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Composition Engineering Opens an Avenue Toward Efficient and Sustainable Nitrogen Fixation

Energy & Environmental Materials 2024年第1期7卷 313-325页

作者： Xiaolin Wang liming Yang Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of EducationWuhan 430074China Hubei Key Laboratory of Materials Chemistry and Service Failure Wuhan 430074China Hubei Key Laboratory of Bioinorganic Chemistry and Materia Medica Wuhan 430074China Hubei Engineering Research Center for Biomaterials and Medical Protective Materials Wuhan 430074China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074China

In this work,we open an avenue toward rational design of potential efficient catalysts for sustainable ammonia synthesis through composition engineering strategy by exploiting the synergistic effects among the active sites as exemplified by diatomic metals anchored graphdiyne via the combination of hierarchical high-throughput screening,first-principles calculations,and molecular dynamics *** 43 highly efficient catalysts feature ultralow onset potentials(|U_(onset)|≤0.40 V)with Rh-Hf and Rh-Ta showing negligible onset potentials of 0 and-0.04 V,*** high catalytic activities of Rh-Hf and Rh-Ta can be ascribed to the synergistic *** forming heteronuclears,the combinations of relatively weak(such as Rh)and relatively strong(such as Hf or Ta)components usually lead to the optimal strengths of adsorption Gibbs free energies of reaction *** origin can be ascribed to the mediate d-band centers of Rh-Hf and Rh-Ta,which lead to the optimal adsorption strengths of intermediates,thereby bringing the high catalytic *** work provides a new and general strategy toward the architecture of highly efficient catalysts not only for electrocatalytic nitrogen reduction reaction(eNRR)but also for other important *** expect that our work will boost both experimental and theoretical efforts in this direction.

关键词： composition engineering strategy diatomic catalysts electrocatalytic nitrogen reduction reaction first-principles calculations graphdiyne hierarchical high-throughput screening synergistic effects

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A low-power Bluetooth-based wireless sensor network and its global confliction-solving impact localization method

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Chinese Journal of Aeronautics 2024年第1期37卷 153-161页

作者： Yuanjia WANG Lei QIU Qiyun XU liming SHI College of Aerospace Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China Department of Electrical and Electronic Engineering University of EdinburghEdinburgh EH89YLUK

During the whole service lifetime of aircraft structures with composite materials,impacts are inevitable and can usually cause severe but barely visible *** the occurrences of impact are random and unpredictable,it is a hotspot direction to develop an online impact monitoring system that can meet strict limitations of aerospace applications including small size,light weight,and low power ***(PZT)sensor,being able to generate impact response signals with no external power and cover a large-scale structure with only a small amount of them,is a promising ***,for real systems,networks with multiple nodes are normally required to monitor large-scale structures in a global way to identify any impact localization confliction,yet the existing studies are mostly evaluated with single nodes instead of ***,in this paper,based on a new low-power node designed,a Bluetooth-based digital impact monitoring PZT sensor network is proposed for the first time with its global confliction-solving impact localization *** of the system as a network are researched and analyzed on a complex real aircraft wing box for a global confliction-solving impact localization,showing a satisfying high accuracy.

关键词： Bluetooth-based low-power design Confliction-solving evaluation Complex composites Piezoelectric sensors Wireless impact monitoring network

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Vitrification cryopreservation of ligaments based on zwitterionic betaine

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Chinese Journal of Chemical Engineering 2024年第8期72卷 1-9页

作者： liming Zhang Xinmeng Liu Haoyue Li Lei Zhang Department of Biochemical Engineering Frontier Science Center for Synthetic Biology and Key Laboratory of Systems Bioengineering(MOE)School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300350China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Ligament cryopreservation enables a prolonged shelf life of allogeneic ligament grafts,which is fundamentally important to ligament ***,conventional cryopreservation techniques fail to eliminate the damage caused by ice crystal growth and the toxicity of cryopreservation agents(CPAs).Here,we report a novel CPA vitrification formulation primarily composed of betaine for ligament *** optimization was conducted on the methods for vitrification and rewarming,as well as the loading and unloading conditions,based on the critical cooling rate(CCR),critical warming rate(CWR),and permeation properties of the *** biomechanical and histological level tests,we demonstrate the superior performance of our method in ligament *** 30 days of vitrification cryopreservation,parameters such as the Young's modulus,tensile stress,denaturation temperature,and glycosaminoglycans content of the ligament remained essentially *** work pioneers the application of ice-free cryopreservation for ligament and holds great potential for improving the long-term storage of ligament,providing valuable insights for future cryopreservation technique development.

关键词： Ligament Betaine Vitrification Cryopreservation

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Sulfated peptides and their receptors:Key regulators of plant development and stress adaptation

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Plant Communications 2024年第6期5卷 44-56页

作者： liming He Liangfan Wu Jia Li Ministry of Education Key Laboratory of Cell Activities and Stress Adaptations School of Life SciencesLanzhou UniversityLanzhou 730000China Guangdong Provincial Key Laboratory of Plant Adaptation and Molecular Design School of Life SciencesGuangzhou UniversityGuangzhou 510006China

Four distinct types of sulfated peptides have been identiﬁed in Arabidopsis *** peptides play crucial roles in regulating plant development and stress *** studies have revealed that Xan-thomonas and Meloidogyne can secrete plant-like sulfated peptides,exploiting the plant sulfated peptide signaling pathway to suppress plant *** the past three decades,receptors for these four types of sulfated peptides have been identiﬁed,all of which belong to the leucine-rich repeat receptor-like protein kinase subfamily.A number of regulatory proteins have been demonstrated to play important roles in their corresponding signal transduction *** this review,we comprehensively summarize the discov-eries of sulfated peptides and their receptors,mainly in Arabidopsis *** also discuss their known biological functions in plant development and stress ***,we put forward a number of ques-tions for reference in future studies.

关键词： peptide hormone sulfated peptide receptor-like protein kinase plant development stress adaptation

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Polyoxometalates for continuous power generation by atmospheric humidity

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Nano Research 2024年第3期17卷 1875-1885页

作者： Tuo Ji Weilin Chen Zhenhui Kang liming Zhang Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Northeast Normal UniversityChangchun 130024China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices DepartmentSoochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyTaipaMacao 999078China Institute of Functional State Key Laboratory of Luminescence and Applications Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China

Atmospheric humidity is a sustainable low-value energy widely existing in natural environment,which is a promising candidate to solve the noncontinuous and low efficiency of low-value energy power *** the mono-substituted Dawson-type polyoxometalates are constructed to be highly dispersed organic ammonium-polyoxoanion clusters and are assembled into thin films power generators with micropores,working in atmospheric *** optimal polyoxometalates generator with the thickness of 7.2μm and the area of 0.36 cm^(2) produces a voltage of 0.68 V and a current density of 19.5μA·cm^(-2) under simulated natural environment,and works continuously and stably under almost all-natural environments(humidity 10%–90%).The highly dispersed polyoxometalate nanoclusters can form microporous in polyoxometalate films to effectively absorb atmospheric humidity and spontaneously form distribution gradient of water,which is the structural basis of power *** continuous power generation may be maintained by the effective adsorption and utilization of H_(2)O,the huge electrostatic field of organic ammonium-polyoxoanion clusters,and the reasonably designed polyoxometalates containing inorganic small ions with high *** is the first humidity generator designed with polyoxometalates,which may provide a new research direction for polyoxometalates in sustainable utilization of low-value energy.

关键词： atmospheric humidity continuous power generations nanomaterials polyoxoanions polyoxometalates

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Cyber-Syndrome:Concept,Theoretical Characterization,and Control Mechanism

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Tsinghua Science and Technology 2024年第3期29卷 721-735页

作者： Feifei Shi Huansheng Ning liming Chen Sahraoui Dhelim School of Computer and Communication Engineering University of Science and Technology BeijingBeijing 100083China Faculty of Computing Ulster UniversityNewtownabbeyBT370QBUK School of Computer Science University College DublinDublinD04 V1W8Ireland

The prevalence of social media and mobile computing has led to intensive user engagement in the emergent Cyber-Physical-Social-Thinking(CPST)***,the easy access,the lack of governance,and excessive use has generated a raft of new behaviors within CPST,which affects users’physical,social,and mental *** this paper,we conceive the Cyber-Syndrome concept to denote the collection of cyber disorders due to excessive or problematic Cyberspace interactions based on CPST *** we characterize the Cyber-Syndrome concept in terms of Maslow’s theory of Needs,from which we establish an in-depth theoretical understanding of Cyber-Syndrome from its etiology,formation,symptoms,and ***,we propose an entropy-based Cyber-Syndrome control mechanism for its computation and *** goal of this study is to give new insights into this rising phenomenon and offer guidance for further research and development.

关键词： Cyber-Syndrome cyber-physical systems Cyber-Physical-Social-Thinking(CPST)space Maslow’sHierarchy of Needs entropy

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Characterization of size-resolved effective density of atmospheric particles in an urban atmosphere in Southern China

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Journal of Environmental Sciences 2024年第7期141卷 194-204页

作者： Tingting Xie liming Cao Jinyi Zheng Peng Xuan Xiaofeng Huang Laboratory of Atmospheric Observation Supersite School of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China

Effective density(ρ_(eff))is one of the most important physical properties of atmospheric particles,providing important references in exploring the emissions and aging processes of fresh *** this study,a combined system of differential mobility analyzer,centrifugal particle mass analyzer,and condensation particle counter was used to periodically measure theρ_(eff)of atmospheric particles in Shenzhen from Oct.2021 to *** showed that theρ_(eff)of particles with various size presented a bimodal distribution,which could be divided into main density(ρ_(m),main peak,corresponding to relatively dense particles after aging)and sub density(ρ_(s),sub peak,corresponding to fresh particles).The occurrence frequencies ofρ_(s)of particles with diameters of 50 and 80 nm were less than 20%,but were as high as about 40%of that with diameters from 120 to 350 ***ρ_(m)showed increasing trend with the size of particles,whileρ_(s)decreased as the increasing of the size of ***ρ_(eff)on pollution day varied significantly with chemical *** increasing of the proportion of sulfate could promote the increasing ofρ_(eff),while black carbon and organic matter caused opposite effects,which may be related to various factors,including the difference of the material density and morphology of various chemical ***ρ_(eff)of 50,80 and 120 nm particles decreased considerably during the new particle formation event,indicating that organic condensation was an important contributor to new particle growth.

关键词： DMA-CPMA-CPC Effective density Main/sub density Size distribution

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Recycling of Silicone Rubber from Composite Insulator with Pyrolysis Method

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CSEE Journal of Power and Energy Systems 2024年第4期10卷 1787-1798页

作者： Ruiqi Shang liming Wang Fanghui Yin Masoud Farzaneh Institute of Advanced Technologies in Energy and Electrical Engineering(IAT3E) Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Department of Applied Sciences(DSA) University of Quebec at ChicoutimiChicoutimiQC G7H2B1Canada

Composite insulators have been widely used in transmission *** being removed from transmission lines,their housing silicone material cannot degrade *** tackle this problem,this paper proposes an effective method to recycle waste insulators by pyrolysis to obtain mullite(3Al_(2)O_(3)·2SiO_(2))with high purity and compact *** recycling process studied will not generate toxic *** thermal degradation process of housing material is investigated by analyzing its degradation products including the gas and residues in *** experimental results indicate that the colorant agent Fe2O3 inside the housing material is beneficial for the generation of mullite by decreasing the temperature of ***,since the transitional alumina generated by the dehydration of aluminum hydroxide(ATH)has a smaller diameter and can better dissolute into the silica phases,ATH is a better choice as the additional aluminum *** comparing the components,structure,and particle size of grains formed at different calcination temperatures,the proposed pyrolysis temperatures of the two stages are 1400◦C and 1600◦C,respectively.

关键词： Composite insulator mullite pyrolysis recycling silicone rubber sintering

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DeciLS-PBO: an effective local search method for pseudo-Boolean optimization

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Frontiers of Computer Science 2024年第2期18卷 239-241页

作者： Luyu JIANG Dantong OUYANG Qi ZHANG liming ZHANG College of Computer Science and Technology Jilin UniversityChangchun 130012China Key Laboratory of Symbolic Computation and Knowledge Engineering(Ministry of Education) Jilin UniversityChangchun 130012China

1 Introduction Local search method is a rising star for solving combinatorial optimization problems in recent years,and the state-of-the-art local search-based incomplete Maximum Satisfiability(MaxSAT)solversshowpromi... 详细信息

关键词： Max optimization local

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Study on detecting main ingredients of silicone rubber based on terahertz spectrum

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High Voltage 2024年第3期9卷 518-527页

作者： Hongwei Mei Lanxin Li Fanghui Yin liming Wang Masoud Farzaneh Shenzhen International Graduate School(SIGS) Tsinghua UniversityShenzhenGuangdongChina Kunming Power Exchange Center KunmingYunnanChina Department of Applied Sciences(DSA) University of Quebec at ChicoutimiChicoutimiQuebecCanada

The authors investigated the ingredient detection technique of silicone rubber based on the Terahertz *** this purpose,18 diverse high-temperature vulcanised silicone rubber(HTVSR)formulations were customised,8 of which are used as calibration set while the rest 10 as prediction *** on the Beer-Lambert Law,the partial-least-square(PLS)regression model and the least-squares support-vector machines(LS-SVM)regression model were used to yield the relationships between the absorption spectrums and the content percentages of polydimethylsiloxane(PDMS),alumina tri-hydrate(ATH),and silica in *** results showed that for the formulations tested,the prediction accuracy of all three main ingredients by the PLS regression model could be improved by changing the spectrum range from 0.2–4 to 0.5–2 *** the data were pre-processed by the Savitzky–Golay smoothing method or multiplicative scatter correction method,the prediction accuracy of PDMS could be further ***,this would lead to a slight decrease in the prediction accuracy of *** the LS-SVM regression model,the radial basis function(RBF)kernel and the linear kernel were *** was found that the prediction accuracy of both kernels was better than that of the PLS regression *** the LS-SVM regression model using the RBF kernel,the correlated coefficients of PDMS and ATH in the prediction set could be up to 0.9915 and 0.9742,respectively.

关键词： rubber spectrum kernel

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