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Ammonia pyrolysis oxidation excited by nanosecond pulsed discharge:Global/fluid models hybrid solution

Journal of Energy Chemistry 2025年第1期100卷 385-396页

作者： Mingming Zhang hanyu Wu Qi Chen Jiaxin Yang Bonan Liu School of Mechanical Electronic and Control Engineering Beijing Jiaotong University China University of Petroleum

The kinetic characteristics of plasma-assisted oxidative pyrolysis of ammonia are studied by using the global/fluid models hybrid solution ***,the stable products of plasma-assisted oxidative pyrolysis of ammonia are *** results show that the consumption of NH3/O2and the production of N2/H2change linearly with the increase of voltage,which indicates the decoupling of nonequilibrium molecular excitation and oxidative pyrolysis of ammonia at low ***,the detailed reaction kinetics mechanism of ammonia oxidative pyrolysis stimulated by a nanosecond pulse voltage at low pressure and room temperature is *** on the reaction path analysis,the simplified mechanism is *** detailed and simplified mechanism simulation results are compared with experimental data to verify the accuracy of the simplified ***,based on the simplified mechanism,the fluid model of ammonia oxidative pyrolysis stimulated by the nanosecond pulse plasma is established to study the pre-sheath/sheath behavior and the resultant consumption and formation of key *** results show that the generation,development,and propagation of the pre-sheath have a great influence on the formation and consumption of *** consumption of NH3by the cathode pre-sheath is greater than that by the anode pre-sheath,but the opposite is true for OH and O（1S）.However,within the sheath,almost all reactions do not ***,by changing the parameters of nanosecond pulse power supply voltage,it is found that the electron number density,electron current density,and applied peak voltages are not the direct reasons for the structural changes of the sheath and ***,the discharge interval has little effect on the sheath structure and gas mixture *** research results of this paper not only help to understand the kinetic promotion of non-equilibrium excitation in the process of oxidative pyrolysis but also help to explore th

关键词： Nanosecond pulsed discharge Ammonia Oxidative pyrolysis Fluid model Global model

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Bioinspired Passive Tactile Sensors Enabled by Reversible Polarization of Conjugated Polymers

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Nano-Micro Letters 2025年第1期17卷 361-377页

作者： Feng He Sitong Chen Ruili Zhou hanyu Diao Yangyang Han Xiaodong Wu School of Mechanical Engineering Sichuan UniversityChengdu 610065People’s Republic of China School of Software Engineering Chongqing University of Posts and TelecommunicationsChongqing 400065People’s Republic of China State Key Laboratory of Polymer Materials Engineering Sichuan UniversityChengdu 610065People’s Republic of China

Tactile perception plays a vital role for the human body and is also highly desired for smart prosthesis and advanced *** to active sensing devices,passive piezoelectric and triboelectric tactile sensors consume less power,but lack the capability to resolve static ***,we address this issue by utilizing the unique polarization chemistry of conjugated polymers for the first time and propose a new type of bioinspired,passive,and bio-friendly tactile sensors for resolving both static and dynamic ***,to emulate the polarization process of natural sensory cells,conjugated polymers(including poly(3,4-ethylenedioxythiophen e):poly(styrenesulfonate),polyaniline,or polypyrrole)are controllably polarized into two opposite states to create artificial potential *** controllable and reversible polarization process of the conjugated polymers is fully in situ ***,a micro-structured ionic electrolyte is employed to imitate the natural ion channels and to encode external touch stimulations into the variation in potential difference *** with the currently existing tactile sensing devices,the developed tactile sensors feature distinct characteristics including fully organic composition,high sensitivity(up to 773 mV N^(−1)),ultralow power consumption(nW),as well as superior *** demonstrations,both single point tactile perception(surface texture perception and material property perception)and two-dimensional tactile recognitions(shape or profile perception)with high accuracy are successfully realized using self-defined machine learning *** tactile sensing concept innovation based on the polarization chemistry of conjugated polymers opens up a new path to create robotic tactile sensors and prosthetic electronic skins.

关键词： Passive tactile sensors Reversible polarization of conjugated polymers Tactile perception Machine learning algorithm Object recognition

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Space advanced technology demonstration satellite

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Science China(Technological Sciences) 2024年第1期67卷 240-258页

作者： ZHANG XiaoFeng CHEN Wen ZHU XiaoCheng MENG Na HE JunWang BI XingZi ZHANG YongHe SHI Qi LI Fei LIU Rui FENG ZhengGong LIU Liu LI JinSong WU HaiChen XU DongXiao LI TaiJie HUANG JiangJiang LIU Shuo LI TianTong YU XianSheng GAO Yang ZHOU Heng ban hanyu ZHANG YanLi ZHANG YueTing YANG YingQuan HE Tao DUAN XuLiang CHEN Xin WANG YaMin SUN AnTai ZHANG KuoXiang SUN Ying WANG YaoBin FAN ChengCheng XIONG ShaoLin LI XinQiao WEN XiangYang LING ZhiXing SUN XiaoJin ZHANG Chen BAI XianYong WANG ZhanShan DENG YuanYong TIAN Hui YANG JianFeng XUE HongBo SANG Peng LIU JinGuo ZHENG HuiLong ZHU Xiang HE JianWu LI Hui XU LuXiang XU ShuYan CHEN WenWu LIU ZhenDong WANG ZhaoLi MAO XiangLong GAO Rong LI ZongXuan DING GuoPeng WANG XinYu DOU RunJiang WENG LuBin LUO Hao WANG YaPing LIANG XianFeng FANG ZiRuo Innovation Academy for Microsatellites Chinese Academy of SciencesShanghai 201203China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China National Astronomical Observatory of China Beijing 100101China Shanghai Institute of Technical Physics Chinese Academy of SciencesShanghai 200083China Institute of Precision Optical Engineering School of Physics Science and EngineeringTongji UniversityShanghai 200092China School of Earth and Space Sciences Peking UniversityBeijing 100871China Xi’an Institute of Optics and Precision Mechanics Chinese Academy of SciencesXi’an 710119China National Space Science Center Chinese Academy of SciencesBeijing 100190China Shenyang Institute of Automation Chinese Academy of SciencesShenyang 110016China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China Institute of Mechanics Chinese Academy of SciencesBeijing 100190China Shanghai Institute of Organic Chemistry Chinese Academy of SciencesShanghai 200032China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou 310024China Nanyang Technological University Singapore 569830Singapore Dalian Institute of Chemical Physics Chinese Academy of SciencesDalian 116023China Technical Institute of Physics and Chemistry Chinese Academy of SciencesBeijing 100049China Changchun Institute of Optics Fine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Institute of Semiconductors Chinese Academy of SciencesBeijing 100083China Institute of Automation Chinese Academy of SciencesBeijing 100190China School of Aeronautics and Astronautics Zhejiang UniversityHangzhou 310058China

The Space Advanced Technology demonstration satellite(SATech-01),a mission for low-cost space science and new technology experiments,organized by Chinese Academy of Sciences(CAS),was successfully launched into a Sun-synchronous orbit at an altitude of~500 km on July 27,2022,from the Jiuquan Satellite Launch *** as an experimental platform for space science exploration and the demonstration of advanced common technologies in orbit,SATech-01 is equipped with 16 experimental payloads,including the solar upper transition region imager(SUTRI),the lobster eye imager for astronomy(LEIA),the high energy burst searcher(HEBS),and a High Precision Magnetic Field Measurement System based on a CPT Magnetometer(CPT).It also incorporates an imager with freeform optics,an integrated thermal imaging sensor,and a multi-functional integrated imager,*** paper provides an overview of SATech-01,including a technical description of the satellite and its scientific payloads,along with their on-orbit performance.

关键词： SATech-01 spacecraft design scientific instruments on-orbit performance

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Advances and applications in single-cell and spatial genomics

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Science China Life Sciences 2025年

作者： Jingjing Wang Fang Ye Haoxi Chai Yujia Jiang Teng Wang Xia Ran Qimin Xia Ziye Xu Yuting Fu Guodong Zhang hanyu Wu Guoji Guo Hongshan Guo Yijun Ruan Yongcheng Wang Dong Xing Xun Xu Zemin Zhang Beijing Advanced Innovation Center for Genomics (ICG) Peking University Guangdong Provincial Key Laboratory of Genome Read and Write BGI Research Bone Marrow Transplantation Center of the First Affiliated Hospital & Liangzhu Laboratory Zhejiang University School of Medicine Life Sciences Institute and The Second Affiliated Hospital Zhejiang University BGI Research Biomedical Pioneering Innovation Center (BIOPIC) and School of Life Sciences Peking University Academy for Advanced Interdisciplinary Studies Peking University Institute of Hematology Zhejiang University Department of Laboratory Medicine of The First Affiliated Hospital & Liangzhu Laboratory Zhejiang University School of Medicine Center for Stem Cell and Regenerative Medicine Zhejiang University School of Medicine Zhejiang Provincial Key Lab for Tissue Engineering and Regenerative Medicine Dr.Li Dak Sum & Yip Yio Chin Center for Stem Cell and Regenerative Medicine

The applications of single-cell and spatial technologies in recent times have revolutionized the present understanding of cellular states and the cellular heterogeneity inherent in complex biological systems. These advancements offer unprecedented resolution in the examination of the functional genomics of individual cells and their spatial context within tissues. In this review, we have comprehensively discussed the historical development and recent progress in the field of single-cell and spatial genomics. We have reviewed the breakthroughs in single-cell multi-omics technologies, spatial genomics methods, and the computational strategies employed toward the analyses of singlecell atlas data. Furthermore, we have highlighted the advances made in constructing cellular atlases and their clinical applications,particularly in the context of disease. Finally, we have discussed the emerging trends, challenges, and opportunities in this rapidly evolving field.

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Determination of 3,4-dichlorinated biphenyl in soil samples by real-time immuno-PCR assay

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Journal of Environmental Sciences 2012年第12期24卷 2191-2197页

作者： hanyu Chen Huisheng Zhuang School of Environmental Science and Engineering Shanghai Jiao Tong University Shanghai 200240 China. E-mail: chypds@ *** Department of Environment and Municipal Engineering Henan University of Urban Construction Henan 467043 China

A real-time fluorescent quantitative immuno-polymerase chain reaction （RT-IPCR） assay was developed for the detection of non-dioxin- like polychlorinated biphenyl （PCB） congener in soil samples. Based on the construction of 3,4-dichlorinated biphenyl （IUPAC PCB 12） hapten and its immunogen, the specific polyclonal antibodies （pAbs） to PCB12 was obtained and used to develop a direct competitive RT-IPCR assay. Using the optimized assay, a standard curve for PCB 12 was prepared. The linear range for the determination of PCB 12 was from 10.0 to 1.0 x l06 fg/mL with a correlation coefficient of 0.98 and a detection limit of 1.53 fg/rnL. The RT-IPCR assays were tested for their cross-reactivity profiles using four selected congeners and four Aroclor products. The results for the soil samples correlated with the concentrations of PCBs obtained by gas chromatography/mass spectrometry. This highly specific, sensitive, and robust assay can be applied to on-site tests of PCBs and serve as a model for other pollutant immunoassays.

关键词： 3,4-dichlorinated biphenyl antigen polyclonal antibody real-time immuno-PCR

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Single-atom catalysis for organic reactions

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Chinese Chemical Letters 2023年第6期34卷 121-129页

作者： hanyu Hu Jiangbo Xi Key Laboratory of Novel Biomass-Based Environmental and Energy Materials in Petroleum and Chemical Industry Key Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationHubei Key Laboratory of Novel Reactor and Green Chemical TechnologySchool of Chemistry and Environmental EngineeringWuhan Institute of TechnologyWuhan 430205China

Metal-based catalysis,including homogeneous and heterogeneous catalysis,plays a significant role in the modern chemical *** catalysis is widely used due to the high efficiency,easy catalyst separation and ***,the metal-utilization efficiency for conventional heterogeneous catalysts needs further improvement compared to homogeneous *** tackle this,the pursing of heterogenizing homogeneous catalysts has always been attractive but *** a recently emerging class of catalytic material,single-atom catalysts(SACs)are expected to bridge homogeneous and heterogeneous catalytic process in organic reactions and have arguably become the most active new frontier in catalysis *** this review,a brief introduction and development history of single-atom catalysis and SACs involved organic reactions are *** addition,recent advances in SACs and their practical applications in organic reactions such as oxidation,reduction,addition,coupling reaction,and other organic reactions are thoroughly *** understand structure-property relationships of single-atom catalysis in organic reactions,active sites or coordination structure,metal atom-utilization efficiency(e.g.,turnover frequency,TOF calculated based on active metal)and catalytic performance(e.g.,conversion and selectivity)of SACs are comprehensively ***,the application limitations,development trends,future challenges and perspective of SAC for organic reaction are discussed.

关键词： Single-atom catalysis Active site Metal utilization Organic reaction Catalytic performance

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Constructing super D-Kaup-Newell hierarchy and its nonlinear integrable coupling with self-consistent sources

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Frontiers of Mathematics in China 2019年第6期14卷 1353-1366页

作者： hanyu WEI Tiecheng XIA College of Mathematics and Statistics Zhoukou Normal UniversityZhoukou 466001China Department of Mathematics Shanghai UniversityShanghai 200444China

How to construct new super integrable equation hierarchy is an important *** this paper,a new Lax pair is proposed and the super D-Kaup-Newell hierarchy is generated,then a nonlinear integrable coupling of the super D-Kaup-Newcll hierarchy is *** super Hamiltonian structures of coupling equation hierarchy is derived with the aid of the super variational ***,the self-consistent sources of super integrable coupling hierarchy is *** is indicated that this method is a straightforward and efficient way to construct the super integrable equation hierarchy.

关键词： Super D-Kaup-Newell hierarchy nonlinear integrable coupling super Hamiltonian structures self-consistent sources

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Modified bottleneck-based heuristic for large-scale job-shop scheduling problems with a single bottleneck

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Journal of Systems Engineering and Electronics 2007年第3期18卷 556-565页

作者： Zuo Yan Gu hanyu Xi Yugeng Inst. of Automation Shanghai Jiaotong Univ. Shanghai 200240 P. R. China

A modified bottleneck-based （MB） heuristic for large-scale job-shop scheduling problems with a welldefined bottleneck is suggested, which is simpler but more tailored than the shifting bottleneck （SB） procedure. In this algorithm, the bottleneck is first scheduled optimally while the non-bottleneck machines are subordinated around the solutions of the bottleneck schedule by some effective dispatching rules. Computational results indicate that the MB heuristic can achieve a better tradeoff between solution quality and computational time compared to SB procedure for medium-size problems. Furthermore, it can obtain a good solution in a short time for large-scale jobshop scheduling problems.

关键词： job shop scheduling problem bottleneck shifting bottleneck procedure.

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Measurements and estimation of flow velocity in mobile bed rills

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International Journal of Sediment Research 2023年第1期38卷 97-104页

作者： Yunyun ban China Agricultural University Key Laboratory of Water Cycle and Related Land Surface Processes Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences

Rills are primary sediment sources and hillslope water/sediment runoff transport channels. Water flow velocities in rills are easily affected by bed condition over eroding and non-eroding slopes, which is an important hydrodynamic process in soil erosion research. This research is done to demonstrate the poorly understood “feedback mechanism” related to slope independence of flow velocity to slope gradient. A series of experiments were done on silt loam soil slopes to measure water flow velocity in rills under nine unit width flow rates(q)(0.17 × 10-3, 0.33 × 10-3, 0.67 × 10-3, 1.33 × 10-3, 2.67 × 10-3,5.33 × 10-3, 10.67 × 10-3, 21.33 × 10-3, and 42.67 × 10-3m3/(s·m)) combined with four slope gradients(8.7%, 17.6%, 26.8%, and 36.4%), in which mobile bed rills were monitored. For unit flow velocity under q ≤ 1.33 × 10-3m2/s, independence of flow velocity to slope was obtained. However, the results indicated that slope gradient combined with a higher unit flow rate contributed to better velocity prediction and fitted with a segmented equation well(R2= 0.95). A feedback mechanism was able to verify that the increase in roughness directly dissipated flow energy to reduce flow velocity, but cannot completely counterbalances steep slope effect. The experimental results showed that erosion-caused morphological changes on soil slopes reduce flow velocity by half due to an increase in bed roughness. Therefore, the current experimental measurements considering a wide range of flow rate and slope gradient conditions is useful to reveal the steep slope effect in mobile bed rills. The analysis showed that, for the investigated conditions, the flow velocity is a slope gradient-and flow ratedependent parameter.

关键词： Flow velocity Flow rate Slope gradient Model fitting Slope morphology

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Solid-state batteries:from 'all-solid' to 'almost-solid'

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National Science Review 2023年第6期10卷 57-59页

作者： hanyu Huo Jürgen Janek Institute of Physical Chemistry Justus Liebig University Giessen Center for Materials Research (ZfM) Justus Liebig University Giessen

Lithium-ion batteries (LIBs) have been the undisputed leading technology in electrochemical energy storage since they were commercialized in *** then,the mass manufacturing of LIBs has reached maturity,and we have also seen the realization of high energy density,long cycling stability and low *** technology enabled the huge success of mobile consumer electronics,with its usage in electric vehicles and other advanced *** to the use of organic solvents for the ele ctrolytes,LIBs are sensitive to high temperatures,lose performance at low temperatures and show inherent safety risks with increasing energy density (Fig.1a).As the performance of current LIBs is also limited,next-generation battery technologies are being intensively investigated,especially given the ever-increasing demand for high energy density as well as high power density.

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