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Plasma science and Technology 2011年第1期13卷 82-87页

作者： sankarsan MOHAPATRO b.s.rajanikanth High Voltage Lab Indian Institute of Science

Improved performance of plasma in raw engine exhaust treatment is reported. A new type of reactor referred to as of cross-flow dielectric barrier discharge （DbD） was used, in which the gas flow is perpendicular to the corona electrode. In raw exhaust environment, the cross-flow （radial-flow） reactor exhibits a superior performance with regard to NOx removal when compared to that with axial flow of gas. Experiments were conducted at different flow rates ranging from 2 L/min to 25 L/min. The plasma assisted barrier discharge reactor has shown encouraging results in NOx removal at high flow rates.

关键词： electric discharges NOx removal, non-thermal plasma, raw diesel engine exhaust

Achieving better NO_x Removal in Discharge Plasma Reactor by Field Enhancement

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Plasma science and Technology 2008年第2期10卷 198-202页

作者： b.s.rajanikanth Dipanwita sINHA High Voltage Laboratory Deptartment of Electrical Engineering Indian Institute of Science Bangalore 560012 India

Application of plasma chemistry for gas cleaning is gaining prominence in recent years, mainly from an energy efficiency point of view. In this paper we conducted a comparative study of NO/NOx removal using two different types of dielectric barrier discharge electrodes, wire- cylinder reactor, pipe-cylinder reactor. Investigations were first carried out with synthetic gases to obtain the baseline information on the NO/NOx removal with respect to the two geometries studied. Further, experiments were carried out with raw diesel exhaust under loaded condition. A high NOx removal efficiency of 90% was observed for the pipe-cylinder reactor as compared to that of 53.4% for the wire-cylinder reactor. Furthermore, for the same energy consumed per NO molecule （about 73 eV/NO molecule）, the removal efficiency increased from 67% for the wire- cylinder to about 98% for the pipe-cylinder which was quite appreciable.

关键词： NOx removal engine exhaust plasma treatment barrier discharge electrodes

DeNOx study in Diesel Engine Exhaust Using barrier Discharge Corona Assisted by V_2O_5/TiO_2 Catalyst

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Plasma science and Technology 2004年第4期6卷 2411-2415页

作者： b.s.rajanikanth V.Ravi Indian Institute of science Bangalore 560012IndiaIndian Institute of ScienceBangalore 560012India

A plasma-assisted catalytic reactor was used to remove nitrogen oxides (NOx)from diesel engine exhaust operated under different load conditions. Initial studies were focused onplasma reactor (a dielectric barrier discharge reactor) treatment of diesel exhaust at varioustemperatures. The nitric oxide (NO) removal efficiency was lowered when high temperature exhaust wastreated using plasma reactor. Also, NO removal efficiency decreased when 45% load exhaust wastreated. studies were then made with plasma reactor combined with a catalytic reactor consisting ofa selective catalytic reduction (sCR) catalyst, V_2O_5/TiO_2. Ammonia was used as a reducing agentfor sCR process in a ratio of 1:1 to NOx. The studies were focused on temperatures of the sCRcatalytic reactor below 200℃. The plasma-assisted catalytic reactor was operated well to remove NOxunder no-load and load conditions. For an energy input of 96 J/l, the NOx removal efficienciesobtained under no-load and load conditions were 90% and 72% respectively at an exhaust temperatureof 100 ℃.

关键词： non-thermal plasma DeNOx barrier discharge diesel exhaust

Discharge Plasma Assisted Adsorbents for Exhaust Treatment: A Comparative Analysis on Enhancing NO_x Removal

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Plasma science and Technology 2008年第3期10卷 307-312页

作者： b.s.rajanikanth Dipanwita sINHA P.EMMANUEL Department of High Voltage Engineering Indian Institute of Science Bangalore 560012 India

An analysis has been made on the discharge plasma coupled with an adsorbent system for NOx removal. The cascaded plasma-adsorbent system may be perceived as a better alternative for the existing adsorbent-based abatement system in the industry. In this study the exhaust is sourced from a diesel generator set. It was observed that better NO removal in a plasma reactor can be made possible by achieving higher average fields and subsequent NO2 removal can be improved using an adsorbent system connected in cascade with the plasma system. The paper describes various findings pertaining to these comparative analyses.

关键词： NOx removal engine exhaust discharge plasma plasma-adsorbent non- thermal plasma

A Cascaded Discharge plasma—Adsorbent Technique for Engine Exhaust Treatment

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Plasma science and Technology 2003年第3期5卷 1825-1833页

作者： b.s.rajanikanth A.D.srinivasan b.AryaNandiny DeptofHighVoltageEngineering IndianInstituteofScienceBangalore560012India

A cascaded system of electrical discharges (non-thermal plasma) andadsorption process was investigated for the removal of oxides of Nitrogen (NO_x) and totalhydrocarbons (THC) from an actual diesel engine exhaust. The non-thermal plasma and adsorptionprocesses were separately studied first and then the cascaded process was studied. In this study,different types of adsorbents were used. The NO_x removal efficiency was higher withplasma-associated adsorption (cascaded) process compared to the individual processes and the removalefficiency was found almost invariant in time. When associated by plasma, among the adsorbentsstudied, activated charcoal and Ms-13X were more effective for NO_x and THC removal *** experiments were conducted at no load and at 50 % load conditions. The plasma reactor was keptat room temperature throughout the experiment, while the temperature of the adsorbent reactor wasvaried. A relative comparison of adsorbents was discussed at the end.

关键词： discharge plasma engine exhaust adsorbent non-thermal plasma

Unfiltered Diesel Engine Exhaust Treatment by Discharge Plasma: Effect of soot Oxidation

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Plasma science and Technology 2004年第5期6卷 2475-2480页

作者： b.s.rajanikanth subhankar Das A.D.srinivasan Dept. of High Voltage Engineering Indian Institute of Science Bangalore 560012 IndiaDept. of High Voltage Engineering Indian Institute of Science Bangalore 560012 IndiaDept. of High Voltage Engineering Indian Institute of Science Bangalore 560012 India

A cascaded system of electrical discharges (Non-thermal plasma), catalyst andadsorption process was investigated for the removal of oxides of nitrogen (NO_x) and carbonmonoxide (CO) from a Diesel engine raw exhaust. The three processes were separately studied first,and then the cascaded processes, namely plasma-catalyst and plasma-adsorbent, were investigated. Inthis paper main emphasis was laid on the effect of carbonaceous soot oxidation on the plasmatreatment process. While the cascaded plasma-catalyst process exhibits a higher CO removal, thecascaded plasma-adsorbent process exhibits a higher NO_x removal. The experiments were conductedunder no-load. The plasma and adsorbent reactors were kept at room temperature throughout theexperiment while the catalyst reactor was kept at 200℃ / 300℃.

关键词： discharge plasma diesel engine exhaust catalyst adsorbent non-thermalplasma

NOx Reduction and Desorption studies Under Electric Discharge Plasma Using a simulated Gas Mixture:A Case study on the Effect of Corona Electrodes

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Plasma science and Technology 2009年第3期11卷 327-333页

作者： K.YOsHIDA b.s.rajanikanth M.OKUbO Plasma and Environmental Engineering Laboratory Department of Electrical and Electronic Systems EngineeringOsaka Institute of Technology High Voltage Laboratory Department of Electrical EngineeringIndian Institute of Science Environmental Protection Engineering Laboratory Department of Mechanical EngineeringOsaka Prefecture University

In this study, reduction and desorption of oxides of nitrogen （NOx） were conducted using an electrical discharge plasma technique. The study was carried out using a simulated gas mixture to explore the possibility of re-generation of used adsorbents by a nonthermal plasma desorption technique. Three different types of corona electrodes, namely, pipe, helical wire, and straight wire, were used for analyzing their effectiveness in NOx reduction/desorption. The pipe- type corona electrode exhibited a nitric oxide （NO） conversion of 50%, which is 1.5 times that of the straight-wire-type electrode at an energy density of 175 J/L. The helical-wire-type corona electrode exhibited a NOx desorption efficiency almost 4 times that of the pipe-type electrode, indicating the possibility that corona-generated species play a crucial role in desorption.

关键词： NOx reduction nonthermal plasma electric discharge application NOx desorption

Catalyst-Packed Non-Thermal Plasma Reactor for Removal of Nitrogen Oxides

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Plasma science and Technology 2003年第1期5卷 1603-1608页

A single-stage plasma-catalytic reactor in which catalytic materials werepacked was used to remove nitrogen oxides. The packing material was scoria being made of variousmetal oxides including Al_2O_3, MgO, TiO_2, etc. scoria was able to act not only as dielectricpellets but also as a catalyst in the presence of reducing agent such as ethylene and *** plasma discharge, scoria did not work well as a catalyst in the temperature range of 100 ℃to 200 ℃, showing less than 10% of NOx removal efficiency. When plasma is produced inside thereactor, the NOx removal efficiency could be increased to 60% in this temperature range.

关键词： plasma catalyst scoria nitrogen oxides removal

studies on Nitrogen Oxides Removal Using Plasma Assisted Catalytic Reactor

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Plasma science and Technology 2003年第6期5卷 2057-2062页

作者： V.Ravi Young sun Mok b.s.rajanikanth Ho-Chul Kang Department of High Voltage Engineering Indian Institute of Science Bangalore-560 012IndiaDepartment of Chemical EngineeringCheju National UniversityAraCheju 690-756South KoreaDepartment of High Voltage EngineeringIndian Institute of Science Bangalore-560 012IndiaDepartment of Chemical EngineeringCheju National UniversityAraCheju 690-756South Korea

An electric discharge plasma reactor combined with a catalytic reactor wasstudied for removing nitrogen oxides. To understand the combined process thoroughly, dischargeplasma and catalytic process were separately studied first, and then the two processes were combinedfor the study. The plasma reactor was able to oxidize NO to NO_2 well although the oxidation ratedecreased with temperature. The plasma reactor alone did not reduce the NO_x (NO+NO_2) leveleffectively, but the increase in the ratio of NO_2 to NO as a result of plasma discharge led to theenhancement of NO_x removal efficiency even at lower temperatures over the catalyst surface(V_2O_5-WO_3/TiO_2). At a gas temperature of 100℃, the NO_x removal efficiency obtained using thecombined plasma catalytic process was 88% for an energy input of 36 eV/molecule or 30 J/l.

关键词： non-thermal plasma catalytic process oxidation NO_x removal

Injection of N-Radicals into Diesel Engine Exhaust Treated by Plasma for Improved NO_x Removal: A Feasibility study

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Plasma science and Technology 2006年第2期8卷 202-206页

作者： b. s. rajanikanth b. R. sUsHMA Dept. of High Voltage Engineering Indian Institute of Science Bangalore 560012 India

Reported in this paper is a feasibility study on the injection of plasma induced N radicals for the abatement of NO and NOx present in the actual diesel exhaust. The radical laden diesel exhaust was further treated by discharge plasma in a dielectric barrier discharge reactor. N radicals were produced in a separate plasma reactor filled with baTiO3 pellets and were then injected into the treatment zone, There was a significant improvement in the efficiency when the radicals were injected compared to that when there was no radical injection. The efficiency of NOx removal at 0 load with plasma alone was 14% whereas with the injection of N radicals it went up to 38%, The results of the experiments conducted at different loads are discussed,

关键词： N-radical diesel engine exhaust NOx removal plasma treatment