegetation is an important constituent of the terrestrial carbon sinks and is significantly influenced by *** the impact of droughts on different types of vegetation GPP provides insight into the spatiotemporal variation of terrestrial carbon sinks,aiding efforts to mitigate the detrimental effects of climate *** this study,we utilized the precipitation and temperature data from the Climatic Research Unit,the standardized precipitation evapotranspiration index(SPEI),the standardized precipitation index(SPI),and the simulated vegetation GPP using the eddy covariance-light use efficiency(EC-LUE)model to analyze the spatiotemporal change of GPP and its response to different drought indices in the Mongolian Plateau during *** main findings indicated that vegetation GPP decreased in 50.53% of the plateau,mainly in its northern and northeastern parts,while it increased in the remaining 49.47%***,meadow steppe(78.92%)and deciduous forest(79.46%)witnessed a significant decrease in vegetation GPP,while alpine steppe(75.08%),cropland(76.27%),and sandy vegetation(87.88%)recovered *** aridification areas accounted for 71.39% of the affected areas,while 28.53% of the areas underwent severe aridification,mainly located in the south and central ***,the warming aridification areas of desert steppe(92.68%)and sandy vegetation(90.24%)were *** warming was found to amplify the sensitivity of coniferous forest,deciduous forest,meadow steppe,and alpine steppe GPP to ***,the drought sensitivity of vegetation GPP in the Mongolian Plateau gradually decreased as altitude *** cumulative effect of drought on vegetation GPP persisted for 3.00-8.00 *** findings of this study will improve the understanding of how drought influences vegetation in arid and semi-arid areas.

关键词： gross primary productivity(GPP) climate change warming aridification areas drought sensitivity cumulative effect duration(CED) Mongolian Plateau

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