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Impact chaos control and stress release——A key for development of ultra fine vibration milling

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Progress in Natural science:Materials International 2002年第5期12卷 18-23页

作者： WANG Shulin(Department of Power Engineering, university of shanghai for science and technology, shanghai 200093, china) shanghai Univ Sci & Technol Dept Power Engn Shanghai 200093 Peoples R China

Through our previous experimental and analytical studies, it has been discovered that the key for the development of vibration milling is the impact chaos control and stress release. The necessities for the chaos control and stress release are: (i) to strictly e-liminate the sub-harmonics; (ii) to control the super-harmonics to a lower level and (iii) to load the system compressively with relatively higher period, in order that the vibration energy can be absorbed by the particles effectively and sufficiently. A new vibration model for ultra fine milling is proposed, which has wide applications in preparing ultra fine particles.

关键词： vibration mills ultra fine milling impact chaos control stress release.

Recovery of Li, Ni, Co and Mn from spent lithium-ion batteries assisted by organic acids: Process optimization and leaching mechanism

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International Journal of Minerals,Metallurgy and Materials 2024年第3期31卷 518-530页

作者： liuyi Ren Bo liu Shenxu bao Wei Ding Yimin Zhang Xiaochuan Hou Chao lin Bo Chen School of Resources and Environmental Engineering Wuhan University of TechnologyWuhan 430070China State Environmental Protection Key Laboratory of Mineral Metallurgical Resources Utilization and Pollution Control Wuhan University of Science and TechnologyWuhan 430081China Zhejiang New Era Zhongneng Recycling technology Co. LtdShaoxing 312000China Shenzhen Water Planning&Design institute Co. LtdShenzhen 518000China

The proper recycling of spent lithium-ion batteries(LIBs)can promote the recovery and utilization of valuable resources,while also negative environmental effects resulting from the presence of toxic and hazardous *** this study,a new environmentally friendly hydro-metallurgical process was proposed for leaching lithium(Li),nickel(Ni),cobalt(Co),and manganese(Mn)from spent LIBs using sulfuric acid with citric acid as a *** effects of the concentration of sulfuric acid,the leaching temperature,the leaching time,the solid-liquid ratio,and the reducing agent dosage on the leaching behavior of the above elements were *** parameters were optimized using response surface methodology(RSM)to maximize the recovery of metals from spent *** maxim-um recovery efficiencies of Li,Ni,Co,and Mn can reach 99.08%,98.76%,98.33%,and 97.63%.under the optimized conditions(the sulfuric acid concentration was 1.16 mol/L,the citric acid dosage was 15wt%,the solid-liquid ratio was 40 g/L,and the temperature was 83℃ for 120 min),*** was found that in the collaborative leaching process of sulfuric acid and citric acid,the citric acid initially provided strong reducing CO_(2)^(-),and the transition metal ions in the high state underwent a reduction reaction to produce transition metal ions in the low ***,citric acid can also act as a proton donor and chelate with lower-priced transition metal ions,thus speeding up the dissolution process.

关键词： spent lithium-ion batteries leaching response surface methodology sulfuric acid citric acid

Risk Factors of Depression Screened by Two-Sample Mendelian Randomization Analysis:A Systematic Review

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Biomedical and Environmental sciences 2024年第1期37卷 85-95页

作者： WANG Han lin XUE Yan Feng CUI bao Qiu liu Hong SHEN Xin Xin Shandong Provincial Research Center for Bioinformatic Engineering and Technique School of Life SciencesShandong University of TechnologyZibo 255049ShandongChina Shanxi Province Cancer Hospital/Shanxi Hospital Affiliated to Cancer Hospital Chinese Academy of Medical Sciences/Cancer Hospital Affiliated to Shanxi Medical UniversityTaiyuan 030013ShanxiChina State Key Laboratory of Infectious Disease Prevention and Control National Institute for Viral Disease Control and PreventionChinese Center for Disease Control and PreventionBeijing 102206China

Objective This study explored the potentially modifiable factors for depression and major depressive disorder(MDD)from the MR-Base database and further evaluated the associations between drug targets with *** We analyzed two-sample of Mendelian randomization(2SMR)using genetic variant depression(n=113,154)and MDD(n=208,811)from Genome-Wide Association Studies(GWAS).Separate calculations were performed with modifiable risk factors from MR-Base for 1,001 *** MR analysis was performed by screening drug targets with MDD in the DrugBank database to explore the therapeutic targets for *** variance weighted(IVW),fixed-effect inverse variance weighted(FE-IVW),MR-Egger,weighted median,and weighted mode were used for complementary *** The potential causal relationship between modifiable risk factors and depression contained 459 results for depression and 424 for ***,the associations between drug targets and MDD showed that SLC6A4,GRIN2A,GRIN2C,SCN10A,and IL1B expression are associated with an increased risk of *** contrast,ADRB1,CHRNA3,HTR3A,GSTP1,and GABRG2 genes are candidate protective factors against *** This study identified the risk factors causally associated with depression and MDD,and estimated 10 drug targets with significant impact on MDD,providing essential information for formulating strategies to prevent and treat depression.

关键词： Risk factors Drug targets Depression Major depressive disorder Two-sample Mendelian randomization

Confined Mn^(2+) enables effective aerobic oxidation catalysis

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science china Chemistry 2024年第5期67卷 1545-1553页

作者： Desheng Yuan Sicong Ma Xiao Kong Chi Zhang lin Chen Chengsheng Yang Lihua Wang Zhen liu lin Ye Yongmei liu Rui Ma Zhi-Pan liu Yifeng Zhu Yong Cao Xinhe bao Department of Chemical Physics University of Science and Technology of ChinaHefei 230026China Department of Chemistry Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsCollaborative Innovation Center of Chemistry for Energy MaterialsFudan UniversityShanghai 200438China Key Laboratory of Synthetic and Self-Assembly Chemistry for Organic Functional Molecules Shanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China School of Materials and Chemistry University of Shanghai for Science and TechnologyShanghai 200093China shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China institute of Advanced Fluorine-Containing Materials Zhejiang Normal UniversityJinhua 321004China State Key Laboratory of Catalysis National Laboratory for Clean EnergyCollaborative Innovation Center of Chemistry for Energy MaterialsDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China

Effective and mild activation of O_(2) is essential but challenging for aerobic oxidation. In heterogeneous catalysis, high-valence manganese oxide(e.g., +4) is known to be active for the oxidation, whereas divalent MnO is ineffective due to its limited capacity to supply surface oxygen and its thermodynamically unstable structure when binding O_(2) in reaction conditions. Inspired by natural enzymes that rely on divalent Mn^(2+), we discovered that confining Mn^(2+) onto the Mn_(2)O_(3) surface through a dedicated calcination process creates highly active catalysts for the aerobic oxidation of 5-hydroxymethylfurfural, benzyl alcohol, and *** Mn_(2)O_(3)-confined Mn^(2+) is undercoordinated and efficiently mediates O_(2) activation, resulting in 2–3 orders of magnitude higher activity than Mn_(2)O_(3) alone. Through low-temperature infrared spectroscopy, we distinguished low-content Mn^(2+) sites at Mn_(2)O_(3) surface, which are difficult to be differentiated by X-ray photoelectron spectroscopy. The combination of in-situ energydispersive X-ray absorption spectroscopy and X-ray diffraction further provides insights into the formation of the newly identified active Mn^(2+) sites. By optimizing the calcination step, we were able to increase the catalytic activity threefold *** finding offers promising frontiers for exploring active oxidation catalysts by utilizing the confinement of Mn^(2+)and oftenignored calcination skills.

关键词： confinement catalysis manganese oxide aerobic oxidation divalent Mn^(2+) operando spectroscopies

EMMA:An Efficient Massive Mapping Algorithm Using Improved Approximate Mapping Filtering

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Acta Biochimica et Biophysica Sinica 2006年第12期38卷 857-864页

作者： Xin ZHANG~1 Zhi-Wei CAO~2 Zhi-Xin lin~3 Qing-Kang WANG~1* Yi-Xue LI~4 1 institute of Micro/Nano science and technology,shanghai Jiaotong university,shanghai 200030,china 2 shanghai Center for Bioinformation technology,shanghai 200235,china 3 College of Life science and technology,shanghai Jiaotong university,shanghai 200030,china 4 Bioinformation Center of shanghai institutes for Biological sciences,Chinese Academy of sciences,shanghai 200031,china institute of Micro/Nano science and technology Shanghai Jiaotong UniversityShanghai 200030 China shanghai Center for Bioinformation technology Shanghai 200235 China College of Life science and technology Shanghai Jiaotong UniversityShanghai 200030 China Bioinformation Center of shanghai institutes for Biological sciences Chinese Academy of SciencesShanghai 200031 China

Efficient massive mapping algorithm (EMMA),an algorithm on efficiently mapping massivecDNAs onto genomic sequences,has recently been *** process of mapping massive cDNAsonto genomic sequences has been improved using more approximate mapping filtering based on an enhancedsuffix array coupled with a pruned fast hash table,algorithms of block alignment extensions,and *** compared with the classical BLAT software in this field,the computing of EMMA ranges fromtwo to forty-one times faster under similar prediction precisions.

关键词： cDNA mapping maximal exact match enhanced suffix array pruned fast hash table extension algorithm

Nonsmooth Equations of K-T Systems for a Constrained Minimax Problem

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Journal of Systems Engineering and Electronics 2003年第2期14卷 31-35页

作者： Gao Yan School of Management, university of shanghai for science and technology, shanghai 200093, P. R. china School of Management University of Shanghai for Science and Technology Shanghai 200093 P. R. China

Using K-T optimality condition of nonsmooth optimization, we establish two equivalent systems of the nonsmooth equations for the constrained minimax problem directly. Then generalized Newton methods are applied to solve these systems of the nonsmooth equations. Thus a new approach to solving the constrained minimax problem is developed.

关键词： Optimization Minimax problems Nonsmooth equations Generalized Newton methods.

Particle size characterization by ultrasonic attenuation spectra

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Particuology 2008年第4期6卷 276-281页

作者： Mingxu Su, Minghua Xue, Xiaoshu Cai, Zhitao Shang, Feng Xu institute of Particle and Two-Phase Flow Measurement, university of shanghai for science and technology, shanghai 200093, china institute of Particle and Two-Phase Flow Measurement University of Shanghai for Science and Technology Shanghai 200093 China

This paper contributes to extracting information from signals of broadband ultrasonic attenuation spectrum for effective utilization in particle size characterization. The single particle scattering model and the coupled-phase model are formulated simultaneously, the relationship between particle size distribution and ultrasonic spectrum is established, and a convergence criterion for calculation is quantified. Demonstration inversion by the optimum regularization factor method is carried out to yield typical numerical results for discussion. With the experimental set-up developed by the institute of Particle and Two-Phase Flow Measurement (IPTFM) at the university of shanghai for science and technology, sand sediment particle size is measured by attenuation spectrum and analyzed using the above inversion algorithm and theoretical models. To validate the proposed ultrasonic spectrum particle sizing method, results are compared with those obtained by microscopy.

关键词： Ultrasonic spectrum Particle Size Inversion

Enhanced activity of yqhD oxidoreductase in synthesis of 1,3-propanediol by error-prone PCR

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Progress in Natural science:Materials International 2008年第12期18卷 1519-1524页

作者： Hongmei Li~a Jia Chen~a Yinghua Li~b a institute of Food science and Biological technology,university of shanghai for science and technology,shanghai 200093,china b institute of Pharmaceutical Engineering,Zhejiang university,Hangzhou 310027,china institute of Food science and Biological technology University of Shanghai for Science and Technology Shanghai 200093 China institute of Pharmaceutical Engineering Zhejiang University Hangzhou 310027 China

yqhD oxidoreductase was determined to be an NADP-dependent dehydrogenase,and was more active toward 3-HPA when compared to 1,3-propanediol *** further improve enzyme activity towards 3-hydroxypropionaldehyde (3-HPA),error-prone PCR was implemented to mutant yqhD *** mutants,D99QN147H and Q202A with increased catalytic and affinity efficiency,were obtained after one round of error-prone polymerase chain *** the catalytic efficiency of the mutant D99QN147H was up to 4-fold greater than the wild enzyme (0.0375 min-1mM-1vs.0.0078 min-1mM-1).The recombined strain containing pEY28yqhD D99QN147H yielded 28 g L-1of 1,3-propanediol in the fed-batch LB cultures (1 L volume) with an initial 3-HPA concentration of 40 g L-1,which was higher than the 21 and 17 g L-1of 1,3-propanediol from the mutant Q202A and the wild-type,*** for propionaldehyde,the optimal mutant D99QN147H also exhibited higher activity on a range of substituted aldehydes than the wild- type.

关键词： yqhD oxidoreductase Error-prone PCR Catalytic efficiency 1,3-Propanediol

Cauchy Problem for Quasilinear Hyperbolic Systems with Higher Order Dissipative Terms

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Acta Mathematicae Applicatae Sinica 2003年第1期19卷 71-82页

作者： Wei-guo ZhangDepartment of Basic sciences, university of shanghai for science and technology, shanghai 200093, china Department of Basic sciences University of Shanghai for Science and Technology Shanghai China

Abstract In this paper, the author studies the global existence, singularities and life span of smooth solutions of the Cauchy problem for a class of quasilinear hyperbolic systems with higher order dissipative terms ... 详细信息

关键词： Keywords Cauchy problem Dissipative term Genuinely nonlinear linearly degenerate