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Phase Patterning of Poly(oxime-ester)for Information Encryption by Photo-induced Isomerization

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Chinese Journal of Polymer Science 2024年第10期42卷 1488-1494,I0010页

作者： Yu-Fan Yang Yun bai Yi-bao Li Chang-Fei He School of Chemistry and Chemical Engineering Gannan Normal UniversityGanzhou341000China

Crystal polymers or liquid crystal elastomers undergo a phase transition that results in a change in the corresponding optical properties,which has the potential to be applied in areas such as information encryption and *** utilization of these materials for patterning purposes requires different phase transition ***,once prepared,altering the phase transition temperature of them presents significant ***,a poly(oxime-ester)(POE)network is developed to achieve high-resolution and multilevel patterning by photo-induced *** as-prepared POE exhibits the ability to transition from an opaque state to a transparent state under temperature stimuli,with the transition temperature and kinetics dependent on UV light exposure ***,complex patterns and information can be encrypted through different selective regional exposure time and decrypted under specific temperature or cooling ***,we illustrate an example of temporal communication,where cooling time or temperature serves as the encoded *** research expands the application scope of advanced encryption materials,showcasing the potential of POE in dynamic information encryption and decryption processes.

关键词： Poly(oxime-ester) Isomerization Phase patterning Information encryption

Reliable calculations of nuclear binding energies by the Gaussian process of machine learning

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Nuclear Science and Techniques 2024年第6期35卷 130-144页

作者： Zi-Yi Yuan dong bai Zhen Wang Zhong-Zhou Ren School of Physics Science and Engineering Tongji UniversityShanghai 200092China College of Science Hohai UniversityNanjing 211100China Key Laboratory of Advanced Micro-Structure Materials Ministry of EducationShanghai 200092China

Reliable calculations of nuclear binding energies are crucial for advancing the research of nuclear physics. Machine learning provides an innovative approach to exploring complex physical problems. In this study, the nuclear binding energies are modeled directly using a machine-learning method called the Gaussian process. First, the binding energies for 2238 nuclei with Z > 20 and N > 20 are calculated using the Gaussian process in a physically motivated feature space, yielding an average deviation of 0.046 MeV and a standard deviation of 0.066 MeV. The results show the good learning ability of the Gaussian process in the studies of binding energies. Then, the predictive power of the Gaussian process is studied by calculating the binding energies for 108 nuclei newly included in AME2020. The theoretical results are in good agreement with the experimental data, reflecting the good predictive power of the Gaussian process. Moreover, the α-decay energies for 1169 nuclei with 50 ≤ Z ≤ 110 are derived from the theoretical binding energies calculated using the Gaussian process. The average deviation and the standard deviation are, respectively, 0.047 MeV and 0.070 MeV. Noticeably, the calculated α-decay energies for the two new isotopes ^ (204 )Ac(Huang et al. Phys Lett B 834, 137484(2022)) and ^ (207) Th(Yang et al. Phys Rev C 105, L051302(2022)) agree well with the latest experimental data. These results demonstrate that the Gaussian process is reliable for the calculations of nuclear binding energies. Finally, the α-decay properties of some unknown actinide nuclei are predicted using the Gaussian process. The predicted results can be useful guides for future research on binding energies and α-decay properties.

关键词： Nuclear binding energies decay Machine learning Gaussian process

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变压器局部放电射频和超声联合检测

沈阳工业大学学报 2009年第1期31卷 11-15,60页

作者：白保东兰云鹏沈阳工业大学生物医学与电磁工程研究所沈阳110178

针对变压器局部放电超声超声检测法在使用中存在灵敏度不高、定位误差过大等不足,提出使用射频和超声联合检测定位的方法.该方法针对超声超声检测定位法产生误差的原因提出相应改进措施,检测中超声波信号和射频电流信号被同时使用来判... 详细信息

针对变压器局部放电超声超声检测法在使用中存在灵敏度不高、定位误差过大等不足,提出使用射频和超声联合检测定位的方法.该方法针对超声超声检测定位法产生误差的原因提出相应改进措施,检测中超声波信号和射频电流信号被同时使用来判断局部放电现象的发生并对放电源进行定位,既具有超声波法便于定位的优点,又具备射频检测法快速检测局部放电发生的高灵敏度,同时还可以简化定位过程,提高系统抗干扰能力和定位实时性,实现对局部放电的在线检测和定位,具有较好的实际应用价值.

关键词：变压器局部放电射频超声波检测

Effects of Fe solid solute on grain boundaries of bi-crystal Cu: A molecular dynamics simulation

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Nano Materials Science 2024年第1期6卷 86-95页

作者： Shuohan Yang Hongwei bao Huizhong bai Yan Li Haodong Xu Fei Ma State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an710049ShaanxiChina

Grain boundaries(GBs)play a crucial role on the structural stability and mechanical properties of Cu and its *** this work,molecular dynamics(MD)simulations are employed to study the effects of Fe solutes on the formation energy,excess volume,dislocations and melting behaviors of GBs in CuFe *** is illustrated that Fe solute affects the structural stability of Cu GBs substantially,the formation energy of GBs is reduced,but the thickness and melting point of GBs are increased,that is,the structural stability of Cu GBs is significantly improved owing to the Fe solutes.A strong scaling law exists between the formation energy,excess volume,thickness and melting point of ***,Fe solid solute plays an important role in the characteristics of GBs in bi-crystal Cu.

关键词： CuFe alloy Grain boundary Structural stability MD simulations

三维瞬态涡流–电路–运动系统耦合问题的新解法

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中国电机工程学报 2008年第9期28卷 139-144页

作者：张洋白保东谢德馨沈阳工业大学电气工程学院辽宁省沈阳市110023

提出一种分析瞬态三维电磁场–电路–运动系统耦合问题的新方法,该方法考虑了外部电路、材料非线性、涡流影响以及运动等因素,适用于工程计算。对于三维瞬态涡流场与电路耦合问题,应用Crank-Nicholson法进行求解;对于运动问题,应用一种... 详细信息

提出一种分析瞬态三维电磁场–电路–运动系统耦合问题的新方法,该方法考虑了外部电路、材料非线性、涡流影响以及运动等因素,适用于工程计算。对于三维瞬态涡流场与电路耦合问题,应用Crank-Nicholson法进行求解;对于运动问题,应用一种非协调网格技术的插值运动边界法进行求解;三维电磁转矩的计算应用节点力法实现。为验证该方法的有效性,将其应用于TeamWork问题10、24以及24的运动模型的分析与计算,得到的结果误差均小于2%且计算时间明显缩短,即该方法能较为高效准确地解决瞬态三维电磁场–电路–运动系统耦合的问题。

关键词：瞬态涡流场耦合运动电磁转矩节点力法

Hydrodynamic analysis of carbon nanotube clusters in distributor-less conical fluidized beds with step-by-step scaling

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Chinese Journal of Chemical Engineering 2024年第3期67卷 117-125页

作者： Tianle Zhang Wenjuan bai Qianpeng dong Dianming Chu Lianlian Wang Yan He Shandong Engineering Laboratory for Preparation and Application of High-performance Carbon-Materials College of Electromechanical EngineeringQingdao University of Science and TechnologyQingdao 266061China Shandong Dazhan Nano Materials Co. Ltd.Binzhou 256220China

As a high-performance material with great application potential,the application of carbon nanotubes has been limited by their production volume.A distributor-less conical fluidized bed is the main equipment used in the industrial production of carbon *** improve the production volume and product quality of carbon nanotubes,the study of fluidized-bed-diameter scaling is *** different diameters of distributor-less conical fluidized beds were established,and then the particle behavior and bubble characteristics of carbon nanotube clusters at these bed diameters were ***-series and wavelet analysis methods were used to analyze the pressure-fluctuation signals inside the fluidized *** showed that the distributor-less design caused the airflow to break through the middle of the bed,which did not change with the change in bed *** powder-bridging phenomenon of carbon nanotube clusters in a 100-mm-diameter fluidized bed was related to the special microstructure of carbon nanotube *** frequency of pressure fluctuations in the bed decreased nonlinearly with increasing bed *** study can guide the design and scale-up of distributor-less conical fluidized beds,especially for the scale-up of carbon nanotube production equipment,which can contribute to the improvement of carbon nanotubes’capacity and quality in industrial production.

关键词： Carbon nanotubes Fluidized bed Multiphase flow Scale-up Multiscale

Crack identification in concrete, using digital image correlation and neural network

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Frontiers of Structural and Civil Engineering 2024年第4期18卷 536-550页

作者： Jingyi WANG dong LEI Kaiyang ZHOU Jintao HE Feipeng ZHU Pengxiang bai College of Mechanics and Materials Hohai UniversityNanjing 211100China

In engineering applications,concrete crack monitoring is very *** methods are of low efficiency,low accuracy,have poor timeliness,and are applicable in only a limited number of ***,more comprehensive detection of concrete damage under different scenarios is of high value for practical engineering *** image correlation(DIC)technology can provide a large amount of experimental data,and neural network(NN)can process very rich ***,NN,including convolutional neural networks(CNN)and back propagation neural networks(BP),can be combined with DIC technology to analyze experimental data of three-point bending of plain concrete and four-point bending of reinforced *** addition,strain parameters can be used for training,and displacement parameters can be added for comprehensive *** data obtained by DIC technology are grouped for training,and the recognition results of NN show that the combination of strain and displacement parameters,i.e.,the response of specimen surface and whole body,can make results more objective and *** identification results obtained by CNN and BP show that these technologies can accurately identify *** identification results for reinforced concrete specimens are less affected by noise than those of plain concrete *** is more convenient because it can identify some features directly from images,recognizing the cracks formed by macro *** can issue early warning of the microscopic cracks,but it requires a large amount of data and *** can be seen that CNN is more intuitive and efficient in image processing,and is suitable when low accuracy is adequate,while BP is suitable for occasions with greater accuracy *** two tools have advantages in different situations,and together they can play an important role in engineering monitoring.

关键词： digital image correlation convolutional neural network back propagation neural neural network damage detection concrete

In-situ construction of PDOL electrolyte with dual-reinforced stable interface for high-voltage lithium metal batteries

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Science China Chemistry 2024年第5期67卷 1664-1671页

作者： Yingkang Wu Yuzhou bai Wujie dong Xue Wang Wenqin Ma Fuqiang Huang State Key Lab of Metal Matrix Composites School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China School of Physical Science and Technology Shanghai Tech UniversityShanghai 201210China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050China

In-situ polymerized electrolytes significantly enhance the interfacial compatibility of lithium metal batteries(LMBs). Typically,in-situ polymerized 1,3-dioxolane(PDOL) exhibits low interfacial resistance, yet still suffers from low ionic conductivity and a narrow electrochemical stability window(ESW). Here, an ultra-stable PDOL-based polymer electrolyte is developed by incorporating plasticizers of tetramethylene sulfone(TMS) and fluorinated ethylene carbonate(FEC) into the 3D cross-linked network, achieving a significant enhancement in the transport capacity and efficiency of Li-ion. The ionic conductivity reaches3.63×10^(-4)S cm^(-1)even at room temperature, and the transference number(tLi^(+)) is even higher at 0.85. Furthermore, the ESW of this electrolyte can be increased to 4.5 V with the addition of TMS, which forms a thin and robust antioxidant cathode-electrolyte interface(CEI) on the surface of high-voltage LiCoO_(2). FEC generates an inorganic-rich solid-electrolyte interface(SEI) on the Li anode, which effectively inhibits the growth of lithium dendrites. Benefiting from the aforementioned advantages, the highvoltage lithium metal battery demonstrates outstanding long-cycle stability, with 93.2% capacity retention after 200 cycles. This work offers a straightforward and accessible method for the practical implementation of high energy density in-situ polymerized solid-state LMBs.

关键词： solid polymer electrolyte in-situ polymerization PDOL high-voltage LMBs

Spherical cationic polymer networks with porphyrin photosensitizer for sustainable and efficient photocatalysis

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Nano Research 2024年第5期17卷 3934-3941页

作者： Lingling Zhang Liwei Wu Junhui bao Longhui Li Zejun Liu Feng bai Jie Ju Xi Yao Key Laboratory for Special Functional Materials of Ministry of Education School of Materials Science and EngineeringHenan UniversityKaifeng 475004China Department of Chemistry City University of Hong KongKowloonHong Kong 999077China

The continuous and sustainable photo-activity on micro-or nano-carriers has always been a key stepping stone in the industrialization of photo-catalysis,photo-synthesis,and ***,we report a new series of positively charged hollow microspheres carrying porphyrin *** hollow spheres are formed through crosslinking of well-ordered porous thin laminates,initiated by co-assembly of regular monomers and those decorated with porphyrin *** the surface of an individual sphere,densely distributed positive sites attract anionic *** superficial porphyrin decomposes the accumulated reactants under 1 *** degradation and release of products,the photoactive sites are thereby *** demonstrate that polymer network(1:10)exhibited superior sustainable photocatalytic performance with complete degradation of methyl orange(MO)in 40 min with no observable performance deterioration after six *** established close loop of adsorption-reaction-release cycle makes possible many efficient and continuous photo-catalytic processes.

关键词： hydrogen bonding assembly porphyrin sustainable photo-activity anionic pollutant